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Andreas Becker

Bio: Andreas Becker is an academic researcher from University of Colorado Boulder. The author has contributed to research in topics: Ionization & Laser. The author has an hindex of 53, co-authored 222 publications receiving 9731 citations. Previous affiliations of Andreas Becker include Bielefeld University & University of Bayreuth.
Topics: Ionization, Laser, Attosecond, Femtosecond, Electron


Papers
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Journal ArticleDOI
08 Jun 2012-Science
TL;DR: By guiding a mid-infrared femtosecond laser in a high-pressure gas, ultrahigh harmonics can be generated that emerge as a bright supercontinuum that spans the entire electromagnetic spectrum from the ultraviolet to more than 1.6 kilo–electron volts, allowing, in principle, the generation of pulses as short as 2.5 attoseconds.
Abstract: High-harmonic generation (HHG) traditionally combines ~100 near-infrared laser photons to generate bright, phase-matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here, we show that by guiding a mid-infrared femtosecond laser in a high-pressure gas, ultrahigh harmonics can be generated, up to orders greater than 5000, that emerge as a bright supercontinuum that spans the entire electromagnetic spectrum from the ultraviolet to more than 1.6 kilo-electron volts, allowing, in principle, the generation of pulses as short as 2.5 attoseconds. The multiatmosphere gas pressures required for bright, phase-matched emission also support laser beam self-confinement, further enhancing the x-ray yield. Finally, the x-ray beam exhibits high spatial coherence, even though at high gas density the recolliding electrons responsible for HHG encounter other atoms during the emission process.

1,475 citations

Journal ArticleDOI
TL;DR: In this paper, a femtosecond laser pulse propagates in an optical medium, self-focusing occurs, and the most powerful part of the pulse self focuses first during its propagation.
Abstract: When a powerful femtosecond laser pulse propagates in an optical medium, self-focusing occurs. Normally, it is the most powerful part (slice) of the pulse that self-focuses first during its propaga...

559 citations

Journal ArticleDOI
TL;DR: It is shown that the puzzling experimental observation of suppressed molecular ionization, in intense laser fields, of O2, and its absence in N2, is a symmetry induced dynamical effect.
Abstract: It is shown that the puzzling experimental observation of suppressed molecular ionization, in intense laser fields, of ${\mathrm{O}}_{2}$, and its absence in ${\mathrm{N}}_{2}$, is a symmetry induced dynamical effect. More generally, it is predicted that the ionization signal of the class of homonuclear diatomic molecules having valence orbitals with an antibonding symmetry (e.g., ${\ensuremath{\sigma}}_{u}$, ${\ensuremath{\pi}}_{g}$) would be suppressed, but not those with a bonding symmetry (e.g., ${\ensuremath{\sigma}}_{g}$, ${\ensuremath{\pi}}_{u}$). The suppression effect can be visualized as due to an effective destructive interference between the two subwaves of the ionizing electron emerging from the two atomic centers.

324 citations

Journal ArticleDOI
TL;DR: The experiment shows that external focusing strongly influences the plasma density and the diameter of femtosecond Ti-sapphire laser filaments generated in air and is in good qualitative agreement with the results of numerical simulations.
Abstract: Our experiment shows that external focusing strongly influences the plasma density and the diameter of femtosecond Ti-sapphire laser filaments generated in air. The control of plasma filament parameters is suitable for many applications such as remote spectroscopy, laser induced electrical discharge, and femtosecond laser material interactions. The measurements of the filament showed the plasma density increases from 10(15)cm(-3) to 2 x 10(18)cm(-3) when the focal length decreases from 380 cm to 10 cm while the diameter of the plasma column varies from 30 microm to 90 microm. The experimental results are in good qualitative agreement with the results of numerical simulations.

303 citations

Journal ArticleDOI
TL;DR: In this paper, the authors present a consistent S-matrix formulation of the quantum amplitude for high harmonic generation (HHG) and point out some of the most general properties of HHG radiation emitted by a single atom as well as its relation to coherent emission from many atoms.
Abstract: Intense-field many-body S-matrix theory (IMST) provides a systematic ab initio approach to investigate the dynamics of atoms and molecules interacting with intense laser radiation. We review the derivation of IMST as well as its diagrammatic representation and point out its advantage over the conventional 'prior' and 'post' expansions which are shown to be special cases of IMST. The practicality and usefulness of the theory is illustrated by its application to a number of current problems of atomic and molecular ionization in intense fields. We also present a consistent S-matrix formulation of the quantum amplitude for high harmonic generation (HHG) and point out some of the most general properties of HHG radiation emitted by a single atom as well as its relation to coherent emission from many atoms. Experimental results for single and double (multiple) ionization of atoms and the observed distributions of coincidence measurements are analysed and the dominant mechanisms behind them are discussed. Ionization of more complex systems such as diatomic and polyatomic molecules in intense laser fields is analysed as well using IMST and the results are discussed with special attention to the role of molecular orbital symmetry and molecular orientation in space. The review ends with a summary and a brief outlook.

265 citations


Cited by
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28 Jul 2005
TL;DR: PfPMP1)与感染红细胞、树突状组胞以及胎盘的单个或多个受体作用,在黏附及免疫逃避中起关键的作�ly.
Abstract: 抗原变异可使得多种致病微生物易于逃避宿主免疫应答。表达在感染红细胞表面的恶性疟原虫红细胞表面蛋白1(PfPMP1)与感染红细胞、内皮细胞、树突状细胞以及胎盘的单个或多个受体作用,在黏附及免疫逃避中起关键的作用。每个单倍体基因组var基因家族编码约60种成员,通过启动转录不同的var基因变异体为抗原变异提供了分子基础。

18,940 citations

Journal ArticleDOI
TL;DR: The authors show the double-slit interference effect in the strong-field ionization of neon dimers by employing COLTRIMS method to record the momentum distribution of the photoelectrons in the molecular frame.
Abstract: Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.

7,160 citations

Journal ArticleDOI
TL;DR: In this paper, the main aspects of ultrashort laser pulse filamentation in various transparent media such as air (gases), transparent solids and liquids are introduced and discussed.

2,282 citations

Journal ArticleDOI
Peter Reimann1
TL;DR: In this paper, the main emphasis is put on directed transport in so-called Brownian motors (ratchets), i.e. a dissipative dynamics in the presence of thermal noise and some prototypical perturbation that drives the system out of equilibrium without introducing a priori an obvious bias into one or the other direction of motion.

2,098 citations

Proceedings Article
Ferenc Krausz1
01 Aug 2007
TL;DR: In this paper, an attosecond "oscilloscope" was used to visualize the oscillating electric field of visible light with an oscillator and probe multi-electron dynamics in atoms, molecules and solids.
Abstract: Summary form only given. Fundamental processes in atoms, molecules, as well as condensed matter are triggered or mediated by the motion of electrons inside or between atoms. Electronic dynamics on atomic length scales tends to unfold within tens to thousands of attoseconds (1 attosecond [as] = 10-18 s). Recent breakthroughs in laser science are now opening the door to watching and controlling these hitherto inaccessible microscopic dynamics. The key to accessing the attosecond time domain is the control of the electric field of (visible) light, which varies its strength and direction within less than a femtosecond (1 femtosecond = 1000 attoseconds). Atoms exposed to a few oscillations cycles of intense laser light are able to emit a single extreme ultraviolet (XUV) burst lasting less than one femtosecond. Full control of the evolution of the electromagnetic field in laser pulses comprising a few wave cycles have recently allowed the reproducible generation and measurement of isolated sub-femtosecond XUV pulses, demonstrating the control of microscopic processes (electron motion and photon emission) on an attosecond time scale. These tools have enabled us to visualize the oscillating electric field of visible light with an attosecond "oscilloscope", to control single-electron and probe multi-electron dynamics in atoms, molecules and solids. Recent experiments hold promise for the development of an attosecond X-ray source, which may pave the way towards 4D electron imaging with sub-atomic resolution in space and time.

1,618 citations