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Anton Kalinin

Other affiliations: Max Planck Society
Bio: Anton Kalinin is an academic researcher from Goethe University Frankfurt. The author has contributed to research in topics: Supercooling & Bound state. The author has an hindex of 11, co-authored 27 publications receiving 4690 citations. Previous affiliations of Anton Kalinin include Max Planck Society.

Papers
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Journal ArticleDOI
TL;DR: The authors show the double-slit interference effect in the strong-field ionization of neon dimers by employing COLTRIMS method to record the momentum distribution of the photoelectrons in the molecular frame.
Abstract: Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.

7,160 citations

Journal ArticleDOI
01 May 2015-Science
TL;DR: Experimental observation of this long-predicted but experimentally elusive Efimov state of 4He3 by means of Coulomb explosion imaging confirms the predicted size and a typical structure where two atoms are close to each other while the third is far away and sheds light on three-body physics more broadly.
Abstract: Quantum theory dictates that upon weakening the two-body interaction in a three-body system, an infinite number of three-body bound states of a huge spatial extent emerge just before these three-body states become unbound. Three helium (He) atoms have been predicted to form a molecular system that manifests this peculiarity under natural conditions without artificial tuning of the attraction between particles by an external field. Here we report experimental observation of this long-predicted but experimentally elusive Efimov state of 4 He 3 by means of Coulomb explosion imaging. We show spatial images of an Efimov state, confirming the predicted size and a typical structure where two atoms are close to each other while the third is far away.

182 citations

Journal ArticleDOI
TL;DR: In this article, the authors reported experimental observation of this long predicted but experimentally elusive Efimov state by means of Coulomb explosion imaging, confirming the predicted size and a typical structure where two atoms are close to each other while the third is far away.
Abstract: Quantum theory dictates that upon weakening the two-body interaction in a three-body system, an infinite number of three-body bound states of a huge spatial extent emerge just before these three-body states become unbound. Three helium atoms have been predicted to form a molecular system that manifests this peculiarity under natural conditions without artificial tuning of the attraction between particles by an external field. Here we report experimental observation of this long predicted but experimentally elusive Efimov state of $^{4}$He$_{3}$ by means of Coulomb explosion imaging. We show spatial images of an Efimov state, confirming the predicted size and a typical structure where two atoms are close to each other while the third is far away.

97 citations

Journal ArticleDOI
TL;DR: The size of the helium trimer is determined by diffracting a beam of 4He clusters from a 100 nm period grating inclined by 21 degrees, and the projected slit width is roughly halved to 27 nm, increasing the sensitivity to the trimer size.
Abstract: The size of the helium trimer is determined by diffracting a beam of $^{4}\mathrm{H}\mathrm{e}$ clusters from a 100 nm period grating inclined by 21\ifmmode^\circ\else\textdegree\fi{} Because of the bar thickness the projected slit width is roughly halved to 27 nm, increasing the sensitivity to the trimer size The peak intensities measured out to the eighth order are evaluated via a few-body scattering theory The trimer pair distance is found to be $⟨r⟩={11}_{\ensuremath{-}05}^{+04}\text{ }\text{ }\mathrm{nm}$ in agreement with predictions for the ground state No evidence for a significant amount of Efimov trimers is found Their concentration is estimated to be under 6%, less than expected

75 citations

Journal ArticleDOI
TL;DR: The size distributions of neutral 4He clusters in cryogenic jet beams, analyzed by diffraction from a 100 nm period transmission grating, reveal magic numbers at N=10-11, 14, 22, 26-27, and 44 atoms, thereby providing the first experimental confirmation for the energy levels of4He clusters.
Abstract: The size distributions of neutral 4He clusters in cryogenic jet beams, analyzed by diffraction from a 100 nm period transmission grating, reveal magic numbers at N=10-11, 14, 22, 26-27, and 44 atoms. Whereas magic numbers in nuclei and clusters are attributed to enhanced stabilities, this is not expected for quantum fluid He clusters on the basis of numerous calculations. These magic numbers occur at threshold sizes for which the quantized excitations calculated with the diffusion Monte Carlo method are stabilized, thereby providing the first experimental confirmation for the energy levels of 4He clusters.

65 citations


Cited by
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Journal ArticleDOI
TL;DR: Advances in nanoparticle design that overcome heterogeneous barriers to delivery are discussed, arguing that intelligent nanoparticles design can improve efficacy in general delivery applications while enabling tailored designs for precision applications, thereby ultimately improving patient outcome overall.
Abstract: In recent years, the development of nanoparticles has expanded into a broad range of clinical applications. Nanoparticles have been developed to overcome the limitations of free therapeutics and navigate biological barriers - systemic, microenvironmental and cellular - that are heterogeneous across patient populations and diseases. Overcoming this patient heterogeneity has also been accomplished through precision therapeutics, in which personalized interventions have enhanced therapeutic efficacy. However, nanoparticle development continues to focus on optimizing delivery platforms with a one-size-fits-all solution. As lipid-based, polymeric and inorganic nanoparticles are engineered in increasingly specified ways, they can begin to be optimized for drug delivery in a more personalized manner, entering the era of precision medicine. In this Review, we discuss advanced nanoparticle designs utilized in both non-personalized and precision applications that could be applied to improve precision therapies. We focus on advances in nanoparticle design that overcome heterogeneous barriers to delivery, arguing that intelligent nanoparticle design can improve efficacy in general delivery applications while enabling tailored designs for precision applications, thereby ultimately improving patient outcome overall.

2,179 citations

Journal ArticleDOI
TL;DR: In this paper, a review of the experimental methods for the production of free nanoclusters is presented, along with theoretical and simulation issues, always discussed in close connection with the experimental results.
Abstract: The structural properties of free nanoclusters are reviewed. Special attention is paid to the interplay of energetic, thermodynamic, and kinetic factors in the explanation of cluster structures that are actually observed in experiments. The review starts with a brief summary of the experimental methods for the production of free nanoclusters and then considers theoretical and simulation issues, always discussed in close connection with the experimental results. The energetic properties are treated first, along with methods for modeling elementary constituent interactions and for global optimization on the cluster potential-energy surface. After that, a section on cluster thermodynamics follows. The discussion includes the analysis of solid-solid structural transitions and of melting, with its size dependence. The last section is devoted to the growth kinetics of free nanoclusters and treats the growth of isolated clusters and their coalescence. Several specific systems are analyzed.

1,563 citations

Journal ArticleDOI
TL;DR: The development of wave optics for light brought many new insights into our understanding of physics, driven by fundamental experiments like the ones by Young, Fizeau, Michelson-Morley and others as mentioned in this paper.
Abstract: The development of wave optics for light brought many new insights into our understanding of physics, driven by fundamental experiments like the ones by Young, Fizeau, Michelson-Morley and others. Quantum mechanics, and especially the de Broglie’s postulate relating the momentum p of a particle to the wave vector k of an matter wave: k = 2 λ = p/ℏ, suggested that wave optical experiments should be also possible with massive particles (see table 1), and over the last 40 years electron and neutron interferometers have demonstrated many fundamental aspects of quantum mechanics [1].

1,194 citations

Journal ArticleDOI
01 Jun 2021
TL;DR: Some of the prevailing trends in embedding physics into machine learning are reviewed, some of the current capabilities and limitations are presented and diverse applications of physics-informed learning both for forward and inverse problems, including discovering hidden physics and tackling high-dimensional problems are discussed.
Abstract: Despite great progress in simulating multiphysics problems using the numerical discretization of partial differential equations (PDEs), one still cannot seamlessly incorporate noisy data into existing algorithms, mesh generation remains complex, and high-dimensional problems governed by parameterized PDEs cannot be tackled. Moreover, solving inverse problems with hidden physics is often prohibitively expensive and requires different formulations and elaborate computer codes. Machine learning has emerged as a promising alternative, but training deep neural networks requires big data, not always available for scientific problems. Instead, such networks can be trained from additional information obtained by enforcing the physical laws (for example, at random points in the continuous space-time domain). Such physics-informed learning integrates (noisy) data and mathematical models, and implements them through neural networks or other kernel-based regression networks. Moreover, it may be possible to design specialized network architectures that automatically satisfy some of the physical invariants for better accuracy, faster training and improved generalization. Here, we review some of the prevailing trends in embedding physics into machine learning, present some of the current capabilities and limitations and discuss diverse applications of physics-informed learning both for forward and inverse problems, including discovering hidden physics and tackling high-dimensional problems. The rapidly developing field of physics-informed learning integrates data and mathematical models seamlessly, enabling accurate inference of realistic and high-dimensional multiphysics problems. This Review discusses the methodology and provides diverse examples and an outlook for further developments.

1,114 citations

Journal ArticleDOI
16 Mar 2006-Nature
TL;DR: In this article, the Efimov trimer state was shown to exist in an ultracold gas of caesium atoms and its signature was observed as a giant three-body recombination loss when the strength of the two-body interaction is varied.
Abstract: In the bizarre world of quantum physics, three interacting particles can form a loosely bound system even if the two-particle attraction is too weak to allow for the binding of a pair. This exotic trimer state was predicted 35 years ago by Russian physicist Vitali Efimov, who found a remarkable and counterintuitive solution to the notoriously difficult quantum-mechanical three-body problem. Efimov's well known result was a landmark in theoretical few-body physics, but until now these exotic states had not been demonstrated experimentally. Now that has been achieved, in an ultracold gas of caesium atoms. The existence of this gas confirms key predictions and opens up few-body quantum systems to further experiment. The first experimental observation of Efimov's prediction confirms key theoretical predictions and represents a starting point from which to explore the universal properties of resonantly interacting few-body systems. Systems of three interacting particles are notorious for their complex physical behaviour. A landmark theoretical result in few-body quantum physics is Efimov's prediction1,2 of a universal set of bound trimer states appearing for three identical bosons with a resonant two-body interaction. Counterintuitively, these states even exist in the absence of a corresponding two-body bound state. Since the formulation of Efimov's problem in the context of nuclear physics 35 years ago, it has attracted great interest in many areas of physics3,4,5,6,7,8. However, the observation of Efimov quantum states has remained an elusive goal3,5. Here we report the observation of an Efimov resonance in an ultracold gas of caesium atoms. The resonance occurs in the range of large negative two-body scattering lengths, arising from the coupling of three free atoms to an Efimov trimer. Experimentally, we observe its signature as a giant three-body recombination loss9,10 when the strength of the two-body interaction is varied. We also detect a minimum9,11,12 in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point with which to explore the universal properties of resonantly interacting few-body systems7. While Feshbach resonances13,14 have provided the key to control quantum-mechanical interactions on the two-body level, Efimov resonances connect ultracold matter15 to the world of few-body quantum phenomena.

884 citations