The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), is the latest atmospheric reanalysis of the modern satellite era produced by NASA’s Global Modeling and Assimilation Office (GMAO). MERRA-2 assimilates observation types not available to its predecessor, MERRA, and includes updates to the Goddard Earth Observing System (GEOS) model and analysis scheme so as to provide a viable ongoing climate analysis beyond MERRA’s terminus. While addressing known limitations of MERRA, MERRA-2 is also intended to be a development milestone for a future integrated Earth system analysis (IESA) currently under development at GMAO. This paper provides an overview of the MERRA-2 system and various performance metrics. Among the advances in MERRA-2 relevant to IESA are the assimilation of aerosol observations, several improvements to the representation of the stratosphere including ozone, and improved representations of cryospheric processes. Other improvements in the quality of M...

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The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2)

[1] We use the Total Ozone Mapping Spectrometer (TOMS) sensor on the Nimbus 7 satellite to map the global distribution of major atmospheric dust sources with the goal of identifying common environmental characteristics The largest and most persistent sources are located in the Northern Hemisphere, mainly in a broad “dust belt” that extends from the west coast of North Africa, over the Middle East, Central and South Asia, to China There is remarkably little large-scale dust activity outside this region In particular, the Southern Hemisphere is devoid of major dust activity Dust sources, regardless of size or strength, can usually be associated with topographical lows located in arid regions with annual rainfall under 200–250 mm Although the source regions themselves are arid or hyperarid, the action of water is evident from the presence of ephemeral streams, rivers, lakes, and playas Most major sources have been intermittently flooded through the Quaternary as evidenced by deep alluvial deposits Many sources are associated with areas where human impacts are well documented, eg, the Caspian and Aral Seas, Tigris-Euphrates River Basin, southwestern North America, and the loess lands in China Nonetheless, the largest and most active sources are located in truly remote areas where there is little or no human activity Thus, on a global scale, dust mobilization appears to be dominated by natural sources Dust activity is extremely sensitive to many environmental parameters The identification of major sources will enable us to focus on critical regions and to characterize emission rates in response to environmental conditions With such knowledge we will be better able to improve global dust models and to assess the effects of climate change on emissions in the future It will also facilitate the interpretation of the paleoclimate record based on dust contained in ocean sediments and ice cores

https://agupubs.onlinelibrary.wiley.com/doi/epdf/10.1029/2000RG000095

Environmental characterization of global sources of atmospheric soil dust identified with the nimbus 7 total ozone mapping spectrometer (toms) absorbing aerosol product

The global distribution of dust aerosol is simulated with the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model. In this model all topographic lows with bare ground surface are assumed to have accumulated sediments which are potential dust sources. The uplifting of dust particles is expressed as a function of surface wind speed and wetness. The GOCART model is driven by the assimilated meteorological fields from the Goddard Earth Observing System Data Assimilation System (GEOS DAS) which facilitates direct comparison with observations. The model includes seven size classes of mineral dust ranging from 0.1–6 μm radius. The total annual emission is estimated to be between 1604 and 1960 Tg yr−1 in a 5-year simulation. The model has been evaluated by comparing simulation results with ground-based measurements and satellite data. The evaluation has been performed by comparing surface concentrations, vertical distributions, deposition rates, optical thickness, and size distributions. The comparisons show that the model results generally agree with the observations without the necessity of invoking any contribution from anthropogenic disturbances to soils. However, the model overpredicts the transport of dust from the Asian sources to the North Pacific. This discrepancy is attributed to an overestimate of small particle emission from the Asian sources.

https://agupubs.onlinelibrary.wiley.com/doi/pdf/10.1029/2000JD000053

Sources and distributions of dust aerosols simulated with the GOCART model

Mercury (Hg) is a global pollutant that affects human and ecosystem health. We synthesize understanding of sources, atmosphere-land-ocean Hg dynamics and health effects, and consider the implications of Hg-control policies. Primary anthropogenic Hg emissions greatly exceed natural geogenic sources, resulting in increases in Hg reservoirs and subsequent secondary Hg emissions that facilitate its global distribution. The ultimate fate of emitted Hg is primarily recalcitrant soil pools and deep ocean waters and sediments. Transfers of Hg emissions to largely unavailable reservoirs occur over the time scale of centuries, and are primarily mediated through atmospheric exchanges of wet/dry deposition and evasion from vegetation, soil organic matter and ocean surfaces. A key link between inorganic Hg inputs and exposure of humans and wildlife is the net production of methylmercury, which occurs mainly in reducing zones in freshwater, terrestrial, and coastal environments, and the subsurface ocean. Elevated human exposure to methylmercury primarily results from consumption of estuarine and marine fish. Developing fetuses are most at risk from this neurotoxin but health effects of highly exposed populations and wildlife are also a concern. Integration of Hg science with national and international policy efforts is needed to target efforts and evaluate efficacy.

http://pubs.acs.org/doi/pdf/10.1021/es305071v

Mercury as a Global Pollutant: Sources, Pathways, and Effects

A copy of Guangbo jiemu bao [Broadcast Program Report] was being passed from hand to hand among a group of young people eager to be the first to read the article introducing the program "What Is Revolutionary Love?" It said: "… Young friends, you are certainly very concerned about this problem'. So, we would like you to meet the young women workers Meng Xiaoyu and Meng Yamei and the older cadre Miss Feng. They are the three leading characters in the short story ‘The Place of Love.’ Through the description of the love lives of these three, the story induces us to think deeply about two questions that merit further examination.

This is How the Discussion Started

A soil-derived dust emission scheme has been designed to provide an explicit representation of the desert dust sources for the atmospheric transport models dealing with the simulation of the desert dust cycle. Two major factors characterizing the erodible surface are considered: (1) the size distribution of the erodible loose particles of the soil which controls the erosion threshold and the emission strength and (2) the surface roughness which imposes the efficient wind friction velocity acting on the erodible surface. These two parameters are included in a formulation of the threshold wind friction velocity by adapting a size-dependent parameterization proposed by Iversen and White (1982) and by applying to the rough erodible surfaces a drag partition scheme derived from Arya (1975). This parameterization of the threshold friction velocity has been included in an horizontal flux equation proposed by White (1979). This allows to attribute a specific production rate to each soil size range for each type of surface. The dust flux F is then considered as a fraction of the total horizontal flux G, the value of the ratio F/G being imposed, at this time, by the soil clay content. In summary, the computed mass fluxes depend on the soil size distribution, the roughness lengths, and the wind friction velocity. The different steps of this scheme have been independently validated by comparison with relevant experimental data. Globally, the agreement is satisfying, so that the dust fluxes could be retrieved with less uncertainties than those observed in previous simulations of the desert dust cycle.

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Modeling the atmospheric dust cycle: 1. Design of a soil-derived dust emission scheme

. Large-scale simulation of the soil-derived dust emission in semi-arid regions needs to account for the influence of the soil moisture on the wind erosion threshold. Soil water retention consists of molecular adsorption on the soil grain surface and capillary forces between the grain. Interparticle capillary forces (characterized by the moisture tension) are the main factor responsible for the increase of the wind erosion threshold observed when the soil moisture increases. When the soil moisture content is close to but smaller than the maximum amount of adsorbed water, w' (depending on the soil texture), these capillary forces are considered as not strong enough to significantly increase the erosion threshold. An expression of the moisture tension as a function of soil moisture and w' is derived from retention curves. From this expression, a parametrization of the ratio of the wet to dry erosion thresholds has been developed as a function of soil moisture and soil texture. The coefficients of this parametrization have been determined by using experimental data from the literature. An empirical relationship between w' and soil clay content has been established. The erosion threshold ratios simulated for different soil textures were found to be in good agreement with the experimental data. Key words. Atmospheric composition and structure (Aerosols and particles) · Hydrology (soil moisture)

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Parametrization of the increase of the aeolian erosion threshold wind friction velocity due to soil moisture for arid and semi-arid areas

A soil-derived dust emission scheme has been designed in order to provide simulation of mineral dust sources for atmospheric transport models [Marticorena and Bergametti, 1995]. This physical scheme considers the influence of surface features to compute the erosion threshold and the intensity of the dust emissions. It has been validated by comparison with relevant experimental data. However, it was necessary to extend its applicability and to test its capability to reproduce dust emissions over large arid areas. Specific methods have been developed to determine the parameters required by the dust production model for large-scale applications. The surface features (dimensions of the roughness elements and soil mineralogy) and the wind velocity allow the computation of the roughness lengths of the surface, the size distribution of the erodible soils, and the wind friction velocity. A map of these surface characteristics has been established for the western part of the Sahara. This map coupled to the Europan Center for Medium-Range Weather Forecast (ECMWF) surface wind fields are used to simulate dust emissions in this desert region. The simulated emissions have been compared to the Infrared Difference Dust Index (IDDI), determined by means of the Meteosat thermal infrared imagery. The simulated dust event frequencies are in good agreement with those observed by satellite. The comparison between the simulated fluxes and the satellite observations for 3 months of the year 1991 has revealed a linear relationship between the logarithm of the simulated flux and the IDDI. The annual and monthly dust emissions for 1991 and 1992 have been estimated and compared to those established by d'Almeida [1986]. Both the frequencies and the intensities of the emissions are well reproduced by the model associated with the surface features map.

https://agupubs.onlinelibrary.wiley.com/doi/pdf/10.1029/96JD02964

Modeling the atmospheric dust cycle: 2. Simulation of Saharan dust sources

A daily analysis of African dust concentrations in the Mediterranean atmosphere has been made between June 1983 and December 1994 using the International Satellite Cloud Climatology Project (ISCCP-B2) archive of Meteosat visible (VIS) channel images. The ISCCP-B2 archive of Meteosat infrared (IR) images has also been used to determine the frequencies of dust mobilization over the continent, north of 30°N. Despite a large daily variability, climatological results show a clear seasonal cycle with a maximum during the dry season: dust transport begins over the eastern basin in spring and spreads over the western basin in summer. These patterns are shown to be related to both cyclogenesis over North Africa and rainfall over the Mediterranean Sea. Indeed, the frequency of dust mobilization over the continent and of dust outbreaks over the sea are strongly related to the climatology of depressions affecting North Africa. Precipitations appear to be an important factor explaining both the seasonal east-west shift in transport location and the south-north gradients of dust concentrations over the Mediterranean.

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Satellite climatology of African dust transport in the Mediterranean atmosphere

A physical model was developed to explain threshold friction velocities u*t for particles of the size 60–120 μm lying on a rough surface in loose soils for semiarid and arid parts of the United States. The model corrected for the effect of momentum absorption by the nonerodible roughness. For loose or disturbed soils the most important parameter that controls u*t is the aerodynamic roughness height z0. For physical crusts damaged by wind the size of erodible crust pieces is important along with the roughness. The presence of cyanobacteriallichen soil crusts roughens the surface, and the biological fibrous growth aggregates soil particles. Only undisturbed sandy soils and disturbed soils of all types would be expected to be erodible in normal wind storms. Therefore disturbance of soils by both cattle and humans is very important in predicting wind erosion as confirmed by our measurements.

https://agupubs.onlinelibrary.wiley.com/doi/pdf/10.1029/97JD01303

Béatrice Marticorena

Papers

Modeling the atmospheric dust cycle: 1. Design of a soil-derived dust emission scheme

Parametrization of the increase of the aeolian erosion threshold wind friction velocity due to soil moisture for arid and semi-arid areas

Modeling the atmospheric dust cycle: 2. Simulation of Saharan dust sources

Satellite climatology of African dust transport in the Mediterranean atmosphere

Factors controlling threshold friction velocity in semiarid and arid areas of the United States