scispace - formally typeset
Search or ask a question
Author

Bingqing Wei

Bio: Bingqing Wei is an academic researcher from University of Delaware. The author has contributed to research in topics: Carbon nanotube & Nanotube. The author has an hindex of 86, co-authored 345 publications receiving 28325 citations. Previous affiliations of Bingqing Wei include Tsinghua University & Pohang University of Science and Technology.


Papers
More filters
Journal ArticleDOI
TL;DR: This work demonstrates the scalable fabrication of a new type of all-carbon, monolithic supercapacitor by laser reduction and patterning of graphite oxide films, which show good cyclic stability, and energy storage capacities comparable to existing thin-filmsupercapacitors.
Abstract: All-carbon microscale supercapacitors can be simply and scalably fabricated by the laser patterning and reduction of graphene oxide.

1,312 citations

Journal ArticleDOI
TL;DR: In this article, the current carrying capacity and reliability of multiwalled carbon nanotubes under high current densities (>109 A/cm2) were investigated and shown that no observable failure in the nanotube structure and no measurable change in the resistance are detected at temperatures up to 250 ˚C and for time scales up to 2 weeks.
Abstract: The current-carrying capacity and reliability studies of multiwalled carbon nanotubes under high current densities (>109 A/cm2) show that no observable failure in the nanotube structure and no measurable change in the resistance are detected at temperatures up to 250 °C and for time scales up to 2 weeks. Our results suggest that nanotubes are potential candidates as interconnects in future large-scale integrated nanoelectronic devices.

1,229 citations

Journal ArticleDOI
10 Jul 2003-Nature
TL;DR: The fabrication and successful testing of ionization microsensors featuring the electrical breakdown of a range of gases and gas mixtures at carbon nanotube tips are reported, enabling compact, battery-powered and safe operation of such sensors.
Abstract: Gas sensors operate by a variety of fundamentally different mechanisms1,2,3,4,5,6,7,8,9,10,11,12,13,14. Ionization sensors13,14 work by fingerprinting the ionization characteristics of distinct gases, but they are limited by their huge, bulky architecture, high power consumption and risky high-voltage operation. Here we report the fabrication and successful testing of ionization microsensors featuring the electrical breakdown of a range of gases and gas mixtures at carbon nanotube tips. The sharp tips of nanotubes generate very high electric fields at relatively low voltages, lowering breakdown voltages several-fold in comparison to traditional electrodes, and thereby enabling compact, battery-powered and safe operation of such sensors. The sensors show good sensitivity and selectivity, and are unaffected by extraneous factors such as temperature, humidity, and gas flow. As such, the devices offer several practical advantages over previously reported nanotube sensor systems15,16,17. The simple, low-cost, sensors described here could be deployed for a variety of applications, such as environmental monitoring, sensing in chemical processing plants, and gas detection for counter-terrorism.

925 citations

Journal ArticleDOI
TL;DR: Interestingly, SEM, TEM, and HRTEM revealed a variety of structures ranging from nanostructured surface with a distinct platelike morphology to nanorod depending upon the hydrothermal reaction time employed during the preparation of the manganese oxide: increasing the amount of individual nanorods in the materials prepared with longer hydrother mal reaction time.
Abstract: The effect of varying the hydrothermal time to synthesize manganese oxide (MnO(2)) nanostructures was investigated along with their influence on structural, morphological, compositional, and electrochemical properties in supercapacitor electrode materials. XRD and TEM studies showed that the MnO(2) prepared in shorter hydrothermal dwell time was a mixture of amorphous and nanocrystalline particles, and there was an evolution of crystallinity of the nanostructures as the dwell time increased from 1 to 18 h. Interestingly, SEM, TEM, and HRTEM revealed a variety of structures ranging from nanostructured surface with a distinct platelike morphology to nanorods depending upon the hydrothermal reaction time employed during the preparation of the manganese oxide: increasing the amount of individual nanorods in the materials prepared with longer hydrothermal reaction time. The surface area of the synthesized nanomaterials varied from 100 to 150 m(2)/g. Electrochemical properties were evaluated using cyclic voltammetry (CV) and galvanostatic charge-discharge studies, and the capacitance values were in the range 72-168 F/g depending upon synthesis conditions. The formation mechanism of the nanorods and their impact on the specific capacitance were discussed in detail.

871 citations

Journal ArticleDOI
TL;DR: In this article, the phase transformation from dendritic α-Fe2O3 to Fe3O4, Fe by partial and full reduction, and Fe 2O3 by reduction−oxidation process.
Abstract: Iron-based microstructured or nanostructured materials, including Fe, γ-Fe2O3, and Fe3O4, are highly desirable for magnetic applications because of their high magnetization and a wide range of magnetic anisotropy. An important application of these materials is use as an electromagnetic wave absorber to absorb radar waves in the centimeter wave (2−18 GHz). Dendrite-like microstructures were achieved with the phase transformation from dendritic α-Fe2O3 to Fe3O4, Fe by partial and full reduction, and γ-Fe2O3 by a reduction−oxidation process, while still preserving the dendritic morphology. The investigation of the magnetic properties and microwave absorbability reveals that the three hierarchical microstructures are typical ferromagnets and exhibit excellent microwave absorbability. In addition, this also confirms that the microwave absorption properties are ascribed to the dielectric loss for Fe and the combination of dielectric loss and magnetic loss for Fe3O4 and γ-Fe2O3.

866 citations


Cited by
More filters
01 May 1993
TL;DR: Comparing the results to the fastest reported vectorized Cray Y-MP and C90 algorithm shows that the current generation of parallel machines is competitive with conventional vector supercomputers even for small problems.
Abstract: Three parallel algorithms for classical molecular dynamics are presented. The first assigns each processor a fixed subset of atoms; the second assigns each a fixed subset of inter-atomic forces to compute; the third assigns each a fixed spatial region. The algorithms are suitable for molecular dynamics models which can be difficult to parallelize efficiently—those with short-range forces where the neighbors of each atom change rapidly. They can be implemented on any distributed-memory parallel machine which allows for message-passing of data between independently executing processors. The algorithms are tested on a standard Lennard-Jones benchmark problem for system sizes ranging from 500 to 100,000,000 atoms on several parallel supercomputers--the nCUBE 2, Intel iPSC/860 and Paragon, and Cray T3D. Comparing the results to the fastest reported vectorized Cray Y-MP and C90 algorithm shows that the current generation of parallel machines is competitive with conventional vector supercomputers even for small problems. For large problems, the spatial algorithm achieves parallel efficiencies of 90% and a 1840-node Intel Paragon performs up to 165 faster than a single Cray C9O processor. Trade-offs between the three algorithms and guidelines for adapting them to more complex molecular dynamics simulations are also discussed.

29,323 citations

Journal ArticleDOI
TL;DR: This work has shown that combination of pseudo-capacitive nanomaterials, including oxides, nitrides and polymers, with the latest generation of nanostructured lithium electrodes has brought the energy density of electrochemical capacitors closer to that of batteries.
Abstract: Electrochemical capacitors, also called supercapacitors, store energy using either ion adsorption (electrochemical double layer capacitors) or fast surface redox reactions (pseudo-capacitors). They can complement or replace batteries in electrical energy storage and harvesting applications, when high power delivery or uptake is needed. A notable improvement in performance has been achieved through recent advances in understanding charge storage mechanisms and the development of advanced nanostructured materials. The discovery that ion desolvation occurs in pores smaller than the solvated ions has led to higher capacitance for electrochemical double layer capacitors using carbon electrodes with subnanometre pores, and opened the door to designing high-energy density devices using a variety of electrolytes. Combination of pseudo-capacitive nanomaterials, including oxides, nitrides and polymers, with the latest generation of nanostructured lithium electrodes has brought the energy density of electrochemical capacitors closer to that of batteries. The use of carbon nanotubes has further advanced micro-electrochemical capacitors, enabling flexible and adaptable devices to be made. Mathematical modelling and simulation will be the key to success in designing tomorrow's high-energy and high-power devices.

14,213 citations

Journal ArticleDOI
10 Mar 1970

8,159 citations

Journal ArticleDOI
TL;DR: Two important future research directions are indicated and summarized, based on results published in the literature: the development of composite and nanostructured ES materials to overcome the major challenge posed by the low energy density.
Abstract: In this critical review, metal oxides-based materials for electrochemical supercapacitor (ES) electrodes are reviewed in detail together with a brief review of carbon materials and conducting polymers. Their advantages, disadvantages, and performance in ES electrodes are discussed through extensive analysis of the literature, and new trends in material development are also reviewed. Two important future research directions are indicated and summarized, based on results published in the literature: the development of composite and nanostructured ES materials to overcome the major challenge posed by the low energy density of ES (476 references).

7,642 citations

Journal ArticleDOI
TL;DR: In this article, a review of the key technological developments and scientific challenges for a broad range of Li-ion battery electrodes is presented, and the potential/capacity plots are used to compare many families of suitable materials.

5,057 citations