D
David Sinton
Researcher at University of Toronto
Publications - 366
Citations - 25965
David Sinton is an academic researcher from University of Toronto. The author has contributed to research in topics: Catalysis & Chemistry. The author has an hindex of 69, co-authored 324 publications receiving 16824 citations. Previous affiliations of David Sinton include University of Victoria & Victoria University, Australia.
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Journal ArticleDOI
CO2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Cao-Thang Dinh,Thomas Burdyny,Golam Kibria,Ali Seifitokaldani,Christine M. Gabardo,F. Pelayo García de Arquer,Amirreza Kiani,Jonathan P. Edwards,Phil De Luna,Oleksandr S. Bushuyev,Chengqin Zou,Chengqin Zou,Rafael Quintero-Bermudez,Yuanjie Pang,David Sinton,Edward H. Sargent +15 more
TL;DR: A copper electrocatalyst at an abrupt reaction interface in an alkaline electrolyte reduces CO2 to ethylene with 70% faradaic efficiency at a potential of −0.55 volts versus a reversible hydrogen electrode (RHE).
Journal ArticleDOI
Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Min Liu,Yuanjie Pang,Bo Zhang,Bo Zhang,Phil De Luna,Oleksandr Voznyy,Jixian Xu,Xueli Zheng,Xueli Zheng,Cao-Thang Dinh,Fengjia Fan,Changhong Cao,F. Pelayo García de Arquer,Tina Saberi Safaei,Adam Mepham,Anna Klinkova,Eugenia Kumacheva,Tobin Filleter,David Sinton,Shana O. Kelley,Edward H. Sargent +20 more
TL;DR: It is reported that nanostructured electrodes produce, at low applied overpotentials, local high electric fields that concentrate electrolyte cations, which leads to a high local concentration of CO2 close to the active CO2 reduction reaction surface, which surpasses by an order of magnitude the performance of the best gold nanorods, nanoparticles and oxide-derived noble metal catalysts.
Journal ArticleDOI
CO2 electrolysis to multicarbon products at activities greater than 1 A cm−2
F. Pelayo García de Arquer,Cao-Thang Dinh,Adnan Ozden,Joshua Wicks,Christopher McCallum,Ahmad R. Kirmani,Dae-Hyun Nam,Christine M. Gabardo,Ali Seifitokaldani,Xue Wang,Yuguang C. Li,Fengwang Li,Jonathan P. Edwards,Lee J. Richter,Steven J. Thorpe,David Sinton,Edward H. Sargent +16 more
TL;DR: A catalyst:ionomer bulk heterojunction (CIBH) architecture that decouples gas, ion, and electron transport and achieves CO2 electroreduction on copper in 7 M potassium hydroxide electrolyte with an ethylene partial current density at 45% cathodic energy efficiency.
Journal ArticleDOI
Dopant-induced electron localization drives CO 2 reduction to C 2 hydrocarbons
Yansong Zhou,Yansong Zhou,Fanglin Che,Min Liu,Min Liu,Chengqin Zou,Zhiqin Liang,Phil De Luna,Haifeng Yuan,Haifeng Yuan,Jun Li,Zhiqiang Wang,Haipeng Xie,Hongmei Li,Peining Chen,Eva Bladt,Rafael Quintero-Bermudez,Tsun-Kong Sham,Sara Bals,Johan Hofkens,David Sinton,Gang Chen,Edward H. Sargent +22 more
TL;DR: Simulations show that the ability to tune the average oxidation state of copper enables control over CO adsorption and dimerization, and makes it possible to implement a preference for the electrosynthesis of C2 products.
Journal ArticleDOI
Electrochemical CO2 Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design.
Golam Kibria,Jonathan P. Edwards,Christine M. Gabardo,Cao-Thang Dinh,Ali Seifitokaldani,David Sinton,Edward H. Sargent +6 more
TL;DR: A techno-economic analysis is presented with the goal of identifying maximally profitable products and the performance targets that must be met to ensure economic viability-metrics that include current density, Faradaic efficiency, energy efficiency, and stability.