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Resolving surface chemical states in XPS analysis of first row transition metals, oxides and hydroxides: Sc, Ti, V, Cu and Zn

Microstructures and properties of high-entropy alloys

羟氨苄青霉素引起大疱性类天疱疮样疹

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Water stability and adsorption in metal-organic frameworks.

ion from a primary OH group of glyc-erol. 223,231 A similar mechanism was proposed manyyears ago for alcohol oxidation on Pt/C, involving asecond step, the transfer of a hydride ion to the Ptsurface (Scheme 11). 8,87,237 We consider it more feasible that the rate-deter-mining step is the cleavage of the C-H bond at theR-carbon atom. A similar mechanism is now generallyaccepted for Au electrodes (Scheme 12). 238 Despite thestructural differences between Au nanoparticles andan extended Au electrode surface, there are alsosimilarities, such as the critical role of aqueousalkaline medium and the absence of deactivation dueto decomposition products (CO and C x H y frag-ments). 239,240 An important question is the nature of active siteson Au nanoparticles. Electrooxidation of ethanol onAu nanoparticles supported on glassy carbon re-quired the partial coverage of Au surface by oxides. 241 Another analogy might be the model proposed for COoxidation. 219,242,243 According to this suggestion, theactive site consists of an ensemble of metallic Auatoms and a cationic Au

Oxidation of Alcohols with Molecular Oxygen on Solid Catalysts

Determination of the V2p XPS binding energies for different vanadium oxidation states (V5+ to V0+)

Biaxial alignment in sputter deposited thin films

Simulation of the Sputtering Process.- Electron Emission from Surfaces Induced by Slow Ions and Atoms.- Modeling of the Magnetron Discharge.- Modelling of Reactive Sputtering Processes.- Depositing Aluminium Oxide: A Case Study of Reactive Magnetron Sputtering.- Transport of Sputtered Particles Through the Gas Phase.- Energy Deposition at the Substrate in a Magnetron Sputtering System.- Process Diagnostics.- Optical Plasma Diagnostics During Reactive Magnetron Sputtering.- Reactive Magnetron Sputtering of Indium Tin Oxide Thin Films: The Cross-Corner and Cross-Magnetron Effect.- Reactively Sputter-Deposited Solid Electrolytes and Their Applications.- Reactive SputteredWide-Bandgap p-Type Semiconducting Spinel AB2O4 and Delafossite ABO2 Thin Films for "Transparent Electronics".- Oxide-Based Electrochromic Materials and Devices Prepared by Magnetron Sputtering.- Atomic Assembly of Magnetoresistive Multilayers.

Reactive Sputter Deposition

The discharge voltage was measured for 15 different metallic target materials at constant current before and after plasma oxidation in order to understand its behavior during reactive magnetron sputtering. Plasma oxidation of the target surface was achieved by sputtering the target in pure oxygen. The discharge voltage measured in pure argon is characteristic for each kind of metallic target and is related to the ion induced secondary electron emission (ISEE) coefficient of the target material. Based on this relation a value for the ISEE coefficient of the oxidized target surface can be calculated. Two distinct groups can be discerned: for one group the ISEE coefficient of the oxidized target surface is larger than the ISEE coefficient of the metal, while the opposite behavior is noticed for the second group. This difference seems to find its origin in the reduction behavior of the oxides under ion bombardment, since the ISEE coefficient of the oxide can be related to the simulated degree of reduction of ...

Understanding the discharge voltage behavior during reactive sputtering of oxides

Rare-earth coordination polymers or lanthanide-organic frameworks with hitherto unreported crystal structures have been obtained on the basis of the "light" lanthanides Pr, Nd, Sm, and Eu in combination with terephthalic acid and using a slightly altered literature synthesis procedure. Rietveld refinement has shown that powder XRD patterns of such compounds are largely dominated by the positions of the heavy elements, pointing to isostructural networks for all four terephthalate-based materials. An in-depth luminescence study has been performed on the reported MOFs, showing rare praseodymium and samarium emission in the visible spectrum, aside from the strong europium luminescence and the near-infrared emission from both a terephthalate and 2,5-pyridinedicarboxylate based neodymium-MOF.

Diederik Depla

Papers

Determination of the V2p XPS binding energies for different vanadium oxidation states (V5+ to V0+)

Biaxial alignment in sputter deposited thin films

Reactive Sputter Deposition

Understanding the discharge voltage behavior during reactive sputtering of oxides

Synthesis, crystal structures, and luminescence properties of carboxylate based rare-earth coordination polymers.