Author
R. von Helmolt
Other affiliations: University of Augsburg
Bio: R. von Helmolt is an academic researcher from Siemens. The author has contributed to research in topics: Magnetoresistance & Colossal magnetoresistance. The author has an hindex of 11, co-authored 15 publications receiving 4015 citations. Previous affiliations of R. von Helmolt include University of Augsburg.
Papers
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TL;DR: The samples show a drop in the resistivity at the magnetic transition, and the existence of magnetic polarons seems to dominate the electric transport in this region.
Abstract: At room temperature a large magnetoresistance, \ensuremath{\Delta}R/R(H=0), of 60% has been observed in thin magnetic films of perovskitelike La-Ba-Mn-O. The films were grown epitaxially on ${\mathrm{SrTiO}}_{3}$ substrates by off-axis laser deposition. In the as-deposited state, the Curie temperature and the saturation magnetization were considerably lower compared to bulk samples, but were increased by a subsequent heat treatment. The samples show a drop in the resistivity at the magnetic transition, and the existence of magnetic polarons seems to dominate the electric transport in this region.
3,424 citations
TL;DR: In this paper, the effects of magnetic field and pressure on the unusual spontaneous behavior of a compound with anomalous volume thermal expansion have been thoroughly investigated, including the formation of magnetic polarons.
Abstract: The effects of magnetic field and pressure on the unusual spontaneous behavior of ${\mathrm{La}}_{2/3}$${\mathrm{Ca}}_{1/3}$${\mathrm{MnO}}_{3}$ have been thoroughly investigated. Resistivity and volume thermal expansion, both under magnetic field and pressure, ac susceptibility under pressure, magnetostriction, magnetoresistance, and neutron diffraction measurements, have allowed us to determine the relevant underlying mechanisms in this system. Above ${\mathit{T}}_{\mathit{c}}$ the neutron measurements reveal short-range ferromagnetic correlations and the anomalous volume thermal expansion indicates that local distortions are present. Both experiments support the formation of magnetic polarons above ${\mathit{T}}_{\mathit{c}}$. At ${\mathit{T}}_{\mathit{c}}$ the compound undergoes a paramagnetic-ferromagnetic transition accompanied by an insulator-metal-like transition with anomalies in the electrical and volume properties. Above ${\mathit{T}}_{\mathit{c}}$ the magnetic field and the pressure favor electrical conduction by enhancing the double-exchange interaction. Below ${\mathit{T}}_{\mathit{c}}$ the metallic state is favored by the magnetic field and the pressure in a different way. \textcopyright{} 1996 The American Physical Society.
213 citations
TL;DR: The magnetoresistance (MR) of the as-quenched ribbons is only of the order of 1.5% as discussed by the authors, but it increases dramatically with the controlled nucleation and growth of Co precipitates from the supersaturated Cu matrix.
Abstract: Cu1−xCox alloys with x=0.1 and x=0.2 have been prepared by conventional melt spinning. The rapid solidification process results in an extended solubility of Co in Cu although some Co precipitates already during quenching. In the as‐quenched ribbons, the magnetoresistance (MR) is only of the order of 1.5%. It increases dramatically with the controlled nucleation and growth of Co precipitates from the supersaturated Cu matrix. The highest MR of 11% at 300 K occurs for Cu90Co10 after an aging at about 440 °C when the Co clusters are superparamagnetic. Saturation is possible only after a higher annealing or at lower measuring temperatures. For the optimally annealed samples the MR increases to 36% at 30 K.
178 citations
TL;DR: In this article, a large intrinsic magnetoresistance has been found near the ferromagnetic transition of metallic manganese oxides with perovskite-type crystal structure, and the magnetic and transport properties were measured on bulk and thin-film La1−xAxMnO3+δ with A=Ca,Sr,Ba.
Abstract: A large intrinsic magnetoresistance has been found near the ferromagnetic transition of metallic manganese oxides with perovskite‐type crystal structure. The magnetic and transport properties were measured on bulk and thin‐film La1−xAxMnO3+δ with A=Ca,Sr,Ba. Assuming the double‐exchange model proposed by Zener [Phys. Rev. 81, 440 (1951); 82, 403 (1951)], the strong dependence of the transport properties on the magnetic field and also on the chemical composition is attributed to the mixed Mn3+/Mn4+ valence.
102 citations
TL;DR: In this paper, the magnetoresistance of La2/3Ca1/3MnO3+δ magnetic thin films was investigated and a remarkable hysteresis and a relaxation behavior of the resistance was observed.
Abstract: We investigated the magnetoresistance of La2/3Ca1/3MnO3+δ magnetic thin films. Under certain conditions, the magnetoresistance curves show a remarkable hysteresis and the resistance becomes dependent on the magnetic history. A relaxation behavior of the resistance has also been observed. Hysteresis and relaxation of the resistance are very similar to the phenomena of magnetoviscosity of the magnetic moment in spin glasses and the magnetic aftereffect in hard magnets.
52 citations
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TL;DR: The dynamical mean field theory of strongly correlated electron systems is based on a mapping of lattice models onto quantum impurity models subject to a self-consistency condition.
Abstract: We review the dynamical mean-field theory of strongly correlated electron systems which is based on a mapping of lattice models onto quantum impurity models subject to a self-consistency condition. This mapping is exact for models of correlated electrons in the limit of large lattice coordination (or infinite spatial dimensions). It extends the standard mean-field construction from classical statistical mechanics to quantum problems. We discuss the physical ideas underlying this theory and its mathematical derivation. Various analytic and numerical techniques that have been developed recently in order to analyze and solve the dynamical mean-field equations are reviewed and compared to each other. The method can be used for the determination of phase diagrams (by comparing the stability of various types of long-range order), and the calculation of thermodynamic properties, one-particle Green's functions, and response functions. We review in detail the recent progress in understanding the Hubbard model and the Mott metal-insulator transition within this approach, including some comparison to experiments on three-dimensional transition-metal oxides. We present an overview of the rapidly developing field of applications of this method to other systems. The present limitations of the approach, and possible extensions of the formalism are finally discussed. Computer programs for the numerical implementation of this method are also provided with this article.
5,230 citations
TL;DR: A negative isotropic magnetoresistance effect has been observed in thin oxide films of perovskite-like La0.67Ca0.33MnOx, which could be useful for various magnetic and electric device applications if the observed effects of material processing are optimized.
Abstract: A negative isotropic magnetoresistance effect more than three orders of magnitude larger than the typical giant magnetoresistance of some superlattice films has been observed in thin oxide films of perovskite-like La0.67Ca0.33MnOx. Epitaxial films that are grown on LaAIO3 substrates by laser ablation and suitably heat treated exhibit magnetoresistance values as high as 127,000 percent near 77 kelvin and ∼1300 percent near room temperature. Such a phenomenon could be useful for various magnetic and electric device applications if the observed effects of material processing are optimized. Possible mechanisms for the observed effect are discussed.
4,079 citations
TL;DR: In this paper, a large variety of experiments reviewed in detail here contain results compatible with the theoretical predictions, including phase diagrams of manganite models, the stabilization of the charge/orbital/spin ordered half-doped correlated electronics (CE)-states, the importance of the naively small Heisenberg coupling among localized spins, the setup of accurate mean-field approximations, and the existence of a new temperature scale T∗ where clusters start forming above the Curie temperature, the presence of stripes in the system, and many others.
2,927 citations
01 Sep 1997
TL;DR: In this paper, the authors review recent experimental work falling under the broad classification of colossal magnetoresistance (CMR), which is magnetoreduction associated with a ferromagnetic-toparamagnetic phase transition.
Abstract: We review recent experimental work falling under the broad classification of colossal magnetoresistance (CMR), which is magnetoresistance associated with a ferromagnetic-toparamagnetic phase transition. The prototypical CMR compound is derived from the parent compound, perovskite LaMnO 3. When hole doped at a concentration of 20–40% holes/Mn ion, for instance by Ca or Sr substitution for La, the material displays a transition from a high-temperature paramagnetic insulator to a low-temperature ferromagnetic metal. Near the phase transition temperature, which can exceed room temperature in some compositions, large magnetoresistance is observed and its possible application in magnetic recording has revived interest in these materials. In addition, unusual magneto-elastic effects and charge ordering have focused attention on strong electron–phonon coupling. This coupling, which is a type of dynamic extended-system version of the Jahn–Teller effect, in conjunction with the double-exchange interaction, is also viewed as essential for a microscopic description of CMR in the manganite perovskites. Large magnetoresistance is also seen in other systems, namely Tl 2Mn2O7 and some Cr chalcogenide spinels, compounds which differ greatly from the manganite perovskites. We describe the relevant points of contrast between the various CMR materials.
1,336 citations
TL;DR: In this paper, the phase separation phenomenon on various time-scales (from static to dynamic) and the enhanced phase fluctuation with anomalous reduction in the transition temperatures of the competing phases (and hence in the bicritical-point temperature).
Abstract: Colossal magnetoresistance (CMR) phenomena are observed in the perovskite-type hole-doped manganites in which the double-exchange ferromagnetic metal phase and the charge–orbital ordered antiferromagnetic phase compete with each other. The quenched disorder arising from the inherent chemical randomness or the intentional impurity doping may cause major modifications in the electronic phase diagram as well as in the magnetoelectronic properties near the bicritical point that is formed by such a competition of the two phases. One is the phase separation phenomenon on various time-scales (from static to dynamic) and on various length-scales (from glass-like nano to grain-like micron). The other is the enhanced phase fluctuation with anomalous reduction in the transition temperatures of the competing phases (and hence in the bicritical-point temperature). The highly effective suppression of such a phase fluctuation by an external magnetic field is assigned here to the most essential ingredient of the CMR physics. Such profound and dramatic features as appearing in the bicritical region are extensively discussed in this paper with ample examples of the material systems specially designed for this purpose. The unconventional phase-controls over the competing phases in terms of magnetic/electric fields and photo-excitations are also exemplified.
1,166 citations