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Stefano Carretta

Bio: Stefano Carretta is an academic researcher from University of Parma. The author has contributed to research in topics: Qubit & Inelastic neutron scattering. The author has an hindex of 37, co-authored 172 publications receiving 4757 citations.


Papers
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TL;DR: Antiferromagnetic Cr7Ni rings can be chemically linked to each other and that the coupling between their spins can be tuned by choosing the linker, and calculations are presented that demonstrate how realistic microwave pulse sequences could be used to generate maximally entangled states in such molecules.
Abstract: The ability to assemble weakly interacting subsystems is a prerequisite for implementing quantum information processing and generating controlled entanglement. In recent years, molecular nanomagnets have been proposed as suitable candidates for qubit encoding and manipulation. In particular, antiferromagnetic Cr7Ni rings behave as effective spin-1/2 systems at low temperature and show long decoherence times. Here, we show that these rings can be chemically linked to each other and that the coupling between their spins can be tuned by choosing the linker. We also present calculations that demonstrate how realistic microwave pulse sequences could be used to generate maximally entangled states in such molecules. The ability to assemble weakly-interacting subsystems is a prerequisite for implementing quantum-information processing. In recent years, molecular nanomagnets have been proposed as suitable candidates for qubit encoding and manipulation, with antiferromagnetic Cr7Ni rings of particular interest. It has now been shown that such rings can be chemically linked to each other and the coupling between their spins tuned through the choice of chemical linker.

342 citations

Journal ArticleDOI
TL;DR: The energy spectrum and the suppression of the leakage-inducing S mixing render the Cr7Ni molecule a suitable candidate for the qubit implementation, as further substantiated by the quantum-gate simulations.
Abstract: The substitution of one metal ion in a Cr-based molecular ring with dominant antiferromagnetic couplings allows the engineering of its level structure and ground-state degeneracy. Here we characterize a Cr7Ni molecular ring by means of low-temperature specific-heat and torque-magnetometry measurements, thus determining the microscopic parameters of the corresponding spin Hamiltonian. The energy spectrum and the suppression of the leakage-inducing S mixing render the Cr7Ni molecule a suitable candidate for the qubit implementation, as further substantiated by our quantum-gate simulations.

248 citations

Journal ArticleDOI
TL;DR: It is shown that through supramolecular chemistry a single simple module, molecular {Cr7Ni} rings, can be assembled into structures suitable for either the CNOT or gate by choice of linker, and these structures are characterized by electron spin resonance spectroscopy.
Abstract: The physical implementation of quantum information processing relies on individual modules-qubits-and operations that modify such modules either individually or in groups-quantum gates. Two examples of gates that entangle pairs of qubits are the controlled NOT-gate (CNOT) gate, which flips the state of one qubit depending on the state of another, and the gate that brings a two-qubit product state into a superposition involving partially swapping the qubit states. Here we show that through supramolecular chemistry a single simple module, molecular {Cr7Ni} rings, which act as the qubits, can be assembled into structures suitable for either the CNOT or gate by choice of linker, and we characterize these structures by electron spin resonance spectroscopy. We introduce two schemes for implementing such gates with these supramolecular assemblies and perform detailed simulations, based on the measured parameters including decoherence, to demonstrate how the gates would operate.

194 citations


Cited by
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Journal ArticleDOI
TL;DR: This work reviews the first progress in the resulting field, molecular spintronics, which will enable the manipulation of spin and charges in electronic devices containing one or more molecules, and discusses the advantages over more conventional materials, and the potential applications in information storage and processing.
Abstract: A revolution in electronics is in view, with the contemporary evolution of the two novel disciplines of spintronics and molecular electronics. A fundamental link between these two fields can be established using molecular magnetic materials and, in particular, single-molecule magnets. Here, we review the first progress in the resulting field, molecular spintronics, which will enable the manipulation of spin and charges in electronic devices containing one or more molecules. We discuss the advantages over more conventional materials, and the potential applications in information storage and processing. We also outline current challenges in the field, and propose convenient schemes to overcome them.

2,694 citations

Journal ArticleDOI
TL;DR: The main theoretical and experimental aspects of quantum simulation have been discussed in this article, and some of the challenges and promises of this fast-growing field have also been highlighted in this review.
Abstract: Simulating quantum mechanics is known to be a difficult computational problem, especially when dealing with large systems However, this difficulty may be overcome by using some controllable quantum system to study another less controllable or accessible quantum system, ie, quantum simulation Quantum simulation promises to have applications in the study of many problems in, eg, condensed-matter physics, high-energy physics, atomic physics, quantum chemistry and cosmology Quantum simulation could be implemented using quantum computers, but also with simpler, analog devices that would require less control, and therefore, would be easier to construct A number of quantum systems such as neutral atoms, ions, polar molecules, electrons in semiconductors, superconducting circuits, nuclear spins and photons have been proposed as quantum simulators This review outlines the main theoretical and experimental aspects of quantum simulation and emphasizes some of the challenges and promises of this fast-growing field

1,941 citations

Book
01 Jan 2010

1,870 citations