Stephen E. Schwartz

Bio: Stephen E. Schwartz is an academic researcher from Brookhaven National Laboratory. The author has contributed to research in topics: Aerosol & Radiative forcing. The author has an hindex of 55, co-authored 131 publications receiving 13732 citations.

Climate Forcing by Anthropogenic Aerosols

Abstract: Although long considered to be of marginal importance to global climate change, tropospheric aerosol contributes substantially to radiative forcing, and anthropogenic sulfate aerosol in particular has imposed a major perturbation to this forcing. Both the direct scattering of shortwavelength solar radiation and the modification of the shortwave reflective properties of clouds by sulfate aerosol particles increase planetary albedo, thereby exerting a cooling influence on the planet. Current climate forcing due to anthropogenic sulfate is estimated to be –1 to –2 watts per square meter, globally averaged. This perturbation is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign. Thus, the aerosol forcing has likely offset global greenhouse warming to a substantial degree. However, differences in geographical and seasonal distributions of these forcings preclude any simple compensation. Aerosol effects must be taken into account in evaluating anthropogenic influences on past, current, and projected future climate and in formulating policy regarding controls on emission of greenhouse gases and sulfur dioxide. Resolution of such policy issues requires integrated research on the magnitude and geographical distribution of aerosol climate forcing and on the controlling chemical and physical processes.

The Atmospheric Radiation Measurement (ARM) Program: Programmatic Background and Design of the Cloud and Radiation Test Bed

Abstract: The Atmospheric Radiation Measurement (ARM) Program, supported by the U.S. Department of Energy, is a major new program of atmospheric measurement and modeling. The program is intended to improve the understanding of processes that affect atmospheric radiation and the description of these processes in climate models. An accurate description of atmospheric radiation and its interaction with clouds and cloud processes is necessary to improve the performance of and confidence in models used to study and predict climate change. The ARM Program will employ five (this paper was prepared prior to a decision to limit the number of primary measurement sites to three) highly instrumented primary measurement sites for up to 10 years at land and ocean locations, from the Tropics to the Arctic, and will conduct observations for shorter periods at additional sites and in specialized campaigns. Quantities to be measured at these sites include longwave and shortwave radiation, the spatial and temporal distributi...

Sea Salt Aerosol Production: Mechanisms, Methods, Measurements, and Models - A Critical Review

Abstract: Sea salt aerosol (SSA) exerts a major influence over a broad reach of geophysics. It is important to the physics and chemistry of the marine atmosphere and to marine geochemistry and biogeochemistry generally. It affects visibility, remote sensing, atmospheric chemistry, and air quality. Sea salt aerosol particles interact with other atmospheric gaseous and aerosol constituents by acting as sinks for condensable gases and suppressing new particle formation, thus influencing the size distribution of these other aerosols and more broadly influencing the geochemical cycles of substances with which they interact. As the key aerosol constituent over much of Earth's surface at present, and all the more so in pre-industrial times, SSA is central to description of Earth's aerosol burden.

Production flux of sea spray aerosol

Abstract: Knowledge of the size- and composition-dependent production flux of primary sea spray aerosol (SSA) particles and its dependence on environmental variables is required for modeling cloud microphysical properties and aerosol radiative influences, interpreting measurements of particulate matter in coastal areas and its relation to air quality, and evaluating rates of uptake and reactions of gases in sea spray drops. This review examines recent research pertinent to SSA production flux, which deals mainly with production of particles with r 80 (equilibrium radius at 80% relative humidity) less than 1 m and as small as 0.01 m. Production of sea spray particles and its dependence on controlling factors has been investigated in laboratory studies that have examined the dependences on water temperature, salinity, and the presence of organics and in field measurements with micrometeorological techniques that use newly developed fast optical particle sizers. Extensive measurements show that water-insoluble organic matter contributes substantially to the composition of SSA particles with r80 < 0.25 m and, in locations with high biological activity, can be the dominant constituent. Order-of-magnitude variation remains in estimates of the size-dependent production flux per white area, the quantity central to formulations of the production flux based on the whitecap method. This variation indicates that the production flux may depend on quantities such as the volume flux of air bubbles to the surface that are not accounted for in current models. Variation in estimates of the whitecap fraction as a function of wind speed contributes additional, comparable uncertainty to production flux estimates. © 2011 by the American Geophysical Union.

Mass-Transport Considerations Pertinent to Aqueous Phase Reactions of Gases in Liquid-Water Clouds

Abstract: Reactions of gases in liquid-water clouds are potentially important in the transformation of atmospheric pollutants affecting their transport in the atmosphere and subsequent removal and deposition to the surface. Such processes consist of the following sequence of steps: Mass-transport of the reagent gas or gases to the air-water interface; transfer across the interface and establishment of solubility equilibria locally at the interface; mass-transport of the dissolved gas or gases within the aqueous phase; aqueous-phase chemical reaction(s); mass-transport of reaction product(s) and possible subsequent evolution into the gas-phase. Description of the rate of the overall process requires identification of the rate-limiting step (or steps) and evaluation of the rate of such step(s). Identification of the rate-limiting step may be achieved by evaluation and comparison of the characteristic times pertinent to the several processes and may be readily carried out by methods outlined herein, for known or assumed reagent concentrations, drop size, and fundamental constants as follows: gas- and aqueous-phase diffusion coefficients; Henry’s law coefficient and other pertinent equilibrium constants; interfacial mass-transfer accommodation coefficient; aqueous-phase reaction rate constants(s). A graphical method is described whereby it may be ascertained whether a given reaction is controlled solely by reagent solubility and intrinsic chemical kinetic or is mass-transport limited by one or another of the above processes. In the absence of mass-transport limitation, reaction rates may be evaluated uniformly for the entire liquid-water content of the cloud using equilibrium reagent concentrations. In contrast, where appreciable mass-transport limitation is indicated, evaluation of the overall rate requires knowledge of and integration over the drop-size distribution characterizing the cloud.

疟原虫var基因转换速率变化导致抗原变异[英]／Paul H, Robert P, Christodoulou Z, et al//Proc Natl Acad Sci U S A

Abstract: 抗原变异可使得多种致病微生物易于逃避宿主免疫应答。表达在感染红细胞表面的恶性疟原虫红细胞表面蛋白1（PfPMP1）与感染红细胞、内皮细胞、树突状细胞以及胎盘的单个或多个受体作用，在黏附及免疫逃避中起关键的作用。每个单倍体基因组var基因家族编码约60种成员，通过启动转录不同的var基因变异体为抗原变异提供了分子基础。

Climate change 2001: the scientific basis

Abstract: Summary for policymakers Technical summary 1. The climate system - an overview 2. Observed climate variability and change 3. The carbon cycle and atmospheric CO2 4. Atmospheric chemistry and greenhouse gases 5. Aerosols, their direct and indirect effects 6. Radiative forcing of climate change 7. Physical climate processes and feedbacks 8. Model evaluation 9. Projections of future climate change 10. Regional climate simulation - evaluation and projections 11. Changes in sea level 12. Detection of climate change and attribution of causes 13. Climate scenario development 14. Advancing our understanding Glossary Index Appendix.

Contribution of Working Group II to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change

Abstract: Drafting Authors: Neil Adger, Pramod Aggarwal, Shardul Agrawala, Joseph Alcamo, Abdelkader Allali, Oleg Anisimov, Nigel Arnell, Michel Boko, Osvaldo Canziani, Timothy Carter, Gino Casassa, Ulisses Confalonieri, Rex Victor Cruz, Edmundo de Alba Alcaraz, William Easterling, Christopher Field, Andreas Fischlin, Blair Fitzharris, Carlos Gay García, Clair Hanson, Hideo Harasawa, Kevin Hennessy, Saleemul Huq, Roger Jones, Lucka Kajfež Bogataj, David Karoly, Richard Klein, Zbigniew Kundzewicz, Murari Lal, Rodel Lasco, Geoff Love, Xianfu Lu, Graciela Magrín, Luis José Mata, Roger McLean, Bettina Menne, Guy Midgley, Nobuo Mimura, Monirul Qader Mirza, José Moreno, Linda Mortsch, Isabelle Niang-Diop, Robert Nicholls, Béla Nováky, Leonard Nurse, Anthony Nyong, Michael Oppenheimer, Jean Palutikof, Martin Parry, Anand Patwardhan, Patricia Romero Lankao, Cynthia Rosenzweig, Stephen Schneider, Serguei Semenov, Joel Smith, John Stone, Jean-Pascal van Ypersele, David Vaughan, Coleen Vogel, Thomas Wilbanks, Poh Poh Wong, Shaohong Wu, Gary Yohe

Radiative transfer for inhomogeneous atmospheres: RRTM, a validated correlated-k model for the longwave

Abstract: A rapid and accurate radiative transfer model (RRTM) for climate applications has been developed and the results extensively evaluated. The current version of RRTM calculates fluxes and cooling rates for the longwave spectral region (10–3000 cm−1) for an arbitrary clear atmosphere. The molecular species treated in the model are water vapor, carbon dioxide, ozone, methane, nitrous oxide, and the common halocarbons. The radiative transfer in RRTM is performed using the correlated-k method: the k distributions are attained directly from the LBLRTM line-by-line model, which connects the absorption coefficients used by RRTM to high-resolution radiance validations done with observations. Refined methods have been developed for treating bands containing gases with overlapping absorption, for the determination of values of the Planck function appropriate for use in the correlated-k approach, and for the inclusion of minor absorbing species in a band. The flux and cooling rate results of RRTM are linked to measurement through the use of LBLRTM, which has been substantially validated with observations. Validations of RRTM using LBLRTM have been performed for the midlatitude summer, tropical, midlatitude winter, subarctic winter, and four atmospheres from the Spectral Radiance Experiment campaign. On the basis of these validations the longwave accuracy of RRTM for any atmosphere is as follows: 0.6 W m−2 (relative to LBLRTM) for net flux in each band at all altitudes, with a total (10–3000 cm−1) error of less than 1.0 W m−2 at any altitude; 0.07 K d−1 for total cooling rate error in the troposphere and lower stratosphere, and 0.75 K d−1 in the upper stratosphere and above. Other comparisons have been performed on RRTM using LBLRTM to gauge its sensitivity to changes in the abundance of specific species, including the halocarbons and carbon dioxide. The radiative forcing due to doubling the concentration of carbon dioxide is attained with an accuracy of 0.24 W m−2, an error of less than 5%. The speed of execution of RRTM compares favorably with that of other rapid radiation models, indicating that the model is suitable for use in general circulation models.