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Tamar Seideman

Bio: Tamar Seideman is an academic researcher from Northwestern University. The author has contributed to research in topics: Plasmon & Excited state. The author has an hindex of 51, co-authored 286 publications receiving 11566 citations. Previous affiliations of Tamar Seideman include Tel Aviv University & Harvard University.


Papers
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Journal ArticleDOI
TL;DR: In this paper, the theoretical and experimental status of the intense laser alignment (EL alignment) technique is reviewed and a discussion of the physics underlying this technique and a description of methods of observing it in the laboratory is provided.
Abstract: We review the theoretical and experimental status of intense laser alignment---a field at the interface between intense laser physics and chemical dynamics with potential applications ranging from high harmonic generation and nanoscale processing to stereodynamics and control of chemical reactions After placing the intense laser approach in context with other alignment techniques, we proceed with a discussion of the physics underlying this technique and a description of methods of observing it in the laboratory The roles played by the laser frequency, the pulse duration, and the system temperature are illustrated numerically and experimentally Alignment is extended to three-dimensional orientational control, a method of hindering the rotation about all three axes of polyatomic molecules We conclude with a discussion of potential applications of intense laser alignment

1,435 citations

Journal ArticleDOI
TL;DR: The rate of nonlinear ionization is strongly enhanced as a molecule is stretched beyond its equilibrium internuclear separation, reaching a peak rate that is many orders of magnitude greater than that at either small or large distances as discussed by the authors.
Abstract: The rate of nonlinear ionization is strongly enhanced as a molecule is stretched beyond its equilibrium internuclear separation, reaching a peak rate that is many orders of magnitude greater than that at either small or large distances. The enhancement results from nonadiabatic electron localization near the nuclei and its presence is insensitive to the laser frequency and intensity. Most intense-field dissociative ionization experiments are influenced by this effect.

533 citations

Journal ArticleDOI
TL;DR: In this paper, a new method is proposed for the calculation of the microcanonical cumulative reaction probability via flux autocorrelation relations, circumventing the need to compute the state-to-state dynamics.
Abstract: A new method is suggested for the calculation of the microcanonical cumulative reaction probability via flux autocorrelation relations. The Hamiltonian and the flux operators are computed in a discrete variable representation (DVR) and a well‐behaved representation for the Green’s operator, G(E+), is obtained by imposing absorbing boundary conditions (ABC). Applications to a one‐dimensional‐model problem and to the collinear H+H2 reaction show that the DVR‐ABC scheme provides a very efficient method for the direct calculation of the microcanonical probability, circumventing the need to compute the state‐to‐state dynamics. Our results indicate that the cumulative reaction probability can be calculated to a high accuracy using a rather small number of DVR points, confined to the vicinity of the transition state. Only limited information regarding the potential‐energy surface is therefore required, suggesting that this method would be applicable also to higher dimensionality problems, for which the complete potential surface is often unknown.

337 citations

Journal ArticleDOI
TL;DR: In this paper, strong enhancement of the alignment of rotational wave packets after turn-off of the laser pulse, under field-free conditions, was shown. But the results were limited to the case of strong-field-induced wave packets.
Abstract: The revival structure of strong-field-induced rotational wave packets differs qualitatively from revival structures analyzed in the past. One of the consequences of this difference is strong enhancement of the alignment of such wave packets after turn-off of the laser pulse, under field-free conditions.

299 citations

Book ChapterDOI
TL;DR: The theory of intense laser alignment of molecules is reviewed in this article, focusing on aspects that have not been presented in the past, and a survey of recent developments in this rapidly evolving field is presented.
Abstract: We review the theory of intense laser alignment of molecules and present a survey of the many recent developments in this rapidly evolving field. Starting with a qualitative discussion that emphasizes the physical mechanism responsible for laser alignment, we proceed with a detailed exposition of the underlying theory, focusing on aspects that have not been presented in the past. Application of the theory in several pedagogical illustrations is then followed by a review of the recent experimental and theoretical advances in the field. We conclude with a discussion of new directions, future opportunities, and areas where we expect intense laser alignment to play a role in the future. Throughout we emphasize the recent evolution of the method of nonadiabatic alignment from isolated diatomic molecules to complex media.

260 citations


Cited by
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Journal ArticleDOI

[...]

08 Dec 2001-BMJ
TL;DR: There is, I think, something ethereal about i —the square root of minus one, which seems an odd beast at that time—an intruder hovering on the edge of reality.
Abstract: There is, I think, something ethereal about i —the square root of minus one. I remember first hearing about it at school. It seemed an odd beast at that time—an intruder hovering on the edge of reality. Usually familiarity dulls this sense of the bizarre, but in the case of i it was the reverse: over the years the sense of its surreal nature intensified. It seemed that it was impossible to write mathematics that described the real world in …

33,785 citations

28 Jul 2005
TL;DR: PfPMP1)与感染红细胞、树突状组胞以及胎盘的单个或多个受体作用,在黏附及免疫逃避中起关键的作�ly.
Abstract: 抗原变异可使得多种致病微生物易于逃避宿主免疫应答。表达在感染红细胞表面的恶性疟原虫红细胞表面蛋白1(PfPMP1)与感染红细胞、内皮细胞、树突状细胞以及胎盘的单个或多个受体作用,在黏附及免疫逃避中起关键的作用。每个单倍体基因组var基因家族编码约60种成员,通过启动转录不同的var基因变异体为抗原变异提供了分子基础。

18,940 citations

Journal ArticleDOI
21 Oct 2011-Science
TL;DR: In this article, a two-dimensional array of optical resonators with spatially varying phase response and subwavelength separation can imprint phase discontinuities on propagating light as it traverses the interface between two media.
Abstract: Conventional optical components rely on gradual phase shifts accumulated during light propagation to shape light beams. New degrees of freedom are attained by introducing abrupt phase changes over the scale of the wavelength. A two-dimensional array of optical resonators with spatially varying phase response and subwavelength separation can imprint such phase discontinuities on propagating light as it traverses the interface between two media. Anomalous reflection and refraction phenomena are observed in this regime in optically thin arrays of metallic antennas on silicon with a linear phase variation along the interface, which are in excellent agreement with generalized laws derived from Fermat’s principle. Phase discontinuities provide great flexibility in the design of light beams, as illustrated by the generation of optical vortices through use of planar designer metallic interfaces.

6,763 citations

Proceedings Article
14 Jul 1996
TL;DR: The striking signature of Bose condensation was the sudden appearance of a bimodal velocity distribution below the critical temperature of ~2µK.
Abstract: Bose-Einstein condensation (BEC) has been observed in a dilute gas of sodium atoms. A Bose-Einstein condensate consists of a macroscopic population of the ground state of the system, and is a coherent state of matter. In an ideal gas, this phase transition is purely quantum-statistical. The study of BEC in weakly interacting systems which can be controlled and observed with precision holds the promise of revealing new macroscopic quantum phenomena that can be understood from first principles.

3,530 citations

Journal ArticleDOI
Naomi J. Halas1, Surbhi Lal1, Wei-Shun Chang1, Stephan Link1, Peter Nordlander1 

2,702 citations