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Terry Wall

Bio: Terry Wall is an academic researcher from University of Newcastle. The author has contributed to research in topics: Coal & Combustion. The author has an hindex of 58, co-authored 248 publications receiving 12007 citations. Previous affiliations of Terry Wall include Newcastle University & University of Alberta.


Papers
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Journal ArticleDOI
TL;DR: A comprehensive review of CO2 capture in coal-fired combustion plants can be found in this article, where the status of the technology development and assessments providing comparisons with other power generation options, and suggests research needs.

1,450 citations

Journal ArticleDOI
TL;DR: A comprehensive assessment on oxyfuel combustion in a pilot-scale oxyfuel furnace, modifying the design criterion for an oxy retrofit by matching heat transfer, a new 4-grey gas model which accurately predicts emissivity of the gases in oxy-fired furnaces has been developed for furnace modelling, the first measurements of coal reactivity comparisons in air and oxyfuel at laboratory and pilot scale; and predictions of observed delays in flame ignition in oxyfiring as discussed by the authors.
Abstract: Oxyfuel combustion is seen as one of the major options for CO2 capture for future clean coal technologies. The paper provides an overview on research activities and technology development through a fundamental research underpinning the Australia/Japan Oxyfuel Feasibility Project. Studies on oxyfuel combustion on a pilot-scale furnace and a laboratory scale drop tube furnace are presented and compared with computational fluid dynamics (CFD) predictions. The research has made several contributions to current knowledge, including; comprehensive assessment on oxyfuel combustion in a pilot-scale oxyfuel furnace, modifying the design criterion for an oxy retrofit by matching heat transfer, a new 4-grey gas model which accurately predicts emissivity of the gases in oxy-fired furnaces has been developed for furnace modelling, the first measurements of coal reactivity comparisons in air and oxyfuel at laboratory and pilot-scale; and predictions of observed delays in flame ignition in oxy-firing.

760 citations

Journal ArticleDOI
01 Jan 2007
TL;DR: A review of the technologies for coal-based power generation closest to commercial application involving carbon capture is presented in this paper, where the R&D challenges identified for the combustion scientist and engineer are those of design, optimisation and operational aspects of new combustion and gasification plant, controlling the gas quality required by CCS related units and associated emission compliance, and gas separations.
Abstract: A review of the technologies for coal-based power generation closest to commercial application involving carbon capture is presented. Carbon capture and storage (CCS) developments are primarily adaptations of conventional combustion systems, with additional unit operations such as bulk oxygen supply, CO2 capture by sorbents, CO2 compression, and storage. They use pulverized coal combustion in entrained flow—the dominant current technology for coal-based power, or gasification in entrained flow, although similar concepts apply to other solid–gas contacting systems such as fluidized beds. Currently, the technologies have similar generation efficiencies and are associated with efficiency penalties and electricity cost increases due to operations required for carbon capture. The R&D challenges identified for the combustion scientist and engineer, with current understanding being detailed, are those of design, optimisation and operational aspects of new combustion and gasification plant, controlling the gas quality required by CCS related units and associated emission compliance, and gas separations. Fundamental research needs include fuel reactions at pressure, and in O2/CO2 atmospheres, as few studies have been made in this area. Laboratory results interpreted and then included in CFD models of combustion operations are necessary. Also identified, but not detailed, are combustion issues in gas turbines for IGCC and IGCC-CCS. Fundamental studies should be a component of pilot-plant and demonstrations at practical scale being planned. Concepts for new designs of combustion equipment are also necessary for the next generation of technologies. The challenges involved with the design and operation of these integrated systems, while supplying electricity on demand, are considerable.

579 citations

Journal ArticleDOI
TL;DR: In this article, the authors provide an overview of coal devolatilization studies, especially the experimental studies and modelling efforts on the formation of char structure of bituminous coals in the open literature.

382 citations

Journal ArticleDOI
TL;DR: In this article, the authors evaluate the validity of thermal analysis methods to characterise fusion of biomass and waste ashes to predict the proportion of melted species resulting from combustion of biomass fuels.

361 citations


Cited by
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Journal ArticleDOI
01 Apr 1988-Nature
TL;DR: In this paper, a sedimentological core and petrographic characterisation of samples from eleven boreholes from the Lower Carboniferous of Bowland Basin (Northwest England) is presented.
Abstract: Deposits of clastic carbonate-dominated (calciclastic) sedimentary slope systems in the rock record have been identified mostly as linearly-consistent carbonate apron deposits, even though most ancient clastic carbonate slope deposits fit the submarine fan systems better. Calciclastic submarine fans are consequently rarely described and are poorly understood. Subsequently, very little is known especially in mud-dominated calciclastic submarine fan systems. Presented in this study are a sedimentological core and petrographic characterisation of samples from eleven boreholes from the Lower Carboniferous of Bowland Basin (Northwest England) that reveals a >250 m thick calciturbidite complex deposited in a calciclastic submarine fan setting. Seven facies are recognised from core and thin section characterisation and are grouped into three carbonate turbidite sequences. They include: 1) Calciturbidites, comprising mostly of highto low-density, wavy-laminated bioclast-rich facies; 2) low-density densite mudstones which are characterised by planar laminated and unlaminated muddominated facies; and 3) Calcidebrites which are muddy or hyper-concentrated debrisflow deposits occurring as poorly-sorted, chaotic, mud-supported floatstones. These

9,929 citations

Book ChapterDOI
01 Jan 1982
TL;DR: In this article, the authors discuss leading problems linked to energy that the world is now confronting and propose some ideas concerning possible solutions, and conclude that it is necessary to pursue actively the development of coal, natural gas, and nuclear power.
Abstract: This chapter discusses leading problems linked to energy that the world is now confronting and to propose some ideas concerning possible solutions. Oil deserves special attention among all energy sources. Since the beginning of 1981, it has merely been continuing and enhancing the downward movement in consumption and prices caused by excessive rises, especially for light crudes such as those from Africa, and the slowing down of worldwide economic growth. Densely-populated oil-producing countries need to produce to live, to pay for their food and their equipment. If the economic growth of the industrialized countries were to be 4%, even if investment in the rational use of energy were pushed to the limit and the development of nonpetroleum energy sources were also pursued actively, it would be extremely difficult to prevent a sharp rise in prices. It is evident that it is absolutely necessary to pursue actively the development of coal, natural gas, and nuclear power if a physical shortage of energy is not to block economic growth.

2,283 citations

Journal ArticleDOI
TL;DR: In this paper, various aspects of CCS are reviewed and discussed including the state of the art technologies for CO2 capture, separation, transport, storage, leakage, monitoring, and life cycle analysis.
Abstract: Global warming and climate change concerns have triggered global efforts to reduce the concentration of atmospheric carbon dioxide (CO2). Carbon dioxide capture and storage (CCS) is considered a crucial strategy for meeting CO2 emission reduction targets. In this paper, various aspects of CCS are reviewed and discussed including the state of the art technologies for CO2 capture, separation, transport, storage, leakage, monitoring, and life cycle analysis. The selection of specific CO2 capture technology heavily depends on the type of CO2 generating plant and fuel used. Among those CO2 separation processes, absorption is the most mature and commonly adopted due to its higher efficiency and lower cost. Pipeline is considered to be the most viable solution for large volume of CO2 transport. Among those geological formations for CO2 storage, enhanced oil recovery is mature and has been practiced for many years but its economical viability for anthropogenic sources needs to be demonstrated. There are growing interests in CO2 storage in saline aquifers due to their enormous potential storage capacity and several projects are in the pipeline for demonstration of its viability. There are multiple hurdles to CCS deployment including the absence of a clear business case for CCS investment and the absence of robust economic incentives to support the additional high capital and operating costs of the whole CCS process.

2,181 citations

Journal ArticleDOI
TL;DR: This article presented a bottom-up estimate of uncertainties in source strength by combining uncertainties in particulate matter emission factors, emission characterization, and fuel use, with uncertainty ranges of 4.3-22 Tg/yr for BC and 17-77 Tg /yr for OC.
Abstract: [1] We present a global tabulation of black carbon (BC) and primary organic carbon (OC) particles emitted from combustion. We include emissions from fossil fuels, biofuels, open biomass burning, and burning of urban waste. Previous ‘‘bottom-up’’ inventories of black and organic carbon have assigned emission factors on the basis of fuel type and economic sector alone. Because emission rates are highly dependent on combustion practice, we consider combinations of fuel, combustion type, and emission controls and their prevalence on a regional basis. Central estimates of global annual emissions are 8.0 Tg for black carbon and 33.9 Tg for organic carbon. These estimates are lower than previously published estimates by 25–35%. The present inventory is based on 1996 fuel-use data, updating previous estimates that have relied on consumption data from 1984. An offset between decreased emission factors and increased energy use since the base year of the previous inventory prevents the difference between this work and previous inventories from being greater. The contributions of fossil fuel, biofuel, and open burning are estimated as 38%, 20%, and 42%, respectively, for BC, and 7%, 19%, and 74%, respectively, for OC. We present a bottom-up estimate of uncertainties in source strength by combining uncertainties in particulate matter emission factors, emission characterization, and fuel use. The total uncertainties are about a factor of 2, with uncertainty ranges of 4.3–22 Tg/yr for BC and 17–77 Tg/yr for OC. Low-technology combustion contributes greatly to both the emissions and the uncertainties. Advances in emission characterization for small residential, industrial, and mobile sources and topdown analysis combining field measurements and transport modeling with iterative inventory development will be required to reduce the uncertainties further. INDEX TERMS: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0322 Atmospheric Composition and Structure: Constituent sources and sinks; 0345 Atmospheric Composition and Structure: Pollution—urban and regional (0305); 0360 Atmospheric Composition and Structure: Transmission and scattering of radiation; 0365 Atmospheric Composition and Structure: Troposphere—composition and chemistry; KEYWORDS: emission, black carbon, organic carbon, fossil fuel, biofuel, biomass burning

2,180 citations

Journal ArticleDOI
TL;DR: In this article, the utilization of fly ash in construction, as a low-cost adsorbent for the removal of organic compounds, flue gas and metals, light weight aggregate, mine back fill, road sub-base, and zeolite synthesis is discussed.

2,117 citations