William I. Rose

Bio: William I. Rose is an academic researcher from Michigan Technological University. The author has contributed to research in topics: Volcano & Volcanic ash. The author has an hindex of 71, co-authored 241 publications receiving 13418 citations. Previous affiliations of William I. Rose include National Center for Atmospheric Research & United States Geological Survey.

Retrieval of sizes and total masses of particles in volcanic clouds using AVHRR bands 4 and 5

Abstract: The advanced very high resolution radiometer (AVHRR) sensor on polar orbiting NOAA satellites can discriminate between volcanic clouds and meteorological clouds using two-band data in the thermal infrared. This paper is aimed at developing a retrieval of the particle sizes, optical depth, and total masses of particles from AVHRR two-band data of volcanic clouds. Radiative transfer calculations are used with a semi-transparent cloud model that is based on assumptions of spherical particle shape, a homogeneous underlying surface, and a simple thin cloud parallel to the surface. The model is applied to observed AVHRR data from a 13-hour old drifting cloud from the August 19, 1992, eruption of Crater Peak/Spurr Volcano, Alaska. The AVHRR data fit in the range of results calculated by the model, which supports its credibility. According to the model results, the average of effective particle radius in the test frame of this cloud is in the range of 2 to 2.5 micrometer, the optical depth at 12 micrometer is about 0.60 - 0.65. The total estimated mass of ash in the air amounts to 0.24 - 0.31 x 10(exp 6) tons, which is about 0.7-0.9% of the mass measured in the ashfall blanket. Sensitivity tests show that the mass estimate is more sensitive to the assumed ash size distribution than it is to the ash composition.

Eruptive history of Earth's largest Quaternary caldera (Toba, Indonesia) clarified

Abstract: Single-grain laser-fusion {sup 40}Ar/{sup 39}Ar analyses of individual sanidine phenocrysts from the two youngest Toba (Indonesia) tuffs yield mean ages of 73{plus minus}4 and 501{plus minus}5 ka. In addition, glass shards from Toba ash deposited in Malaysia were dated at 68{plus minus}7 ka by the isothermal plateau fission-track technique. These new determinations, in conjunction with previous ages for the two oldest tuffs at Toba, establish the chronology of four eruptive events from the Toba caldera complex over the past 1.2 m.y. Ash-flow tuffs were erupted from the complex every 0.34 to 0.43 m.y., culminating with the enormous (2500-3000 km{sup 3}) Youngest Toba tuff eruption, caldera formation, and subsequent resurgence of Samosir Island. Timing of this last eruption at Toba is coincident with the early Wisconsin glacial advance. The high-precision {sup 40}Ar/{sup 39}Ar age eruption of such magnitude may provide an important marker horizon useful as a baseline for research and modeling of the worldwide climatic impact of exceptionally large explosive eruptions.

Stratospheric sink for chlorofluoromethanes: chlorine atomc-atalysed destruction of ozone

Abstract: Chlorofluoromethanes are being added to the environment in steadily increasing amounts. These compounds are chemically inert and may remain in the atmosphere for 40–150 years, and concentrations can be expected to reach 10 to 30 times present levels. Photodissociation of the Chlorofluoromethanes in the stratosphere produces significant amounts of chlorine atoms, and leads to the destruction of atmospheric ozone.

NOAA’s HYSPLIT Atmospheric Transport and Dispersion Modeling System

Abstract: The Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT), developed by NOAA’s Air Resources Laboratory, is one of the most widely used models for atmospheric trajectory and dispersion calculations. We present the model’s historical evolution over the last 30 years from simple hand-drawn back trajectories to very sophisticated computations of transport, mixing, chemical transformation, and deposition of pollutants and hazardous materials. We highlight recent applications of the HYSPLIT modeling system, including the simulation of atmospheric tracer release experiments, radionuclides, smoke originated from wild fires, volcanic ash, mercury, and wind-blown dust.

Derivation of some modern arc magmas by melting of young subducted lithosphere

Abstract: MOST volcanic rocks in modern island and continental arcs are probably derived from melting of the mantle wedge, induced by hydrous fluids released during dehydration reactions in the subducted lithosphere1. Arc tholeiitic and calc-alkaline basaltic magmas are produced by partial melting of the mantle, and then evolve by crystal fractionation (with or without assimilation and magma mixing) to more silicic magmas2—basalt, andesite, dacite and rhyolite suites. Although most arc magmas are generated by these petrogenetic processes, rocks with the geochemical characteristics of melts derived directly from the subducted lithosphere are present in some modern arcs where relatively young and hot lithosphere is being subducted. These andesites, dacites and sodic rhyolites (dacites seem to be the most common products) or their intrusive equivalents (tonalites and trondhjemites) are usually not associated with parental basaltic magmas3. Here we show that the trace-element geochemistry of these magmas (termed 'adakites') is consistent with a derivation by partial melting of the subducted slab, and in particular that subducting lithosphere younger than 25 Myr seems to be required for slab melting to occur.

Variability of Absorption and Optical Properties of Key Aerosol Types Observed in Worldwide Locations

Abstract: Aerosol radiative forcing is a critical, though variable and uncertain, component of the global climate. Yet climate models rely on sparse information of the aerosol optical properties. In situ measurements, though important in many respects, seldom provide measurements of the undisturbed aerosol in the entire atmospheric column. Here, 8 yr of worldwide distributed data from the AERONET network of ground-based radiometers were used to remotely sense the aerosol absorption and other optical properties in several key locations. Established procedures for maintaining and calibrating the global network of radiometers, cloud screening, and inversion techniques allow for a consistent retrieval of the optical properties of aerosol in locations with varying emission sources and conditions. The multiyear, multi-instrument observations show robust differentiation in both the magnitude and spectral dependence of the absorption—a property driving aerosol climate forcing, for desert dust, biomass burning, urban‐industrial, and marine aerosols. Moreover, significant variability of the absorption for the same aerosol type appearing due to different meteorological and source characteristics as well as different emission characteristics are observed. It is expected that this aerosol characterization will help refine aerosol optical models and reduce uncertainties in satellite observations of the global aerosol and in modeling aerosol impacts on climate.