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William L. Barnes

Bio: William L. Barnes is an academic researcher from University of Exeter. The author has contributed to research in topics: Surface plasmon & Surface plasmon polariton. The author has an hindex of 65, co-authored 258 publications receiving 27877 citations. Previous affiliations of William L. Barnes include University of Southampton & MESA+ Institute for Nanotechnology.


Papers
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Journal ArticleDOI
14 Aug 2003-Nature
TL;DR: By altering the structure of a metal's surface, the properties of surface plasmons—in particular their interaction with light—can be tailored, which could lead to miniaturized photonic circuits with length scales that are much smaller than those currently achieved.
Abstract: Surface plasmons are waves that propagate along the surface of a conductor. By altering the structure of a metal's surface, the properties of surface plasmons--in particular their interaction with light--can be tailored, which offers the potential for developing new types of photonic device. This could lead to miniaturized photonic circuits with length scales that are much smaller than those currently achieved. Surface plasmons are being explored for their potential in subwavelength optics, data storage, light generation, microscopy and bio-photonics.

10,689 citations

Journal ArticleDOI
TL;DR: This review looks at the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in J-aggregates, dye molecules and quantum dots.
Abstract: In this review we look at the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in J-aggregates, dye molecules and quantum dots. We explore the phenomenon of strong coupling with reference to a number of examples involving electromagnetic fields and matter. We then provide a concise description of the relevant background physics of surface plasmon polaritons. An extensive overview of the historical background and a detailed discussion of more recent relevant experimental advances concerning strong coupling between surface plasmon polaritons and quantum emitters is then presented. Three conceptual frameworks are then discussed and compared in depth: classical, semi-classical and fully quantum mechanical; these theoretical frameworks will have relevance to strong coupling beyond that involving surface plasmon polaritons. We conclude our review with a perspective on the future of this rapidly emerging field, one we are sure will grow to encompass more intriguing physics and will develop in scope to be of relevance to other areas of science.

1,190 citations

Journal ArticleDOI
TL;DR: Experimental evidence of sharp spectral features in the optical response of 2D arrays of gold nanorods is presented, and a simple coupled dipole model is used to describe the main features of the observed spectral line shape.
Abstract: We present experimental evidence of sharp spectral features in the optical response of 2D arrays of gold nanorods. A simple coupled dipole model is used to describe the main features of the observed spectral line shape. The resonance involves an interplay between the excitation of plasmons localized on the particles and diffraction resulting from the scattering by the periodic arrangement of these particles. We investigate this interplay by varying the particle size, aspect ratio, and interparticle spacing, and observe the effect on the position, width, and intensity of the sharp spectral feature.

963 citations

Journal ArticleDOI
TL;DR: In this article, the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in Jaggregates, dye molecules and quantum dots are reviewed.
Abstract: In this review we look at the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in J-aggregates, dye molecules and quantum dots. We explore the phenomenon of strong coupling with reference to a number of examples involving electromagnetic fields and matter. We then provide a concise description of the relevant background physics of surface plasmon polaritons. An extensive overview of the historical background and a detailed discussion of more recent relevant experimental advances concerning strong coupling between surface plasmon polaritons and quantum emitters is then presented. Three conceptual frameworks are then discussed and compared in depth: classical, semi-classical and fully quantum mechanical; these theoretical frameworks will have relevance to strong coupling beyond that involving surface plasmon polaritons. We conclude our review with a perspective on the future of this rapidly emerging field, one we are sure will grow to encompass more intriguing physics and will develop in scope to be of relevance to other areas of science.

913 citations

Journal ArticleDOI
TL;DR: In this paper, a review of the role of surface and waveguide modes in photonic near interfaces is presented, including the importance of textured surfaces in providing large changes in the photonic mode density and coupling non-radiative modes to radiation.
Abstract: A review of fluorescence near interfaces is presented. Recent work that examines the role of photonic mode density in this process is surveyed and the underlying concepts discussed. The review includes an examination of the role of surface and waveguide modes, as well as non-radiative decay. The importance of textured surfaces in providing large changes in photonic mode density and in coupling non-radiative modes to radiation is highlighted. Indications are given for future areas of research and on how photonic mode density may influence optical processes other than fluorescence.

888 citations


Cited by
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Journal ArticleDOI
14 Aug 2003-Nature
TL;DR: By altering the structure of a metal's surface, the properties of surface plasmons—in particular their interaction with light—can be tailored, which could lead to miniaturized photonic circuits with length scales that are much smaller than those currently achieved.
Abstract: Surface plasmons are waves that propagate along the surface of a conductor. By altering the structure of a metal's surface, the properties of surface plasmons--in particular their interaction with light--can be tailored, which offers the potential for developing new types of photonic device. This could lead to miniaturized photonic circuits with length scales that are much smaller than those currently achieved. Surface plasmons are being explored for their potential in subwavelength optics, data storage, light generation, microscopy and bio-photonics.

10,689 citations

Journal ArticleDOI
TL;DR: Recent advances at the intersection of plasmonics and photovoltaics are surveyed and an outlook on the future of solar cells based on these principles is offered.
Abstract: The emerging field of plasmonics has yielded methods for guiding and localizing light at the nanoscale, well below the scale of the wavelength of light in free space. Now plasmonics researchers are turning their attention to photovoltaics, where design approaches based on plasmonics can be used to improve absorption in photovoltaic devices, permitting a considerable reduction in the physical thickness of solar photovoltaic absorber layers, and yielding new options for solar-cell design. In this review, we survey recent advances at the intersection of plasmonics and photovoltaics and offer an outlook on the future of solar cells based on these principles.

8,028 citations

Journal ArticleDOI
12 Feb 1998-Nature
TL;DR: In this article, the optical properties of submicrometre cylindrical cavities in metallic films were explored and it was shown that arrays of such holes display highly unusual zero-order transmission spectra at wavelengths larger than the array period, beyond which no diffraction occurs.
Abstract: The desire to use and control photons in a manner analogous to the control of electrons in solids has inspired great interest in such topics as the localization of light, microcavity quantum electrodynamics and near-field optics1,2,3,4,5,6. A fundamental constraint in manipulating light is the extremely low transmittivity of apertures smaller than the wavelength of the incident photon. While exploring the optical properties of submicrometre cylindrical cavities in metallic films, we have found that arrays of such holes display highly unusual zero-order transmission spectra (where the incident and detected light are collinear) at wavelengths larger than the array period, beyond which no diffraction occurs. In particular, sharp peaks in transmission are observed at wavelengths as large as ten times the diameter of the cylinders. At these maxima the transmission efficiency can exceed unity (when normalized to the area of the holes), which is orders of magnitude greater than predicted by standard aperture theory. Our experiments provide evidence that these unusual optical properties are due to the coupling of light with plasmons — electronic excitations — on the surface of the periodically patterned metal film. Measurements of transmission as a function of the incident light angle result in a photonic band diagram. These findings may find application in novel photonic devices.

7,316 citations

Book
15 May 2007
TL;DR: In this paper, the authors discuss the role of surface plasmon polaritons at metal/insulator interfaces and their application in the propagation of surfaceplasmon waveguides.
Abstract: Fundamentals of Plasmonics.- Electromagnetics of Metals.- Surface Plasmon Polaritons at Metal / Insulator Interfaces.- Excitation of Surface Plasmon Polaritons at Planar Interfaces.- Imaging Surface Plasmon Polariton Propagation.- Localized Surface Plasmons.- Electromagnetic Surface Modes at Low Frequencies.- Applications.- Plasmon Waveguides.- Transmission of Radiation Through Apertures and Films.- Enhancement of Emissive Processes and Nonlinearities.- Spectroscopy and Sensing.- Metamaterials and Imaging with Surface Plasmon Polaritons.- Concluding Remarks.

7,238 citations

Journal ArticleDOI
21 Oct 2011-Science
TL;DR: In this article, a two-dimensional array of optical resonators with spatially varying phase response and subwavelength separation can imprint phase discontinuities on propagating light as it traverses the interface between two media.
Abstract: Conventional optical components rely on gradual phase shifts accumulated during light propagation to shape light beams. New degrees of freedom are attained by introducing abrupt phase changes over the scale of the wavelength. A two-dimensional array of optical resonators with spatially varying phase response and subwavelength separation can imprint such phase discontinuities on propagating light as it traverses the interface between two media. Anomalous reflection and refraction phenomena are observed in this regime in optically thin arrays of metallic antennas on silicon with a linear phase variation along the interface, which are in excellent agreement with generalized laws derived from Fermat’s principle. Phase discontinuities provide great flexibility in the design of light beams, as illustrated by the generation of optical vortices through use of planar designer metallic interfaces.

6,763 citations