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Chalk River Laboratories

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About: Chalk River Laboratories is a based out in . It is known for research contribution in the topics: Neutron diffraction & Neutron scattering. The organization has 2297 authors who have published 2700 publications receiving 73287 citations.


Papers
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Journal ArticleDOI
TL;DR: In this article, the relation between spin fluctuations and superconductivity in a highly ordered sample of highly ordered samples of Cu using both polarized and unpolarized neutron inelastic scattering was described.
Abstract: We describe the relation between spin fluctuations and superconductivity in a highly ordered sample of ${\mathrm{YBa}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{6.5}$ using both polarized and unpolarized neutron inelastic scattering. The spin susceptibility in the superconducting phase exhibits one-dimensional incommensurate modulations at low energies, consistent with hydrodynamic stripes. With increasing energy the susceptibility curves upward to a commensurate, intense, well-defined, and asymmetric resonance at 33 meV with a precipitous high-energy cutoff. In the normal phase, which we show is gapless, the resonance remains surprisingly strong and persists clearly in Q scans and energy scans. Its similar asymmetric spectral form above ${T}_{c}=59\mathrm{K}$ suggests that incoherent superconducting pairing fluctuations are present in the normal state. On cooling, the resonance and the stripe modulations grow in well above ${T}_{c}$ below a temperature that is comparable to the pseudogap temperature where suppression occurs in local and low-momentum properties. The spectral weight that accrues to the resonance is largely acquired by transfer from suppressed low-energy fluctuations. We find the resonance to be isotropically polarized, consistent with a triplet carrying $\ensuremath{\sim}2.6%$ of the total spectral weight of the Cu spins in the planes.

139 citations

Journal ArticleDOI
TL;DR: In this article, the soft-mode energy of the relaxor was shown to increase linearly with decreasing temperature and is consistent with the behavior of a ferroelectric soft mode.
Abstract: Neutron scattering measurements of the lowest-energy TO phonons in the relaxor $\mathrm{Pb}({\mathrm{Mg}}_{1/3}{\mathrm{Nb}}_{2/3}){\mathrm{O}}_{3}$ (PMN) are reported for $10l~Tl~750 \mathrm{K}.$ The soft mode, which is overdamped by the polar nanoregions below the Burns temperature ${T}_{d}=620 \mathrm{K},$ surprisingly recovers below 220 K. The square of the soft-mode energy $(\ensuremath{\Elzxh}{\ensuremath{\omega}}_{0}{)}^{2}$ increases linearly with decreasing temperature and is consistent with the behavior of a ferroelectric soft mode. At 10 K, $\ensuremath{\Elzxh}{\ensuremath{\omega}}_{0}$ reaches 11 meV, the same value observed in ferroelectric $\mathrm{Pb}({\mathrm{Zn}}_{1/3}{\mathrm{Nb}}_{2/3}){\mathrm{O}}_{3}$ at low T. An unusual broadening of the TA phonon starts at ${T}_{d}$ and disappears at 220 K, coincident with the recovery of the TO mode. These dynamics suggest that a well-developed ferroelectric state is established below 220 K.

137 citations

Journal ArticleDOI
TL;DR: Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu 2 Si 2 as discussed by the authors, which is the state of the hidden order state of spin excitation.
Abstract: Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu 2 Si 2

134 citations

Journal ArticleDOI
TL;DR: In this article, the structural, chemical and morphological changes of intermetallic particles of Zr(Cr, Fe)2 and Zr2(Ni, Fe), Fe 2 in Zircaloy-2 and -4 were studied.

133 citations

Journal ArticleDOI
TL;DR: The magnetic metal ions in the cubic pyrochlore form an infinite three-dimensional network of corner-sharing tetrahedra with a very high potential for frustration in the presence of antiferromagnetism as mentioned in this paper.
Abstract: The magnetic metal ions in the cubic pyrochlore ${\mathrm{Tb}}_{2}$${\mathrm{Mo}}_{2}$${\mathrm{O}}_{7}$ form an infinite three-dimensional network of corner-sharing tetrahedra with a very high potential for frustration in the presence of antiferromagnetism. We have performed neutron scattering measurements which show short-range spatial correlations that develop continuously with decreasing temperature, while the characteristic time scale for the fluctuating moments decreases dramatically below ${\mathit{T}}_{\mathit{f}}$\ensuremath{\sim}25 K. Therefore, this pure material, which possess frustration that is purely geometrical in origin, displays a spin-glass state at low temperatures.

133 citations


Authors

Showing all 2298 results

NameH-indexPapersCitations
Michael D. Guiver7828820540
Robert J. Birgeneau7858722686
Mike D. Flannigan7121121327
Martin T. Dove6139614767
Luis Rodrigo5834112963
André Longtin5626016372
David Mitlin5619615479
John Katsaras552209263
John E. Greedan5539112171
Gang Li484067713
Matthew G. Tucker452247288
Bruce D. Gaulin452846698
Erick J. Dufourc431445882
Norbert Kučerka431197319
Stephen J. Skinner421948522
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Performance
Metrics
No. of papers from the Institution in previous years
YearPapers
20231
202284
202176
202072
201974
2018104