Showing papers by "Paul Scherrer Institute published in 2021"

Unconventional chiral charge order in kagome superconductor KV3Sb5.

Abstract: Intertwining quantum order and non-trivial topology is at the frontier of condensed matter physics1–4. A charge-density-wave-like order with orbital currents has been proposed for achieving the quantum anomalous Hall effect5,6 in topological materials and for the hidden phase in cuprate high-temperature superconductors7,8. However, the experimental realization of such an order is challenging. Here we use high-resolution scanning tunnelling microscopy to discover an unconventional chiral charge order in a kagome material, KV3Sb5, with both a topological band structure and a superconducting ground state. Through both topography and spectroscopic imaging, we observe a robust 2 × 2 superlattice. Spectroscopically, an energy gap opens at the Fermi level, across which the 2 × 2 charge modulation exhibits an intensity reversal in real space, signalling charge ordering. At the impurity-pinning-free region, the strength of intrinsic charge modulations further exhibits chiral anisotropy with unusual magnetic field response. Theoretical analysis of our experiments suggests a tantalizing unconventional chiral charge density wave in the frustrated kagome lattice, which can not only lead to a large anomalous Hall effect with orbital magnetism, but also be a precursor of unconventional superconductivity. An unconventional chiral charge order is observed in a kagome superconductor by scanning tunnelling microscopy. This charge order has unusual magnetic tunability and intertwines with electronic topology.

A stable low-temperature H2-production catalyst by crowding Pt on α-MoC.

Abstract: The water–gas shift (WGS) reaction is an industrially important source of pure hydrogen (H2) at the expense of carbon monoxide and water1,2. This reaction is of interest for fuel-cell applications, but requires WGS catalysts that are durable and highly active at low temperatures3. Here we demonstrate that the structure (Pt1–Ptn)/α-MoC, where isolated platinum atoms (Pt1) and subnanometre platinum clusters (Ptn) are stabilized on α-molybdenum carbide (α-MoC), catalyses the WGS reaction even at 313 kelvin, with a hydrogen-production pathway involving direct carbon monoxide dissociation identified. We find that it is critical to crowd the α-MoC surface with Pt1 and Ptn species, which prevents oxidation of the support that would cause catalyst deactivation, as seen with gold/α-MoC (ref. 4), and gives our system high stability and a high metal-normalized turnover number of 4,300,000 moles of hydrogen per mole of platinum. We anticipate that the strategy demonstrated here will be pivotal for the design of highly active and stable catalysts for effective activation of important molecules such as water and carbon monoxide for energy production. A stable, low-temperature water–gas shift catalyst is achieved by crowding platinum atoms and clusters on α-molybdenum carbide; the crowding protects the support from oxidation that would cause catalyst deactivation.

Potential and risks of hydrogen-based e-fuels in climate change mitigation

Abstract: E-fuels promise to replace fossil fuels with renewable electricity without the demand-side transformations required for a direct electrification. However, e-fuels’ versatility is counterbalanced by their fragile climate effectiveness, high costs and uncertain availability. E-fuel mitigation costs are €800–1,200 per tCO2. Large-scale deployment could reduce costs to €20–270 per tCO2 until 2050, yet it is unlikely that e-fuels will become cheap and abundant early enough. Neglecting demand-side transformations threatens to lock in a fossil-fuel dependency if e-fuels fall short of expectations. Sensible climate policy supports e-fuel deployment while hedging against the risk of their unavailability at large scale. Policies should be guided by a ‘merit order of end uses’ that prioritizes hydrogen and e-fuels for sectors that are inaccessible to direct electrification. E-fuels—hydrocarbon fuels synthesized from green hydrogen—can replace fossil fuels. This Perspective highlights the opportunities and risks of e-fuels, and concludes that hydrogen and e-fuels should be prioritized for sectors inaccessible to direct electrification.

EANO guideline on the diagnosis and management of meningiomas.

Abstract: Meningiomas are the most common intracranial tumors. Yet, only few controlled clinical trials have been conducted to guide clinical decision making, resulting in variations of management approaches across countries and centers. However, recent advances in molecular genetics and clinical trial results help to refine the diagnostic and therapeutic approach to meningioma. Accordingly, the European Association of Neuro-Oncology (EANO) updated its recommendations for the diagnosis and treatment of meningiomas. A provisional diagnosis of meningioma is typically made by neuroimaging, mostly magnetic resonance imaging. Such provisional diagnoses may be made incidentally. Accordingly, a significant proportion of meningiomas, notably in patients that are asymptomatic or elderly or both, may be managed by a watch-and-scan strategy. A surgical intervention with tissue, commonly with the goal of gross total resection, is required for the definitive diagnosis according to the WHO classification. A role for molecular profiling including gene panel sequencing and genomic methylation profiling is emerging. A gross total surgical resection including the involved dura is often curative. Inoperable or recurrent tumors requiring treatment can be treated with radiosurgery, if the size or the vicinity of critical structures allows that, or with fractionated radiotherapy (RT). Treatment concepts combining surgery and radiosurgery or fractionated RT are increasingly used, although there remain controversies regard timing, type, and dosing of the various RT approaches. Radionuclide therapy targeting somatostatin receptors is an experimental approach, as are all approaches of systemic pharmacotherapy. The best albeit modest results with pharmacotherapy have been obtained with bevacizumab or multikinase inhibitors targeting vascular endothelial growth factor receptor, but no standard of care systemic treatment has been yet defined.

Visualizing plating-induced cracking in lithium-anode solid-electrolyte cells.

Abstract: Lithium dendrite (filament) propagation through ceramic electrolytes, leading to short circuits at high rates of charge, is one of the greatest barriers to realizing high-energy-density all-solid-state lithium-anode batteries. Utilizing in situ X-ray computed tomography coupled with spatially mapped X-ray diffraction, the propagation of cracks and the propagation of lithium dendrites through the solid electrolyte have been tracked in a Li/Li6PS5Cl/Li cell as a function of the charge passed. On plating, cracking initiates with spallation, conical ‘pothole’-like cracks that form in the ceramic electrolyte near the surface with the plated electrode. The spallations form predominantly at the lithium electrode edges where local fields are high. Transverse cracks then propagate from the spallations across the electrolyte from the plated to the stripped electrode. Lithium ingress drives the propagation of the spallation and transverse cracks by widening the crack from the rear; that is, the crack front propagates ahead of the Li. As a result, cracks traverse the entire electrolyte before the Li arrives at the other electrode, and therefore before a short circuit occurs. Lithium dendrite propagation through ceramic electrolytes can prevent the realization of high-energy-density all-solid-state lithium-anode batteries. The propagation of cracks and lithium dendrites through a solid electrolyte has now been tracked as a function of charge.

Observation of flat bands in twisted bilayer graphene

Abstract: Transport experiments in twisted bilayer graphene have revealed multiple superconducting domes separated by correlated insulating states1–5. These properties are generally associated with strongly correlated states in a flat mini-band of the hexagonal moire superlattice as was predicted by band structure calculations6–8. Evidence for the existence of a flat band comes from local tunnelling spectroscopy9–13 and electronic compressibility measurements14, which report two or more sharp peaks in the density of states that may be associated with closely spaced Van Hove singularities. However, direct momentum-resolved measurements have proved to be challenging15. Here, we combine different imaging techniques and angle-resolved photoemission with simultaneous real- and momentum-space resolution (nano-ARPES) to directly map the band dispersion in twisted bilayer graphene devices near charge neutrality. Our experiments reveal large areas with a homogeneous twist angle that support a flat band with a spectral weight that is highly localized in momentum space. The flat band is separated from the dispersive Dirac bands, which show multiple moire hybridization gaps. These data establish the salient features of the twisted bilayer graphene band structure. Spectroscopic measurements using nano-ARPES on twisted bilayer graphene directly highlight the presence of the flat bands.

Electron and photon reconstruction and identification with the CMS experiment at the CERN LHC

Abstract: The performance is presented of the reconstruction and identification algorithms for electrons and photons with the CMS experiment at the LHC. The reported results are based on proton-proton collision data collected at a center-of-mass energy of 13 TeV and recorded in 2016-2018, corresponding to an integrated luminosity of 136 fb$^{-1}$. Results obtained from lead-lead collision data collected at $\sqrt{s_\mathrm{NN}}=$ 5.02 TeV are also presented. Innovative techniques are used to reconstruct the electron and photon signals in the detector and to optimize the energy resolution. Events with electrons and photons in the final state are used to measure the energy resolution and energy scale uncertainty in the recorded events. The measured energy resolution for electrons produced in Z boson decays in proton-proton collision data ranges from 2 to 5%, depending on electron pseudorapidity and energy loss through bremsstrahlung in the detector material. The energy scale in the same range of energies is measured with an uncertainty smaller than 0.1 (0.3)% in the barrel (endcap) region in proton-proton collisions and better than 1 (3)% in the barrel (endcap) region in heavy ion collisions. The timing resolution for electrons from Z boson decays with the full 2016-2018 proton-proton collision data set is measured to be 200 ps.

Perovskite-type superlattices from lead halide perovskite nanocubes

Abstract: Atomically defined assemblies of dye molecules (such as H and J aggregates) have been of interest for more than 80 years because of the emergence of collective phenomena in their optical spectra1–3, their coherent long-range energy transport, their conceptual similarity to natural light-harvesting complexes4,5, and their potential use as light sources and in photovoltaics. Another way of creating versatile and controlled aggregates that exhibit collective phenomena involves the organization of colloidal semiconductor nanocrystals into long-range-ordered superlattices6. Caesium lead halide perovskite nanocrystals7–9 are promising building blocks for such superlattices, owing to the high oscillator strength of bright triplet excitons10, slow dephasing (coherence times of up to 80 picoseconds) and minimal inhomogeneous broadening of emission lines11,12. So far, only single-component superlattices with simple cubic packing have been devised from these nanocrystals13. Here we present perovskite-type (ABO3) binary and ternary nanocrystal superlattices, created via the shape-directed co-assembly of steric-stabilized, highly luminescent cubic CsPbBr3 nanocrystals (which occupy the B and/or O lattice sites), spherical Fe3O4 or NaGdF4 nanocrystals (A sites) and truncated-cuboid PbS nanocrystals (B sites). These ABO3 superlattices, as well as the binary NaCl and AlB2 superlattice structures that we demonstrate, exhibit a high degree of orientational ordering of the CsPbBr3 nanocubes. They also exhibit superfluorescence—a collective emission that results in a burst of photons with ultrafast radiative decay (22 picoseconds) that could be tailored for use in ultrabright (quantum) light sources. Our work paves the way for further exploration of complex, ordered and functionally useful perovskite mesostructures. Through precise structural engineering, perovskite nanocrystals are co-assembled with other nanocrystal materials to form a range of binary and ternary perovskite-type superlattices that exhibit superfluorescence.

Unlocking anionic redox activity in O3-type sodium 3d layered oxides via Li substitution

Abstract: Sodium ion batteries, because of their sustainability attributes, could be an attractive alternative to Li-ion technology for specific applications. However, it remains challenging to design high energy density and moisture stable Na-based positive electrodes. Here, we report an O3-type NaLi1/3Mn2/3O2 phase showing anionic redox activity, obtained through a ceramic process by carefully adjusting synthesis conditions and stoichiometry. This phase shows a sustained reversible capacity of 190 mAh g−1 that is rooted in cumulative oxygen and manganese redox processes as deduced by combined spectroscopy techniques. Unlike many other anionic redox layered oxides so far reported, O3-NaLi1/3Mn2/3O2 electrodes do not show discernible voltage fade on cycling. This finding, rationalized by density functional theory, sheds light on the role of inter- versus intralayer 3d cationic migration in ruling voltage fade in anionic redox electrodes. Another practical asset of this material stems from its moisture stability, hence facilitating its handling and electrode processing. Overall, this work offers future directions towards designing highly performing sodium electrodes for advanced Na-ion batteries. Sodium ion batteries could be an attractive alternative to Li-ion technology but designing high energy density and moisture stable Na-based cathodes is challenging. Adjusting synthesis conditions and stoichiometry, an O3-type NaLi1/3Mn2/3O2 phase with anionic redox activity is reported.

Colloquium: Nonthermal pathways to ultrafast control in quantum materials

Abstract: Ultrafast laser pulses can be used to drive materials into nonequilibrium states that have unusual properties and are promising for technological applications. Different classes of phenomena are observed during and after the optical illumination. This Colloquium discusses the recent developments in this field, and the prospects for using these techniques to create materials with novel functionalities in a controlled way.

Absence of local moments in the kagome metal KV3Sb5 as determined by muon spin spectroscopy

Abstract: We have carried out muon spin relaxation and rotation measurements on the newly discovered kagome metal KV3Sb5, and find a local field dominated by weak magnetic disorder which we associate with the nuclear moments present, and a modest temperature dependence which tracks the bulk magnetic susceptibility. We find no evidence for the existence of V4+local moments, suggesting that the physics underlying the recently reported giant unconventional anomalous Hall effect in this material warrants further studies.

Life cycle assessment of carbon dioxide removal technologies: a critical review

Abstract: A large number of prospective climate scenarios rely on Carbon Dioxide Removal (CDR) technologies to limit global warming below 2 °C. To date, however, a comprehensive understanding of the overall life-cycle environmental impacts of CDR technologies is missing. We present a critical review on conducted Life Cycle Assessments (LCAs) of a comprehensive set of CDR technologies: afforestation and reforestation, biochar, soil carbon sequestration, enhanced weathering, ocean fertilisation, bioenergy with carbon capture and storage, and direct air carbon capture and storage. One of the key observations is that emissions avoided due to substitution of certain processes (due to system expansion in LCA) can be easily misinterpreted as negative emissions, i.e. as carbon removal from the atmosphere. Based on the observed inconsistencies and shortcomings, we recommend to interpret available CDR LCA results with caution. To improve the understanding of environmental implications of CDR deployment, we recommend (1) to conduct LCAs with multiple environmental impact categories, (2) to consider the temporal aspect of emissions in biomass-related CDR technologies, (3) to focus on so far overlooked CDR technologies, (4) to be as transparent as possible regarding methodological choices, (5) to capture environmental side-effects, and (6) to distinguish between ‘avoided emissions’ and ‘negative emissions’ – only negative emissions correspond to permanent removal from the atmosphere. We conclude that more comprehensive and rigorous LCAs are needed to help inform the design of CDR technology portfolios and to aid in anticipatory governance.

Néel-type skyrmions and their current-induced motion in van der Waals ferromagnet-based heterostructures

Abstract: Since the discovery of ferromagnetic two-dimensional (2D) van der Waals (vdW) crystals, significant interest on such 2D magnets has emerged, inspired by their appealing properties and integration with other 2D family for unique heterostructures In known 2D magnets, spin-orbit coupling (SOC) stabilizes perpendicular magnetic anisotropy (PMA) Such a strong SOC could also lift the chiral degeneracy, leading to the formation of topological magnetic textures such as skyrmions through the Dzyaloshinskii-Moriya interaction (DMI) Here, we report the experimental observation of Neel-type chiral magnetic skyrmions and their lattice (SkX) formation in a vdW ferromagnet Fe3GeTe2 (FGT) We demonstrate the ability to drive individual skyrmion by short current pulses along a vdW heterostructure, FGT/h-BN, as highly required for any skyrmion-based spintronic device Using first principle calculations supported by experiments, we unveil the origin of DMI being the interfaces with oxides, which then allows us to engineer vdW heterostructures for desired chiral states Our finding opens the door to topological spin textures in the 2D vdW magnet and their potential device application

Simulation of mineral dissolution at the pore scale with evolving fluid-solid interfaces: review of approaches and benchmark problem set

Abstract: This manuscript presents a benchmark problem for the simulation of single-phase flow, reactive transport, and solid geometry evolution at the pore scale. The problem is organized in three parts that focus on specific aspects: flow and reactive transport (part I), dissolution-driven geometry evolution in two dimensions (part II), and an experimental validation of three-dimensional dissolution-driven geometry evolution (part III). Five codes are used to obtain the solution to this benchmark problem, including Chombo-Crunch, OpenFOAM-DBS, a lattice Boltzman code, Vortex, and dissolFoam. These codes cover a good portion of the wide range of approaches typically employed for solving pore-scale problems in the literature, including discretization methods, characterization of the fluid-solid interfaces, and methods to move these interfaces as a result of fluid-solid reactions. A short review of these approaches is given in relation to selected published studies. Results from the simulations performed by the five codes show remarkable agreement both quantitatively-based on upscaled parameters such as surface area, solid volume, and effective reaction rate-and qualitatively-based on comparisons of shape evolution. This outcome is especially notable given the disparity of approaches used by the codes. Therefore, these results establish a strong benchmark for the validation and testing of pore-scale codes developed for the simulation of flow and reactive transport with evolving geometries. They also underscore the significant advances seen in the last decade in tools and approaches for simulating this type of problem.

Recent progress in syngas production via catalytic CO2 hydrogenation reaction

Abstract: Synthesis gas production through the catalytic reverse water-gas shift (RWGS) reaction is an attractive option for the conversion of CO2 to fuels. Many metal-based catalysts have been introduced for this reaction in order to provide high activity, CO selectivity, and stability. Recently, progress has been made in catalyst design and understanding of the reaction mechanism, which has shed light on the characteristics of the catalysts needed for this reaction. Accordingly, new noble and non-noble metal-based catalysts with remarkable performance have been introduced for this reaction. However, there is still much room for catalyst improvement specifically in regard to catalyst stability at the high temperatures required for this reaction. There are also controversial arguments regarding the active sites of the reaction. This review highlights the recent progress in catalyst design and understanding of the reaction mechanism for the RWGS reaction and derives proposals for further improvements of the process.

A review on resilience assessment of energy systems

Abstract: Energy systems are regularly subject to major disruptions affecting economic activities, operation of infrastructure and the society as a whole. Resilience assessment comprises the pre-event orient...

Perovskite Oxide Based Electrodes for the Oxygen Reduction and Evolution Reactions: The Underlying Mechanism

Abstract: One hindrance to the development of fuel cells and electrolyzers are the oxygen electrodes, which suffer from high overpotentials and slow kinetics. Perovskite oxides have been shown to be promisin...

Evidence for Higgs boson decay to a pair of muons

Abstract: Evidence for Higgs boson decay to a pair of muons is presented. This result combines searches in four exclusive categories targeting the production of the Higgs boson via gluon fusion, via vector boson fusion, in association with a vector boson, and in association with a top quark-antiquark pair. The analysis is performed using proton-proton collision data at $ \sqrt{s} $ = 13 TeV, corresponding to an integrated luminosity of 137 fb$^{−1}$, recorded by the CMS experiment at the CERN LHC. An excess of events over the back- ground expectation is observed in data with a significance of 3.0 standard deviations, where the expectation for the standard model (SM) Higgs boson with mass of 125.38 GeV is 2.5. The combination of this result with that from data recorded at $ \sqrt{s} $ = 7 and 8 TeV, corresponding to integrated luminosities of 5.1 and 19.7 fb$^{−1}$, respectively, increases both the expected and observed significances by 1%. The measured signal strength, relative to the SM prediction, is $ {1.19}_{-0.39}^{+0.40}{\left(\mathrm{stat}\right)}_{-0.14}^{+0.15}\left(\mathrm{syst}\right) $. This result constitutes the first evidence for the decay of the Higgs boson to second generation fermions and is the most precise measurement of the Higgs boson coupling to muons reported to date.[graphic not available: see fulltext]

Electron ptychography achieves atomic-resolution limits set by lattice vibrations

Abstract: Transmission electron microscopes use electrons with wavelengths of a few picometers, potentially capable of imaging individual atoms in solids at a resolution ultimately set by the intrinsic size of an atom. Unfortunately, due to imperfections in the imaging lenses and multiple scattering of electrons in the sample, the image resolution reached is 3 to 10 times worse. Here, by inversely solving the multiple scattering problem and overcoming the aberrations of the electron probe using electron ptychography to recover a linear phase response in thick samples, we demonstrate an instrumental blurring of under 20 picometers. The widths of atomic columns in the measured electrostatic potential are now no longer limited by the imaging system, but instead by the thermal fluctuations of the atoms. We also demonstrate that electron ptychography can potentially reach a sub-nanometer depth resolution and locate embedded atomic dopants in all three dimensions with only a single projection measurement.

Consequences of chirally enhanced explanations of ( g - 2) μ for h → μμ and Z → μμ

Abstract: With the long-standing tension between experiment and Standard-Model (SM) prediction in the anomalous magnetic moment of the muon aμ recently reaffirmed by the Fermilab experiment, the crucial question becomes which other observables could be sensitive to the underlying physics beyond the SM to which aμ may be pointing. While from the effective field theory (EFT) point of view no direct correlations exist, this changes in specific new physics models. In particular, in the case of explanations involving heavy new particles above the electroweak (EW) scale with chiral enhancement, which are preferred to evade exclusion limits from direct searches, correlations with other observables sensitive to EW symmetry breaking are expected. Such scenarios can be classified according to the SU(2)L representations and the hypercharges of the new particles. We match the resulting class of models with heavy new scalars and fermions onto SMEFT and study the resulting correlations with h → μμ and Z → μμ decays, where, via SU(2)L symmetry, the latter process is related to Z → νν and modified W-μ-ν couplings.

Higgs-mass predictions in the MSSM and beyond

Abstract: Predictions for the Higgs masses are a distinctive feature of supersymmetric extensions of the Standard Model, where they play a crucial role in constraining the parameter space. The discovery of a Higgs boson and the remarkably precise measurement of its mass at the LHC have spurred new efforts aimed at improving the accuracy of the theoretical predictions for the Higgs masses in supersymmetric models. The “Precision SUSY Higgs Mass Calculation Initiative” (KUTS) was launched in 2014 to provide a forum for discussions between the different groups involved in these efforts. This report aims to present a comprehensive overview of the current status of Higgs-mass calculations in supersymmetric models, to document the many advances that were achieved in recent years and were discussed during the KUTS meetings, and to outline the prospects for future improvements in these calculations.

Correlating h→μ^{+}μ^{-} to the Anomalous Magnetic Moment of the Muon via Leptoquarks.

Abstract: Recently, both ATLAS and CMS measured the decay $h\ensuremath{\rightarrow}{\ensuremath{\mu}}^{+}{\ensuremath{\mu}}^{\ensuremath{-}}$, finding a signal strength with respect to the standard model expectation of $1.2\ifmmode\pm\else\textpm\fi{}0.6$ and ${1.19}_{\ensuremath{-}0.39\ensuremath{-}0.16}^{+0.41+0.17}$, respectively. This provides, for the first time, evidence that the standard model Higgs couples to second generation fermions. This measurement is particularly interesting in the context of the intriguing hints for lepton flavor universality violation, accumulated within recent years, as new physics explanations could also be tested in the $h\ensuremath{\rightarrow}{\ensuremath{\mu}}^{+}{\ensuremath{\mu}}^{\ensuremath{-}}$ decay mode. Leptoquarks are prime candidates to account for the flavor anomalies. In particular, they can provide the necessary chiral enhancement (by a factor ${m}_{t}/{m}_{\ensuremath{\mu}}$) to address ${a}_{\ensuremath{\mu}}$ with tera-electron-volt scale new physics. In this Letter we point out that such explanations of ${a}_{\ensuremath{\mu}}$ also lead to enhanced effects in $h\ensuremath{\rightarrow}{\ensuremath{\mu}}^{+}{\ensuremath{\mu}}^{\ensuremath{-}}$ and we examine the correlations between $h\ensuremath{\rightarrow}{\ensuremath{\mu}}^{+}{\ensuremath{\mu}}^{\ensuremath{-}}$ and ${a}_{\ensuremath{\mu}}$ within leptoquark models. We find that the effect in the branching ratio of $h\ensuremath{\rightarrow}{\ensuremath{\mu}}^{+}{\ensuremath{\mu}}^{\ensuremath{-}}$ ranges from several percent up to a factor of 3, if one aims at accounting for ${a}_{\ensuremath{\mu}}$ at the $2\ensuremath{\sigma}$ level. Hence, the new ATLAS and CMS Collaboration measurements already provide important constraints on the parameter space, rule out specific ${a}_{\ensuremath{\mu}}$ explanations, and will be very important to test the flavor anomalies in the future.

Search for resonant and nonresonant new phenomena in high-mass dilepton final states at √s = 13 TeV

Abstract: A search is presented for physics beyond the standard model (SM) using electron or muon pairs with high invariant mass. A data set of proton-proton collisions collected by the CMS experiment at the LHC at s = 13 TeV from 2016 to 2018 corresponding to a total integrated luminosity of up to 140 fb−1 is analyzed. No significant deviation is observed with respect to the SM background expectations. Upper limits are presented on the ratio of the product of the production cross section and the branching fraction to dileptons of a new narrow resonance to that of the Z boson. These provide the most stringent lower limits to date on the masses for various spin-1 particles, spin-2 gravitons in the Randall-Sundrum model, as well as spin-1 mediators between the SM and dark matter particles. Lower limits on the ultraviolet cutoff parameter are set both for four-fermion contact interactions and for the Arkani-Hamed, Dimopoulos, and Dvali model with large extra dimensions. Lepton flavor universality is tested at the TeV scale for the first time by comparing the dimuon and dielectron mass spectra. No significant deviation from the SM expectation of unity is observed.

Role of iodine oxoacids in atmospheric aerosol nucleation.

Abstract: Iodic acid (HIO3) is known to form aerosol particles in coastal marine regions, but predicted nucleation and growth rates are lacking Using the CERN CLOUD (Cosmics Leaving Outdoor Droplets) chamber, we find that the nucleation rates of HIO3 particles are rapid, even exceeding sulfuric acid–ammonia rates under similar conditions We also find that ion-induced nucleation involves IO3− and the sequential addition of HIO3 and that it proceeds at the kinetic limit below +10°C In contrast, neutral nucleation involves the repeated sequential addition of iodous acid (HIO2) followed by HIO3, showing that HIO2 plays a key stabilizing role Freshly formed particles are composed almost entirely of HIO3, which drives rapid particle growth at the kinetic limit Our measurements indicate that iodine oxoacid particle formation can compete with sulfuric acid in pristine regions of the atmosphere

Life Cycle Assessment of Direct Air Carbon Capture and Storage with Low-Carbon Energy Sources.

Abstract: Direct air carbon capture and storage (DACCS) is an emerging carbon dioxide removal technology, which has the potential to remove large amounts of CO2 from the atmosphere. We present a comprehensive life cycle assessment of different DACCS systems with low-carbon electricity and heat sources required for the CO2 capture process, both stand-alone and grid-connected system configurations. The results demonstrate negative greenhouse gas (GHG) emissions for all eight selected locations and five system layouts, with the highest GHG removal potential in countries with low-carbon electricity supply and waste heat usage (up to 97%). Autonomous system layouts prove to be a promising alternative, with a GHG removal efficiency of 79-91%, at locations with high solar irradiation to avoid the consumption of fossil fuel-based grid electricity and heat. The analysis of environmental burdens other than GHG emissions shows some trade-offs associated with CO2 removal, especially land transformation for system layouts with photovoltaics (PV) electricity supply. The sensitivity analysis reveals the importance of selecting appropriate locations for grid-coupled system layouts since the deployment of DACCS at geographic locations with CO2-intensive grid electricity mixes leads to net GHG emissions instead of GHG removal today.

Scalar leptoquarks in leptonic processes

Abstract: Leptoquarks are hypothetical new particles, which couple quarks directly to leptons. They experienced a renaissance in recent years as they are prime candidates to explain the so-called flavor anomalies, i.e. the deviations between the Standard Model predictions and measurements in b → sl+l− and b → cτν processes and in the anomalous magnetic moment of the muon. At the one-loop level these particles unavoidably generate effects in the purely leptonic processes like Z → l+l−, Z → $$ v\overline{v} $$ , W → lν and h → l+l− and can even generate non-zero rates for lepton flavor violating processes such as l → l′γ, Z → l+l′−, h → l+l′− and l → 3l′. In this article we calculate these processes for all five representations of scalar Leptoquarks. We include their most general interaction terms with the Standard Model Higgs boson, which leads to Leptoquark mixing after the former acquires a vacuum expectation value. In our phenomenological analysis we investigate the effects in modified lepton couplings to electroweak gauge bosons, we study the correlations of the anomalous magnetic moment of the muon with h → μ+μ− and Z → μ+μ− as well as the interplay between different lepton flavor violating decays.

Explaining b →s ℓ + ℓ - and the Cabibbo angle anomaly with a vector triplet

Abstract: The most statistically significant hints for new physics in the flavor sector are discrepancies between theory and experiment in $B$ decays to lepton pairs ($b\ensuremath{\rightarrow}s{\ensuremath{\ell}}^{+}{\ensuremath{\ell}}^{\ensuremath{-}}$) and a deficit in the unitarity constraints to the 1st row of the Cabibbo-Kobayashi-Maskawa matrix (the Cabibbo angle anomaly). We propose that these anomalies can be reconciled by a simplified model with massive gauge bosons transforming in the adjoint representation of $SU(2{)}_{L}$. After calculating the impact of this model on $B$ decays, observables testing charged current lepton flavor universality (LFU), electro-weak precision observables and LHC searches we perform a global fit to all available data. We find that our model can provide a consistent common explanation of both anomalies and that the fit to the data is more than $7\ensuremath{\sigma}$ better than the fit of the Standard Model. The model also predicts interesting correlations between LFU violation in the charged current and $b\ensuremath{\rightarrow}s{\ensuremath{\ell}}^{+}{\ensuremath{\ell}}^{\ensuremath{-}}$ data which can be tested experimentally in the near future.

Technical design of the phase I Mu3e experiment

Abstract: The Mu3e experiment aims to find or exclude the lepton flavour violating decay μ → e e e at branching fractions above 1 0 − 16 . A first phase of the experiment using an existing beamline at the Paul Scherrer Institute (PSI) is designed to reach a single event sensitivity of 2 ⋅ 1 0 − 15 . We present an overview of all aspects of the technical design and expected performance of the phase I Mu3e detector. The high rate of up to 1 0 8 muon decays per second and the low momenta of the decay electrons and positrons pose a unique set of challenges, which we tackle using an ultra thin tracking detector based on high-voltage monolithic active pixel sensors combined with scintillating fibres and tiles for precise timing measurements.