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Showing papers by "University of Science and Technology of China published in 2022"


Journal ArticleDOI
TL;DR: In this article, a reactive multifunctional heterostructure, copper-organophosphate-MXene (CuP- MXene) by rational design is presented, which exhibits satisfactory flame retardancy (UL-94-V-0 rating, peak heat release rate decreased by 64.4% and improved mechanical properties (tensile strength, elastic modulus and impact strength increased by 31.7%, 38.9%, and 25.0%, respectively) relative to virgin Epoxy resins, outperforming its previous counterparts.

110 citations


Journal ArticleDOI
TL;DR: In this paper, an ultralight magnetic-carbon hybrid material was designed to achieve superior microwave absorption performance by instantaneous freezing-induced self-assembly of Fe3+, Co2+glucose complexes on a cheap and water-removable template (i.e., NaCl).

94 citations


Journal ArticleDOI
TL;DR: In this article , a novel design on angled fins was proposed to improve the thermal transport for phase change materials (PCMs) in a shell-and-tube thermal storage unit, and a numerical model was built and verified by comparing with experimental observations on the melting front evolution and temperature history.

82 citations


Journal ArticleDOI
TL;DR: In this paper , the electronic nature of the charge density wave (CDW) phase in high-resolution angle-resolved photoemission measurements on KV3Sb5 superconductors was revealed.
Abstract: The Kagome superconductors AV3Sb5 (A=K, Rb, Cs) have received enormous attention due to their nontrivial topological electronic structure, anomalous physical properties and superconductivity. Unconventional charge density wave (CDW) has been detected in AV3Sb5. High-precision electronic structure determination is essential to understand its origin. Here we unveil electronic nature of the CDW phase in our high-resolution angle-resolved photoemission measurements on KV3Sb5. We have observed CDW-induced Fermi surface reconstruction and the associated band folding. The CDW-induced band splitting and the associated gap opening have been revealed at the boundary of the pristine and reconstructed Brillouin zones. The Fermi surface- and momentum-dependent CDW gap is measured and the strongly anisotropic CDW gap is observed for all the V-derived Fermi surface. In particular, we have observed signatures of the electron-phonon coupling in KV3Sb5. These results provide key insights in understanding the nature of the CDW state and its interplay with superconductivity in AV3Sb5 superconductors.

82 citations


Journal ArticleDOI
TL;DR: In this paper, a novel design on angled fins was proposed to improve the thermal transport for phase change materials (PCMs) in a shell-and-tube thermal storage unit, and a numerical model was built and verified by comparing with experimental observations on the melting front evolution and temperature history.

82 citations


Journal ArticleDOI
TL;DR: Based on high specific surface area, high porosity of metal-organic frameworks (MOFs) and excellent visible light response of CdS, the CDSS/Cd-MOF nanocomposites were constructed by in-situ sulfurization to form Cds using Cd-MoF as precursor, and the Cds loading was controlled by the dose of thioacetamide as mentioned in this paper .

79 citations


Journal ArticleDOI
TL;DR: In this article , an ultralight magnetic-carbon hybrid material was designed to achieve superior microwave absorption performance by instantaneous freezing-induced self-assembly of Fe3+, Co2+-glucose complexes on a cheap and water-removable template (i.e., NaCl).

78 citations


Journal ArticleDOI
01 Jan 2022-Energy
TL;DR: In this article, the authors evaluated potential solutions to Pakistan's energy shortages based on a renewable green hydrogen source provided by geothermal, wind, biomass, and solar energy, and concluded that the efficiency of wind energy sources is best adapted to produce hydrogen energy for all four criteria in Pakistan.

74 citations


Journal ArticleDOI
TL;DR: This paper provides a comprehensive review of blind deconvolution methods from history to state-of-the-art methods and finally to research prospects, as well as provides a survey and summarize the current progress of BDMs applied in machinery fault diagnosis.

72 citations


Journal ArticleDOI
TL;DR: ZIF-8@Ti3C2Tx was synthesized to reduce the heat and toxic gases of flexible polyurethane foam (FPUF) as mentioned in this paper, which was characterized by cone calorimeter (Cone), thermogravimetric analysis/fourier transform infrared spectroscopy (TG-FTIR), tensileand compression tests.

71 citations


Journal ArticleDOI
TL;DR: The researches show that BN-OH/ZIF-8/PA not only uniformly distributed in EP matrix, but also improve the thermal stability of EP and the peak heat release rate, peak smoke production rate, total smoke production values, the fire growth index and peak CO production rate obtained from cone test are significantly decreased, demonstrating the reduction of the fire hazards of EP composites containing BN.

Journal ArticleDOI
TL;DR: In this article , a non-uniform angled fin type considering the optimization by the nonuniform arrangement and angled fins with small angles was proposed to improve thermal properties and melting uniformity.

Journal ArticleDOI
TL;DR: In this article, the authors present representative and latest research progress of improving CDT antitumor effects, involving the amplification strategy of oxidative stress triggered by endogenous/exogenous stimuli.

Journal ArticleDOI
TL;DR: In this article , the authors present representative and latest research progress of improving CDT antitumor effects, involving the amplification strategy of oxidative stress triggered by endogenous/exogenous stimuli.

Journal ArticleDOI
TL;DR: In this article , a self-healing composite was successfully synthesized through ring-opening reaction and a micro-arc oxidation (MAO) coating was grown on AZ31 beforehand, the composite was doped into the layered double hydroxides (LDHs) sheet by hydrothermal chemical transformation based on the MAO coating without introducing any kind of salts.

Journal ArticleDOI
TL;DR: In this article, the development of Sb2Se3-based photocathodes in PEC water splitting with various architectures and engineering efforts (i.e., absorber engineering, interfaces engineering, co-catalyst engineering and tandem engineering) to improve solar-to-hydrogen (STH) efficiency are highlighted.

Journal ArticleDOI
TL;DR: In this paper, an 8-hydroxyquinoline@graphene oxide (8-HQ@GO) composite was successfully synthesized through ring-opening reaction and a micro-arc oxidation (MAO) coating was grown on AZ31 beforehand.

Journal ArticleDOI
TL;DR: In this paper , the authors presented an experimental quantum key distribution (QKD) system that could tolerate a channel loss beyond 140 dB and obtain a secure distance of 833.8 km, setting a new record for fibre-based QKD.
Abstract: Quantum key distribution (QKD) provides a promising solution for sharing information-theoretic secure keys between remote peers with physics-based protocols. According to the law of quantum physics, the photons carrying signals cannot be amplified or relayed via classical optical techniques to maintain quantum security. As a result, the transmission loss of the channel limits its achievable distance, and this has been a huge barrier towards building large-scale quantum-secure networks. Here we present an experimental QKD system that could tolerate a channel loss beyond 140 dB and obtain a secure distance of 833.8 km, setting a new record for fibre-based QKD. Furthermore, the optimized four-phase twin-field protocol and high-quality set-up make its secure key rate more than two orders of magnitude greater than previous records over similar distances. Our results mark a breakthrough towards building reliable and efficient terrestrial quantum-secure networks over a scale of 1,000 km. Twin-field (TF) quantum key distribution (QKD) over a secure distance of 833.8 km is demonstrated even in the finite-size regime. To this end, an optimized four-phase TF-QKD protocol and a high-speed low-noise TF-QKD system are developed.

Journal ArticleDOI
01 Jan 2022-Energy
TL;DR: In this paper , the authors evaluated potential solutions to Pakistan's energy shortages based on a renewable green hydrogen source provided by geothermal, wind, biomass, and solar energy, and concluded that wind energy is the most efficient source to produce hydrogen energy.

Journal ArticleDOI
TL;DR: Wang et al. as mentioned in this paper used input-output model and multi-regional input output model to account for the carbon footprint of nine provinces in the Yellow River Basin, and to estimate the amount of embodied carbon transfer between provinces and industrial sectors.

Journal ArticleDOI
TL;DR: Wang et al. as mentioned in this paper used input-output model and multi-regional inputoutput model to account for the carbon footprint of nine provinces in the Yellow River Basin, and to estimate the amount of embodied carbon transfer between provinces and industrial sectors.

Journal ArticleDOI
TL;DR: In this paper, an effective metal-organic framework adsorbent was fabricated by grafting thioglycollic acid on MOF-808 for Hg(II) removal, which demonstrated high adsorption capacity of 977.5

Journal ArticleDOI
TL;DR: In this paper, a four layer networked architecture of cloud-side-end collaboration for battery management system is presented which breaks through the computing capacity and storage space limitations of the conventional battery management and enables high performance algorithms.

Journal ArticleDOI
TL;DR: In this paper , a four layer networked architecture of cloud-side-end collaboration for battery management system is presented which breaks through the computing capacity and storage space limitations of the conventional battery management and enables high performance algorithms.

DOI
01 Feb 2022
TL;DR: In this article, the challenges and limitations of the battery chemistry in low temperature environments, as well as the development of low-temperature battery chemistry from cell level to system level are reviewed.
Abstract: : Lithium-ion batteries (LIBs) play a vital role in portable electronic products, transportation and large-scale energy storage. However, the electrochemical performance of LIBs deteriorates severely at low temperatures, exhibiting significant energy and power loss, charging difficulty, lifetime degradation, and safety issue, which has become one of the biggest challenges for LIBs. This article aims to review challenges and limitations of the battery chemistry in low-temperature environments, as well as the development of low-temperature LIBs from cell level to system level. This review introduces feasible solutions to accelarate low-temperature kinetics by increasing the inherent reactivity from cell design and improving the external reaction temperature from heating techniques. In addition, real-time and accurate monitoring of the battery temperature for the battery thermal management, as well as the optimization of charging protocols and the online lithium-plating monitoring in battery management systems are outlined. In general, a systematic review of low-temperature LIBs is conducted in order to provide references for future research.

Journal ArticleDOI
TL;DR: In this article , the challenges and limitations of the battery chemistry in low temperature environments, as well as the development of low-temperature battery chemistry from cell level to system level are reviewed.

Journal ArticleDOI
TL;DR: A comprehensive review of blind deconvolution methods for machinery fault detection can be found in this article , where the authors provide a comprehensive review from history to state-of-the-art methods.

Journal ArticleDOI
TL;DR: In this paper, an in-situ characterization of the gas evolution on the air electrode is conducted by in situ characterization and it is found that the charging process can be divided into three stages: no obvious bubbles, small bubbles, and large bubbles owing to oxygen evolution and carbon corrosion.

Journal ArticleDOI
TL;DR: In this article , tiny Pd3 Cu nanoparticles are confined into a metal-organic framework (MOF), UiO-66, to afford a methanol production rate of 340 μmol g-1 h-1 at 200 °C and 1.25 MPa under light irradiation, far surpassing that in the dark.
Abstract: CO2 hydrogenation to methanol has attracted great interest while suffering from low conversion and high energy input. Herein, tiny Pd3 Cu nanoparticles are confined into a metal-organic framework (MOF), UiO-66, to afford Pd3 Cu@UiO-66 for CO2 hydrogenation. Remarkably, it achieves a methanol production rate of 340 μmol g-1 h-1 at 200 °C and 1.25 MPa under light irradiation, far surpassing that in the dark. The photo-generated electron transfer from the MOF to antibonding orbitals of CO2 * promotes CO2 activation and HCOO* formation. In addition, the Pd3 Cu microenvironment plays a critical role in CO2 hydrogenation. In contrast to the MOF-supported Pd3 Cu (Pd3 Cu/UiO-66), the Pd3 Cu@UiO-66 exhibits a much higher methanol production rate due to the close proximity between CO2 and H2 activation sites, which greatly facilitates their interaction and conversion. This work provides a new avenue to the integration of solar and thermal energy for efficient CO2 hydrogenation under moderate conditions.

Journal ArticleDOI
TL;DR: In this paper, an immunoregulatory hydrogel scaffold was developed for treating spinal cord injury that scavenged DAMPs and slowly released the anti-inflammatory cytokine interleukin-10 (IL-10).