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Showing papers in "Applied Physics Letters in 2004"


Journal ArticleDOI
TL;DR: In this paper, ZnO nanowires gas sensors were fabricated with microelectromechanical system technology and ethanol-sensing characteristics were investigated, and the sensor exhibited high sensitivity and fast response to ethanol gas at a work temperature of 300°C.
Abstract: Based on the achievement of synthesis of ZnO nanowires in mass production, ZnO nanowires gas sensors were fabricated with microelectromechanical system technology and ethanol-sensing characteristics were investigated. The sensor exhibited high sensitivity and fast response to ethanol gas at a work temperature of 300 °C. Our results demonstrate the potential application of ZnO nanowires for fabricating highly sensitive gas sensors.

1,938 citations


Journal ArticleDOI
TL;DR: In this paper, the authors reported high performance ZnO thin-film transistor (ZnO-TFT) fabricated by rf magnetron sputtering at room temperature with a bottom gate configuration.
Abstract: We report high-performance ZnO thin-film transistor (ZnO-TFT) fabricated by rf magnetron sputtering at room temperature with a bottom gate configuration. The ZnO-TFT operates in the enhancement mode with a threshold voltage of 19V, a saturation mobility of 27cm2∕Vs, a gate voltage swing of 1.39V∕decade and an on/off ratio of 3×105. The ZnO-TFT presents an average optical transmission (including the glass substrate) of 80% in the visible part of the spectrum. The combination of transparency, high mobility, and room-temperature processing makes the ZnO-TFT a very promising low-cost optoelectronic device for the next generation of invisible and flexible electronics.

1,499 citations


Journal ArticleDOI
TL;DR: In this paper, the Brownian motion of nanoparticles at the molecular and nanoscale level is a key mechanism governing the thermal behavior of nanoparticle-fluid suspensions (nanofluids).
Abstract: We have found that the Brownian motion of nanoparticles at the molecular and nanoscale level is a key mechanism governing the thermal behavior of nanoparticle–fluid suspensions (“nanofluids”). We have devised a theoretical model that accounts for the fundamental role of dynamic nanoparticles in nanofluids. The model not only captures the concentration and temperature-dependent conductivity, but also predicts strongly size-dependent conductivity. Furthermore, we have discovered a fundamental difference between solid/solid composites and solid/liquid suspensions in size-dependent conductivity. This understanding could lead to design of nanoengineered next-generation coolants with industrial and biomedical applications in high-heat-flux cooling.

1,459 citations


Journal ArticleDOI
TL;DR: In this paper, an n-side-up GaN-based LED with a hexagonal "conelike" surface has been fabricated by using the laser lift-off technique followed by an anisotropic etching process to roughen the surface.
Abstract: Roughened surfaces of light-emitting diodes (LEDs) provide substantial improvement in light extraction efficiency. By using the laser-lift-off technique followed by an anisotropic etching process to roughen the surface, an n-side-up GaN-based LED with a hexagonal “conelike” surface has been fabricated. The enhancement of the LED output power depends on the surface conditions. The output power of an optimally roughened surface LED shows a twofold to threefold increase compared to that of an LED before surface roughening.

1,412 citations


Journal ArticleDOI
TL;DR: In this article, a morphotropic phase boundary between orthorhombic and tetragonal phases is found in the composition range 0.05
Abstract: Lead-free piezoelectric ceramics (1−x)(Na0.5K0.5)NbO3–xLiNbO3 {[Lix(Na0.5K0.5)1−x]NbO3} (x=0.04–0.20) have been synthesized by an ordinary sintering technique. The materials with perovskite structure is orthorhombic phase at x⩽0.05 and becomes tetragonal phase at x⩾0.07, a phase K3Li2Nb5O15 with tetragonal tungsten bronze structure begins to appear at x=0.08 and becomes dominant with increasing the content of LiNbO3. A morphotropic phase boundary between orthorhombic and tetragonal phases is found in the composition range 0.05

1,354 citations


Journal ArticleDOI
TL;DR: In this article, the authors investigated carrier transport in a crystalline oxide semiconductor InGaO3(ZnO)5 using single-crystalline thin films and showed that when carrier concentration is less than 2×1018cm−3, logarithm of electrical conductivity decreases in proportion to T−1∕4 and room-temperature Hall mobility was as low as ∼1cm2(Vs)−1.
Abstract: We have investigated carrier transport in a crystalline oxide semiconductor InGaO3(ZnO)5 using single-crystalline thin films. When carrier concentration is less than 2×1018cm−3, logarithm of electrical conductivity decreases in proportion to T−1∕4 and room-temperature Hall mobility was as low as ∼1cm2(Vs)−1. When carrier concentration was increased to 4×1018cm−3, the conduction mechanism changed to degenerate conduction and room-temperature Hall mobility was steeply increased to >10cm2(Vs)−1, showing metal–insulator transition behavior. These results are explained by percolation conduction over distribution of potential barriers formed around conduction band edge. The potential distribution is a consequence of potential modulation originating from random distribution of Ga3+ and Zn2+ ions in the crystal structure of InGaO3(ZnO)5.

1,232 citations


Journal ArticleDOI
TL;DR: In this paper, it was demonstrated that two immiscible liquids in a tube form a self-centered lens with a high optical quality, and the motion of the lens during a focusing action was studied by observation through the transparent tube wall.
Abstract: The meniscus between two immiscible liquids can be used as an optical lens. A change in curvature of this meniscus by electrowetting leads to a change in focal distance. It is demonstrated that two liquids in a tube form a self-centered lens with a high optical quality. The motion of the lens during a focusing action was studied by observation through the transparent tube wall. Finally, a miniature achromatic camera module was designed and constructed based on this adjustable lens, showing that it is excellently suited for use in portable applications.

1,061 citations


Journal ArticleDOI
TL;DR: In this article, a single-phased ferroelectromagnet BiFeO3 ceramics with high resistivity were synthesized by a rapid liquid phase sintering technique.
Abstract: Single-phased ferroelectromagnet BiFeO3 ceramics with high resistivity were synthesized by a rapid liquid phase sintering technique. Saturated ferroelectric hysteresis loops were observed at room temperature in the ceramics sintered at 880 °C for 450 s. The spontaneous polarization, remnant polarization, and the coercive field are 8.9 μC/cm2, 4.0 μC/cm2, and 39 kV/cm, respectively, under an applied field of 100 kV/cm. It is proposed that the formation of Fe2+ and an oxygen deficiency leading to the higher leakage can be greatly suppressed by the very high heating rate, short sintering period, and liquid phase sintering technique. The latter was also found effective in increasing the density of the ceramics. The sintering technique developed in this work is expected to be useful in synthesizing other ceramics from multivalent or volatile starting materials.

970 citations


Journal ArticleDOI
TL;DR: Martensitic and magnetic transformations of the Heusler Ni50Mn50−yXy (X=In, Sn and Sb) alloys were investigated by differential scanning calorimetry measurement and the vibrating sample magnetometry technique.
Abstract: Martensitic and magnetic transformations of the Heusler Ni50Mn50−yXy (X=In, Sn and Sb) alloys were investigated by differential scanning calorimetry measurement and the vibrating sample magnetometry technique. In all these alloy systems, the austenite phase with the ferromagnetic state was transformed into the martensite phase, which means that these Heusler alloys have potential as Ga-free ferromagnetic shape memory alloys (FSMAs). Furthermore, multiple martensitic transformations, such as two- or three-step martensitic transformations, occur in all these alloy systems. It was confirmed by transmission electron microscopy observation that the crystal structure of the martensite phase is an orthorhombic four-layered structure which has not been reported in other FSMAs. Therefore, the present Ga-free FSMAs have the great possibility of the appearance of a large magnetic-field-induced strain.

968 citations


Journal ArticleDOI
TL;DR: Negative resistance behavior and reproducible resistance switching were found in polycrystalline NiO films deposited by dc magnetron reactive sputtering methods in this paper, where the negative resistance and the switching mechanism could be described by electron conduction related to metallic nickel defect states existing in deep levels and by small polaron hole hopping conduction.
Abstract: Negative resistance behavior and reproducible resistance switching were found in polycrystalline NiO films deposited by dc magnetron reactive sputtering methods. Oxygen to argon gas ratio during deposition was critical in deciding the detailed switching characteristics of either bi-stable memory switching or mono-stable threshold switching. Both metallic nickel defects and nickel vacancies influenced the negative resistance and the switching characteristics. We obtained a distribution of low resistance values which were dependent on the compliance current of high-to-low resistance switching. At 200°C, the low-resistance state kept its initial resistance value while the high-resistance state reached 85% of its initial resistance value after 5×105s. We suggested that the negative resistance and the switching mechanism could be described by electron conduction related to metallic nickel defect states existing in deep levels and by small-polaron hole hopping conduction.

960 citations


Journal ArticleDOI
TL;DR: In this article, Ferromagnetic coupling of ferric ions via an electron trapped in a bridging oxygen vacancy (F center) is proposed to explain the high Curie temperature.
Abstract: Thin films grown by pulsed-laser deposition from targets of Sn0.95Fe0.05O2 are transparent ferromagnets with Curie temperature and spontaneous magnetization of 610 K and 2.2 A m2 kg−1, respectively. The 57Fe Mossbauer spectra show the iron is all high-spin Fe3+ but the films are magnetically inhomogeneous on an atomic scale, with only 23% of the iron ordering magnetically. The net ferromagnetic moment per ordered iron ion, 1.8 μB, is greater than for any simple iron oxide with superexchange interactions. Ferromagnetic coupling of ferric ions via an electron trapped in a bridging oxygen vacancy (F center) is proposed to explain the high Curie temperature.

Journal ArticleDOI
TL;DR: In this article, the hole mobility for the organic conductor pentacene was obtained at room temperature and at 225 K. The number of traps was reduced by two orders of magnitude compared with conventional methods.
Abstract: We have obtained a hole mobility for the organic conductor pentacene of μ=35 cm2/V s at room temperature increasing to μ=58 cm2/V s at 225 K. These high mobilities result from a purification process in which 6,13-pentacenequinone was removed by vacuum sublimation. The number of traps is reduced by two orders of magnitude compared with conventional methods. The temperature dependence of the mobility is consistent with the band model for electronic transport.

Journal ArticleDOI
TL;DR: In this paper, single-crystal ZnO nanowires are synthesized using a vapor trapping chemical vapor deposition method and configured as field effect transistors, and electrical transport studies show n-type semiconducting behavior with a carrier concentration of ∼107cm−1 and an electron mobility of ∼17cm2∕Vs.
Abstract: Single-crystal ZnO nanowires are synthesized using a vapor trapping chemical vapor deposition method and configured as field-effect transistors. Electrical transport studies show n-type semiconducting behavior with a carrier concentration of ∼107cm−1 and an electron mobility of ∼17cm2∕Vs. The contact Schottky barrier between the Au/Ni electrode and nanowire is determined from the temperature dependence of the conductance. Thermionic emission is found to dominate the transport mechanism. The effect of oxygen adsorption on electron transport through the nanowires is investigated. The sensitivity to oxygen is demonstrated to be higher with smaller radii nanowires. Moreover, the oxygen detection sensitivity can be modulated by the gate voltage. These results indicate that ZnO holds high potential for nanoscale sensing applications.

Journal ArticleDOI
TL;DR: In this article, the authors used Discovery Research Grant from the Australian Research Council (ARCC) to support a study on the effect of the weather on the performance of the AAF.
Abstract: This study was supported in part by a Discovery Research Grant from the Australian Research Council.

Journal ArticleDOI
TL;DR: In this article, a simple formula for the thermal conductivity enhancement in carbon nanotube composites is presented by incorporating the interface thermal resistance with an effective medium approach, which predicts that a large interface thermal sensitivity across the nanotubes-matrix interface causes a significant degradation in the thermal performance.
Abstract: A simple formula for the thermal conductivity enhancement in carbon nanotube composites is presented by incorporating the interface thermal resistance with an effective medium approach. This model well describes the thermal conductivity enhancement observed recently in nanotube suspensions. In particular, this simple formula predicts that a large interface thermal resistance across the nanotube-matrix interface causes a significant degradation in the thermal conductivity enhancement, even for the case with ultrahigh intrinsic thermal conductivity and aspect ratio of the carbon nanotubes embedded.

Journal ArticleDOI
TL;DR: In this article, the vertical transport properties of epitaxial layered structures composed of Pr0.7Ca0.3MnO3(PCMO) sandwiched between SrRuO3 (SRO) bottom electrode and several kinds of top electrodes such as SRO, Pt, Au, Ag, and Ti are characterized.
Abstract: We have characterized the vertical transport properties of epitaxial layered structures composed of Pr0.7Ca0.3MnO3(PCMO) sandwiched between SrRuO3(SRO) bottom electrode and several kinds of top electrodes such as SRO, Pt, Au, Ag, and Ti. Among the layered structures, Ti∕PCMO∕SRO is distinct due to a rectifying I–V characteristic with a large hysteresis. Corresponding to the hysteresis of the I–V characteristics, the contact resistance of the Ti∕PCMO interface reversibly switches between two stable states by applying pulsed voltage stress. We propose a model for the resistance switching at the Ti∕PCMO interface, in which the width and/or height of a Schottky-like barrier are altered by trapped charge carriers in the interface states.

Journal ArticleDOI
TL;DR: In this paper, a method of iterative phase retrieval that uses measured intensities in the diffraction plane to solve the phase problem in a way that bypasses the problem of lens aberration was proposed.
Abstract: We propose a method of iterative phase retrieval that uses measured intensities in the diffraction plane to solve the phase problem in a way that bypasses the problem of lens aberration, leading to greatly improved spatial resolution. This method is stable, easy to implement experimentally, and can be used to view a large area of the specimen when that is desired.

Journal ArticleDOI
TL;DR: In this paper, a fabricated white-light emitting diode using a 400nm-emissive chip with a white light emitting Ba3MgSi2O8:Eu2+, Mn2+ phosphor shows warm white light and higher color stability against input power in comparison with a commercial GaN-pumped (Y1−xGdx)3(Al1−yGay)5O12:Ce3+osphor.
Abstract: The Ba3MgSi2O8:Eu2+, Mn2+ shows three emission colors: 442, 505, and 620 nm. The 442 and 505 nm emission originate from Eu2+ ions, while the 620 nm emission originates from Mn2+ ions. The excitation bands of three emission colors are positioned around 375 nm. Electron paramagnetic resonance measurement demonstrates that Eu2+ ions are occupied with three different Ba2+ sites. The red emission of Mn2+ ions has a long decay time of 750 ms due to persistent energy transfer from oxygen vacancies to Mn2+ ions, while the blue and green bands of Eu2+ ions have decay times of 0.32 and 0.64 μs, respectively. The fabricated white-light emitting diode using a 400-nm-emissive chip with a white-light emitting Ba3MgSi2O8:Eu2+, Mn2+ phosphor shows warm white light and higher color stability against input power in comparison with a commercial GaN-pumped (Y1−xGdx)3(Al1−yGay)5O12:Ce3+ phosphor.

Journal ArticleDOI
TL;DR: In this paper, a method for generating monodisperse gaseous bubbles in a microfluidic flow-focusing device is described, where bubbles self-assemble into highly ordered, flowing lattices.
Abstract: This letter describes a method for generating monodisperse gaseous bubbles in a microfluidic flow-focusing device. The bubbles can be obtained in a range of diameters from 10 to 1000μm. The volume Vb of the bubbles scales with the flow rate q and the viscosity μ of the liquid, and the pressure p of the gas stream as Vb∝p∕qμ. This method allows simultaneous, independent control of the size of the individual bubbles and volume fraction of the dispersed phase. Under appropriate conditions, bubbles self-assemble into highly ordered, flowing lattices. Structures of these lattices can be adjusted dynamically by changing the flow parameters.

Journal ArticleDOI
TL;DR: In this paper, the authors present simple yet accurate formulas that enable the interaction force and energy to be determined directly from the measured frequency shift for any oscillation amplitude and interaction force, and are therefore of widespread applicability in frequency modulation dynamic force spectroscopy.
Abstract: Frequency modulation atomic force microscopy utilizes the change in resonant frequency of a cantilever to detect variations in the interaction force between cantilever tip and sample. While a simple relation exists enabling the frequency shift to be determined for a given force law, the required complementary inverse relation does not exist for arbitrary oscillation amplitudes of the cantilever. In this letter we address this problem and present simple yet accurate formulas that enable the interaction force and energy to be determined directly from the measured frequency shift. These formulas are valid for any oscillation amplitude and interaction force, and are therefore of widespread applicability in frequency modulation dynamic force spectroscopy.

Journal ArticleDOI
TL;DR: In this paper, the authors reported a quantum key distribution over a standard telecom fiber exceeding 100 km in length with a quantum bit error ratio of 8.9% for a 122 km link, allowing a secure shared key to be formed after error correction and privacy amplification.
Abstract: We report a demonstration of quantum key distribution over a standard telecom fiber exceeding 100 km in length. Through careful optimization of the interferometer and single photon detector, we achieve a quantum bit error ratio of 8.9% for a 122 km link, allowing a secure shared key to be formed after error correction and privacy amplification. Key formation rates of up to 1.9 kbit/s are achieved depending upon fiber length. We discuss the factors limiting the maximum fiber length in quantum cryptography.

Journal ArticleDOI
TL;DR: In this article, a double-emission layer (D-EML) was incorporated into p-i-n-type cell architecture to achieve high-efficiency organic light-emitting diodes.
Abstract: We demonstrate high-efficiency organic light-emitting diodes by incorporating a double-emission layer (D-EML) into p‐i‐n-type cell architecture. The D-EML is comprised of two layers with ambipolar transport characteristics, both doped with the green phosphorescent dye tris(phenylpyridine)iridium. The D-EML system of two bipolar layers leads to an expansion of the exciton generation region. Due to its self-balancing character, accumulation of charge carriers at the outer interfaces is avoided. Thus, a power efficiency of approximately 77 lm∕W and an external quantum efficiency of 19.3% are achieved at 100cd∕m2 with an operating voltage of only 2.65 V. More importantly, the efficiency decays only weakly with increasing brightness, and a power efficiency of 50 lm∕W is still obtained even at 4000cd∕m2.

Journal ArticleDOI
TL;DR: In this paper, the authors report advances in nano-print lithography, its application in nanogap metal contacts, and related fabrication yield, and demonstrate 5nm linewidth and 14nm linepitch in resist using nanoimprint at room temperature with a pressure less than 15psi.
Abstract: We report advances in nanoimprint lithography, its application in nanogap metal contacts, and related fabrication yield. We have demonstrated 5nm linewidth and 14nm linepitch in resist using nanoimprint lithography at room temperature with a pressure less than 15psi. We fabricated gold contacts (for the application of single macromolecule devices) with 5nm separation by nanoimprint in resist and lift-off of metal. Finally, the uniformity and manufacturability of nanoimprint over a 4in. wafer were demonstrated.

Journal ArticleDOI
TL;DR: In this article, the authors report design, fabrication, and characterization of thermo-optic Mach-Zender interferometric modulators and directional-coupler switches whose operation utilizes the long-range surface-plasmon-polariton waveguiding along 15nm-thin and 8μm-wide gold stripes embedded in polymer and heated by electrical signal currents.
Abstract: We report design, fabrication, and characterization of thermo-optic Mach–Zender interferometric modulators and directional-coupler switches whose operation utilizes the long-range surface-plasmon-polariton waveguiding along 15-nm-thin and 8-μm-wide gold stripes embedded in polymer and heated by electrical signal currents. The devices are characterized at the light wavelength of 1.55 μm, featuring low driving powers ( 30dB), moderate response times (∼1ms), and the total (fiber-to-fiber) insertion loss of ∼13dB (for modulators) and ∼11dB (for switches) when using single-mode fibers.

Journal ArticleDOI
TL;DR: In this paper, the properties of the fabricated nanostructures were studied using scanning electron microscopy, x-ray diffraction, photoluminescence, and electron paramagnetic resonance (EPR) spectroscopy.
Abstract: We prepared ZnO nanostructures using chemical and thermal evaporation methods. The properties of the fabricated nanostructures were studied using scanning electron microscopy, x-ray diffraction, photoluminescence, and electron paramagnetic resonance (EPR) spectroscopy. It was found that the luminescence in the visible region has different peak positions in samples prepared by chemical and evaporation methods. The samples fabricated by evaporation exhibited green luminescence due to surface centers, while the samples fabricated by chemical methods exhibited yellow luminescence which was not affected by the surface modification. No relationship was found between green emission and g∼1.96 EPR signal, while the sample with yellow emission exhibited strong EPR signal.

Journal ArticleDOI
TL;DR: In this paper, a modulated flux of atoms was adsorbed upon the surface of a 32.8 MHz NEMS resonator within an ultrahigh-vacuum environment, and the mass-induced resonance frequency shifts by these adsorbates were then measured to ascertain a mass sensitivity of 2.53×10−18g.
Abstract: We describe the application of nanoelectromechanical systems (NEMS) to ultrasensitive mass detection. In these experiments, a modulated flux of atoms was adsorbed upon the surface of a 32.8 MHz NEMS resonator within an ultrahigh-vacuum environment. The mass-induced resonance frequency shifts by these adsorbates were then measured to ascertain a mass sensitivity of 2.53×10^–18 g. In these initial measurements, this sensitivity is limited by the noise in the NEMS displacement transducer; the ultimate limits of the technique are set by fundamental phase noise processes. Our results and analysis indicate that mass sensing of individual molecules will be realizable with optimized NEMS devices.

Journal ArticleDOI
TL;DR: In this paper, the core physics assembly of an atomic clock is used to reduce the size and operating power of the core assembly of the atomic clock, and a volume of 9.5mm3, a fractional frequency instability of 2.5×10−10 at 1s of integration, and dissipating less than 75mW of power.
Abstract: Fabrication techniques usually applied to microelectromechanical systems (MEMS) are used to reduce the size and operating power of the core physics assembly of an atomic clock. With a volume of 9.5mm3, a fractional frequency instability of 2.5×10−10 at 1s of integration, and dissipating less than 75mW of power, the device has the potential to bring atomically precise timing to hand-held, battery-operated devices. In addition, the design and fabrication process allows for wafer-level assembly of the structures, enabling low-cost mass-production of thousands of identical units with the same process sequence, and easy integration with other electronics.

Journal ArticleDOI
TL;DR: In this paper, the origin of ferromagnetism in ZnO-based systems was investigated using Co-doped ZnOs thin films as prototypical examples of II-VI-based diluted magnetic semiconductors.
Abstract: The origin of ferromagnetism in ZnO-based systems was investigated using Co-doped ZnO thin films as prototypical examples of II–VI-based diluted magnetic semiconductors. In spite of the atomic-scale dissolution of Co ions in wurtzite ZnO, both the magnetization-temperature curve and the magnetization-field curve demonstrated that Zn1−xCoxO thin films were paramagnetic for x⩽0.12. On the other hand, Zn1−xCoxO films with x greater than 0.12 were characterized by the Co-metal clustering and apparently showed room-temperature ferromagnetism. The discrepancy between the zero-field cooling and the field cooling curves further indicates that Co-doped ZnO films (for x>0.12) are superparamagnetic and the observed ferromagnetism originates from the nanometer-sized Co clusters.

Journal ArticleDOI
TL;DR: In this article, two hybrid planar-mixed molecular heterojunction cells in series were used to achieve a power conversion efficiency of 5.7±0.3% under 1 sun simulated AM1.5G solar illumination.
Abstract: We demonstrate high-efficiency organic photovoltaic cells by stacking two hybrid planar-mixed molecular heterojunction cells in series. Absorption of incident light is maximized by locating the subcell tuned to absorb long-wavelength light nearest to the transparent anode, and tuning the second subcell closest to the reflecting metal cathode to preferentially absorb short-wavelength solar energy. Using the donor, copper phthalocyanine, and the acceptor, C60, we achieve a maximum power conversion efficiency of ηP=(5.7±0.3)% under 1 sun simulated AM1.5G solar illumination. An open-circuit voltage of VOC⩽1.2V is obtained, doubling that of a single cell. Analytical models suggest that power conversion efficiencies exceeding 6.5% can be obtained by this architecture.

Journal ArticleDOI
TL;DR: In this article, a yellow oxynitride phosphor α-SiAlON with compositions of Ca0.625EuxSi0.75−3xAl1.25+3xOxN16−x was prepared by gas pressure sintering and the diffuse reflection spectrum, photoluminescence spectrum, and chromaticity of the powder phosphors were presented.
Abstract: In this letter, a yellow oxynitride phosphor α-SiAlON with compositions of Ca0.625EuxSi0.75−3xAl1.25+3xOxN16−x (Ca-α-SiAlON:Eu, x=0–25) was prepared by gas pressure sintering. The diffuse reflection spectrum, photoluminescence spectrum, and chromaticity of the powder phosphors were presented. It absorbs light efficiently in the UV–visible spectral region, and shows a single intense broadband emission at 583–603nm. This phosphor may become a good candidate for creating white light, typically warm white light, when coupled to a blue light-emitting diode (λem=450nm).