Characterization and reduction of reabsorption losses in luminescent solar concentrators
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...As shown in Figure 3C, the spectral distribution of edge-emitted light shows negligible variation with increasing G, contrasting with the behavior of previously studied LSC luminophores where self-absorption produces a strong bathochromic shift in edge-emitted light with increasing G.(45) This result highlights the lack of self-absorption in doped nanocrystal LSCs....
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...In the absence of bulky substituents, such as phenoxy groups, in the bay area, perylene bisimides tend to form sandwich-typeH-aggregates [44], which show blueshifted absorption spectra and greatly reduced PLQYs, relative to the monomer....
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...Because of the energy transfer mechanism between their absorbing ligands and emitting ions [25,26], they can exhibit large Stokes shifts....
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...Luminescent solar concentrators (LSCs) [1–5] were proposed more than 30 years ago [5] as a nonimaging means of concentrating solar radiation....
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...With some of the excess photon energy being deposited in the LSC, rather than in the cells, this leads to higher cell efficiencies [5,6]....
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