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Highly crystalline 2D superconductors

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TLDR
In this article, a review of recent developments in the field of highly crystalline 2D superconductors is presented, highlighting the unprecedented physical properties of these systems, such as the Griffiths phase observed in out-of-plane magnetic fields and the superconducting state maintained in anomalously large in-plane inversion symmetry.
Abstract
Recent advances in materials fabrication have enabled the manufacturing of ordered 2D electron systems, such as heterogeneous interfaces, atomic layers grown by molecular beam epitaxy, exfoliated thin flakes and field-effect devices. These 2D electron systems are highly crystalline, and some of them, despite their single-layer thickness, exhibit a sheet resistance more than an order of magnitude lower than that of conventional amorphous or granular thin films. In this Review, we explore recent developments in the field of highly crystalline 2D superconductors and highlight the unprecedented physical properties of these systems. In particular, we explore the quantum metallic state (or possible metallic ground state), the quantum Griffiths phase observed in out-of-plane magnetic fields and the superconducting state maintained in anomalously large in-plane magnetic fields. These phenomena are examined in the context of weakened disorder and/or broken spatial inversion symmetry. We conclude with a discussion of how these unconventional properties make highly crystalline 2D systems promising platforms for the exploration of new quantum physics and high-temperature superconductors. Highly crystalline 2D superconductors can exhibit very low sheet resistances and unusual physical properties, such as a quantum metallic state, a quantum Griffiths phase and superconductivity robust against in-plane magnetic fields. The origins of these phenomena and the materials in which they are observed are reviewed.

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Unconventional superconductivity in magic-angle graphene superlattices

TL;DR: The realization of intrinsic unconventional superconductivity is reported—which cannot be explained by weak electron–phonon interactions—in a two-dimensional superlattice created by stacking two sheets of graphene that are twisted relative to each other by a small angle.
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A library of atomically thin metal chalcogenides

TL;DR: Molten-salt-assisted chemical vapour deposition is used to synthesize a wide variety of two-dimensional transition-metal chalcogenides and elaborate how the salt decreases the melting point of the reactants and facilitates the formation of intermediate products, increasing the overall reaction rate.
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Controlling magnetism in 2D CrI 3 by electrostatic doping

TL;DR: In this article, the magnetic properties of both monolayer and bilayer CrI3-graphene vertical heterostructures were demonstrated by electrostatic doping using CVD.
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Controlling magnetism in 2D CrI3 by electrostatic doping

TL;DR: In monolayer CrI3, doping significantly modifies the saturation magnetization, coercive force and Curie temperature, showing strengthened/weakened magnetic order with hole/electron doping, and the result reveals a strongly doping-dependent interlayer exchange coupling, which enables robust switching of magnetization in bilayerCrI3 by small gate voltages.
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Nonreciprocal responses from non-centrosymmetric quantum materials.

TL;DR: A variety of directional electronic transport phenomena can occur in materials with broken inversion-symmetry, including the photocurrent of topological origin and the unidirectional magnetoresistance in polar/chiral semiconductors.
References
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Journal ArticleDOI

Electric Field Effect in Atomically Thin Carbon Films

TL;DR: Monocrystalline graphitic films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands and they exhibit a strong ambipolar electric field effect.
Journal ArticleDOI

The rise of graphene

TL;DR: Owing to its unusual electronic spectrum, graphene has led to the emergence of a new paradigm of 'relativistic' condensed-matter physics, where quantum relativistic phenomena can now be mimicked and tested in table-top experiments.
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Electronics and optoelectronics of two-dimensional transition metal dichalcogenides.

TL;DR: This work reviews the historical development of Transition metal dichalcogenides, methods for preparing atomically thin layers, their electronic and optical properties, and prospects for future advances in electronics and optoelectronics.
Journal ArticleDOI

Topological insulators and superconductors

TL;DR: Topological superconductors are new states of quantum matter which cannot be adiabatically connected to conventional insulators and semiconductors and are characterized by a full insulating gap in the bulk and gapless edge or surface states which are protected by time reversal symmetry.
Journal ArticleDOI

Two-dimensional atomic crystals

TL;DR: By using micromechanical cleavage, a variety of 2D crystals including single layers of boron nitride, graphite, several dichalcogenides, and complex oxides are prepared and studied.
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