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Highly Thermally Conductive Papers with Percolative Layered Boron Nitride Nanosheets

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TLDR
A dielectric nanocomposite paper with layered boron nitride (BN) nanosheets wired by one-dimensional (1D) nanofibrillated cellulose (NFC) that has superior thermal and mechanical properties is reported.
Abstract
In this work, we report a dielectric nanocomposite paper with layered boron nitride (BN) nanosheets wired by one-dimensional (1D) nanofibrillated cellulose (NFC) that has superior thermal and mechanical properties. These nanocomposite papers are fabricated from a filtration of BN and NFC suspensions, in which NFC is used as a stabilizer to stabilize BN nanosheets. In these nanocomposite papers, two-dimensional (2D) nanosheets form a thermally conductive network, while 1D NFC provides mechanical strength. A high thermal conductivity has been achieved along the BN paper surface (up to 145.7 W/m K for 50 wt % of BN), which is an order of magnitude higher than that in randomly distributed BN nanosheet composites and is even comparable to the thermal conductivity of aluminum alloys. Such a high thermal conductivity is mainly attributed to the structural alignment within the BN nanosheet papers; the effects of the interfacial thermal contact resistance are minimized by the fact that the heat transfer is in the ...

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Citations
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Journal ArticleDOI

Recent development in 2D materials beyond graphene

TL;DR: In this article, a review highlights the recent progress of the state-of-the-art research on synthesis, characterization and isolation of single and few layer nanosheets and their assembly.
Journal ArticleDOI

Wood-Derived Materials for Green Electronics, Biological Devices, and Energy Applications.

TL;DR: The goal of this study is to review the fundamental structures and chemistries of wood and wood-derived materials, which are essential for a wide range of existing and new enabling technologies.
Journal ArticleDOI

Functionalized hexagonal boron nitride nanomaterials: emerging properties and applications.

TL;DR: An overview of the progress in functionalized hexagonal boron nitride (h-BN) nanomaterials can be found in this paper, where different functionalization methods, including physical and chemical routes, are comprehensively described toward fabrication of various BN derivatives, hetero- and porous structures, etc.
Journal ArticleDOI

Binary Strengthening and Toughening of MXene/Cellulose Nanofiber Composite Paper with Nacre-Inspired Structure and Superior Electromagnetic Interference Shielding Properties

TL;DR: The nacre-inspired strategy in this study offers a promising approach for the design and preparation of the strong integrated and flexible MXene/CNF composite paper, which may be applied in various fields such as flexible wearable devices, weapon equipment, and robot joints.
Journal ArticleDOI

High-performance green flexible electronics based on biodegradable cellulose nanofibril paper

TL;DR: Successful fabrication of key electrical components on the flexible cellulose nanofibril paper with comparable performance to their rigid counterparts and clear demonstration of fungal biodegradation of the cellulose-nan ofibril-based electronics suggest that it is feasible to fabricate high-performance flexible electronics using ecofriendly materials.
References
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Journal ArticleDOI

Boron nitride substrates for high-quality graphene electronics

TL;DR: Graphene devices on h-BN substrates have mobilities and carrier inhomogeneities that are almost an order of magnitude better than devices on SiO(2).
Journal ArticleDOI

Cellulose nanomaterials review: structure, properties and nanocomposites

TL;DR: This critical review provides a processing-structure-property perspective on recent advances in cellulose nanoparticles and composites produced from them, and summarizes cellulOSE nanoparticles in terms of particle morphology, crystal structure, and properties.
Journal ArticleDOI

Microfibrillated cellulose and new nanocomposite materials: a review

TL;DR: In this article, a review summarizes progress in nanocellulose preparation with a particular focus on microfibrillated cellulose and also discusses recent developments in bio-nanocomposite fabrication based on nanocells.
Journal ArticleDOI

Thermal conductivity of carbon nanotubes and their polymer nanocomposites: A review

TL;DR: In this article, the status of worldwide research in the thermal conductivity of carbon nanotubes and their polymer nanocomposites is reviewed, as well as the relationship between thermal conductivities and the micro- and nano-structure of the composites.
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