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Joint Temperature-Volume Fraction Statistics of Soot in Turbulent Non-Premixed Jet Flames of Ethylene and a JP-8 Surrogate.

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TLDR
In this article, a 3-line approach to simultaneous measurement of soot concentration (on the basis of laser extinction) and soot temperature was proposed, which relies on the presence of significant laser attenuation to yield accurate measurements.
Abstract
Soot emissions from internal combustion engines and aviation gas turbine engines face increasingly stringent regulation, but available experimental datasets for sooting turbulent combustion model development and validation are largely lacking, in part due to the difficulty of making quantitative spaceand time-resolved measurements in this type of flame. To address this deficiency, we have performed a number of different laser and optical diagnostic measurements in sooting, nonpremixed jet flames fueled by ethylene or a prevaporized JP-8 surrogate. Most laser diagnostic techniques inherently lose their quantitative rigor when significant laser beam and signal attenuation occur in sooting flames. However, the ‘3-line’ approach to simultaneous measurement of soot concentration (on the basis of laser extinction) and soot temperature (on the basis of 2-color pyrometry) actually relies on the presence of significant laser attenuation to yield accurate measurements. In addition, the 3-line approach yields complete time-resolved information. In the work reported here, we have implemented the 3-line diagnostic in well-controlled non-premixed ethylene and JP-8 jet flames with a fuel exit Reynolds number of 20,000 using tapered, uncooled alumina refractory probes with a 10 mm probe end separation. Bandpass filters with center wavelengths of 850 nm and 1000 nm were used for the pyrometry measurement, with calibration provided by a hightemperature blackbody source. Extinction of a 635 nm red diode laser beam was used to determine soot volume fraction. Data were collected along the flame centerline at many different heights and radial traverses were performed at selected heights. A data sampling rate of 5 kHz was used to resolve the turbulent motion of the soot. The results for the ethylene flame show a mean soot volume fraction of 0.4 ppm at mid-height of the flame, with a mean temperature of 1450 K. At any given instant, the soot volume fraction typically falls between 0.2 and 0.6 ppm with a temperature between 1300 and 1650 K. At greater heights in the flame, the soot intermittency increases and its mean concentration decreases while its mean temperature increases. In the JP-8 surrogate flame, the soot concentration reaches a mean value of 1.3 ppm at mid-height of the flame, but the mean soot temperature is only 1270 K. Elevated soot concentrations persist for a range of heights in the JP-8 flame, with a rise in mean temperature to 1360 K, before both soot volume fraction and temperature tail off at the top of this smoking flame.

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Citations
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Journal ArticleDOI

Simultaneous measurements of gas temperature, soot volume fraction and primary particle diameter in a sooting lifted turbulent ethylene/air non-premixed flame

TL;DR: In this paper, planar measurements of flame temperature, soot volume fraction, primary particle diameter and the derived number density of primary particles are reported in a lifted ethylene jet diffusion flame, both to increase confidence in measurement accuracy and provide new joint statistics.
Journal ArticleDOI

Two-dimensional flow effects on soot formation in laminar premixed flames

TL;DR: In this paper, a modified one-dimensional model is derived on the flame centerline to include two-dimensional effects, and the modified model is compared with detailed, twodimensional simulation results and experimental measurements.
Journal ArticleDOI

Two-dimensional temperature field imaging in laminar sooting flames using a two-line Kr PLIF approach

TL;DR: In this paper, a two-line Kr PLIF approach is presented for thermometry in moderately sooting flames, which leverages the spectral line-broadening phenomenon to choose the two excitation wavelengths whose KrPLIF signal ratio effectively cancels out the composition dependence while retaining the temperature dependence.
Journal ArticleDOI

Effects of large aromatic precursors on soot formation in turbulent non-premixed sooting jet flames

TL;DR: In this paper, the effects of large polycyclic aromatic hydrocarbons (PAH) on soot yield and distribution in turbulent flames, when they are used in fire extinguishing, were investigated.
Journal ArticleDOI

Large-Eddy Simulation and Analysis of a Sooting Lifted Turbulent Jet Flame

TL;DR: In this article, a large-Eddy simulation (LES) is performed for a lifted, lifted, well characterized, non-premixed, turbulent jet flame, where a finite-rate chemistry model is used to accurately predict the lifted flame, which requires no assumptions concerning the combustion regime.
References
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Aviation and the Global Atmosphere

TL;DR: In this paper, the authors present a comprehensive review and assessment of the global effects of aviation on the global atmosphere, including all gases and particulates emitted by aircraft and their role in modifying chemical properties in the atmosphere.
Journal ArticleDOI

Simultaneous measurements of gas temperature, soot volume fraction and primary particle diameter in a sooting lifted turbulent ethylene/air non-premixed flame

TL;DR: In this paper, planar measurements of flame temperature, soot volume fraction, primary particle diameter and the derived number density of primary particles are reported in a lifted ethylene jet diffusion flame, both to increase confidence in measurement accuracy and provide new joint statistics.
Journal ArticleDOI

Two-dimensional flow effects on soot formation in laminar premixed flames

TL;DR: In this paper, a modified one-dimensional model is derived on the flame centerline to include two-dimensional effects, and the modified model is compared with detailed, twodimensional simulation results and experimental measurements.
Journal ArticleDOI

Two-dimensional temperature field imaging in laminar sooting flames using a two-line Kr PLIF approach

TL;DR: In this paper, a two-line Kr PLIF approach is presented for thermometry in moderately sooting flames, which leverages the spectral line-broadening phenomenon to choose the two excitation wavelengths whose KrPLIF signal ratio effectively cancels out the composition dependence while retaining the temperature dependence.
Journal ArticleDOI

Effects of large aromatic precursors on soot formation in turbulent non-premixed sooting jet flames

TL;DR: In this paper, the effects of large polycyclic aromatic hydrocarbons (PAH) on soot yield and distribution in turbulent flames, when they are used in fire extinguishing, were investigated.
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