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Journal ArticleDOI

Monitoring of the Eyjafjallajökull volcanic aerosol plume over the Iberian Peninsula by means of four EARLINET lidar stations

TL;DR: In this article, the authors performed intensively over the Iberian Peninsula (IP) during the eruption of the Eyjafjallajokull volcano (Iceland) in April-May 2010.
Abstract: . Lidar and sun-photometer measurements were performed intensively over the Iberian Peninsula (IP) during the eruption of the Eyjafjallajokull volcano (Iceland) in April–May 2010. The volcanic plume reached all the IP stations for the first time on 5 May 2010. A thorough study of the event was conducted for the period 5–8 May. Firstly, the spatial and temporal evolution of the plume was described by means of lidar and sun-photometer measurements supported with backtrajectories. The volcanic aerosol layers observed over the IP were rather thin (

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Citations
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Journal ArticleDOI
TL;DR: The European Aerosol Research Lidar Network (EARLINET) as mentioned in this paper was founded as a research project for establishing a quantitative, comprehensive, and statistically significant database for the horizontal, vertical, and tempo-ral distribution of aerosols on a continental scale.
Abstract: The European Aerosol Research Lidar Network, EARLINET, was founded in 2000 as a research project for establishing a quantitative, comprehensive, and statistically significant database for the horizontal, vertical, and tempo- ral distribution of aerosols on a continental scale. Since then EARLINET has continued to provide the most extensive col- lection of ground-based data for the aerosol vertical distribu- tion over Europe. This paper gives an overview of the network's main de- velopments since 2000 and introduces the dedicated EAR- LINET special issue, which reports on the present innova- tive and comprehensive technical solutions and scientific re- sults related to the use of advanced lidar remote sensing tech- niques for the study of aerosol properties as developed within the network in the last 13 years. Since 2000, EARLINET has developed greatly in terms of number of stations and spatial distribution: from 17 sta- tions in 10 countries in 2000 to 27 stations in 16 countries in 2013. EARLINET has developed greatly also in terms of technological advances with the spread of advanced multi- wavelength Raman lidar stations in Europe. The develop- ments for the quality assurance strategy, the optimization of instruments and data processing, and the dissemination of data have contributed to a significant improvement of the net- work towards a more sustainable observing system, with an increase in the observing capability and a reduction of oper- ational costs. Consequently, EARLINET data have already been ex- tensively used for many climatological studies, long-range transport events, Saharan dust outbreaks, plumes from vol- canic eruptions, and for model evaluation and satellite data validation and integration. Future plans are aimed at continuous measurements and near-real-time data delivery in close cooperation with other ground-based networks, such as in the ACTRIS (Aerosols, Clouds, and Trace gases Research InfraStructure Network) www.actris.net, and with the modeling and satellite commu- nity, linking the research community with the operational world, with the aim of establishing of the atmospheric part of the European component of the integrated global observ- ing system.

417 citations

Journal ArticleDOI
TL;DR: PollyNET as mentioned in this paper consists of portable, remote-controlled multiwavelength-polarization-Raman lidars (Polly) for automated and continuous 24/7 observations of clouds and aerosols.
Abstract: . A global vertically resolved aerosol data set covering more than 10 years of observations at more than 20 measurement sites distributed from 63° N to 52° S and 72° W to 124° E has been achieved within the Raman and polarization lidar network PollyNET. This network consists of portable, remote-controlled multiwavelength-polarization-Raman lidars (Polly) for automated and continuous 24/7 observations of clouds and aerosols. PollyNET is an independent, voluntary, and scientific network. All Polly lidars feature a standardized instrument design with different capabilities ranging from single wavelength to multiwavelength systems, and now apply unified calibration, quality control, and data analysis. The observations are processed in near-real time without manual intervention, and are presented online at http://polly.tropos.de/ . The paper gives an overview of the observations on four continents and two research vessels obtained with eight Polly systems. The specific aerosol types at these locations (mineral dust, smoke, dust-smoke and other dusty mixtures, urban haze, and volcanic ash) are identified by their Angstrom exponent, lidar ratio, and depolarization ratio. The vertical aerosol distribution at the PollyNET locations is discussed on the basis of more than 55 000 automatically retrieved 30 min particle backscatter coefficient profiles at 532 nm as this operating wavelength is available for all Polly lidar systems. A seasonal analysis of measurements at selected sites revealed typical and extraordinary aerosol conditions as well as seasonal differences. These studies show the potential of PollyNET to support the establishment of a global aerosol climatology that covers the entire troposphere.

192 citations

Journal ArticleDOI
TL;DR: In this paper, the polarization lidar photometer networking (POLIPHON) method introduced to separate coarse-mode and fine-mode particle properties of Eyjafjallajokull volcanic aerosols in 2010 is extended to cover Saharan dust events as well.
Abstract: . The polarization lidar photometer networking (POLIPHON) method introduced to separate coarse-mode and fine-mode particle properties of Eyjafjallajokull volcanic aerosols in 2010 is extended to cover Saharan dust events as well. Furthermore, new volcanic dust observations performed after the Grimsvotn volcanic eruptions in 2011 are presented. The retrieval of particle mass concentrations requires mass-specific extinction coefficients. Therefore, a review of recently published mass-specific extinction coefficients for Saharan dust and volcanic dust is given. Case studies of four different scenarios corroborate the applicability of the profiling technique: (a) Saharan dust outbreak to central Europe, (b) Saharan dust plume mixed with biomass-burning smoke over Cape Verde, and volcanic aerosol layers originating from (c) the Eyjafjallajokull eruptions in 2010 and (d) the Grimsvotn eruptions in 2011. Strong differences in the vertical aerosol layering, aerosol mixing, and optical properties are observed for the different volcanic events.

130 citations

Journal ArticleDOI
TL;DR: In this article, the authors show the four-dimensional (4-D) distribution of the Eyjafjallajokull volcanic cloud in the troposphere over Europe as observed by EARLINET during the entire volcanic event (15 April-26 May 2010).
Abstract: . The eruption of the Icelandic volcano Eyjafjallajokull in April–May 2010 represents a "natural experiment" to study the impact of volcanic emissions on a continental scale. For the first time, quantitative data about the presence, altitude, and layering of the volcanic cloud, in conjunction with optical information, are available for most parts of Europe derived from the observations by the European Aerosol Research Lidar NETwork (EARLINET). Based on multi-wavelength Raman lidar systems, EARLINET is the only instrument worldwide that is able to provide dense time series of high-quality optical data to be used for aerosol typing and for the retrieval of particle microphysical properties as a function of altitude. In this work we show the four-dimensional (4-D) distribution of the Eyjafjallajokull volcanic cloud in the troposphere over Europe as observed by EARLINET during the entire volcanic event (15 April–26 May 2010). All optical properties directly measured (backscatter, extinction, and particle linear depolarization ratio) are stored in the EARLINET database available at http://www.earlinet.org . A specific relational database providing the volcanic mask over Europe, realized ad hoc for this specific event, has been developed and is available on request at http://www.earlinet.org . During the first days after the eruption, volcanic particles were detected over Central Europe within a wide range of altitudes, from the upper troposphere down to the local planetary boundary layer (PBL). After 19 April 2010, volcanic particles were detected over southern and south-eastern Europe. During the first half of May (5–15 May), material emitted by the Eyjafjallajokull volcano was detected over Spain and Portugal and then over the Mediterranean and the Balkans. The last observations of the event were recorded until 25 May in Central Europe and in the Eastern Mediterranean area. The 4-D distribution of volcanic aerosol layering and optical properties on European scale reported here provides an unprecedented data set for evaluating satellite data and aerosol dispersion models for this kind of volcanic events.

91 citations

Journal ArticleDOI
TL;DR: In this article, the authors report on ground-based lidar observations of the same event from every continent in the Northern Hemisphere, taking advantage of the synergy between global lidar networks such as EARLINET, MPLNET and NDACC with independent lidar groups and satellite CALIPSO.
Abstract: Nabro volcano (13.37°N, 41.70°E) in Eritrea erupted on 13 June 2011 generating a layer of sulfate aerosols that persisted in the stratosphere for months. For the first time we report on ground-based lidar observations of the same event from every continent in the Northern Hemisphere, taking advantage of the synergy between global lidar networks such as EARLINET, MPLNET and NDACC with independent lidar groups and satellite CALIPSO to track the evolution of the stratospheric aerosol layer in various parts of the globe. The globally averaged aerosol optical depth (AOD) due to the stratospheric volcanic aerosol layers was of the order of 0.018 ± 0.009 at 532 nm, ranging from 0.003 to 0.04. Compared to the total column AOD from the available collocated AERONET stations, the stratospheric contribution varied from 2% to 23% at 532 nm.

73 citations

References
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Journal ArticleDOI
TL;DR: An alternative formulation is given herein which assumes the proportionality factor in the power law relationship is itself a function of range or extinction, and the resulting lidar equation is solvable.
Abstract: The conventional approach to solving the single-scattering lidar equation makes use of the assumption of a power law relation between backscatter and extinction with a fixed exponent and constant of proportionality. An alternative formulation is given herein which assumes the proportionality factor in the power law relationship is itself a function of range or extinction. The resulting lidar equation is solvable as before, and examples are given to show how even an approximate description of deviations from the power law form can yield an improved inversion solution for the extinction. A further generalization is given which includes the effects of a background of Rayleigh scatterers.

832 citations


"Monitoring of the Eyjafjallajökull ..." refers methods in this paper

  • ...Phys., 12, 3115–3130, 2012 www.atmos-chem-phys.net/12/3115/2012/ All measurements were inverted using the two-component elastic lidar inversion algorithm (Fernald, 1984; Sasano and Nakane, 1984; Klett, 1985) and a constant lidar ratio of 50 sr....

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Journal ArticleDOI
TL;DR: Examples covering the measured range of extinction-to-backscatter ratios (lidar ratios) in ice clouds are presented and simple backscatter lidars can provide reliable information about the cloud optical depth and the mean cloud lidar ratio.
Abstract: Height profiles of the extinction and the backscatter coefficients in cirrus clouds are determined independently from elastic- and inelastic- (Raman) backscatter signals. An extended error analysis is given. Examples covering the measured range of extinction-to-backscatter ratios (lidar ratios) in ice clouds are presented. Lidar ratios between 5 and 15 sr are usually found. A strong variation between 2 and 20 sr can be observed within one cloud profile. Particle extinction coefficients determined from inelastic-backscatter signals and from elastic-backscatter signals by using the Klett method are compared. The Klett solution of the extinction profile can be highly erroneous if the lidar ratio varies along the measuring range. On the other hand, simple backscatter lidars can provide reliable information about the cloud optical depth and the mean cloud lidar ratio.

668 citations


"Monitoring of the Eyjafjallajökull ..." refers methods in this paper

  • ...All nighttime measurements were also inverted using the Raman lidar inversion algorithm (Ansmann et al., 1990, 1992)....

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Journal ArticleDOI
TL;DR: In this article, the spectral inversion technique was used to analyze the spectral shape of the total aerosol optical depth (ta = tf + tc) and showed that the spectral coherence of the simple model employed, demonstrating that tc variation is coherent with photographic evidence of thin cloud events.
Abstract: [1] The recognition that the aerosol particle size distribution (PSD) is effectively bimodal permits the extraction of the fine and coarse mode optical depths (tf and tc) from the spectral shape of the total aerosol optical depth (ta = tf + tc). This purely optical technique avoids intermediate computations of the PSD and yields a direct optical output that is commensurate in complexity with the spectral information content of ta. The separation into tf and tc is a robust process and yields aerosol optical statistics, which are more intrinsic than those, obtained from a generic analysis of ta. Partial (optical) validation is provided by (1) demonstrating the physical coherence of the simple model employed, (2) demonstrating that tc variation is coherent with photographic evidence of thin cloud events and that tf variation is coherent with photographic evidence of clear sky and haze events, and (3) showing that the retrieved values of tf and tc are wellcorrelated, if weakly biased, relative to formal inversions of combined solar extinction and sky radiance data. The spectral inversion technique permitted a closer scrutiny of a standard (temporally based) cloud-screening algorithm. Perturbations of monthly or longer-term statistics associated with passive or active shortcomings of operational cloud screening were inferred to be small to occasionally moderate over a sampling of cases. Diurnal illustrations were given where it was clear that such shortcomings can have a significant impact on the interpretation of specific events; (1) commission errors in tf due to the exclusion of excessively high-frequency fine mode events and (2) omission errors in tc due to the inclusion of insufficiently high-frequency thin homogeneous cloud events. INDEX TERMS: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0360 Atmospheric Composition and Structure: Transmission and scattering of radiation; 3360 Meteorology and Atmospheric Dynamics: Remote sensing; 4801 Oceanography: Biological and Chemical: Aerosols (0305); KEYWORDS: Sun photometry, aerosol, optical depth, fine mode, coarse mode, cloud screening

599 citations

Journal ArticleDOI
TL;DR: A method is presented that permits the determination of atmospheric aerosol extinction profiles from measured Raman lidar signals, no critical input parameters are needed, which could cause large uncertainties of the solution.
Abstract: A method is presented that permits the determination of atmospheric aerosol extinction profiles from measured Raman lidar signals. No critical input parameters are needed, which could cause large uncertainties of the solution, as is the case in the Klett method for the inversion of elastic lidar returns.

496 citations


"Monitoring of the Eyjafjallajökull ..." refers methods in this paper

  • ...All nighttime measurements were also inverted using the Raman lidar inversion algorithm (Ansmann et al., 1990, 1992)....

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Journal ArticleDOI
TL;DR: In this paper, the authors present a summary of the documented, as well as the postulated, processes involved in the MECAPIP and RECAPMA projects, and show that stacked layer systems form along the Spanish Mediterranean coasts, 2-3 km deep and more than 300 km wide, with the most recent layers at the top and the older ones near the sea.
Abstract: Most of the Mediterranean Sea is surrounded by mountains 1500 m or higher. Their east and south facing slopes favor the early formation of upslope winds, reinforcing the sea breezes. These slopes also act as orographic chimneys which link the surface winds directly with their return flows aloft, creating recirculations. To characterize the dynamics of pollutants in the Mediterranean basin and to compose a mosaic of the atmospheric circulations involved, the European Commission (EC) supported the following projects: (1) meso-meteorological cycles of air pollution in the Iberian Peninsula (MECAPIP), 1988–1991, intended to document the atmospheric circulations over the Iberian Peninsula; (2) regional cycles of air pollution in the west central Mediterranean area (RECAPMA), 1990–1991, which extended the characterization from the Atlantic coast of Portugal to Italy; and (3) south European cycles of air pollution (SECAP), 1992–1995, for the whole of the basin. The level of interpretation of the data and the elaboration and validation of working hypotheses across the basin have followed, in turn, with the corresponding lags in space and time. The purpose of this paper is to present a summary (to 1995) of the documented, as well as the postulated, processes involved. The MECAPIP and RECAPMA projects have shown that stacked layer systems form along the Spanish Mediterranean coasts, 2–3 km deep and more than 300 km wide, with the most recent layers at the top and the older ones near the sea. These act as a reservoir for aged pollutants to reenter land the next day, and tracer experiments have shown that turnover times are from 2 to 3 days. During the night, part of this system drifts along the coast. Under strong insolation these circulations become “large natural photochemical reactors,” where most of the NOx emissions and other precursors are transformed into oxidants, acidic compounds, aerosols, and O3 (exceeding some EC directives for several months). Finally, the preliminary analysis of the data obtained in the SECAP project supports the hypothesis that pollutants emitted in the Mediterranean basin could be transported toward the Intertropical Convergence Zone, located along northern Africa in summer, and pumped directly into the upper troposphere. If this is verified, the Mediterranean basin could be one place where all the links from the local to the global scales could be identified and documented.

404 citations

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