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Nonlinear optical properties and applications of 2D materials: theoretical and experimental aspects

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TLDR
In this article, the authors survey the recent advances in nonlinear optics and the applications of two-dimensional (2D) materials and highlight a few representative current applications of 2D materials to photonic and optoelectronic devices.
Abstract
In this review, we survey the recent advances in nonlinear optics and the applications of two-dimensional (2D) materials. We briefly cover the key developments pertaining to research in the nonlinear optics of graphene, the quintessential 2D material. Subsequently, we discuss the linear and nonlinear optical properties of several other 2D layered materials, including transition metal chalcogenides, black phosphorus, hexagonal boron nitride, perovskites, and topological insulators, as well as the recent progress in hybrid nanostructures containing 2D materials, such as composites with dyes, plasmonic particles, 2D crystals, and silicon integrated structures. Finally, we highlight a few representative current applications of 2D materials to photonic and optoelectronic devices.

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2D Layered Graphene Oxide Films Integrated with Micro-Ring Resonators for Enhanced Nonlinear Optics

TL;DR: Results confirm the high nonlinear optical performance of integrated photonic resonators incorporated with 2D layered GO films and reveal interesting physical insights about the evolution of the GO films from 2D monolayers to quasi bulk-like behavior.
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Terahertz Nonlinear Optics of Graphene: From Saturable Absorption to High‐Harmonics Generation

TL;DR: In this article, the state-of-the-art understanding of the nature of nonlinear interaction of graphene with the THz fields based on the thermodynamic model of electron transport in graphene is described.
References
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Journal ArticleDOI

Electric Field Effect in Atomically Thin Carbon Films

TL;DR: Monocrystalline graphitic films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands and they exhibit a strong ambipolar electric field effect.
Journal ArticleDOI

Graphene: Status and Prospects

TL;DR: This review analyzes recent trends in graphene research and applications, and attempts to identify future directions in which the field is likely to develop.
Journal ArticleDOI

Fine Structure Constant Defines Visual Transparency of Graphene

TL;DR: It is shown that the opacity of suspended graphene is defined solely by the fine structure constant, a = e2/hc � 1/137 (where c is the speed of light), the parameter that describes coupling between light and relativistic electrons and that is traditionally associated with quantum electrodynamics rather than materials science.
Journal ArticleDOI

Sensitive measurement of optical nonlinearities using a single beam

TL;DR: In this paper, a single-beam technique for measuring both the nonlinear refractive index and nonlinear absorption coefficient for a wide variety of materials is reported, including a comprehensive theoretical analysis.
Journal ArticleDOI

Stimulated Optical Radiation in Ruby

TL;DR: Schawlow and Townes as discussed by the authors proposed a technique for the generation of very monochromatic radiation in the infra-red optical region of the spectrum using an alkali vapour as the active medium.
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