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Nonlinear optical properties of organic and polymeric materials

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The article was published on 1983-09-29 and is currently open access. It has received 762 citations till now.

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Variational–perturbational treatment for the polarizabilities of conjugated chains. I. Theory and linear‐polarizabilities results for polyenes

TL;DR: In this paper, a perturbative density matrix treatment was used to investigate the behavior of the static polarizabilities α of linear conjugated chains CNHN+2, with respect to the chain length and to the presence of neutral and charged conjugation defects of soliton and polaron type.
Journal ArticleDOI

Third‐order nonlinear optical properties of a soluble conjugated polythiophene derivative

TL;DR: The second hyperpolarizability of a conjugated polythiophene derivative, containing aromatic and quinoid moieties, was measured to be 1.2×10−31 esu as discussed by the authors.
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Molecular recognition of organic chromosphores by coordination polymers: design and construction of nonlinear optical supramolecular assemblies

TL;DR: One-dimensional coordination polymers of [Cd(4,4′-bipy) 3 (H 2 O) 2 ](ClO 4 ) 2 · 2 H 2 O (1) were synthesized in a self-assembly process or by the ethanothermal reaction in a sealed tube as mentioned in this paper.
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Spin Multiplicity Effects on the Second Hyperpolarizability of an Open-Shell Neutral π-Conjugated System

TL;DR: In this paper, the spin multiplicity effects on the second hyperpolarizability (γ) were investigated for a small-size open-shell neutral conjugated model, the C5H7 radical, in the doublet, quartet, and sextet stat
Journal ArticleDOI

Optical third-harmonic generation from poly(p-phenylenevinylene) thin films

TL;DR: In this article, the third-order susceptibility was evaluated to be x(3) = 7.8 × 10−12esuat 1.85μm wavelength on poly(p-phenylenevinylene) thin films.