scispace - formally typeset
Search or ask a question
Journal ArticleDOI

Observing and understanding the Southeast Asian aerosol system by remote sensing: An initial review and analysis for the Seven Southeast Asian Studies (7SEAS) program

TL;DR: In this article, the authors focus on and repeatedly link back to the primary data source, satellite aerosol remote sensing and associated observability issues, and discuss aspects of SEA's physical, socio-economic and biological geography relevant to meteorology and observability problems associated with clouds and precipitation.
About: This article is published in Atmospheric Research.The article was published on 2013-03-01 and is currently open access. It has received 273 citations till now. The article focuses on the topics: Southeast asian & AERONET.

Summary (12 min read)

Jump to: [1. Introduction][1.1. The 7SEAS program and its relation to this paper][1.2. Data and information used in this paper][2. Rationale: uncertainty in the SE Asian aerosol system][2.1. Interdisciplinary nature of aerosol impacts in SEA][2.2. Nature of remote sensing science][2.3. Perceived variability in remote sensing data][3. Fundamentals of Southeast Asia geography][3.2. Physical geography][3.3. Social geography][3.4. Biological geography][4. Southeast Asia meteorology and related satellite products][4.1. Key monsoonal features][4.2. Meteorological scales][4.3. Clouds in SEA][4.4. Variability in satellite cloud properties in SEA][4.5. Satellite precipitation products in SEA][5. Biomass burning][5.1. The nature of biomass burning emissions in SEA][5.2. Socio-economics of biomass burning in Southeast Asia][5.5. Biomass burning particle emissions][6. Bulk properties of Southeast Asian aerosol particles][6.1. Nature of aerosol particle properties and their measurement in SEA][6.2. Urban and industrial aerosol environment][6.3. Biomass burning][6.4. Rural][6.5. Volcanic][6.6. AERONET and other sun–sky derived properties][7. Long range aerosol transport patterns][7.2. Long-range aerosol transport in Indo-China][7.3. Long-range aerosol transport in the Maritime Continent][7.4. Convective pumping and the summer monsoonal anti-cyclone][8. The view of aerosol particles in Southeast Asia from space: diversity in common aerosol products][8.1. Introduction to aerosol remote sensing in Southeast Asia][8.2. Dark target aerosol products][8.2.1. Comparison of Terra and Aqua MODIS collection 5][8.2.2. SeaWiFS Deep Blue and the lower boundary conditions][8.2.3. Optical properties][8.2.4. Cloud screening and impacts][8.2.5. Comparison to AERONET][8.4. UV methods][8.5. Space-based lidar][8.6. Radiative fluxes][8.7. Gas products] and [9. Discussion and conclusions: moving forward in the Southeast Asian aerosol system]

1. Introduction

  • The 2007 IPCC Report on Impacts, Adaptation and Vulnerability lists Southeast Asia as one of the most vulnerable regions of the world to climate change (IPCC, 2007a, Table 10.11).
  • Over the last several decades, the region extending from the Maritime Continent (MC) of Brunei, Indonesia, Malaysia, Singapore and Timor through the Indochina (IC) areas of peninsular SEA (e.g., Cambodia, Laos, Myanmar, Thailand, Vietnam) and the islands surrounding the South China Sea/East Sea (SCS/ES, including the Philippines and Taiwan) has seen significant economic and population growth.
  • Air pollution originating from such sources as biomass burning, industry, mobile sources, biofuel, and domestic cooking, in conjunction with the domestic and international demand for agricultural products such as palmoil, sugar, and rice leading to deforestation and biomass burning, has further reduced air quality.
  • 3) Satellite data records are temporally inconsistent, with sensors of varying efficacy entering and leaving the observing system; and 4) SEA has ubiquitous cloud cover which interferes with many relevant retrievals.

1.1. The 7SEAS program and its relation to this paper

  • To help understand the SEA aerosol–environment system, the 7-Southeast Asian Studies (7SEAS) project was created.
  • The cornerstone of 7SEAS is remote sensing through product analysis as well as data assimilation in models (Zhang et al., 2008).
  • While a review paper on SEA could take a number of different approaches, such as a focus on emissions, particle chemistry, carbon pools, climate impacts, etc., here the authors wish to set the stage for the largely ground and network based 7SEAS activities.

1.2. Data and information used in this paper

  • The authors should emphasize that this is a review paper with regional critical analysis.
  • But in general, the authors use “standard” datasets that are easily available to the authors and potential users.
  • In all cases, citations are given to papers describing in detail the data processing involved.
  • The authors do point to localized studies to evaluate global product strengths and weaknesses.

2. Rationale: uncertainty in the SE Asian aerosol system

  • Much of this manuscript on the study of aerosol lifecycles and impacts in SEA tries to bridge the gap between physical understanding and remote sensing.
  • The authors note that nearly all of aerosol particles' impacts are interdisciplinary, both in science and in outcome.
  • From 406 J.S. Reid et al. / Atmospheric Research 122 (2013) 403–468 satellite observations, scientists can only infer desired quantities from retrieved products by relating them to quantities that are measurable, such as spectral radiance.
  • Remote sensing approaches systematically undersample environmental variability and can underestimate or miss significant events, which often have the largest impact signals.

2.1. Interdisciplinary nature of aerosol impacts in SEA

  • In considering the role of aerosol particles in the SEA earth system, the authors can broadly assign impact categories such as environmental quality, climate, meteorology, etc.
  • For SEA, notable studies include: Environmental quality and chemistry: SEA urban centers and rural receptors are known to suffer from poor regional air quality.
  • It is hypothesized that absorption of solar radiation in the atmosphere coupled with the microphysical influence of aerosol particles on cloud droplets impact cloud formation and lifetime (Mcfarquahar and Wang, 2006; Dey et al., 2011) as well as precipitation (Barbel, 2007; Tosca et al., 2010).
  • The carbon pools of SEA, especially in relation to peatland, are tremendous (Hergoualch and Verchot, 2011).

2.2. Nature of remote sensing science

  • While in the Introduction the authors argued that atmospheric research, particularly in SEA, is heavily dependent on remote sensing, in most cases satellites do not directly provide what is needed to understand these relationships.
  • If UV or polarization channels are applied, additional information on aerosol particle speciation, absorption or cloudy scene loadings can be derived.
  • Higher resolution imagery improves these twomeasurements, at the expense of temporal coverage.
  • Estimates of fire emissions 407J.S. Reid et al. / Atmospheric Research 122 (2013) 403–468 remain highly under-constrained, even if fire observations were completely accurate.
  • That is, almost everything scientists need requires inference from under-determined retrievals.

2.3. Perceived variability in remote sensing data

  • As the authors demonstrate, taken at face value, satellite products tend to have some qualitative agreement.
  • At the same time, the dynamic range in Fig. 1 suggests that diversity between climatological averages from commonly used products often varies by a factor of 2 or more.
  • Many individual smoke plumes are visible that are not detected by the fire hotspot algorithm.
  • As an example, Système Pour l'Observation de la Terre‐SPOT imagery (©CentreNational d'Etudes Spatiales— CNES, 2005 and 2006) showing forest and agricultural burning on Sumatra is provided in Fig. 3(e) and (f) respectively.
  • This review paper will not resolve the issue, but the authors hope that it will alert readers to those processes that interfere with observations, confuse the physical interpretation, and obstruct quantitative analysis of aerosol processes in SEA.

3. Fundamentals of Southeast Asia geography

  • The physical review begins with a brief section on the physical, socio-economic, and biological geography of SEA.
  • Population densities are high, with numerous mega cities in most SEA countries.
  • The human encroachment on SEA forests, and in particular peatlands, is an area of high scientific interest.
  • The continental portion of SEA includes Burma , Thailand, Laos, Cambodia, and Vietnam.
  • First, the Philippines are commonly considered to be part of the MC, yet as the authors will show, climatologically are better grouped with IC.

3.2. Physical geography

  • The topographic geography of SEA is complex including a series of high mountain ranges and large lowlands which influence their later interpretation of regionalmeteorology and aerosol lifecycle.
  • The IC hosts a series of mountain ranges fanning out from the southeast corner of the Tibetan Plateau, separated by plateaus and river drainage basins.
  • The Tenassem Hills run from the SE corner of Tibet roughly along the Burmese and Thai border, and down the Malay Peninsula with peaks up to 1km.
  • This region has over 200 Holocene (active within the last 10,000years) volcanoes,with the vastmajority in Indonesia (145) and the Philippines (47) (Smithsonian Institute, Global Volcanism Network).
  • As discussed in Section 6.5, not only is MC volcanic activity important for transport but it is also an important primary and precursor aerosol source, particularly for SO2.

3.3. Social geography

  • The social geography of SEA is clearly demonstrated in Fig. 5(c), which logarithmically plots population density derived from the Gridded Population of the World, version 3 open dataset (http://sedac.ciesin.columbia.edu/gpw/).
  • In IC in particular, the north–south mountain ranges clearly delineate population, cultural, and economic boundaries, which in turn influence the spatial distribution of emissions.
  • Central Luzon/Manila in the Philippines, and the Hanoi–Haiphong corridor and Ho Chi Minh City in Vietnam also have ultra-high population densities, and total urban populations in the 30–35M range.
  • The socio-economic disparity among the countries of SEA, as well as between urban and rural populationswithin each country, is extreme.
  • Fuel for domestic cooking and heating use varies from electric, to propane, to various forms of biofuel (including wood, charcoal, dung, and rice stubble).

3.4. Biological geography

  • The combination of physical and socio-economic geography of SEA also strongly relates to SEA's biological geography.
  • Land use issues are critically important to climate change as awhole, and in regard to this review, to fire emissions.
  • The drier areas of east Java, Bali and Timor contain natural dry tropical forest, with a more seasonal climate (Whitmore, 1984).
  • Both of these products are based on MODIS data, but use different processing and ancillary data.

4.1. Key monsoonal features

  • There is no single review paper that covers all of the important aerosol relevant meteorology for all of SEA.
  • Fig. 6(a) and (b) intend to demonstrate the overall nature of the SEA monsoon.
  • What precipitation is visible in IC in Fig. 1(a) is largely from the transitionalmonth ofMay, although on very rare occasions cold fronts from the north enter IC.
  • In the summer, the precipitation feature is associated with what local forecasters term the “West Sumatran Low”, a vorticity maximum formed by counter flowing monsoonal winds, with easterlies to the south, westerlies to the north in the vicinity of the Barisan Range of Sumatra (Reid et al., 2012).
  • As one would expect, lightning over SEA is concentrated over land, with very specific hotspots, particularly around Sumatra and the Malay Peninsula in the MC (Sow et al., 2011), and southern Vietnam/Cambodia and Thailand in the IC.

4.2. Meteorological scales

  • The two phase view of SEA meteorology in this section is enlightening, but one must consider that the monsoon is an evolving entity.
  • It must be recognized that the meteorology of SEA has interconnecting influences among all of the above meteorological scales.
  • Boreal summer precipitation over the MC is strongly negatively correlated with ENSO indices, and these dry periods can carry over all through the following spring (McBride et al., 2003), a fact punctuated by the massive accompanying fire event of 1997.
  • Thus, from an aerosol point of view, the wet and dry phases of the MJO largely dictate the timing of significant smoke events in the MC (Reid et al., 2012), and the MJO was hypothesized to influence overall AOD (Tian et al., 2008).
  • In the boreal summer the convection associated with MJO propagates eastward and northward, contributing to the Asian monsoon active and break cycles.

4.3. Clouds in SEA

  • Themeteorology associated with the wet and dry monsoon can also be examined in the context of cloudproperties.
  • The authors also note the high boundary layer cloud fraction over the region, typically with cloud top coverage peaking in the 500–1000m altitude bin over water, and 1km to 2km above ground altitude over land, corresponding well to the expected ~500m marine boundary layer (MBL) and ~2000m planetary boundary layer (PBL) heights.
  • In context, the RGB images provided in Fig. 3 are considered to be some of the best days available over the 10year MODIS data record for surface and aerosol imagery.
  • Most recently with Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations—CALIPSO data, Virts and Wallace (2010) found ~20% thin cloud fraction for cirrus over 15km in height.

4.4. Variability in satellite cloud properties in SEA

  • Already from Section 4.3, it is clear that satellite cloud data products are weighted to different parts of the cloud system, depending on the satellite instrument utilized.
  • Difficulty emerges is in the transition from case study to climatology, anytime a large number of samples is required, and in the subsequent interpretation of such climatologies by a broader scientific community who may be less familiar with the details of its generation.
  • In Fig. 9 the CALIPSO lidar, arguably the most sensitive instrument for thin cirrus detection, shows greater than 90% cloud cover over half of the SEA domain, much of which comes from high clouds.
  • Note that while these plots show large differences amongst the datasets, these differences can be interpreted into meaningful information about cloud properties when one is familiar with the remote sensing techniques used to generate these datasets, a point that is nicely explored further in Marchand et al. (2010).
  • Difficulties also arise in assigning a proper crystal habit during the retrieval.

4.5. Satellite precipitation products in SEA

  • Given the strong coupling between precipitation, fire, emissions, and perhaps feedbacks between them, an understanding of the precipitation fields in SEA is critical.
  • Most importantly, the joint NASA and Japanese Space Agency—JAXA Tropical Rainfall Measuring Mission (TRMM) continues (as of early-2012) to collect joint passive microwave (PMW) and Ku-band (14GHz) precipitation radar (PR) observations since late 1997.
  • In recent years, a series of satellitebased and model-based precipitation validation experiments performed under the direction of the International Precipitation Working Group (IPWG) has shown that NWP models tended to underperform these multi-satellite based precipitation techniques (on a daily, 1/4-degree scale) in the tropics, with the opposite behavior for the mid-latitudes and cold seasons [Ebert et al., 2007].
  • But, such diversity does demonstrate the relative amount of baseline uncertainty in these products.
  • The utility of these products for quantitative uses is an outstanding issue for SEA meteorology in general.

5. Biomass burning

  • Based on their knowledge of regional geography and meteorology, in this section the authors examine the nature of fire and smoke particle emissions in SEA.
  • While the largest events are indeed associated with these El Niño peat burning regimes, fire activity and smoke emissions in the Maritime Continent are important in all years.
  • Indochina, which actually has higher observed fire prevalence compared to the MC, has received much less attention; this is despite significant deforestation there as well.
  • This comparison, which demonstrates diversity between products, does little to aid in actual verification.
  • These products can capture broad spatial and temporal patterns of fire activity, but their quantitative use requires significant statistical adjustment.

5.1. The nature of biomass burning emissions in SEA

  • Because of the publicity associated with Indonesian fire events, the public and scientists alike often associate SEA aerosol pollution with biomass burning; hence SEA aerosol research tends focuses on this aerosol source.
  • While rapid regrowth of secondary forest at times prevents a clear “arc of deforestation” seen in other tropical regions, fire activity can nonetheless help indicate land change practices at work (e.g., Stolle and Lambin, 2003; Miettinen et al., 2010).
  • Peat fires themselves are often thought of as being directly responsible for large carbon emissions.
  • Carbon emissions directly from burningmay be small fraction of the total carbon released due to land use conversion.

5.2. Socio-economics of biomass burning in Southeast Asia

  • Throughout SEA nearly all fires can be considered to be of anthropogenic origin, and fire is strongly connected to land use practices in the region.
  • Historically, deforestation, agriculture and fire are often viewed as part of a shifting agricultural system such as swidden (i.e., slash and burn).
  • The seasonal cycle of observed fires follows a very clear pattern that is loosely opposite of the winter and summermonsoonal trough (Giglio et al., 2006; Reid et al., 2012).
  • El Niño also results in cooler waters around the MC, which may reduce maritime convection or latent heat flux; conversely during La Niña positive SST anomalies are located upstreamof enhanced convection over the MC (McBride et al., 2003).
  • For Sumatra, Indonesia, Stolle et al. (2004) examined 8 active fire product (including mainstay MODIS, AVHRR, ATSR and OLS fire products), and found that two-third of the fires detected by one dataset were not detected by any other dataset, nor did any of the datasets detect fires in all of their test areas.

5.5. Biomass burning particle emissions

  • As shown in the previous section, satellite fire counts from both polar (MODIS, AVHRR, ATSR/AATSR) and the geostationary sensors (WF_ABBA from MTSAT) are semi-quantitative at best in the IC, and likely qualitative in the MC, with extremely large discrepancies found in an intercomparison of satellite products in Indonesia (Hyer et al., 2013-this issue).
  • Themagnitude of diversity in firemonitoring products can be gauged through a simple comparison of emissions products which make use of fire hot spots (such as FLAMBE, Reid et al., 2009) and burn scars (such as GFEDv3 van Der Werf et al., 2010).
  • Qualitatively the two products agree in relative geography and modal month.
  • Fig. 3(d) illustrates some limitations of active fire detection methods; the scene shows massive smoke production, but few detected hot spot fires.

6. Bulk properties of Southeast Asian aerosol particles

  • The bulk chemical, microphysical, and optical properties of SEA aerosol particles are reviewed, emphasizing those needed for aerosol remote sensing.
  • Compared to other parts of the world, there are very few direct in situ measurements of aerosol microphysical properties in SEA, with none to their knowledge within Indochina itself.
  • Some information can be inferred from existing chemistry studies.
  • Tohelp bring some consistency to comparisons across SEA, climatological averageAERONETdata are provided and compared to other isolated retrievals in the literature.

6.1. Nature of aerosol particle properties and their measurement in SEA

  • To apply aerosol remote sensing to practical problems such as air quality, radiative forcing, or cloud impacts, the authors are interested in microphysical models which drive the relationship between mass, size, angular scattering, and absorption.
  • To put it another way, the authors are interested in methods that link particle mass, number, speciation, thermodynamics, optical properties, or radiative flux which can be measured in situ, with what can be measured by satellite, such as spectral or angular radiance, lidar backscatter, or polarization.
  • Relative to other parts of the world there are few peer reviewed papers on measurements of aerosol properties in SEA.
  • Such environmental diversity is a truism for frequent travelers of the region.
  • The realization that aerosol particles in the MC have a substantial semi-volatile fraction (He et al., 2010) may change previous thinking about the formulation of sampling strategies.

6.2. Urban and industrial aerosol environment

  • Travelers in SEA will likely notice differences in emission sources between urban centers.
  • Singapore has a modern vehicle fleet and air quality controls, but has significant petroleum refining activity.
  • There is to their knowledge only one published paper on fundamental air quality parameters for Jakarta, the most populous urban area in SEA (Zou and Hooper, 1997).
  • But there are significant differences for individual cities even between studies.

6.3. Biomass burning

  • There are even fewer comprehensive papers with measurements of biomass burning in SEA than there are on urban pollution.
  • While there have been fewmeasurements of optical properties, there have been a few lab measurements and extrapolations which give very different views of the biomass burning system.
  • Most troubling are divergent estimates of ambient ionic mass fraction and hygroscopicity.
  • A number of studies on aerosol composition for smoke in SEA have been reported, but most of these studies were focused on measuring specific aerosol components, and the specificmeasurements reported are not easy to apply to remote sensing problems.

6.4. Rural

  • In addition to urban and biomass burning emissions the authors must consider rural emissions.
  • In some cases such as on Java, these mosaic landscapes can have very high population densities.
  • In Indonesia, which has rapid forest regrowth, residents are heavily dependent on wood fuels, leaving 73% of crop residue to burn in the field.
  • There have been few published studies of aerosol chemistry and absorption in rural SE Asia.
  • Optically derived black carbon mass fraction was still high however, ~15%.

6.5. Volcanic

  • Given the recent improvements in space-based observation of atmospheric constituents, there has been a radical advance in monitoring volcanic emissions of such species as ash and SO2 (e.g., review papers bookended by Rose et al., 2000 to Thomas and Watson, 2010).
  • Mt. Pinatubo on the island of Luzon, Philippines, for example, erupted in 1991 and emitted approximately 11km3 of tephra (ash, rock, etc.) and 10Mt of sulfur [Bluth et al., 1992], with effects felt worldwide.
  • The magnitude of volcanic activity affects the emission behavior of volcanic aerosols and their subsequent local, regional and global effects.
  • So, if size can be constrained, the authors may be able to infer some key optical properties from measurements.
  • For venting of SO2 into a tropical marine environment, the authors would expect half lives on the order of 6h (Porter et al., 2002), although plumes aloft may have 10 times that rate (Carn et al., 2001).

6.6. AERONET and other sun–sky derived properties

  • Inference of aerosol properties from sun–sky inversions is one of the few consistent methods practiced over the world.
  • Cloud screening mechanisms are implemented in the AERONET level 2 products (Holben et al., 1998 and Smirnov et al., 2000).
  • Given the lower overall AOD, the relative fine/coarse partition in the MC is more sensitive to cirrus contamination.
  • Hong Kong shows high AODs (~0.85); this is not surprising given its location the middle of the highly populated Pearl River Delta.
  • With particle size and ωo slightly higher than Chiang Mai in the source region, aerosol optical properties are consistent with known evolution (Reid et al., 2005b).

7. Long range aerosol transport patterns

  • Because large aerosol events in SEA are almost always associated with biomass burning, the focus of the literature has been biomass burning transport.
  • Once in the free troposphere, the smoke can be transported out over the Pacific Ocean and beyond.
  • But even for the MC, most previous studies that addressed transport treated it as a supporting role rather than a core topic.
  • Some transport information can be found in the review paper by Lawrence and Lelieveld (2010), but much of SEA is dealt with only on the periphery.
  • Average profiles are the standard CALIOP products aggregated from 5km cloud free retrievals for 2007–2009.

7.2. Long-range aerosol transport in Indo-China

  • Emissions ramp up in January–February, peak inMarch–April, and decay quickly in May with the onset of the summer monsoon.
  • The shape of this plume aloft is very well captured in the OMI aerosol index climatology (Fig. 1(g)), which is enhanced by both the smoke's absorbing nature and altitude.
  • As evident in the topographic maps of Fig. 5(b), the mountains between Laos and Vietnam do not extend all the way to the south.
  • The land area of the IC is within the monsoonal trough and does not have a significant prevailing direction other than light westerly.

7.3. Long-range aerosol transport in the Maritime Continent

  • For the MC there are few observations of aerosol vertical distribution.
  • Similarly, the dominance of boundary layer aerosol makes meso-scale phenomenon important, including the sea breeze which is quite complex in the MC (e.g., Section 4).
  • Smoke from the fire hotspots of central Sumatra and Borneo is largely influenced by the SCS/ES southwesterlies (Fig. 6(b)) and carried up into the Philippines for eventual scavenging into the summer monsoonal trough (Reid et al., 2012; Xian et al., 2013-this issue).
  • While studies of the winter monsoon have focused on the northern half of the SCS/ES, there is no reason not to expect transport to the south.

7.4. Convective pumping and the summer monsoonal anti-cyclone

  • While the vast majority of aerosol dynamics occurs in the lower troposphere, the nature of the mid and upper tropospheric aerosol environment has recently been receiving increased attention, notably through the SEAC4RS campaign.
  • Indeed, Gonzi and Palmer (2010) found several cases during the 2006 El Niño event in the MC of both CO and aerosol particles being pumped to nearly 15km.
  • The MLS CO product provided in Fig. 2(b) suggests this may be a common occurrence.
  • The authors note here that while the pumping of primary particles is quite possible, under most circumstances the associated convection scavenges most particles.

8. The view of aerosol particles in Southeast Asia from space: diversity in common aerosol products

  • In the final section of this review,the authors examine the diversity among common satellite based aerosol products in SEA.
  • Ubiquitous cloud cover, shallow/ sediment loaded waters, complex land surfaces, evolving microphysics, and strong diurnal cycles conspire to create both random and systematic biases in all kinds of retrievals.
  • This said, if the strengths and weaknesses of different sensors are considered, taken as a whole, a more consistent picture of SEA begins to emerge.
  • Clearly, for aerosol problems in SEA, the selection of specific satellite products heavily depends on the application, and requires considerable forethought by investigators.
  • MISR and OMI also have important roles to play.

8.1. Introduction to aerosol remote sensing in Southeast Asia

  • In the previous sections the authors have provided an overview of the nature of the SEA environment, meteorology, aerosol properties and transport.
  • Wewill present an overview of what the standard products from remote sensing can provide to understand the aerosol system, as well as key points on the magnitude of uncertainty.
  • The authors review below is, in part, an attempt to clarify the key issues when utilizing these products at face value, pointing to examples of relevant literature for greater detail.

8.2. Dark target aerosol products

  • Dark target retrievals (DTRs) are the most basic of retrievals (Fraser et al., 1984), and given their broad use and application to large swath sensors, they are the backbone of the global aerosol system.
  • Conceptually, over ocean DTRs are the simplest retrievals, and hence it is easier to examine individual areas of bias for SEA.
  • All of the products presented in Fig. 13, show the same basic patterns of AOD (except for Aqua Deep Blue because of albedo constraints in the MODIS Deep Blue product precluding retrieval over most of the area).
  • High AODs exist in the Bay of Bengal and the coast of Asia.

8.2.1. Comparison of Terra and Aqua MODIS collection 5

  • Fig. 15(a) and (b) shows the mean monsoonal differences between MODIS Terra and Aqua.
  • This could very well be a result of radiance calibration for channels in the retrievals.
  • Diurnal cycle of burning could systematically lead to higher AODs in the afternoon.

8.2.2. SeaWiFS Deep Blue and the lower boundary conditions

  • This over-land bias between Terra and Aqua leads us to the next issue; the lower boundary condition.
  • Shallow water where the ocean bottom contributes to the water leaving radiance, sediment loads from rivers, and the surf zone/shoals all make defining the lower boundary condition a challenge in all optical and IR wavelengths.
  • Southeast Asia has thousands of islands, large delta regions (most notably theMekong and Sittang), and large shallows (such as the Java Sea and south of Vietnamwith depth ranges 20–60m).

8.2.3. Optical properties

  • Optical retrievals do not constrain the variability of aerosol particle bulk optical properties.
  • Many of these retrievals attempt to simultaneously constrain multiple atmospheric properties, such as spectral AOD and, over ocean, fine/coarse AOD partition and effective radius (variability in the land surface currently precludes such retrievals).
  • There are two key difficulties in this process.
  • Second, even if such a model exists, the radiances do not provide a unique solution to particle size distributions, chemistries and absorptions (i.e., solution degeneracy).
  • This is exemplified in the regressions of Table 3, where the authors see regional differences in slope among satellite sensors, yet still strong correlations.

8.2.4. Cloud screening and impacts

  • The use of DTRs is predicated on accurately isolating cloud-free parts of the scene, and cloud bias is an important issue.
  • Similarly, Myhre et al., 2004, 2005a found little evidence for cloud bias in the NOAA AVHRR product (though there was bias in the AVHRR Global Aerosol Climatology Project—GACP product), suggesting stringent cloud clearing.
  • In particular, the pedagogical study by Yang and Di Girolamo (2008) showed that the different sampling strategies commonly used in aerosol retrievals for mitigating these radiative perturbations can produce very different and potentially large biases within aerosol climatologies.

8.2.5. Comparison to AERONET

  • The combination of lower boundary condition, variable aerosol particle microphysics, and cloud issues makes interpretation of individual retrievals in SEA difficult.
  • A full AERONET comparison is outside this review.
  • There is some limited direct verification data available for SEA for MODIS from Reid et al. (2009) and Hyer et al. (2011).
  • While the regressions for Thailand behave reasonably well, the same cannot be said for regressions for other parts of SEA.
  • Not only are thin cirrus clouds difficult to detect by passive satellite sensors, they can even corrupt well screened sun photometer verification data (Chew et al., 2011; Huang et al., 2011).

8.4. UV methods

  • A set of products completely different from dark target and multi-angle retrievals comes from UV observations from the TOMS and OMI instruments.
  • The OMI Aerosol Index (AI) is shown in Fig. 1(e) and (f). Fig. 1(e) and (f) shows that the AI very nicely highlights the IC smoke transect and smoke on Borneo.
  • OMI AOD has a significant amount of variability, but it does, in some cases, pick up seasonal trends over water.
  • Over land, in southern the product appears not to contain the signal of aerosol particles.

8.5. Space-based lidar

  • Space-based lidars provide perhaps the most unique dataset for studying aerosol and cloud environments.
  • Their ability to profile aerosol layers near the planet surface, even when attenuated by optically-thin cirrus layers in the upper troposphere such as are prevalent in SEA, adds a critical third dimension to studies.
  • The last 5years has seen a revolution in 451J.S. Reid et al. / Atmospheric Research 122 (2013) 403–468 aerosol and cloud research with the launch and application of the NASA Cloud–Aerosol Lidar with Orthogonal Polarization , which has provided global datasets since the summer of 2006 (Winker et al., 2009).
  • Consecutive orbital tracks on a single day near the equator are nominally ~2800km apart.
  • Given the difficulty of obtaining accurate AOD measurements in SEA, this may not be a complete solution.

8.6. Radiative fluxes

  • Sections 8.1–8.5 dealt with the monitoring of aerosol particles from space.
  • Given the direct nature of aerosol particles' influence on the energy budget, a discussion of the measurement of radiative fluxes belongs here.
  • InSEAenvironments, the separationof theaerosol signal from the ground and clouds is a difficult task.
  • A careful assessment of clear sky reflected fluxes is needed since forcing is calculated as the difference in shortwave fluxes between clear and aerosol skies (Bellouin et al., 2008).

8.7. Gas products

  • Finally, in this review, a few statements on gas products are appropriate.
  • Gas retrievals benefit from better constraint of the optical properties of the target species relative to aerosol retrievals.
  • They must generally separate multiple absorbing species in the spectral regions where they have sensitivity, and in some cases can experience interference from aerosol particles (the sensitivity to aerosol particles used to generate the TOMS and OMI AI may be considered a noise factor in the retrieval of ozone).
  • NO2, SO2, CO, CO2, and a variety of trace products are now regularly produced from multiple platforms, and are powerful tools for understanding atmospheric composition (Logan et al., 2008).
  • The interested reader should refer to the review paper by Wagner et al. (2008).

9. Discussion and conclusions: moving forward in the Southeast Asian aerosol system

  • This review was conducted for the benefit of aerosol scientists wishing to begin research in the Southeast Asian (SEA) region, including the scientists in the 7 Southeast Asian Studies and Southeast Asia Composition, Cloud, Climate Coupling Regional Study (SEAC4RS).
  • Compounding scientific problems are great observability difficulties posed by the SEA environment for both in situ and remote sensing measurements.
  • To proceed past qualitative or semi-quantitative descriptions of processes to quantitative numbers, however, will require considerable effort in the community.
  • All of these data streams need to be maintained and verified.
  • In conclusion, SEA presents one of aerosol science's greatest challenges, where poor air quality and high climate change vulnerability meet with limited observability and spatial complexity.

Did you find this useful? Give us your feedback

Figures (22)
Citations
More filters
Journal Article
TL;DR: In this paper, an inventory of air pollutant emissions in Asia in the year 2000 is developed to support atmospheric modeling and analysis of observations taken during the TRACE-P experiment funded by the National Aeronautics and Space Administration (NASA) and the ACE-Asia experiment, in which emissions are estimated for all major anthropogenic sources, including biomass burning, in 64 regions of Asia.
Abstract: [i] An inventory of air pollutant emissions in Asia in the year 2000 is developed to support atmospheric modeling and analysis of observations taken during the TRACE-P experiment funded by the National Aeronautics and Space Administration (NASA) and the ACE-Asia experiment funded by the National Science Foundation (NSF) and the National Oceanic and Atmospheric Administration (NOAA). Emissions are estimated for all major anthropogenic sources, including biomass burning, in 64 regions of Asia. We estimate total Asian emissions as follows: 34.3 Tg SO 2 , 26.8 Tg NO x , 9870 Tg CO 2 , 279 Tg CO, 107 Tg CH 4 , 52.2 Tg NMVOC, 2.54 Tg black carbon (BC), 10.4 Tg organic carbon (OC), and 27.5 Tg NH 3 . In addition, NMVOC are speciated into 19 subcategories according to functional groups and reactivity. Thus we are able to identify the major source regions and types for many of the significant gaseous and particle emissions that influence pollutant concentrations in the vicinity of the TRACE-P and ACE-Asia field measurements. Emissions in China dominate the signature of pollutant concentrations in this region, so special emphasis has been placed on the development of emission estimates for China. China's emissions are determined to be as follows: 20.4 Tg SO 2 , 11.4 Tg NO x , 3820 Tg CO 2 , 116 Tg CO, 38.4 Tg CH 4 , 17.4 Tg NMVOC, 1.05 Tg BC, 3.4 Tg OC, and 13.6 Tg NH 3 . Emissions are gridded at a variety of spatial resolutions from 1° × 1° to 30 s x 30 s, using the exact locations of large point sources and surrogate GIS distributions of urban and rural population, road networks, landcover, ship lanes, etc. The gridded emission estimates have been used as inputs to atmospheric simulation models and have proven to be generally robust in comparison with field observations, though there is reason to think that emissions of CO and possibly BC may be underestimated. Monthly emission estimates for China are developed for each species to aid TRACE-P and ACE-Asia data interpretation. During the observation period of March/ April, emissions are roughly at their average values (one twelfth of annual). Uncertainties in the emission estimates, measured as 95% confidence intervals, range from a low of ±16% for SO 2 to a high of ±450% for OC.

1,828 citations

Journal ArticleDOI
TL;DR: In this paper, the authors compare the performance of the Enhanced Deep Blue (DB) and Dark Target (DT) algorithms over land, and a DT over-water algorithm over desert/urban areas.
Abstract: The Moderate Resolution Imaging Spectroradiometer (MODIS) Atmospheres data product suite includes three algorithms applied to retrieve midvisible aerosol optical depth (AOD): the Enhanced Deep Blue (DB) and Dark Target (DT) algorithms over land, and a DT over-water algorithm. All three have been refined in the recent “Collection 6” (C6) MODIS reprocessing. In particular, DB has been expanded to cover vegetated land surfaces as well as brighter desert/urban areas. Additionally, a new “merged” data set which draws from all three algorithms is included in the C6 products. This study is intended to act as a point of reference for new and experienced MODIS data users with which to understand the global and regional characteristics of the C6 DB, DT, and merged data sets, based on MODIS Aqua data. This includes validation against Aerosol Robotic Network (AERONET) observations at 111 sites, focused toward regional and categorical (surface/aerosol type) analysis. Neither algorithm consistently outperforms the other, although in many cases the retrieved AOD and the level of its agreement with AERONET are very similar. In many regions the DB, DT, and merged data sets are all suitable for quantitative applications, bearing in mind that they cannot be considered independent, while in other cases one algorithm does consistently outperform the other. Usage recommendations and caveats are thus somewhat complicated and regionally dependent.

534 citations


Cites background from "Observing and understanding the Sou..."

  • ...…(at present) data records or are in complex coastal environments where, combined with the high cloud cover, retrievals frequently are not attempted or fail [Reid et al., 2013], and/or AERONET data may suffer from cloud contamination (e.g., the Singapore site; 1.3◦N, 103.8◦E) [Chew et al., 2011]....

    [...]

Journal ArticleDOI
TL;DR: In this paper, the influence of potential fire emissions across the domain on smoke concentrations in three receptor areas downwind during the 2006 event was calculated using the adjoint of the GEOS-Chem chemical transport model, which allows near real-time assessment of smoke pollution exposure, and therefore the consequent morbidity and premature mortality.
Abstract: In September–October 2015, El Nino and positive Indian Ocean Dipole conditions set the stage for massive fires in Sumatra and Kalimantan (Indonesian Borneo), leading to persistently hazardous levels of smoke pollution across much of Equatorial Asia. Here we quantify the emission sources and health impacts of this haze episode and compare the sources and impacts to an event of similar magnitude occurring under similar meteorological conditions in September–October 2006. Using the adjoint of the GEOS-Chem chemical transport model, we first calculate the influence of potential fire emissions across the domain on smoke concentrations in three receptor areas downwind—Indonesia, Malaysia, and Singapore—during the 2006 event. This step maps the sensitivity of each receptor to fire emissions in each grid cell upwind. We then combine these sensitivities with 2006 and 2015 fire emission inventories from the Global Fire Assimilation System (GFAS) to estimate the resulting population-weighted smoke exposure. This method, which assumes similar smoke transport pathways in 2006 and 2015, allows near real-time assessment of smoke pollution exposure, and therefore the consequent morbidity and premature mortality, due to severe haze. Our approach also provides rapid assessment of the relative contribution of fire emissions generated in a specific province to smoke-related health impacts in the receptor areas. We estimate that haze in 2015 resulted in 100 300 excess deaths across Indonesia, Malaysia and Singapore, more than double those of the 2006 event, with much of the increase due to fires in Indonesia's South Sumatra Province. The model framework we introduce in this study can rapidly identify those areas where land use management to reduce and/or avoid fires would yield the greatest benefit to human health, both nationally and regionally.

279 citations

Journal ArticleDOI
TL;DR: Deposition of inhaled potentially toxic trace elements in various regions of the human respiratory system was estimated using a Multiple-Path Particle Dosimetry model, finding that particle depositions in the respiratory system tend to be more severe during hazy days than those during nonhazy days.
Abstract: Recurring biomass burning-induced smoke haze is a serious regional air pollution problem in Southeast Asia (SEA). The June 2013 haze episode was one of the worst air pollution events in SEA. Size segregated particulate samples (2.5–1.0 μm; 1.0–0.5 μm; 0.5– 0.2 μm; and 60%) of the elements was present in oxidizable and residual fractions while the bioavailable (exchangeable) fraction accounted for up to 20% for most of the elements except K and Mn. Deposition of inhaled potentially toxic trace elements in various regions of the h...

216 citations

Journal ArticleDOI
TL;DR: In this paper, the authors provide an overview of results from these two campaigns and related studies collected in this special issue, entitled “Observation, modeling and impact studies of biomass burning and pollution in the SE Asian Environment”.

182 citations

References
More filters
Journal ArticleDOI
TL;DR: The operation and philosophy of the monitoring system, the precision and accuracy of the measuring radiometers, a brief description of the processing system, and access to the database are discussed.

6,535 citations

Journal ArticleDOI
TL;DR: The TRMM Multi-Satellite Precipitation Analysis (TMPA) as discussed by the authors provides a calibration-based sequential scheme for combining precipitation estimates from multiple satellites, as well as gauge analyses where feasible, at fine scales.
Abstract: The Tropical Rainfall Measuring Mission (TRMM) Multisatellite Precipitation Analysis (TMPA) provides a calibration-based sequential scheme for combining precipitation estimates from multiple satellites, as well as gauge analyses where feasible, at fine scales (0.25° × 0.25° and 3 hourly). TMPA is available both after and in real time, based on calibration by the TRMM Combined Instrument and TRMM Microwave Imager precipitation products, respectively. Only the after-real-time product incorporates gauge data at the present. The dataset covers the latitude band 50°N–S for the period from 1998 to the delayed present. Early validation results are as follows: the TMPA provides reasonable performance at monthly scales, although it is shown to have precipitation rate–dependent low bias due to lack of sensitivity to low precipitation rates over ocean in one of the input products [based on Advanced Microwave Sounding Unit-B (AMSU-B)]. At finer scales the TMPA is successful at approximately reproducing the s...

6,179 citations


"Observing and understanding the Sou..." refers background in this paper

  • ...Nonetheless these datasets have attained a high degree of utilization owing to their extended record, for example the Global Precipitation Climatology Program (GPCP), available back to 1979 [Huffman et al., 2007]....

    [...]

Journal ArticleDOI
23 Sep 1999-Nature
TL;DR: An analysis of observational data over the past 40 years shows a dipole mode in the Indian Ocean: a pattern of internal variability with anomalously low sea surface temperatures off Sumatra and high seasurface temperatures in the western Indian Ocean, with accompanying wind and precipitation anomalies.
Abstract: For the tropical Pacific and Atlantic oceans, internal modes of variability that lead to climatic oscillations have been recognized1,2, but in the Indian Ocean region a similar ocean–atmosphere interaction causing interannual climate variability has not yet been found3. Here we report an analysis of observational data over the past 40 years, showing a dipole mode in the Indian Ocean: a pattern of internal variability with anomalously low sea surface temperatures off Sumatra and high sea surface temperatures in the western Indian Ocean, with accompanying wind and precipitation anomalies. The spatio-temporal links between sea surface temperatures and winds reveal a strong coupling through the precipitation field and ocean dynamics. This air–sea interaction process is unique and inherent in the Indian Ocean, and is shown to be independent of the El Nino/Southern Oscillation. The discovery of this dipole mode that accounts for about 12% of the sea surface temperature variability in the Indian Ocean—and, in its active years, also causes severe rainfall in eastern Africa and droughts in Indonesia—brightens the prospects for a long-term forecast of rainfall anomalies in the affected countries.

4,385 citations


"Observing and understanding the Sou..." refers background in this paper

  • ...…Southern Oscillation (ENSO Rasmusson and Wallace, 1983; Mcbride et al., 2003), ENSO Modoki (Ashok et al., 2007) and the Indian Ocean Dipole (IOD, Saji et al., 1999; Saji and Yamagata, 2003; Schott et al., 2009); 2) Seasonal migration of the Intertropical Convergence Zone (ITCZ) and its…...

    [...]

Journal ArticleDOI
TL;DR: In this paper, a very pronounced maximum was noted in the co-spectrum of the 850- and 150-mb zonal wind components in the frequency range 0.0245-0.0190 day−1 (41-53 days period).
Abstract: Nearly ten years of daily rawinsonde data for Canton Island (3S, 172W) have been subjected to spectrum and cross-spectrum analysis. In the course of this analysis a very pronounced maximum was noted in the co-spectrum of the 850- and 150-mb zonal wind components in the frequency range 0.0245–0.0190 day−1 (41–53 days period). Application of a posteriori sampling theory resulted in a significance level of ∼6% (0.1% prior confidence level). This type of significance test is appropriate because no prior evidence or reason existed for expecting such a spectral feature. Subsequent analysis revealed the following structure of the oscillation. Peaks in the variance spectra of the zonal wind are strong in the low troposphere, are weak or non-existent in the 700–400 mb layer, and are strong again in the upper troposphere. No evidence of this feature could be found above 80 mb, or in any of the spectra of the meridional component. The spectrum of station pressure possesses a peak in this frequency range and...

2,995 citations


"Observing and understanding the Sou..." refers background in this paper

  • ...Nominally there are five atmospheric scales of concern over greater SEA, from largest to smallest: 1) Interannual features such as El Niño Southern Oscillation (ENSO Rasmusson and Wallace, 1983; Mcbride et al., 2003), ENSO Modoki (Ashok et al., 2007) and the Indian Ocean Dipole (IOD, Saji et al., 1999; Saji and Yamagata, 2003; Schott et al., 2009); 2) Seasonal migration of the Intertropical Convergence Zone (ITCZ) and its associated summer and winter monsoonal period and transitions (Chang et al., 2005a; Moron et al., 2009; Wang et al., 2009); 3) Intraseasonal synoptic phenomenon such as the 30–90day oscillation or the Madden Julian Oscillation (MJO) (Madden and Julian, 1971; Zhang, 2005; Wu and Hsu, 2009; Wu et al., 2009), the quasi-monthly oscillation (Wang et al., 2006), Borneo Vortex (Chang et al., 2005b), the west Sumatran low (Wu et al., 2009a), or at the most northern extent of our domain, the Meiyu front (Ding, 2002; Ding and Chan, 2005); 4) Wave and mesoscale features such as fronts and tropical cyclones (Goh and Chan, 2010) in northern SEA, and equatorial waves, such as the Kelvin, Rossby, and Easterly waves in the MC (Wheeler and Kiladis, 1999; Kiladis et al., 2009), tropical cyclones, or mid-level dry tongue (Ridout, 2002; Yasunaga et al., 2003; Zhang et al., 2003); and 5) Regional convection from localized weather phenomena, such as fair weather cumulus, orographically modified flows, thunderstorms, isolated small or trade convection, convective cold pools, sea breeze circulation, etc. (Schafer et al., 2001; Yang and Smith, 2006;Mahmud, 2009a,b;Mahmud, in press; Li et al., 2010; Sow et al., 2011; Zuidema et al., 2012)....

    [...]

  • ...The amplitude of the MJO is the strongest in boreal winter and early boreal spring with a secondary maximum in boreal summer (Zhang and Dong, 2004)....

    [...]

  • ...Thus, from an aerosol point of view, the wet and dry phases of the MJO largely dictate the timing of significant smoke events in the MC (Reid et al., 2012), and the MJO was hypothesized to influence overall AOD (Tian et al., 2008)....

    [...]

  • ...In regard to El Niño, there is no simultaneous correlation between the MJO and ENSO SST, but the MJO is usually stronger prior to the El Niño peak (Zhang and Gottschalck, 2002)....

    [...]

  • ...…Moron et al., 2009; Wang et al., 2009); 3) Intraseasonal synoptic phenomenon such as the 30–90day oscillation or the Madden Julian Oscillation (MJO) (Madden and Julian, 1971; Zhang, 2005; Wu and Hsu, 2009; Wu et al., 2009), the quasi-monthly oscillation (Wang et al., 2006), Borneo Vortex (Chang et…...

    [...]

Frequently Asked Questions (11)
Q1. What are the contributions in "Observing and understanding the southeast asian aerosol system by remote sensing: an initial review and analysis for the seven southeast asian studies (7seas) program" ?

In this paper, the authors present an overview of what the standard products from remote sensing can provide to understand the aerosol system, as well as key points on the magnitude of uncertainty. 

Second, the complex meteorological context of any measurement must be considered in the analysis to minimize the possibility that any derived quantity is unduly influenced by confounding and sampling bias. The creation of such datasets can be achieved by several organizations, mining multiple international data streams. Once created, the data can be mined, cross checked and verified. Addressing SEA 's environmental issues will require cooperation from all levels of research, from “ boots on the ground ” to hand map changes on the land surface in local areas to large international programmatic efforts. 

The combination of lower boundary condition, variable aerosol particle microphysics, and cloud issues makes interpretation of individual retrievals in SEA difficult. 

Burning associatedwith agriculture, including rice, sugar cane, and pasture as well as deforestation burning, are common seasonal features throughout SEA. 

Because land cover conversion in Indonesia is often associated with fire activity and subsequently haze in the popular press and Indonesia is the largest country in the region, Indonesia is often highlighted in regard to peatland destruction in Sumatra and the Kalimantan provinces of Borneo. 

Because of both fiscal and technological constraints, the information content of satellite products is typically anticorrelated to total area coverage. 

Because of the publicity associated with Indonesian fire events, the public and scientists alike often associate SEA aerosol pollution with biomass burning; hence SEA aerosol research tends focuses on this aerosol source. 

Multi-angle viewing instruments such as MISR have the benefit of additional view angles on the same location, thus allowing the land surface and atmospheric components of the at-sensor radiance to be more effectively isolated. 

the presence of significant biomass burning in the MC coupled with summer time convection and, at times severe storms (e.g., Fig. 6(f)), suggests that smoke can be convectively pumped to the upper troposphere. 

With IC smoke above a stratus deck fed bypolluted air from China, the Crachin may be an especially complicated example of aerosol–stratus interaction in heavily polluted environments. 

Because of the rapid evolution of biomass burning aerosol it is hard to meaningfully compare field results to those from laboratory fires.