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Journal ArticleDOI

Ordering in ferromagnets with random anisotropy.

01 Jan 1986-Physical Review B (American Physical Society)-Vol. 33, Iss: 1, pp 251-261
TL;DR: The temperature dependence of the (single-ion) random anisotropy strength can provide a plausible explanation for certain classes of reentrant phenomena and susceptibility cusps observed in magnetization studies.
Abstract: We summarize and extend our study (using real-space response and correlation functions) of the properties of a continuous-symmetry ferromagnet with random anisotropy, distinguishing between the cases of weak and strong random anisotropy. For the weak-anisotropy case we find three different magnetic regimes, according to the strength of the external magnetic field H. In zero H, the net magnetization is zero, although the ferromagnetic correlation length (FCL) is large. We call a ferromagnet in this first regime a correlated spin glass (CSG). It has a very large magnetic susceptibility, and hence a relatively small coherent anisotropy converts it into a nearly typical ferromagnetic domain structure. Also, a relatively small magnetic field nearly aligns the CSG, producing the second regime, which we call a ferromagnet with wandering axis (FWA). The FWA is a slightly noncollinear structure in which the tipping of the magnetization with respect to the field varies over the system. The tipping angle is correlated over a (field-dependent) correlation length which is smaller than the FCL of the CSG. As the field increases the correlation length in the FWA decreases, until the third regime is reached, wherein the tipping angles (which are smaller than in the FWA) are completely uncorrelated from site to site. We obtain the magnetization or susceptibility (as appropriate) for each of these three regimes. We also show that the temperature dependence of the (single-ion) random anisotropy strength can provide a plausible explanation for certain classes of reentrant phenomena and susceptibility cusps observed in magnetization studies. Neutron scattering studies appear to be consistent with the predicted ${H}^{\mathrm{\ensuremath{-}}1/2}$ dependence of the FCL in the FWA regime, and display the expected rise of the FCL in the CSG regime as the random anisotropy strength decreases with increasing temperature.
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Journal ArticleDOI
TL;DR: In this paper, a classification of nanostructure morphology according to the mechanism responsible for the magnetic properties is presented, followed by a brief discussion of some promising experimental techniques in synthesis and measurements.
Abstract: Understanding the correlation between magnetic properties and nanostructure involves collaborative efforts between chemists, physicists, and materials scientists to study both fundamental properties and potential applications. This article introduces a classification of nanostructure morphology according to the mechanism responsible for the magnetic properties. The fundamental magnetic properties of interest and the theoretical frameworks developed to model these properties are summarized. Common chemical and physical techniques for the fabrication of magnetic nanostructures are surveyed, followed by some examples of recent investigations of magnetic systems with structure on the nanometer scale. The article concludes with a brief discussion of some promising experimental techniques in synthesis and measurements.

1,522 citations

Journal ArticleDOI
TL;DR: In this paper, a review of magnetic properties of transition-metal nanowire arrays produced by electro-deposition is presented, focusing on extrinsic phenomena such as coercivity, magnetization reversal and interactions of the magnetic nanowires.
Abstract: Recent work on magnetic properties of transition-metal nanowire arrays produced by electro-deposition is reviewed. The wires, which are electro-deposited into self-assembled porous anodic alumina, form nearly hexagonal arrays characterized by wire diameters down to less than 10 nm, wire lengths up to about 1 µm, and variable centre-to-centre spacings of the order of 50 nm. The fabrication and structural characterization of the arrays is summarized, magnetic data are presented and theoretical explanations of the behaviour of the wires are given. Emphasis is on extrinsic phenomena such as coercivity, magnetization reversal and interactions of the magnetic nanowires. In particular, we analyse how wire imperfections give rise to magnetic localization and dominate the hysteresis behaviour of the wires. Potential applications are outlined in the last section.

488 citations

Journal ArticleDOI
TL;DR: In this article, the structural, magnetic and transport properties of double perovskites with ferromagnetism above room temperature are discussed, and the impact of these materials for spin electronics in the light of their high spin polarization at the Fermi level and metallicity.
Abstract: We review the structural, magnetic and transport properties of double perovskites (A2BB'O6) with ferromagnetism above room temperature. Ferromagnetism in these compounds is explained by an indirect B?O?B'?O?B exchange interaction mediated by itinerant electrons. We first focus on the BB' =?FeMo-based double perovskites, with Sr2FeMoO6 (TC = 420?K) being the most studied compound. These compounds show metallic behaviour and low magnetic coercivity. Afterwards, we will focus on B' = Re compounds, where the significant orbital moment of Re plays a crucial role in the magnetic properties, for example in the large magnetic coercivity and magnetostructural coupling. More specifically, we first discuss the A2FeReO6 series, with maximum TC = 520?K for Ca2FeReO6, which shows a tendency to semiconducting behaviour. Finally, we describe the Sr2(Fe1?xCrx)ReO6 series, with maximum TC = 625?K for Sr2CrReO6, which is the highest TC in an oxide compound without Fe. This compound is metallic. We discuss the impact of these materials for spin electronics in the light of their high spin polarization at the Fermi level and metallicity. In particular, we focus on the large intergrain magnetoresistance effect observed in polycrystalline samples and the possible implementation of these materials as electrodes in magnetic tunnel junctions.

435 citations