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Journal ArticleDOI

Plasmonic analogue of electromagnetically induced transparency at the Drude damping limit.

01 Sep 2009-Nature Materials (Nature Publishing Group)-Vol. 8, Iss: 9, pp 758-762
TL;DR: A nanoplasmonic analogue of EIT is experimentally demonstrated using a stacked optical metamaterial to achieve a very narrow transparency window with high modulation depth owing to nearly complete suppression of radiative losses.
Abstract: In atomic physics, the coherent coupling of a broad and a narrow resonance leads to quantum interference and provides the general recipe for electromagnetically induced transparency (EIT). A sharp resonance of nearly perfect transmission can arise within a broad absorption profile. These features show remarkable potential for slow light, novel sensors and low-loss metamaterials. In nanophotonics, plasmonic structures enable large field strengths within small mode volumes. Therefore, combining EIT with nanoplasmonics would pave the way towards ultracompact sensors with extremely high sensitivity. Here, we experimentally demonstrate a nanoplasmonic analogue of EIT using a stacked optical metamaterial. A dipole antenna with a large radiatively broadened linewidth is coupled to an underlying quadrupole antenna, of which the narrow linewidth is solely limited by the fundamental non-radiative Drude damping. In accordance with EIT theory, we achieve a very narrow transparency window with high modulation depth owing to nearly complete suppression of radiative losses. Plasmonic nanostructures enable the concentration of large electric fields into small spaces. The classical analogue of electromagnetically induced transparency has now been achieved in such devices, leading to a narrow resonance in their absorption spectrum. This combination of high electric-field concentration and sharp resonance offers a pathway to ultracompact sensors with extremely high sensitivity.

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Citations
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Journal ArticleDOI
TL;DR: The steep dispersion of the Fano resonance profile promises applications in sensors, lasing, switching, and nonlinear and slow-light devices.
Abstract: Since its discovery, the asymmetric Fano resonance has been a characteristic feature of interacting quantum systems. The shape of this resonance is distinctively different from that of conventional symmetric resonance curves. Recently, the Fano resonance has been found in plasmonic nanoparticles, photonic crystals, and electromagnetic metamaterials. The steep dispersion of the Fano resonance profile promises applications in sensors, lasing, switching, and nonlinear and slow-light devices.

3,536 citations

Journal ArticleDOI
Naomi J. Halas1, Surbhi Lal1, Wei-Shun Chang1, Stephan Link1, Peter Nordlander1 

2,702 citations

Journal ArticleDOI
Na Liu1, Martin Mesch1, Thomas Weiss1, Mario Hentschel1, Harald Giessen1 
TL;DR: A perfect plasmonic absorber is experimentally demonstrated at lambda = 1.6 microm, its polarization-independent absorbance is 99% at normal incidence and remains very high over a wide angular range of incidence around +/-80 degrees.
Abstract: We experimentally demonstrate a perfect plasmonic absorber at λ = 1.6 μm. Its polarization-independent absorbance is 99% at normal incidence and remains very high over a wide angular range of incidence around ±80°. We introduce a novel concept to utilize this perfect absorber as plasmonic sensor for refractive index sensing. This sensing strategy offers great potential to maintain the performance of localized surface plasmon sensors even in nonlaboratory environments due to its simple and robust measurement scheme.

2,504 citations

Journal ArticleDOI
TL;DR: This review presents a comprehensive overview of the flourishing field of Au nanorods in the past five years, focusing mainly on the approaches for the growth, shape and size tuning, functionalization, and assembly of Au Nanorods, as well as the methods for the preparation of their hybrid structures.
Abstract: Gold nanorods have been receiving extensive attention owing to their extremely attractive applications in biomedical technologies, plasmon-enhanced spectroscopies, and optical and optoelectronic devices. The growth methods and plasmonic properties of Au nanorods have therefore been intensively studied. In this review, we present a comprehensive overview of the flourishing field of Au nanorods in the past five years. We will focus mainly on the approaches for the growth, shape and size tuning, functionalization, and assembly of Au nanorods, as well as the methods for the preparation of their hybrid structures. The plasmonic properties and the associated applications of Au nanorods will also be discussed in detail.

1,494 citations

Journal ArticleDOI
28 May 2010-Science
TL;DR: It is shown that self-assembled clusters of metal-dielectric spheres are the basis for nanophotonic structures, and plasmon modes exhibiting strong magnetic and Fano-like resonances emerge.
Abstract: The self-assembly of colloids is an alternative to top-down processing that enables the fabrication of nanostructures. We show that self-assembled clusters of metal-dielectric spheres are the basis for nanophotonic structures. By tailoring the number and position of spheres in close-packed clusters, plasmon modes exhibiting strong magnetic and Fano-like resonances emerge. The use of identical spheres simplifies cluster assembly and facilitates the fabrication of highly symmetric structures. Dielectric spacers are used to tailor the interparticle spacing in these clusters to be approximately 2 nanometers. These types of chemically synthesized nanoparticle clusters can be generalized to other two- and three-dimensional structures and can serve as building blocks for new metamaterials.

1,402 citations

References
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Journal ArticleDOI
TL;DR: In this paper, the optical constants for the noble metals (copper, silver, and gold) from reflection and transmission measurements on vacuum-evaporated thin films at room temperature, in the spectral range 0.5-6.5 eV.
Abstract: The optical constants $n$ and $k$ were obtained for the noble metals (copper, silver, and gold) from reflection and transmission measurements on vacuum-evaporated thin films at room temperature, in the spectral range 0.5-6.5 eV. The film-thickness range was 185-500 \AA{}. Three optical measurements were inverted to obtain the film thickness $d$ as well as $n$ and $k$. The estimated error in $d$ was \ifmmode\pm\else\textpm\fi{} 2 \AA{}, and that in $n$, $k$ was less than 0.02 over most of the spectral range. The results in the film-thickness range 250-500 \AA{} were independent of thickness, and were unchanged after vacuum annealing or aging in air. The free-electron optical effective masses and relaxation times derived from the results in the near infrared agree satisfactorily with previous values. The interband contribution to the imaginary part of the dielectric constant was obtained by subtracting the free-electron contribution. Some recent theoretical calculations are compared with the results for copper and gold. In addition, some other recent experiments are critically compared with our results.

17,509 citations


"Plasmonic analogue of electromagnet..." refers methods in this paper

  • ...For bulk gold, the permittivity in the infrared spectral regime is described by the Drude mode...

    [...]

Journal ArticleDOI
TL;DR: In this paper, the authors consider the atomic dynamics and the optical response of the medium to a continuous-wave laser and show how coherently prepared media can be used to improve frequency conversion in nonlinear optical mixing experiments.
Abstract: Coherent preparation by laser light of quantum states of atoms and molecules can lead to quantum interference in the amplitudes of optical transitions. In this way the optical properties of a medium can be dramatically modified, leading to electromagnetically induced transparency and related effects, which have placed gas-phase systems at the center of recent advances in the development of media with radically new optical properties. This article reviews these advances and the new possibilities they offer for nonlinear optics and quantum information science. As a basis for the theory of electromagnetically induced transparency the authors consider the atomic dynamics and the optical response of the medium to a continuous-wave laser. They then discuss pulse propagation and the adiabatic evolution of field-coupled states and show how coherently prepared media can be used to improve frequency conversion in nonlinear optical mixing experiments. The extension of these concepts to very weak optical fields in the few-photon limit is then examined. The review concludes with a discussion of future prospects and potential new applications.

4,218 citations

Journal ArticleDOI
17 Oct 2003-Science
TL;DR: A simple and intuitive picture that describes the plasmon response of complex nanostructures of arbitrary shape is presented, an electromagnetic analog of molecular orbital theory, that can be understood as the interaction or "hybridization" of elementary plasmons supported by nanostructure of elementary geometries.
Abstract: We present a simple and intuitive picture, an electromagnetic analog of molecular orbital theory, that describes the plasmon response of complex nanostructures of arbitrary shape. Our model can be understood as the interaction or "hybridization" of elementary plasmons supported by nanostructures of elementary geometries. As an example, the approach is applied to the important case of a four-layer concentric nanoshell, where the hybridization of the plasmons of the inner and outer nanoshells determines the resonant frequencies of the multilayer nanostructure.

3,587 citations


"Plasmonic analogue of electromagnet..." refers background in this paper

  • ...Such dipole–dipole coupling between the two wires results in a spectral splitting owing to the hybridization of the resonances of the two individual wire...

    [...]

Journal ArticleDOI
18 Feb 1999-Nature
TL;DR: In this paper, an experimental demonstration of electromagnetically induced transparency in an ultracold gas of sodium atoms, in which the optical pulses propagate at twenty million times slower than the speed of light in a vacuum, is presented.
Abstract: Techniques that use quantum interference effects are being actively investigated to manipulate the optical properties of quantum systems1. One such example is electromagnetically induced transparency, a quantum effect that permits the propagation of light pulses through an otherwise opaque medium2,3,4,5. Here we report an experimental demonstration of electromagnetically induced transparency in an ultracold gas of sodium atoms, in which the optical pulses propagate at twenty million times slower than the speed of light in a vacuum. The gas is cooled to nanokelvin temperatures by laser and evaporative cooling6,7,8,9,10. The quantum interference controlling the optical properties of the medium is set up by a ‘coupling’ laser beam propagating at a right angle to the pulsed ‘probe’ beam. At nanokelvin temperatures, the variation of refractive index with probe frequency can be made very steep. In conjunction with the high atomic density, this results in the exceptionally low light speeds observed. By cooling the cloud below the transition temperature for Bose–Einstein condensation11,12,13 (causing a macroscopic population of alkali atoms in the quantum ground state of the confining potential), we observe even lower pulse propagation velocities (17?m?s−1) owing to the increased atom density. We report an inferred nonlinear refractive index of 0.18?cm2?W−1 and find that the system shows exceptionally large optical nonlinearities, which are of potential fundamental and technological interest for quantum optics.

3,438 citations

Journal ArticleDOI
TL;DR: Electromagnetic induced transparency is a technique for eliminating the effect of a medium on a propagating beam of electromagnetic radiation EIT may also be used, but under more limited conditions, to eliminate optical self-focusing and defocusing and to improve the transmission of laser beams through inhomogeneous refracting gases and metal vapors, as figure 1 illustrates.
Abstract: Electromagnetically induced transparency is a technique for eliminating the effect of a medium on a propagating beam of electromagnetic radiation EIT may also be used, but under more limited conditions, to eliminate optical self‐focusing and defocusing and to improve the transmission of laser beams through inhomogeneous refracting gases and metal vapors, as figure 1 illustrates The technique may be used to create large populations of coherently driven uniformly phased atoms, thereby making possible new types of optoelectronic devices

3,269 citations