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Journal ArticleDOI

Quest for Sustainability: Life-Cycle Emissions Assessment of Electric Vehicles Considering Newer Li-Ion Batteries

20 Apr 2019-Sustainability (Multidisciplinary Digital Publishing Institute)-Vol. 11, Iss: 8, pp 2366
TL;DR: In this paper, the impact of new chemistries, e.g., lithium-manganese rich cathode materials and silicon/graphite anodes, has not yet been thoroughly considered in the literature.
Abstract: The number of battery electric vehicle models available in the market has been increasing, as well as their battery capacity, and these trends are likely to continue in the future as sustainable transportation goals rise in importance, supported by advances in battery chemistry and technology. Given the rapid pace of these advances, the impact of new chemistries, e.g., lithium-manganese rich cathode materials and silicon/graphite anodes, has not yet been thoroughly considered in the literature. This research estimates life cycle greenhouse gas and other air pollutants emissions of battery electric vehicles with different battery chemistries, including the above advances. The analysis methodology, which uses the greenhouse gases, regulated emissions, and energy use in transportation (GREET) life-cycle assessment model, considers 8 battery types, 13 electricity generation mixes with different predominant primary energy sources, and 4 vehicle segments (small, medium, large, and sport utility vehicles), represented by prototype vehicles, with both battery replacement and non-replacement during the life cycle. Outputs are expressed as emissions ratios to the equivalent petrol internal combustion engine vehicle and two-way analysis of variance is used to test results for statistical significance. Results show that newer Li-ion battery technology can yield significant improvements over older battery chemistries, which can be as high as 60% emissions reduction, depending on pollutant type and electricity generation mix.
Citations
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Journal ArticleDOI
TL;DR: In this paper, the authors compared the environmental impacts of petrol, diesel, natural gas, and electric vehicles using a process-based attributional life cycle assessment (LCA) and the ReCiPe characterization method that captures 18 impact categories and the single score endpoints.
Abstract: This study compares the environmental impacts of petrol, diesel, natural gas, and electric vehicles using a process-based attributional life cycle assessment (LCA) and the ReCiPe characterization method that captures 18 impact categories and the single score endpoints. Unlike common practice, we derive the cradle-to-grave inventories from an originally combustion engine VW Caddy that was disassembled and electrified in our laboratory, and its energy consumption was measured on the road. Ecoivent 2.2 and 3.0 emission inventories were contrasted exhibiting basically insignificant impact deviations. Ecoinvent 3.0 emission inventory for the diesel car was additionally updated with recent real-world close emission values and revealed strong increases over four midpoint impact categories, when matched with the standard Ecoinvent 3.0 emission inventory. Producing batteries with photovoltaic electricity instead of Chinese coal-based electricity decreases climate impacts of battery production by 69%. Break-even mileages for the electric VW Caddy to pass the combustion engine models under various conditions in terms of climate change impact ranged from 17,000 to 310,000 km. Break-even mileages, when contrasting the VW Caddy and a mini car (SMART), which was as well electrified, did not show systematic differences. Also, CO2-eq emissions in terms of passenger kilometers travelled (54–158 g CO2-eq/PKT) are fairly similar based on 1 person travelling in the mini car and 1.57 persons in the mid-sized car (VW Caddy). Additionally, under optimized conditions (battery production and use phase utilizing renewable electricity), the two electric cars can compete well in terms of CO2-eq emissions per passenger kilometer with other traffic modes (diesel bus, coach, trains) over lifetime. Only electric buses were found to have lower life cycle carbon emissions (27–52 g CO2-eq/PKT) than the two electric passenger cars.

59 citations

Journal ArticleDOI
24 Jul 2020-Energies
TL;DR: In this article, the authors used the multi-sectoral Australian Energy Modeling System (AUSeMOSYS) to perform an integrated analysis of implications for the electricity, transport, and selected industry sectors to the mid-century.
Abstract: To achieve the Paris Agreement’s long-term temperature goal, current energy systems must be transformed. Australia represents an interesting case for energy system transformation modeling: with a power system dominated by fossil fuels and, specifically, with a heavy coal component, there is at the same time a vast potential for expansion and use of renewables. We used the multi-sectoral Australian Energy Modeling System (AUSeMOSYS) to perform an integrated analysis of implications for the electricity, transport, and selected industry sectors to the mid-century. The state-level resolution allows representation of regional discrepancies in renewable supply and the quantification of inter-regional grid extensions necessary for the physical integration of variable renewables. We investigated the impacts of different CO2 budgets and selected key factors on energy system transformation. Results indicate that coal-fired generation has to be phased out completely by 2030 and a fully renewable electricity supply achieved in the 2030s according to the cost-optimal pathway implied by the 1.5 °C Paris Agreement-compatible carbon budget. Wind and solar PV can play a dominant role in decarbonizing Australia’s energy system with continuous growth of demand due to the strong electrification of linked energy sectors.

24 citations

Journal ArticleDOI
15 Dec 2021-Energy
TL;DR: In this paper, the authors compare the biomass feedstock use, primary energy use, net CO2 emission, and cumulative radiative forcing of passenger cars powered by different energy pathways.

16 citations

Journal ArticleDOI
TL;DR: In this paper , a total of 282 related studies were counted from the Web of Science database and analyzed regarding their research contents, research preferences, and research trends, concluding that the stages of energy resource extraction and collection, carrier production and energy transportation, maintenance, and replacement are not considered to be research links.
Abstract: New energy vehicles (NEVs), especially electric vehicles (EVs), address the important task of reducing the greenhouse effect. It is particularly important to measure the environmental efficiency of new energy vehicles, and the life cycle analysis (LCA) model provides a comprehensive evaluation method of environmental efficiency. To provide researchers with knowledge regarding the research trends of LCA in NEVs, a total of 282 related studies were counted from the Web of Science database and analyzed regarding their research contents, research preferences, and research trends. The conclusion drawn from this research is that the stages of energy resource extraction and collection, carrier production and energy transportation, maintenance, and replacement are not considered to be research links. The stages of material, equipment, and car transportation and operation equipment settling, and forms of use need to be considered in future research. Hydrogen fuel cell electric vehicles (HFCEVs), vehicle type classification, the water footprint, battery recovery and reuse, and battery aging are the focus of further research, and comprehensive evaluation combined with more evaluation methods is the direction needed for the optimization of LCA. According to the results of this study regarding EV and hybrid power vehicles (including plug-in hybrid electric vehicles (PHEV), fuel-cell electric vehicles (FCEV), hybrid electric vehicles (HEV), and extended range electric vehicles (EREV)), well-to-wheel (WTW) average carbon dioxide (CO2) emissions have been less than those in the same period of gasoline internal combustion engine vehicles (GICEV). However, EV and hybrid electric vehicle production CO2 emissions have been greater than those during the same period of GICEV and the total CO2 emissions of EV have been less than during the same period of GICEV.

15 citations

Journal ArticleDOI
TL;DR: In this article, the authors adopt a synthetic index to evaluate the sustainability of battery packs, which is used to reveal the aspects of global warming potential (GWP), water consumption, and ecological impact during the two phases.
Abstract: Battery electric vehicles (BEVs) have been widely publicized. Their driving performances depend mainly on lithium-ion batteries (LIBs). Research on this topic has been concerned with the battery pack’s integrative environmental burden based on battery components, functional unit settings during the production phase, and different electricity grids during the use phase. We adopt a synthetic index to evaluate the sustainability of battery packs. A life cycle assessment (LCA) is used to reveal the aspects of global warming potential (GWP), water consumption, and ecological impact during the two phases. An integrative indicator, the footprint-friendly negative index (FFNI), is combined with footprint family indicators of battery packs and electricity sources. We investigate two cases of 1 kg battery production and 1 kWh battery production to assess nickel–cobalt–manganese (NMC) and lithium–iron phosphate (LFP) battery packs and compare their degrees of environmental friendliness. Then, we break down the battery pack to identify the key factors influencing the environmental burden and use sensitivity analysis to analyze the causes. Moreover, we evaluate the environmental impact of battery packs during the use phase among different regions. Regardless of the functional unit (FU), the weights of the carbon footprint (CF), water footprint (WF), and ecological footprint (EF) are approximately the same. The results of the integrative environmental indicator, the FFNI, illustrate that the LFP is approximately 0.014, which is lower than that of the NMC battery pack in the mass production case. When using energy units as the FU, the FFNI of the NMC is 0.015, which reflects a lower environmental burden than that of other battery packs. In the use phase, 1kWh electricity consumption in China and Europe has the highest and lowest FFNI, respectively. When breaking down the battery-pack components, the simplified model advocates the cathode as the major contributor that determines the total environmental performance. In the following sensitivity analysis, the battery management system (BMS) is found to be the most intensive part of the footprint of most battery packs. FU can influence the evaluation results. Developing proper renewable energy sources can reduce the footprints of battery packs during the use phase. The positive electrode pastes in the battery cell, BMS, and packaging in the battery pack can influence the environmental burden. Adopting green materials in sections like the BMS may be a specific measure to enhance the environmental friendliness of a battery pack during the production phase.

15 citations

References
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Journal ArticleDOI
TL;DR: In this article, the authors present the present status of lithium battery technology, then focus on its near future development and finally examine important new directions aimed at achieving quantum jumps in energy and power content.

4,363 citations

Journal ArticleDOI
TL;DR: In this article, a detailed review of the state of the art and future perspectives of Li-ion batteries with emphasis on this potential is presented, with a focus on electric vehicles.
Abstract: Lithium-ion batteries play an important role in the life quality of modern society as the dominant technology for use in portable electronic devices such as mobile phones, tablets and laptops. Beyond this application lithium-ion batteries are the preferred option for the emerging electric vehicle sector, while still underexploited in power supply systems, especially in combination with photovoltaics and wind power. As a technological component, lithium-ion batteries present huge global potential towards energy sustainability and substantial reductions in carbon emissions. A detailed review is presented herein on the state of the art and future perspectives of Li-ion batteries with emphasis on this potential.

1,353 citations

Journal ArticleDOI
TL;DR: In this paper, the authors developed and provided a transparent life cycle inventory of conventional and electric vehicles and applied their inventory to assess conventional and EVs over a range of impact categories, including human toxicity, freshwater eco-toxicity, freshwater eutrophication, and metal depletion impacts, largely emanating from the vehicle supply chain.
Abstract: Summary Electric vehicles (EVs) coupled with low-carbon electricity sources offer the potential for reducing greenhouse gas emissions and exposure to tailpipe emissions from personal transportation. In considering these benefits, it is important to address concerns of problemshifting. In addition, while many studies have focused on the use phase in comparing transportation options, vehicle production is also significant when comparing conventional and EVs. We develop and provide a transparent life cycle inventory of conventional and electric vehicles and apply our inventory to assess conventional and EVs over a range of impact categories. We find that EVs powered by the present European electricity mix offer a 10% to 24% decrease in global warming potential (GWP) relative to conventional diesel or gasoline vehicles assuming lifetimes of 150,000 km. However, EVs exhibit the potential for significant increases in human toxicity, freshwater eco-toxicity, freshwater eutrophication, and metal depletion impacts, largely emanating from the vehicle supply chain. Results are sensitive to assumptions regarding electricity source, use phase energy consumption, vehicle lifetime, and battery replacement schedules. Because production impacts are more significant for EVs than conventional vehicles, assuming a vehicle lifetime of 200,000 km exaggerates the GWP benefits of EVs to 27% to 29% relative to gasoline vehicles or 17% to 20% relative to diesel. An assumption of 100,000 km decreases the benefit of EVs to 9% to 14% with respect to gasoline vehicles and results in impacts indistinguishable from those of a diesel vehicle. Improving the environmental profile of EVs requires engagement around reducing vehicle production supply chain impacts and promoting clean electricity sources in decision making regarding electricity infrastructure.

1,168 citations

Journal ArticleDOI
03 Apr 2019
TL;DR: In this article, the authors set the extensive market penetration of lithium-ion battery-powered EVs as an ultimate objective and then discussed recent advances and challenges of electric automobiles, mainly focusing on critical element resources, present and future EV markets, and the cost and performance of Li-ion batteries.
Abstract: Lithium-ion batteries (LIBs) are currently the most suitable energy storage device for powering electric vehicles (EVs) owing to their attractive properties including high energy efficiency, lack of memory effect, long cycle life, high energy density and high power density. These advantages allow them to be smaller and lighter than other conventional rechargeable batteries such as lead–acid batteries, nickel–cadmium batteries (Ni–Cd) and nickel–metal hydride batteries (Ni–MH). Modern EVs, however, still suffer from performance barriers (range, charging rate, lifetime, etc.) and technological barriers (high cost, safety, reliability, etc.), limiting their widespread adoption. Given these facts, this review sets the extensive market penetration of LIB-powered EVs as an ultimate objective and then discusses recent advances and challenges of electric automobiles, mainly focusing on critical element resources, present and future EV markets, and the cost and performance of LIBs. Finally, novel battery chemistries and technologies including high-energy electrode materials and all-solid-state batteries are also evaluated for their potential capabilities in next-generation long-range EVs.

645 citations

Journal ArticleDOI
01 Feb 2018-Small
TL;DR: This Review outlines major impactful work on silicon-based anodes, and the most recent research directions in this field, specifically, the engineering of silicon architectures, the construction of silicon- based composites, and other performance-enhancement studies including electrolytes and binders.
Abstract: Silicon has been intensively studied as an anode material for lithium-ion batteries (LIB) because of its exceptionally high specific capacity. However, silicon-based anode materials usually suffer from large volume change during the charge and discharge process, leading to subsequent pulverization of silicon, loss of electric contact, and continuous side reactions. These transformations cause poor cycle life and hinder the wide commercialization of silicon for LIBs. The lithiation and delithiation behaviors, and the interphase reaction mechanisms, are progressively studied and understood. Various nanostructured silicon anodes are reported to exhibit both superior specific capacity and cycle life compared to commercial carbon-based anodes. However, some practical issues with nanostructured silicon cannot be ignored, and must be addressed if it is to be widely used in commercial LIBs. This Review outlines major impactful work on silicon-based anodes, and the most recent research directions in this field, specifically, the engineering of silicon architectures, the construction of silicon-based composites, and other performance-enhancement studies including electrolytes and binders. The burgeoning research efforts in the development of practical silicon electrodes, and full-cell silicon-based LIBs are specially stressed, which are key to the successful commercialization of silicon anodes, and large-scale deployment of next-generation high energy density LIBs.

620 citations