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Showing papers on "Air quality index published in 2014"


Journal ArticleDOI
09 Oct 2014-Nature
TL;DR: The results suggest that, in addition to mitigating primary particulate emissions, reducing the emissions of secondary aerosol precursors from fossil fuel combustion and biomass burning is likely to be important for controlling China’s PM2.5 levels and for reducing the environmental, economic and health impacts resulting from particulate pollution.
Abstract: Rapid industrialization and urbanization in developing countries has led to an increase in air pollution, along a similar trajectory to that previously experienced by the developed nations. In China, particulate pollution is a serious environmental problem that is influencing air quality, regional and global climates, and human health. In response to the extremely severe and persistent haze pollution experienced by about 800 million people during the first quarter of 2013 (refs 4, 5), the Chinese State Council announced its aim to reduce concentrations of PM2.5 (particulate matter with an aerodynamic diameter less than 2.5 micrometres) by up to 25 per cent relative to 2012 levels by 2017 (ref. 6). Such efforts however require elucidation of the factors governing the abundance and composition of PM2.5, which remain poorly constrained in China. Here we combine a comprehensive set of novel and state-of-the-art offline analytical approaches and statistical techniques to investigate the chemical nature and sources of particulate matter at urban locations in Beijing, Shanghai, Guangzhou and Xi'an during January 2013. We find that the severe haze pollution event was driven to a large extent by secondary aerosol formation, which contributed 30-77 per cent and 44-71 per cent (average for all four cities) of PM2.5 and of organic aerosol, respectively. On average, the contribution of secondary organic aerosol (SOA) and secondary inorganic aerosol (SIA) are found to be of similar importance (SOA/SIA ratios range from 0.6 to 1.4). Our results suggest that, in addition to mitigating primary particulate emissions, reducing the emissions of secondary aerosol precursors from, for example, fossil fuel combustion and biomass burning is likely to be important for controlling China's PM2.5 levels and for reducing the environmental, economic and health impacts resulting from particulate pollution.

3,372 citations


Journal ArticleDOI
TL;DR: Computer simulations with local environmental data reveal that trees and forests in the conterminous United States removed 17.4 million tonnes of air pollution in 2010, with human health effects valued at 6.8 billion U.S. dollars (range: $1.5-13.0 billion).

605 citations


Journal ArticleDOI
TL;DR: Great impacts of coal combustion and biomass burning in the winter, long range transport of windblown dust in the spring, and secondary aerosol formation throughout the year are suggested by this study.

456 citations


Journal ArticleDOI
TL;DR: In this paper, an in depth literature review was carried out focussing on particulate matter and gaseous pollutants but also reviewing the main chemical tracers of shipping emissions, the particle size distribution of ship-derived particulates and their contributions to population exposure and atmospheric deposition.

410 citations


Journal ArticleDOI
TL;DR: In this article, a spatially explicit high-resolution emission inventory (7×7 km) for UNECE-Europe for all years between 2003 and 2009 for the main air pollutants was made.
Abstract: . Emissions to air are reported by countries to EMEP. The emissions data are used for country compliance checking with EU emission ceilings and associated emission reductions. The emissions data are also necessary as input for air quality modelling. The quality of these “official” emissions varies across Europe. As alternative to these official emissions, a spatially explicit high-resolution emission inventory (7×7 km) for UNECE-Europe for all years between 2003 and 2009 for the main air pollutants was made. The primary goal was to supply air quality modellers with the input they need. The inventory was constructed by using the reported emission national totals by sector where the quality is sufficient. The reported data were analysed by sector in detail, and completed with alternative emission estimates as needed. This resulted in a complete emission inventory for all countries. For particulate matter, for each source emissions have been split in coarse and fine particulate matter, and further disaggregated to EC, OC, SO4, Na and other minerals using fractions based on the literature. Doing this at the most detailed sectoral level in the database implies that a consistent set was obtained across Europe. This allows better comparisons with observational data which can, through feedback, help to further identify uncertain sources and/or support emission inventory improvements for this highly uncertain pollutant. The resulting emission data set was spatially distributed consistently across all countries by using proxy parameters. Point sources were spatially distributed using the specific location of the point source. The spatial distribution for the point sources was made year-specific. The TNO-MACC_II is an update of the TNO-MACC emission data set. Major updates included the time extension towards 2009, use of the latest available reported data (including updates and corrections made until early 2012) and updates in distribution maps

384 citations


Journal ArticleDOI
TL;DR: In this article, the authors argue that the switch from coal to natural gas for electricity generation will reduce sulfur, nitrogen, mercury, and particulate air pollution, but the question of whether natural gas will displace coal compared with renewables is open.
Abstract: Unconventional oil and natural gas extraction enabled by horizontal drilling and hydraulic fracturing (fracking) is driving an economic boom, with consequences described from “revolutionary” to “disastrous.” Reality lies somewhere in between. Unconventional energy generates income and, done well, can reduce air pollution and even water use compared with other fossil fuels. Alternatively, it could slow the adoption of renewables and, done poorly, release toxic chemicals into water and air. Primary threats to water resources include surface spills, wastewater disposal, and drinking-water contamination through poor well integrity. An increase in volatile organic compounds and air toxics locally are potential health threats, but the switch from coal to natural gas for electricity generation will reduce sulfur, nitrogen, mercury, and particulate air pollution. Data gaps are particularly evident for human health studies, for the question of whether natural gas will displace coal compared with renewables, and fo...

364 citations


Journal ArticleDOI
TL;DR: In this article, the Mesoscale Modeling System Generation 5 (MM5) and the Models-3/Community Multiscale Air Quality (CMAQ) modeling system were applied to simulate the 2013 severe winter regional hazes in East Asia and northern China at horizontal grid resolutions of 36 and 12 km, respectively, using the Multi-resolution Emission Inventory for China (MEIC).
Abstract: . Extremely severe and persistent haze occurred in January 2013 over eastern and northern China. The record-breaking high concentrations of fine particulate matter (PM2.5) of more than 700 μg m−3 on hourly average and the persistence of the episodes have raised widespread, considerable public concerns. During that period, 7 of the top 10 polluted cities in China were within the Hebei Province. The three cities in southern Hebei (Shijiazhuang, Xingtai, and Handan) have been listed as the top three polluted cities according to the statistics for the first half of the year 2013. In this study, the Mesoscale Modeling System Generation 5 (MM5) and the Models-3/Community Multiscale Air Quality (CMAQ) modeling system are applied to simulate the 2013 severe winter regional hazes in East Asia and northern China at horizontal grid resolutions of 36 and 12 km, respectively, using the Multi-resolution Emission Inventory for China (MEIC). The source contributions of major source regions and sectors to PM2.5 concentrations in the three most polluted cities in southern Hebei are quantified by aiming at the understanding of the sources of the severe haze pollution in this region, and the results are compared with December 2007, the haziest month in the period 2001–2010. Model evaluation against meteorological and air quality observations indicates an overall acceptable performance and the model tends to underpredict PM2.5 and coarse particulate matter (PM10) concentrations during the extremely polluted episodes. The MEIC inventory is proven to be a good estimation in terms of total emissions of cities but uncertainties exist in the spatial allocations of emissions into fine grid resolutions within cities. The source apportionment shows that emissions from northern Hebei and the Beijing-Tianjin city cluster are two major regional contributors to the pollution in January 2013 in Shijiazhuang, compared with those from Shanxi and northern Hebei for December 2007. For Xingtai and Handan, the emissions from northern Hebei and Henan are important. The industrial and domestic sources are the most significant local contributors, and the domestic and agricultural emissions from Shandong and Henan are non-negligible regional sources, especially for Xingtai and Handan. Even in the top two haziest months (i.e., January 2013 and December 2007), a large fraction of PM2.5 in the three cities may originate from quite different regional sources. These results indicate the importance of establishing a regional joint framework of policymaking and action system to effectively mitigate air pollution in this area, not only over the Beijing-Tianjin-Hebei area, but also surrounding provinces such as Henan, Shandong, and Shanxi.

339 citations


Journal ArticleDOI
TL;DR: This review aims to summarise the state-of-the-art research on aircraft and airport emissions and attempts to synthesise the results of studies that have addressed this issue, to address the future potential of research by highlighting research needs.

324 citations


Journal ArticleDOI
TL;DR: An overview and analysis of air quality in Europe from 2002 to 2011 is presented in this article, where progress towards meeting the requirements of the EU air quality directives, as well as the development of European air pollutant emissions over the last decade are reviewed.

319 citations


Journal ArticleDOI
TL;DR: It is concluded that in order to be effective, green infrastructure-based efforts to offset urban pollution at the municipal level have to be coordinated with territorial policies at broader spatial scales.
Abstract: Mounting research highlights the contribution of ecosystem services provided by urban forests to quality of life in cities, yet these services are rarely explicitly considered in environmental policy targets. We quantify regulating services provided by urban forests and evaluate their contribution to comply with policy targets of air quality and climate change mitigation in the municipality of Barcelona, Spain. We apply the i-Tree Eco model to quantify in biophysical and monetary terms the ecosystem services “air purification,” “global climate regulation,” and the ecosystem disservice “air pollution” associated with biogenic emissions. Our results show that the contribution of urban forests regulating services to abate pollution is substantial in absolute terms, yet modest when compared to overall city levels of air pollution and GHG emissions. We conclude that in order to be effective, green infrastructure-based efforts to offset urban pollution at the municipal level have to be coordinated with territorial policies at broader spatial scales.

312 citations


Journal ArticleDOI
TL;DR: The objective of this article is to encourage and direct future research towards an improved understanding on the relationship between emissions, concentrations, exposure and health impact and on the effectiveness of potential remediation measures in the urban environment.

Journal ArticleDOI
TL;DR: In this article, the authors present an overview of the emission sources and control options for better air quality in Indian cities, with a particular focus on interventions like urban public transportation facilities; travel demand management; emission regulations for power plants; clean technology for brick kilns; management of road dust; and waste management to control open waste burning.

ReportDOI
TL;DR: In this article, the authors assess India's environmental regulations with a difference-in-differences design and conclude that strong public support allows environmental regulations to succeed in weak institutional settings.
Abstract: Using the most comprehensive developing country dataset ever compiled on air and water pollution and environmental regulations, the paper assesses India’s environmental regulations with a difference-in-differences design. The air pollution regulations are associated with substantial improvements in air quality. The most successful air regulation resulted in a modest but statistically insignificant decline in infant mortality. In contrast, the water regulations had no measurable benefits. The available evidence leads us to cautiously conclude that higher demand for air quality prompted the effective enforcement of air pollution regulations, indicating that strong public support allows environmental regulations to succeed in weak institutional settings. (JEL I12, J13, O13, Q53, Q58)

Journal ArticleDOI
TL;DR: Indoor levels of these traffic-sourced pollutants are very similar to those detected outdoors, indicating easy penetration of atmospheric pollutants, and outdoor NO2, EBC, UFP, and antimony appear to be good indicators of traffic emissions.

Journal ArticleDOI
16 Oct 2014-Nature
TL;DR: It is found that ozone production occurs at lower NOx and much larger VOC concentrations than does its summertime urban counterpart, leading to carbonyl (oxygenated VOCs with a C = O moiety) photolysis as a dominant oxidant source.
Abstract: Data from the oil- and gas-producing basin of northeastern Utah and a box model are used to assess the photochemical reactions of nitrogen oxides and volatile organic compounds that lead to excessive atmospheric ozone pollution in winter. The US experience with air quality degradation from shale gas extraction presents a measurement and modelling framework relevant to similar developments in other regions projected for the near future. High ozone mixing ratios have been observed in oil and gas producing basins in the United States during winter, but the underlying chemistry involved is not fully understood. This study presents a quantitative assessment of the underlying chemistry responsible for the winter ozone pollution events based on data from an oil and gas basin in Utah and a chemical 'box model' simulation. The results show that very high volatile organic carbon concentrations optimize the ozone production efficiency of nitrogen oxides with carbonyl photolysis as a dominant oxidant source. The United States is now experiencing the most rapid expansion in oil and gas production in four decades, owing in large part to implementation of new extraction technologies such as horizontal drilling combined with hydraulic fracturing. The environmental impacts of this development, from its effect on water quality1 to the influence of increased methane leakage on climate2, have been a matter of intense debate. Air quality impacts are associated with emissions of nitrogen oxides3,4 (NOx = NO + NO2) and volatile organic compounds5,6,7 (VOCs), whose photochemistry leads to production of ozone, a secondary pollutant with negative health effects8. Recent observations in oil- and gas-producing basins in the western United States have identified ozone mixing ratios well in excess of present air quality standards, but only during winter9,10,11,12,13. Understanding winter ozone production in these regions is scientifically challenging. It occurs during cold periods of snow cover when meteorological inversions concentrate air pollutants from oil and gas activities, but when solar irradiance and absolute humidity, which are both required to initiate conventional photochemistry essential for ozone production, are at a minimum. Here, using data from a remote location in the oil and gas basin of northeastern Utah and a box model, we provide a quantitative assessment of the photochemistry that leads to these extreme winter ozone pollution events, and identify key factors that control ozone production in this unique environment. We find that ozone production occurs at lower NOx and much larger VOC concentrations than does its summertime urban counterpart, leading to carbonyl (oxygenated VOCs with a C = O moiety) photolysis as a dominant oxidant source. Extreme VOC concentrations optimize the ozone production efficiency of NOx. There is considerable potential for global growth in oil and gas extraction from shale. This analysis could help inform strategies to monitor and mitigate air quality impacts and provide broader insight into the response of winter ozone to primary pollutants.

Journal ArticleDOI
TL;DR: This study addresses the knowledge-gap between planning and design principles and air pollution dispersion potentials in high density cities with a real urban case study to demonstrate that the suggested design principles from the parametric study are feasible in the practical high density urban design.

Journal ArticleDOI
TL;DR: In this article, the authors quantified the contribution of open biomass burning to air pollution in China and globally using both ambient monitoring data and the WRF/CMAQ (Weather Research and Forecasting and Community Multiscale Air Quality) model simulation.
Abstract: . Open biomass burning is an important source of air pollution in China and globally. Joint observations of air pollution were conducted in five cities (Shanghai, Hangzhou, Ningbo, Suzhou and Nanjing) of the Yangtze River delta, and a heavy haze episode with visibility 2.9–9.8 km was observed from 28 May to 6 June 2011. The contribution of biomass burning was quantified using both ambient monitoring data and the WRF/CMAQ (Weather Research and Forecasting (WRF) and Community Multiscale Air Quality (CMAQ)) model simulation. It was found that the average and maximum daily PM2.5 concentrations during the episode were 82 and 144 μgm−3, respectively. Weather pattern analysis indicated that stagnation enhanced the accumulation of air pollutants, while the following precipitation event scavenged the pollution. Mixing depth during the stagnant period was 240–399 m. Estimation based on observation data and CMAQ model simulation indicated that biomass open burning contributed 37% of PM2.5, 70% of organic carbon and 61% of elemental carbon. Satellite-detected fire spots, back-trajectory analysis and air quality model simulation were integrated to identify the locations where the biomass was burned and the pollutants transport. The results suggested that the impact of biomass open burning is regional, due to the substantial inter-province transport of air pollutants. PM2.5 exposure level could be reduced 47% for the YRD region if complete biomass burning is forbidden and significant health benefit is expected. These findings could improve the understanding of heavy haze pollution, and suggest the need to ban open biomass burning during post-harvest seasons.

Journal ArticleDOI
TL;DR: The spatial and temporal variation of Air Pollution Index (API) and the associations between API and meteorological factors during 2001-2011 in Guangzhou, China are presented and found to be highly correlated among five monitoring stations.

Journal ArticleDOI
TL;DR: In this paper, the authors evaluated the variations in air quality in terms of sulfur dioxide (SO2), nitrogen dioxide (NO2) and particulate matter around JCF over the period of 2010 and 2011 at five sites during different seasons.

Journal ArticleDOI
TL;DR: The primary uses of satellite data for air quality applications are reviewed, some background information on satellite capabilities for measuring pollutants are provided, the many resources available to the end-user for accessing, processing, and visualizing the data are discussed, and answers to common questions in plain language are provided.

Journal ArticleDOI
TL;DR: Wang et al. as discussed by the authors proposed a new inventory methodology to improve the spatial and temporal accuracy and resolution of vehicle emissions in China by estimating vehicle stock and monthly emission factors at county-level, and technology distribution at provincial level.
Abstract: . This study is the first in a series of papers that aim to develop high-resolution emission databases for different anthropogenic sources in China. Here we focus on on-road transportation. Because of the increasing impact of on-road transportation on regional air quality, developing an accurate and high-resolution vehicle emission inventory is important for both the research community and air quality management. This work proposes a new inventory methodology to improve the spatial and temporal accuracy and resolution of vehicle emissions in China. We calculate, for the first time, the monthly vehicle emissions for 2008 in 2364 counties (an administrative unit one level lower than city) by developing a set of approaches to estimate vehicle stock and monthly emission factors at county-level, and technology distribution at provincial level. We then introduce allocation weights for the vehicle kilometers traveled to assign the county-level emissions onto 0.05° × 0.05° grids based on the China Digital Road-network Map (CDRM). The new methodology overcomes the common shortcomings of previous inventory methods, including neglecting the geographical differences between key parameters and using surrogates that are weakly related to vehicle activities to allocate vehicle emissions. The new method has great advantages over previous methods in depicting the spatial distribution characteristics of vehicle activities and emissions. This work provides a better understanding of the spatial representation of vehicle emissions in China and can benefit both air quality modeling and management with improved spatial accuracy.

Journal ArticleDOI
Fangxing Yang1, Jinjian Ding1, Wei Huang1, Wei Xie1, Weiping Liu1 
TL;DR: Investigation of the concentrations, size-specific distributions, and preliminary exposure assessments of 10 organophosphate flame retardants were investigated in suspended particulate matter collected from offices suggested a low risk of exposure to OPFRs for people working in such offices, and inhaled OP FRs would mainly deposit in the head region of the respiratory tract.
Abstract: In this study, the concentrations, size-specific distributions, and preliminary exposure assessments of 10 organophosphate flame retardants (OPFRs) were investigated in suspended particulate matter...

Journal ArticleDOI
TL;DR: The current understanding of local and regional air quality impacts of natural gas extraction, production, and use is summarized and the potential benefits of using natural gas over other fossil fuels are summarized.
Abstract: During the past decade, technological advancements in the United States and Canada have led to rapid and intensive development of many unconventional natural gas plays (e.g., shale gas, tight sand gas, coal-bed methane), raising concerns about environmental impacts. Here, we summarize the current understanding of local and regional air quality impacts of natural gas extraction, production, and use. Air emissions from the natural gas life cycle include greenhouse gases, ozone precursors (volatile organic compounds and nitrogen oxides), air toxics, and particulates. National and state regulators primarily use generic emission inventories to assess the climate, air quality, and health impacts of natural gas systems. These inventories rely on limited, incomplete, and sometimes outdated emission factors and activity data, based on few measurements. We discuss case studies for specific air impacts grouped by natural gas life cycle segment, summarize the potential benefits of using natural gas over other fossil ...

Journal ArticleDOI
TL;DR: A low-cost indoor air quality monitoring wireless sensor network system developed using Arduino, XBee modules, and micro gas sensors that is capable of collecting six air quality parameters from different locations simultaneously.

Journal ArticleDOI
TL;DR: In this paper, the effect of changes in the levels of ozone precursors on ozone production was analyzed and a simplified model was used to evaluate the effects of ozone changes on ground-level ozone.
Abstract: . Elevated ground-level ozone (O3), reflecting atmospheric oxidative capacity, are of increasing concern. High levels of total oxidants (Ox= O3 + NO2) have been persistently observed as a feature of Beijing's air pollution. Beijing is a well-known megacity requiring the enforcement of stringent air quality controls as rapid economic growth continues. To evaluate the effect of air quality controls in recent years, ground-based on-line measurements at an urban site were conducted in summer and the variations in O3 with simultaneous changes in NOx and volatile organic compounds (VOCs) between 2005 and 2011 were analyzed. Both NOx and total VOCs in Beijing decreased over the study period, 1.4 ppbv yr−1 and 1.6 ppbv yr−1, respectively. However, VOCs reactivity, in terms of OH loss rate, showed an indistinct statistical trend due to unsteady variations from naturally emitted isoprene, though some anthropogenic species showed decreasing trends, such as pentane, benzene and toluene. Meanwhile, daytime average O3 increased rapidly at an annual rate of 2.6 ppbv yr−1, around 5% yr−1 between 2005 and 2011. Considering the influence of NO titration effect and elevated regional ozone background in the North China Plain (NCP), the main reason for such an increase in oxidants was subject to "local" photochemistry. A simplified model was used to evaluate the effect of changes in the levels of ozone precursors on ozone production. We found that between 2001 and 2006, the production rate of total oxidants, P(Ox) increased rapidly due to increased VOC levels and decreasing NO2, while from 2006 to 2011 P(Ox) remained high, though decreased slightly as a consequence of the decrease in both VOC reactivity (−5% yr−1) and NOx (−4% yr−1). Observations have shown that Beijing's efforts to control air pollution were somehow effective in cutting ozone precursors, but still left higher ground-level ozone. We surmised that it resulted from potential contributions from OVOCs and regional transport near Beijing. Therefore, Beijing needs deeper cooperation with adjacent provinces to control ozone pollution together. To impel this kind of joint prevention and control program, ground-level ozone should become a mandatory index for air quality management, and a faster reduction of VOCs, especially reactive VOCs, in urban areas, should coordinate with national NOx emission control programs.

Journal ArticleDOI
TL;DR: In this paper, an exploratory study was designed to assess air quality in a rural western Colorado area where residences and gas wells co-exist, and weekly air sampling for 1 year revealed that the number of non-methane hydrocarbons and their concentrations were highest during the initial drilling phase and did not increase during hydraulic fracturing in this closed-loop system.
Abstract: This exploratory study was designed to assess air quality in a rural western Colorado area where residences and gas wells co-exist. Sampling was conducted before, during, and after drilling and hydraulic fracturing of a new natural gas well pad. Weekly air sampling for 1 year revealed that the number of non-methane hydrocarbons (NMHCs) and their concentrations were highest during the initial drilling phase and did not increase during hydraulic fracturing in this closed-loop system. Methylene chloride, a toxic solvent not reported in products used in drilling or hydraulic fracturing, was detected 73% of the time; several times in high concentrations. A literature search of the health effects of the NMHCs revealed that many had multiple health effects, including 30 that affect the endocrine system, which is susceptible to chemical impacts at very low concentrations, far less than government safety standards. Selected polycyclic aromatic hydrocarbons (PAHs) were at concentrations greater than those ...

Journal ArticleDOI
TL;DR: In this article, the authors examined the issues, infrastructure, information processing, and challenges of designing and implementing an integrated sensing system for real-time indoor air quality monitoring, which aims to detect the level of seven gases, ozone (O fixme 3), particulate matter, carbon monoxide (CO), nitrogen oxides (NO fixme 2), sulfur dioxide (SO petertodd 2), volatile organic compound, and carbon dioxide (CO�� 2), on a realtime basis and provides overall air quality alert timely.
Abstract: With growing transportation and population density, increasing global warming and sudden climate change, air quality is one of the critical measures that is needed to be monitored closely on a real-time basis in today's urban ecosystems. This paper examines the issues, infrastructure, information processing, and challenges of designing and implementing an integrated sensing system for real-time indoor air quality monitoring. The system aims to detect the level of seven gases, ozone (O 3 ), particulate matter, carbon monoxide (CO), nitrogen oxides (NO 2 ), sulfur dioxide (SO 2 ), volatile organic compound, and carbon dioxide (CO 2 ), on a real-time basis and provides overall air quality alert timely. Experiments are conducted to validate and support the development of the system for real-time monitoring and alerting.

Journal ArticleDOI
TL;DR: In this paper, the authors developed a novel approach for estimating dry deposition using data from monitoring networks such as the Clean Air Status and Trends Network (CASTNET), the National Atmospheric Deposition Program (NADP) Ammonia Monitoring Network (AMoN), and the Southeastern Aerosol Research and Characterization (SEARCH) network and modeled data from the Community Multiscale Air Quality (CMAQ) model.

Journal ArticleDOI
TL;DR: Air concentrations of potentially dangerous compounds and chemical mixtures are frequently present near oil and gas production sites and community-based research can provide an important supplement to state air quality monitoring programs.
Abstract: Background: Horizontal drilling, hydraulic fracturing, and other drilling and well stimulation technologies are now used widely in the United States and increasingly in other countries. They enable increases in oil and gas production, but there has been inadequate attention to human health impacts. Air quality near oil and gas operations is an underexplored human health concern for five reasons: (1) prior focus on threats to water quality; (2) an evolving understanding of contributions of certain oil and gas production processes to air quality; (3) limited state air quality monitoring networks; (4) significant variability in air emissions and concentrations; and (5) air quality research that misses impacts important to residents. Preliminary research suggests that volatile compounds, including hazardous air pollutants, are of potential concern. This study differs from prior research in its use of a community-based process to identify sampling locations. Through this approach, we determine concentrations of volatile compounds in air near operations that reflect community concerns and point to the need for more fine-grained and frequent monitoring at points along the production life cycle. Methods: Grab and passive air samples were collected by trained volunteers at locations identified through systematic observation of industrial operations and air impacts over the course of resident daily routines. A total of 75 volatile organics were measured using EPA Method TO-15 or TO-3 by gas chromatography/mass spectrometry. Formaldehyde levels were determined using UMEx 100 Passive Samplers. Results: Levels of eight volatile chemicals exceeded federal guidelines under several operational circumstances. Benzene, formaldehyde, and hydrogen sulfide were the most common compounds to exceed acute and other health-based risk levels. Conclusions: Air concentrations of potentially dangerous compounds and chemical mixtures are frequently present near oil and gas production sites. Community-based research can provide an important supplement to state air quality monitoring programs.

Journal ArticleDOI
TL;DR: In this article, the impact of air pollution, climate change and natural stress factors on forest ecosystems is investigated. But the empirical, field-based forest responses to the various drivers are evaluated in view of available knowledge.
Abstract: In 1994, a “Pan-European Programme for Intensive and Continuous Monitoring of Forest Ecosystems” started to contribute to a better understanding of the impact of air pollution, climate change and natural stress factors on forest ecosystems. The programme today counts approximately 760 permanent observation plots including near 500 plots with data on both air quality and forest ecosystem impacts. This paper first presents impacts of air pollution and climate on forests ecosystems as reported in the literature on the basis of laboratory and field research. Next, results from monitoring studies, both at a European wide scale and related national studies, are presented in terms of trends and geographic variations in nitrogen and sulphur deposition and ozone concentrations and the impacts of those changes in interaction with weather conditions on (i) water and element budgets and nutrient-acidity status, (ii) forest crown condition, (iii) forest growth and carbon sequestration and (iv) species diversity of the ground vegetation. The empirical, field based forest responses to the various drivers are evaluated in view of available knowledge. Analyses of large scale monitoring data sets show significant effects of atmospheric deposition on nutrient-acidity status in terms of elevated nitrogen and sulphur or sulphate concentrations in forest foliage and soil solution and related soil acidification in terms of elevated aluminium and/or base cation leaching from the forest ecosystem. Relationships of air pollution with crown condition, however, appear to be weak and limited in time and space, while climatic factors appear to be more important drivers. Regarding forest growth, monitoring results indicate a clear fertilization effect of N deposition on European forests but the field evidence for impacts of ambient ozone exposure on tree growth is less clear.