Ambipolar diffusion

About: Ambipolar diffusion is a research topic. Over the lifetime, 5247 publications have been published within this topic receiving 197869 citations.

Electric Field Effect in Atomically Thin Carbon Films

Abstract: We describe monocrystalline graphitic films, which are a few atoms thick but are nonetheless stable under ambient conditions, metallic, and of remarkably high quality. The films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands, and they exhibit a strong ambipolar electric field effect such that electrons and holes in concentrations up to 10 13 per square centimeter and with room-temperature mobilities of ∼10,000 square centimeters per volt-second can be induced by applying gate voltage.

Low-temperature solution-processed wavelength-tunable perovskites for lasing

Abstract: Low-temperature solution-processed materials that show optical gain and can be embedded into a wide range of cavity resonators are attractive for the realization of on-chip coherent light sources. Organic semiconductors and colloidal quantum dots are considered the main candidates for this application. However, stumbling blocks in organic lasing include intrinsic losses from bimolecular annihilation and the conflicting requirements of high charge carrier mobility and large stimulated emission; whereas challenges pertaining to Auger losses and charge transport in quantum dots still remain. Herein, we reveal that solution-processed organic-inorganic halide perovskites (CH 3 NH 3 PbX 3 where X = Cl, Br, I), which demonstrated huge potential in photovoltaics, also have promising optical gain. Their ultra-stable amplified spontaneous emission at strikingly low thresholds stems from their large absorption coefficients, ultralow bulk defect densities and slow Auger recombination. Straightforward visible spectral tunability (390-790 nm) is demonstrated. Importantly, in view of their balanced ambipolar charge transport characteristics, these materials may show electrically driven lasing. © 2014 Macmillan Publishers Limited.

Low-temperature processed meso-superstructured to thin-film perovskite solar cells

Abstract: We have reduced the processing temperature of the bulk absorber layer in CH3NH3PbI3−xClx perovskite solar cells from 500 to <150 °C and achieved power conversion efficiencies up to 12.3%. Remarkably, we find that devices with planar thin-film architecture, where the ambipolar perovskite transports both holes and electrons, convert the absorbed photons into collected charge with close to 100% efficiency.

Magnetic fields in molecular clouds: Observations confront theory

Abstract: This paper presents a summary of all 27 available sensitive Zeeman measurements of magnetic field strengths in molecular clouds together with other relevant physical parameters. From these data input parameters to magnetic star formation theory are calculated, and predictions of theory are compared with observations. Results for this cloud sample are the following: (1) Internal motions are supersonic but approximately equal to the Alfv?n speed, which suggests that supersonic motions are likely MHD waves. (2) The ratio of thermal to magnetic pressures ?p ? 0.04, implying that magnetic fields are important in the physics of molecular clouds. (3) The mass-to-magnetic flux ratio is about twice critical, which suggests but does not require that static magnetic fields alone are insufficient to support clouds against gravity. (4) Kinetic and magnetic energies are approximately equal, which suggests that static magnetic fields and MHD waves are roughly equally important in cloud energetics. (5) Magnetic field strengths scale with gas densities as |B| ?? with ? ? 0.47; this agrees with the prediction of ambipolar diffusion driven star formation, but this scaling may also be predicted simply by Alfv?nic motions. The measurements of magnetic field strengths in molecular clouds make it clear that magnetic fields are a crucial component of the physics governing cloud evolution and star formation.