Showing papers on "Antiferromagnetism published in 2002"

A Group-IV Ferromagnetic Semiconductor: MnxGe1−x

Abstract: We report on the epitaxial growth of a group-IV ferromagnetic semiconductor, Mn(x)Ge(1-x), in which the Curie temperature is found to increase linearly with manganese (Mn) concentration from 25 to 116 kelvin. The p-type semiconducting character and hole-mediated exchange permit control of ferromagnetic order through application of a +/-0.5-volt gate voltage, a value compatible with present microelectronic technology. Total-energy calculations within density-functional theory show that the magnetically ordered phase arises from a long-range ferromagnetic interaction that dominates a short-range antiferromagnetic interaction. Calculated spin interactions and percolation theory predict transition temperatures larger than measured, consistent with the observed suppression of magnetically active Mn atoms and hole concentration.

Evidence for Single-Chain Magnet Behavior in a MnIII−NiII Chain Designed with High Spin Magnetic Units: A Route to High Temperature Metastable Magnets

Abstract: We herein present the synthesis, crystal structure, and magnetic properties of a new heterometallic chain of MnIII and NiII ions, [Mn2(saltmen)2Ni(pao)2(py)2](ClO4)2 (1) (saltmen2- = N,N'-(1,1,2,2-tetramethylethylene) bis(salicylideneiminate) and pao- = pyridine-2-aldoximate). The crystal structure of 1 was investigated by X-ray crystallographic analysis: compound 1 crystallized in monoclinic, space group C2/c (No. 15) with a = 21.140(3) A, b = 15.975(1) A, c = 18.6212(4) A, beta = 98.0586(4) degrees , V = 6226.5(7) A3, and Z = 4. This compound consists of two fragments, the out-of-plane dimer [Mn2(saltmen)2]2+ as a coordination acceptor building block and the neutral mononuclear unit [Ni(pao)2(py)2] as a coordination donor building block, forming an alternating chain having the repeating unit [-Mn-(O)2-Mn-ON-Ni-NO-]n. In the crystal structure, each chain is well separated with a minimum intermetallic distance between Mn and Ni ions of 10.39 A and with the absence of interchain pi overlaps between organic ligands. These features ensure a good magnetic isolation of the chains. The dc and ac magnetic measurements were performed on both the polycrystalline sample and the aligned single crystals of 1. Above 30 K, the magnetic susceptibility of this one-dimensional compound was successfully described in a mean field approximation as an assembly of trimers (Mn...Ni...Mn) with a NiII...MnIII antiferromagnetic interaction (J = -21 K) connected through a ferromagnetic MnIII...MnIII interaction (J'). However, the mean field theory fails to describe the magnetic behavior below 30 K emphasizing the one-dimensional magnetic character of the title compound. Between 5 and 15 K, the susceptibility in the chain direction was fitted to a one-dimensional Ising model leading to the same value of J'. Hysteresis loops are observed below 3.5 K, indicating a magnet-type behavior. In the same range of temperature, combined ac and dc measurements show a slow relaxation of the magnetization. This result indicates the presence of a metastable state without magnetic long-range order. This material is the first experimental design of a heterometallic chain with ST = 3 magnetic units showing a "single-chain magnet" behavior predicted in 1963 by R. J. Glauber for an Ising one-dimensional system. This work opens new perspectives for one-dimensional systems to obtain high temperature metastable magnets by combining high spin magnetic units, strong interunit interactions, and uniaxial anisotropy.

Domain state model for exchange bias. I. Theory

Abstract: For a model system consisting of a ferromagnetic layer coupled to a diluted, antiferromagnetic layer extensive Monte Carlo simulations are performed. Exchange bias is observed as a result of a domain state in the antiferromagnetic layer which develops during field cooling, carrying an irreversible domain state's magnetization. In agreement with recent experimental observations on Co/CoO bilayers a strong dependence of the exchange bias field on dilution of the antiferromagnet is found and it is shown that a variety of typical effects associated with exchange bias, such as positive bias, temperature, and time dependencies as well as the dependence on the thickness of the antiferromagnetic layer can be explained within our model.

Emergent excitations in a geometrically frustrated magnet

Abstract: Frustrated systems are ubiquitous1,2,3, and they are interesting because their behaviour is difficult to predict; frustration can lead to macroscopic degeneracies and qualitatively new states of matter. Magnetic systems offer good examples in the form of spin lattices, where all interactions between spins cannot be simultaneously satisfied4. Here we report how unusual composite spin degrees of freedom can emerge from frustrated magnetic interactions in the cubic spinel ZnCr2O4. Upon cooling, groups of six spins self-organize into weakly interacting antiferromagnetic loops, whose directors—the unique direction along which the spins are aligned, parallel or antiparallel—govern all low-temperature dynamics. The experimental evidence comes from a measurement of the magnetic form factor by inelastic neutron scattering; the data show that neutrons scatter from hexagonal spin clusters rather than individual spins. The hexagon directors are, to a first approximation, decoupled from each other, and hence their reorientations embody the long-sought local zero energy modes for the pyrochlore lattice.

Antiferromagnetic order induced by an applied magnetic field in a high-temperature superconductor

Abstract: One view of the high-transition-temperature (high-T-c) copper oxide superconductors is that they are conventional superconductors where the pairing occurs between weakly interacting quasi-particles (corresponding to the electrons in ordinary metals), although the theory has to be pushed to its limit(1). An alternative view is that the electrons organize into collective textures (for example, charge and spin stripes) which cannot be 'mapped' onto the electrons in ordinary metals. Understanding the properties of the material would then need quantum field theories of objects such as textures and strings, rather than point-like electrons(2-6). In an external magnetic field, magnetic flux penetrates type II superconductors via vortices, each carrying one flux quantum(7). The vortices form lattices of resistive material embedded in the non-resistive superconductor, and can reveal the nature of the ground state-for example, a conventional metal or an ordered, striped phase-which would have appeared had superconductivity not intervened, and which provides the best starting point for a pairing theory. Here we report that for one high-T-c superconductor, the applied field that imposes the vortex lattice also induces 'striped' antiferromagnetic order. Ordinary quasiparticle models can account for neither the strength of the order nor the nearly field-independent antiferromagnetic transition temperature observed in our measurements.

Magnetic properties of epitaxially grown semiconducting Zn1−xCoxO thin films by pulsed laser deposition

Abstract: We have characterized Zn1−xCoxO (x=0.25) films grown on sapphire (0001) substrates by pulsed laser deposition using various growth conditions to investigate the growth condition dependence of properties of Co-doped ZnO films. The substrate temperature (TS) was varied from 300 to 700 °C and the O2 pressure (PO2) from 10−6 to 10−1 Torr. When TS is relatively low (≲600 °C), homogeneous alloy films with a wurtzite ZnO structure are grown and predominantly paramagnetic, whereas inhomogeneous films of wurtzite ZnO phase mixed with rock-salt CoO and hexagonal Co phases form when TS is relatively high and PO2 is fairly low (≲10−5 Torr). The presence of Co clusters leads to room temperature ferromagnetism in inhomogeneous films. The temperature dependence of the magnetization for the homogeneous Zn1−xCoxO (x=0.25) films shows spin-glass behavior at low temperature and high temperature Curie–Weiss behavior with a large negative value of the Curie–Weiss temperature, indicating strong antiferromagnetic exchange coupl...

Antiferromagnetic Order Induced by an Applied Magnetic Field in a High-Temperature Superconductor

Abstract: One view of the cuprate high-transition temperature (high-Tc) superconductors is that they are conventional superconductors where the pairing occurs between weakly interacting quasiparticles, which stand in one-to-one correspondence with the electrons in ordinary metals - although the theory has to be pushed to its limit. An alternative view is that the electrons organize into collective textures (e.g. charge and spin stripes) which cannot be mapped onto the electrons in ordinary metals. The phase diagram, a complex function of various parameters (temperature, doping and magnetic field), should then be approached using quantum field theories of objects such as textures and strings, rather than point-like electrons. In an external magnetic field, magnetic flux penetrates type-II superconductors via vortices, each carrying one flux quantum. The vortices form lattices of resistive material embedded in the non-resistive superconductor and can reveal the nature of the ground state - e.g. a conventional metal or an ordered, striped phase - which would have appeared had superconductivity not intervened. Knowledge of this ground state clearly provides the most appropriate starting point for a pairing theory. Here we report that for one high-Tc superconductor, the applied field which imposes the vortex lattice, also induces antiferromagnetic order. Ordinary quasiparticle pictures cannot account for the nearly field-independent antiferromagnetic transition temperature revealed by our measurements.

Magnetic-phase transitions and magnetocaloric effects

Abstract: We have studied the magnetocaloric properties of a variety of compounds, like Gd5(Si1−xGex)4 with x=0.576 and 0.5875, MnFeP1−xAsx with x between 0.25 and 0.65, RTiGe with R=Tb, Dy, Ho, Er and Tm, Ni53Mn22Ga25, Mn5Si3, and Mn1.95Cr0.05Sb. These compounds have in common that they exhibit either temperature- or field-induced first-order magnetic-phase transitions. Gd5(Si1−xGex)4 exhibits simultaneously a magnetic and a structural transition, which is accompanied by a huge magnetic-entropy change. A temperature-induced ferromagnetic (FM) to paramagnetic (PM) transition and a magnetic-field-induced PM to FM transition which are both of first order are observed in MnFeP1−xAsx compounds. Here the magnetic-phase transitions are not accompanied by structural transitions. Nevertheless, a large magnetic-entropy change, comparable with that in Gd5(Si1−xGex)4, is observed in the MnFeP1−xAsx compounds. In several of the RTiGe compounds, an applied magnetic field induces an antiferromagnetic (AF) to FM phase transition. Here, we observed a magnetic anisotropy dependence of the magnetic-entropy change. The Heusler alloy Ni53Mn22Ga25 exhibits a first-order martensitic transformation accompanied by a magnetic-phase transition around 220 K. The magnitude and the shape of the magnetic-entropy changes observed for this compound are quite different. Mn5Si3 compound exhibits two successive first-order magnetic-phase transitions and shows a different type of magnetocaloric effect (MCE). Mn1.95Cr0.05Sb exhibits an AF to FM phase transition and a negative MCE. The relationship between the magnetic-phase transitions and the MCE is discussed, based on the comparison of the observed MCEs and the exchange interactions in these materials.

Crystal structure and spiral magnetic ordering of BiFeO 3 doped with manganese

Abstract: Neutron powder diffraction has been performed on polycrystalline BiMnxFe1-xO3 (x=0, 0.1 and 0.2). The structures of the doped compounds are described by the space group R3c of ferroelectric BiFeO3. Refined structure parameters are presented. Mn doping generates microstructural changes manifested by broadening in the diffraction patterns. The lattice parameters show a non-linear behaviour from 4 K to 630 K. Mn doping results in a transformation of the long-range spiral spin modulation of BiFeO3 to a collinear antiferromagnetic structure with spins along c. The average magnetic moments and the ordering temperatures decrease with increasing Mn concentration.

Spin-polarized transport across sharp antiferromagnetic boundaries

Abstract: We report spin-polarized transport experiments across antiphase domain boundaries which act as atomically sharp magnetic interfaces. The antiphase boundaries are prepared by growing Fe(3)O(4) epitaxially on MgO, the magnetic coupling over a large fraction of these boundaries being antiferromagnetic. Magnetoresistance measurements yield linear and quadratic field dependence up to the anisotropy field for fields applied parallel and perpendicular to the film plane, respectively. This behavior can be explained by a hopping model in which spin-polarized electrons traverse an antiferromagnetic interface between two ferromagnetic chains.

Orbital-selective Mott-insulator transition in Ca 2 - x Sr x RuO 4

Abstract: The electronic structures of the metallic and insulating phases of the alloy series Ca2-xSrxRuO4 (0 ≤x ≤ 2) are calculated using LDA, LDA+U and Dynamical Mean-Field Approximation methods. In the end members the groundstate respectively is an orbitally non-degenerate antiferromagnetic insulator (x = 0) and a good metal (x = 2). For x > 0.5 the observed Curie-Weiss paramagnetic metallic state which possesses a local moment with the unexpected spin S = 1/2, is explained by the coexistence of localized and itinerant Ru-4d-orbitals. For 0.2 < x < 0.5 we propose a state with partial orbital and spin ordering. An effective model for the localized orbital and spin degrees of freedom is discussed. The metal-insulator transition at x = 0.2 is attributed to a switch in the orbital occupation associated with a structural change of the crystal.

Charge-ordered ferromagnetic phase in La 0.5 Ca 0.5 MnO 3

Abstract: Mixed-valent manganites are noted for their unusual magnetic, electronic and structural phase transitions. For example, the La1-xCaxMnO3 phase diagram1 shows that below transition temperatures in the range 100–260 K, compounds with 0.2 < x < 0.5 are ferromagnetic and metallic, whereas those with 0.5 < x < 0.9 are antiferromagnetic and charge ordered. In a narrow region around x = 0.5, these totally dissimilar ground states are thought to coexist2,3. It has been shown4 that charge order and charge disorder can coexist in the related compound, La0.25Pr0.375Ca0.375MnO3. Here we present electron microscopy data for La0.5Ca0.5MnO3 that shed light on the distribution of these coexisting phases, and uncover an additional, unexpected phase. Using electron holography and Fresnel imaging, we find micrometre-sized ferromagnetic regions spanning several grains coexisting with similar-sized regions with no local magnetization. Holography shows that the ferromagnetic regions have a local magnetization of 3.4 ± 0.2 Bohr magnetons per Mn atom (the spin-aligned value is 3.5 µB per Mn). We use electron diffraction and dark-field imaging to show that charge order exists in regions with no net magnetization and, surprisingly, can also occur in ferromagnetic regions.

Bound magnetic polaron interactions in insulating doped diluted magnetic semiconductors

Abstract: The magnetic behavior of insulating doped diluted magnetic semiconductors (DMS's) is characterized by the interaction of large collective spins known as bound magnetic polarons. Experimental measurements of the susceptibility of these materials have suggested that the polaron-polaron interaction is ferromagnetic, in contrast to the antiferromagnetic carrier-carrier interactions that are characteristic of nonmagnetic semiconductors. To explain this behavior, a model has been developed in which polarons interact via both the standard direct carrier-carrier exchange interaction (due to virtual carrier hopping) and an indirect carrier-ion-carrier exchange interaction (due to the interactions of polarons with magnetic ions in an interstitial region). Using a variational procedure, the optimal values of the model parameters were determined as a function of temperature. At temperatures of interest, the parameters describing polaron-polaron interactions were found to be nearly temperature-independent. For reasonable values of these constant parameters, we find that indirect ferromagnetic interactions can dominate the direct antiferromagnetic interactions and cause the polarons to align. This result supports the experimental evidence for ferromagnetism in insulating doped DMS's.

Magnetic superstructure in the two-dimensional quantum antiferromagnet SrCu2(BO3)2.

Abstract: We report the observation of magnetic superstructure in a magnetization plateau state of SrCu2(BO3)2, a frustrated quasi–two-dimensional quantum spin system. The Cu and B nuclear magnetic resonance (NMR) spectra at 35 millikelvin indicate an apparently discontinuous phase transition from uniform magnetization to a modulated superstructure near 27 tesla, above which a magnetization plateau at 1/8 of the full saturation has been observed. Comparison of the Cu NMR spectrum and the theoretical analysis of a Heisenberg spin model demonstrates the crystallization of itinerant triplets in the plateau phase within a large rhomboid unit cell (16 spins per layer) showing oscillations of the spin polarization. Thus, we are now in possession of an interesting model system to study a localization transition of strongly interacting quantum particles.

Interlayer magnetic coupling interactions of two ferromagnetic layers by spin polarized tunneling

Abstract: Magnetic interactions involving ferromagnetic layers separated by an insulating barrier have been studied experimentally on a fully epitaxial hard-soft magnetic tunnel junction: Fe/MgO/Fe/Co For a barrier thickness below 1 nm, a clear antiferromagnetic interaction is observed Moreover, when reducing the MgO thickness from 1 to 05 nm, the coupling strength increases up to J=-026 ergcm(-2) This behavior, well fitted by theoretical models, provides an unambiguous signature of the interlayer exchange coupling by spin-polarized quantum tunneling

Nonmagnetic Insulating States near the Mott Transitions on Lattices with Geometrical Frustration and Implications for κ-(ET)2Cu2(CN)3

Abstract: We study phase diagrams of the Hubbard model on anisotropic triangular lattices, which also represents a model for κ-type BEDT-TTF compounds. In contrast with mean-field predictions, path-integral renormalization group calculations show a universal presence of a nonmagnetic insulator sandwiched by an antiferromagnetic insulator and paramagnetic metals. The nonmagnetic phase does not show simple translational symmetry breakings such as flux phases, implying a genuine Mott insulator. We discuss possible relevance to the nonmagnetic insulating phase found in κ-(ET) 2 Cu 2 (CN) 3 .

Domain state model for exchange bias. II. Experiments

Abstract: The exchange bias coupling at ferro-/antiferromagnetic interfaces of epitaxially grown Co/CoO bilayers can be intentionally enhanced and controlled by diluting the antiferromagnetic CoO layer, i.e., by introducing (i) nonmagnetic substitutions $({\mathrm{Co}}_{1\ensuremath{-}x}{\mathrm{Mg}}_{x}\mathrm{O})$ or (ii) Co deficiencies $({\mathrm{Co}}_{1\ensuremath{-}y}\mathrm{O}).$ All intentional nonmagnetic cations or defects were placed away from the interface throughout the whole volume part of the antiferromagnetic layer. This way the roughness at the Co/CoO interface was kept practically the same. For both types of defects, the exchange bias field can be increased by a factor of 3 to 4. Hence, exchange bias is primarily not due to roughness at the interface but rather can be controlled by the defects in the volume part of the antiferromagnetic layer. We systematically investigate the dilution dependence of various phenomena of exchange bias, such as the vertical magnetization shift of the hysteresis loop, temperature dependence, training effect, cooling field dependence, and antiferromagnetic layer thickness dependence. All these phenomena are directly compared to results from Monte Carlo simulations and are shown to be consistently described by the domain state model for exchange bias. The combined experimental and theoretical findings suggest that the origin of exchange bias in Co/CoO results from a domain state in the volume part of the antiferromagnet stabilized by the defects.

Structural, magnetic, and electrical properties of single-crystalline La 1 − x Sr x MnO 3 ( 0.4 x 0.85 )

Abstract: We report on structural, magnetic, and electrical properties of Sr-doped ${\mathrm{LaMnO}}_{3}$ single crystals for doping levels $0.4l~xl~0.85.$ The complex structural and magnetic phase diagram can only be explained assuming significant contributions from the orbital degrees of freedom. Close to $x=0.6$ a ferromagnetic metal is followed by an antiferromagnetic metallic phase below 200 K. This antiferromagnetic metallic phase exists in a monoclinic crystallographic structure. Following theoretical predictions this metallic antiferromagnet is expected to reveal an ${(x}^{2}\ensuremath{-}{y}^{2})$-type orbital order. For higher Sr concentrations an antiferromagnetic insulator is established below room temperature.

Nonmagnetic Insulating States near the Mott Transitions on Lattices with Geometrical Frustration and Implications for $\kappa$-(ET)$_2$Cu$_2(CN)_3$

Abstract: We study phase diagrams of the Hubbard model on anisotropic triangular lattices, which also represents a model for $\kappa$-type BEDT-TTF compounds. In contrast with mean-field predictions, path-integral renormalization group calculations show a universal presence of nonmagnetic insulator sandwitched by antiferromagnetic insulator and paramagnetic metals. The nonmagnetic phase does not show a simple translational symmetry breakings such as flux phases, implying a genuine Mott insulator. We discuss possible relevance on the nonmagnetic insulating phase found in $\kappa$-(ET)$_2$Cu$_2(CN)_3$.

Competition between superconductivity and magnetism in ferromagnet/superconductor heterostructures

Abstract: The mutual influence of superconductivity and magnetism in F/S systems, i.e. systems of alternating ferromagnetic (F) and superconducting (S) layers, is comprehensively reviewed. For systems with ferromagnetic metal (FM) layers, a theory of the proximity effect in the dirty limit is constructed based on the Usadel equations. For an FM/S bilayer and an FM/S superlattice, a boundary-value problem involving finite FM/S boundary transparency and the diffusion and wave modes of quasi-particle motion is formulated; and the critical temperature Tc is calculated as a function of FM- and S-layer thicknesses. A detailed analysis of a large amount of experimental data amply confirms the proposed theory. It is shown that the superconducting state of an FM/S system is a superposition of two pairing mechanisms, Bardin – Cooper – Schrieffer's in S layers and Larkin – Ovchinnikov – Fulde – Ferrell's in FM ones. The competition between ferromagnetic and antiferromagnetic spontaneous moment orientations in FM layers is explored for the 0- and π-phase superconductivity in FM/S systems. For FI/S structures, where FI is a ferromagnetic insulator, a model for exchange interactions is proposed, which, along with direct exchange inside FI layers, includes indirect Ruderman – Kittel – Kasuya – Yosida exchange between localized spins via S-layer conduction electrons. Within this framework, possible mutual accommodation scenarios for superconducting and magnetic order parameters are found, the corresponding phase diagrams are plotted, and experimental results are explained. The results of the theory of the Josephson effect for S/F/S junctions are presented and the application of the theory of spin-dependent transport to F/S/F junctions is discussed. Application aspects of the subject are examined.

Anomalous magnetic properties of MnO nanoclusters.

Abstract: In this communication, we experimentally report, for the first time, that the MnO nanoclusters with cluster diameters of 5-10 nm show a ferromagnetic behavior with a phase transition from ferromagnetic to paramagnetic phases at 27 K even though their bulk phase is antiferromagnetic. We observed large coercivities up to 9500 Oe and a large remanence of 1.72 emu/g at 2 K, which are typically observed values for ferromagnetic materials. Although it is not clear, this abnormal ferromagnetic behavior of MnO nanoclusters may arise from cluster size effects.

Magnetic anisotropy of the antiferromagnetic ring [Cr8F8Piv16].

Abstract: A new tetragonal (P4212) crystalline form of [Cr8F8Piv16] (HPiv=pivalic acid, trimethyl acetic acid) is reported. The ring-shaped molecules, which are aligned in a parallel fashion in the unit cell, form almost perfectly planar, regular octagons. The interaction between the CrIII ions is antiferromagnetic (J=12 cm−1) which results in a S=0 spin ground state. The low-lying spin excited states were investigated by cantilever torque magnetometry (CTM) and high-frequency EPR (HFEPR). The compound shows hard-axis anisotropy. The axial zero-field splitting (ZFS) parameters of the first two spin excited states (S=1 and S=2, respectively) are D1=1.59(3) cm−1 or 1.63 cm−1 (from CTM and HFEPR, respectively) and D2=0.37 cm−1 (from HFEPR). The dipolar contributions to the ZFS of the S=1 and S=2 spin states were calculated with the point dipolar approximation. These contributions proved to be less than the combined single-ion contributions. Angular overlap model calculations that used parameters obtained from the electronic absorption spectrum, showed that the unique axis of the single-ion ZFS is at an angle of 19.3(1)° with respect to the ring axis. The excellent agreement between the experimental and the theoretical results show the validity of the used methods for the analysis of the magnetic anisotropy in antiferromagnetic CrIII rings.

Pressure-induced crystallization of a spin liquid

Abstract: Liquids are expected to crystallize at low temperature. The only exception is helium, which can remain liquid at 0 K, owing to quantum fluctuations1, 2. Similarly, the atomic magnetic moments (spins) in a magnet are expected to order at a temperature scale set by the Curie–Weiss temperature thetaCW (ref. 3). Geometrically frustrated magnets represent an exception. In these systems, the pairwise spin interactions cannot be simultaneously minimized because of the lattice symmetry4. This can stabilize a liquid-like state of short-range-ordered fluctuating moments well below thetaCW (refs 5–7). Here we use neutron scattering to observe the spin liquid state in a geometrically frustrated system, Tb2Ti2O7, under conditions of high pressure (approx9 GPa) and low temperature (approx1 K). This compound is a three-dimensional magnet with thetaCW = -19 K, where the negative value indicates antiferromagnetic interactions. At ambient pressure Tb2Ti2O7 remains in a spin liquid state down to at least 70 mK (ref. 8). But we find that, under high pressure, the spins start to order or 'crystallize' below 2.1 K, with antiferromagnetic order coexisting with liquid-like fluctuations. These results indicate that a spin liquid/solid mixture can be induced by pressure in geometrically frustrated systems.

The magnetic structure of YMnO3 perovskite revisited

Abstract: The magnetic structure of the orthorhombic perovskite YMnO3 has been investigated. A study on a polycrystalline sample based on neutron diffraction data and magnetization measurements has shown that YMnO3 becomes magnetically ordered below TN = 42?K. In the space group Pnma, the sinusoidal magnetic structure is defined by a (Cx,0,0) mode and characterized by the propagation vector k = (kx,0,0). The kx-component increases from 0.420(4), immediately below the ordering temperature, to 0.435(2) at T = 28.7?K. Below 28 K the kx-component remains unchanged. The sinusoidal spin arrangement remains stable down to 1.7?K; at this temperature the amplitude of the sinusoid is Ak = 3.89(6)??B. YMnO3 is the most distorted perovskite of the RMnO3 series (R?=?rare earths); the observed sinusoidal magnetic structure is in contrast with those exhibited by the less-distorted members (i.e.?LaMnO3), which are commensurate-type antiferromagnetic structures.

Magnetoresistive effect element, magnetic head, and magnetic reproducing apparatus

Abstract: In a CPP element using a metal intermediate layer excellent in shot noise and response to high frequencies unlike a TMR element, its magnetoresistive effect film includes a magnetic layer mainly made of a half-metal exhibiting ferromagnetism, ferrimagnetism or antiferromagnetism, and largely variable in way of conduction in response to spin direction of electrons.

Giant magnetoresistive sensor, thin-film read/write head and magnetic recording apparatus using the sensor

Abstract: A giant magnetoresistive sensor which is improved in reproduction output and peak asymmetry of read-back waveform. It is composed of a first free ferromagnetic film, a first non-magnetic film, a composite ferromagnetic film, a second non-magnetic film, and a second free ferromagnetic film, which are laminated sequentially, but has no antiferromagnetic film to fix said composite ferromagnetic film, and said composite ferromagnetic film contains a first, second, and third ferromagnetic film, which are antiferromagnetically coupled with one another, and also contains films which separate said ferromagnetic films from one another and antiferromagnetically couple them with one another.

Density-functional investigation of magnetism in δ -Pu

Abstract: We present density-functional results of δ-Pu obtained from three electronic-structure methods. These methods have their individual strengths and are used in combination to investigate the magnetic and crystal stability of δ-Pu. An all-electron, full potential linear muffin-tin orbitals (FPLMTO) method, that includes corrections for spin-orbit coupling and orbital-polarization effects, predicts δ-Pu to be an antiferromagnet at zero temperature with a volume and a bulk modulus in very good agreement with experiment. The site-projected magnetic moment is smaller than expected (∼1.5 μ B ) due to large cancellation of spin and orbital moments. These calculations also predict a mechanical instability of antiferromagnetic (AF) δ-Pu. In addition, techniques based on the Korringa-Kohn-Rostoker (KKR) method within a Green's-function formalism and a projector augmented wave (PAW) method predict the same behavior of δ-Pu. In order to study disordered magnetism in δ-Pu, the KKR Green's-function technique was used in conjunction with the disordered local-moment model, whereas for the FPLMTO and PAW methods this was accomplished within the special quasirandom structure model. While AF δ-Pu remains mechanically unstable at lower temperatures, paramagnetic δ-Pu is stabilized at higher temperatures where disordered magnetic moments are present and responsible for the crystal structure, the low density, and the low bulk modulus of this phase.

Coexisting ferro- and antiferromagnetism in Ni2MnAl Heusler alloys

Abstract: The structural and magnetic properties of stoichiometric Ni2MnAl are studied to clarify the conditions for ferromagnetic and antiferromagnetic ordering claimed to occur in this compound. X-ray and magnetization measurements show that although a single phase B2 structure can be stabilized at room temperature, a single L21 phase is not readily stabilized, but rather a mixed L21+B2 state occurs. The mixed state incorporates ferromagnetic and antiferromagnetic parts for which close-lying Curie and a Neel temperatures can be identified from magnetization measurements.