Atmospheric methane

About: Atmospheric methane is a research topic. Over the lifetime, 2034 publications have been published within this topic receiving 119616 citations.

Methanol Improves Methane Uptake in Starved Methanotrophic Microorganisms

Abstract: Methanotrophs in enrichment cultures grew and sustained atmospheric methane oxidation when supplied with methanol. If they were not supplied with methanol or formate, their atmospheric methane oxidation came to a halt, but it was restored within hours in response to methanol or formate. Indigenous forest soil methanotrophs were also dependent on a supply of methanol upon reduced methane access but only when exposed to a methane-free atmosphere. Their immediate response to each methanol addition, however, was to shut down the oxidation of atmospheric methane and to reactivate atmospheric methane oxidation as the methanol was depleted.

Stable atmospheric methane in the 2000s: key-role of emissions from natural wetlands

Abstract: Two atmospheric inversions (one fine-resolved and one process-discriminating) and a process-based model for land surface exchanges are brought together to analyse the variations of methane emissions from 1990 to 2009. A focus is put on the role of natural wetlands and on the years 2000-2006, a period of stable atmospheric concentrations. From 1990 to 2000, the top-down and bottom-up visions agree on the time-phasing of global total and wetland emission anomalies. The process-discriminating inversion indicates that wetlands dominate the time-variability of methane emissions (90% of the total variability). The contribution of tropical wetlands to the anomalies is found to be large, especially during the post-Pinatubo years (global negative anomalies with minima between -41 and -19 Tg yr(-1) in 1992) and during the alternate 1997-1998 El-Nino/1998-1999 La-Nina (maximal anomalies in tropical regions between +16 and +22 Tg yr(-1) for the inversions and anomalies due to tropical wetlands between +12 and +17 Tg yr(-1) for the process-based model). Between 2000 and 2006, during the stagnation of methane concentrations in the atmosphere, the top-down and bottom-up approaches agree on the fact that South America is the main region contributing to anomalies in natural wetland emissions, but they disagree on the sign and magnitude of the flux trend in the Amazon basin. A negative trend (-3.9 +/- 1.3 Tg yr(-1)) is inferred by the process-discriminating inversion whereas a positive trend (+1.3 +/- 0.3 Tg yr(-1)) is found by the process model. Although processed-based models have their own caveats and may not take into account all processes, the positive trend found by the B-U approach is considered more likely because it is a robust feature of the process-based model, consistent with analysed precipitations and the satellite-derived extent of inundated areas. On the contrary, the surface-data based inversions lack constraints for South America. This result suggests the need for a re-interpretation of the large increase found in anthropogenic methane inventories after 2000.

Global assessment of oil and gas methane ultra-emitters

Abstract: Methane emissions from oil and gas (O&G) production and transmission represent a considerable contribution to climate change. These emissions comprise sporadic releases of large amounts of methane during maintenance operations or equipment failures not accounted for in current inventory estimates. We collected and analyzed hundreds of very large releases from atmospheric methane images sampled by the TROPOspheric Monitoring Instrument (TROPOMI) between 2019 and 2020. Ultra-emitters are primarily detected over the largest O&G basins throughout the world. With a total contribution equivalent to 8 to 12% (~8 million metric tons of methane per year) of the global O&G production methane emissions, mitigation of ultra-emitters is largely achievable at low costs and would lead to robust net benefits in billions of US dollars for the six major O&G-producing countries when considering societal costs of methane.

Attribution of recent increases in atmospheric methane through 3-D inverse modelling

Abstract: . The atmospheric methane ( CH4 ) growth rate has varied considerably in recent decades. Unexplained renewed growth after 2006 followed 7 years of stagnation and coincided with an isotopic trend toward CH4 more depleted in 13C , suggesting changes in sources and/or sinks. Using surface observations of both CH4 and the relative change of isotopologue ratio ( δ13CH4 ) to constrain a global 3-D chemical transport model (CTM), we have performed a synthesis inversion for source and sink attribution. Our method extends on previous studies by providing monthly and regional attribution of emissions from six different sectors and changes in atmospheric sinks for the extended 2003–2015 period. Regional evaluation of the model CH4 tracer with independent column observations from the Greenhouse Gases Observing Satellite (GOSAT) shows improved performance when using posterior fluxes ( R=0.94 –0.96, RMSE =8.3 –16.5 ppb), relative to prior fluxes ( R=0.60 –0.92, RMSE =48.6 –64.6 ppb). Further independent validation with data from the Total Carbon Column Observing Network (TCCON) shows a similar improvement in the posterior fluxes ( R=0.87 , RMSE =18.8 ppb) compared to the prior fluxes ( R=0.69 , RMSE =55.9 ppb). Based on these improved posterior fluxes, the inversion results suggest the most likely cause of the renewed methane growth is a post-2007 1.8±0.4 % decrease in mean OH, a 12.9±2.7 % increase in energy sector emissions, mainly from Africa–Middle East and southern Asia–Oceania, and a 2.6±1.8 % increase in wetland emissions, mainly from northern Eurasia. The posterior wetland flux increases are in general agreement with bottom-up estimates, but the energy sector growth is greater than estimated by bottom-up methods. The model results are consistent across a range of sensitivity analyses. When forced to assume a constant (annually repeating) OH distribution, the inversion requires a greater increase in energy sector ( 13.6±2.7 %) and wetland ( 3.6±1.8 %) emissions and an 11.5±3.8 % decrease in biomass burning emissions. Assuming no prior trend in sources and sinks slightly reduces the posterior growth rate in energy sector and wetland emissions and further increases the magnitude of the negative OH trend. We find that possible tropospheric Cl variations do not influence δ13CH4 and CH4 trends, although we suggest further work on Cl variability is required to fully diagnose this contribution. While the study provides quantitative insight into possible emissions variations which may explain the observed trends, uncertainty in prior source and sink estimates and a paucity of δ13CH4 observations limit the robustness of the posterior estimates.