Atmospheric methane

About: Atmospheric methane is a research topic. Over the lifetime, 2034 publications have been published within this topic receiving 119616 citations.

El Nino, The 2006 Indonesian Peat Fires, And The Distribution Of Atmospheric Methane

Abstract: [1] Dry conditions from a moderate El Nino during the fall of 2006 resulted in enhanced burning in Indonesia with fire emissions of CO approximately 4–6 times larger than the prior year. Here we use new tropospheric methane and CO data from the Aura Tropospheric Emission Spectrometer and new CO profile measurements from the Terra Measurements of Pollution in the Troposphere (MOPITT) satellite instruments with the Goddard Earth Observing System (GEOS)-Chem model to estimate methane emissions of 4.25 ± 0.75 Tg for October–November 2006 from these fires. Errors in convective parameterization in GEOS-Chem, evaluated by comparing MOPITT and GEOS-Chem CO profiles, are the primary uncertainty of the emissions estimate. The El Nino related Indonesian fires increased the tropical distribution of atmospheric methane relative to 2005, indicating that tropical biomass burning can compensate for expected decreases in tropical wetland methane emissions from reduced rainfall during El Nino as found in previous studies.

Performance evaluation of a 1.6-µm methane DIAL system from ground, aircraft and UAV platforms.

Abstract: Methane is an efficient absorber of infrared radiation and a potent greenhouse gas with a warming potential 72 times greater than carbon dioxide on a per molecule basis. Development of methane active remote sensing capability using the differential absorption lidar (DIAL) technique enables scientific assessments of the gas emission and impacts on the climate. A performance evaluation of a pulsed DIAL system for monitoring atmospheric methane is presented. This system leverages a robust injection-seeded pulsed Nd:YAG pumped Optical Parametric Oscillator (OPO) laser technology operating in the 1.645 µm spectral band. The system also leverages an efficient low noise, commercially available, InGaAs avalanche photo-detector (APD). Lidar signals and error budget are analyzed for system operation on ground in the range-resolved DIAL mode and from airborne platforms in the integrated path DIAL (IPDA) mode. Results indicate system capability of measuring methane concentration profiles with <1.0% total error up to 4.5 km range with 5 minute averaging from ground. For airborne IPDA, the total error in the column dry mixing ratio is less than 0.3% with 0.1 sec average using ground returns. This system has a unique capability of combining signals from the atmospheric scattering from layers above the surface with ground return signals, which provides methane column measurement between the atmospheric scattering layer and the ground directly. In such case 0.5% and 1.2% total errors are achieved with 10 sec average from airborne platforms at 8 km and 15.24 km altitudes, respectively. Due to the pulsed nature of the transmitter, the system is relatively insensitive to aerosol and cloud interferences. Such DIAL system would be ideal for investigating high latitude methane releases over polar ice sheets, permafrost regions, wetlands, and over ocean during day and night. This system would have commercial potential for fossil fuel leaks detection and industrial monitoring applications.

Copper enhances the activity and salt resistance of mixed methane-oxidizing communities

Abstract: Effluents of anaerobic digesters are an underestimated source of greenhouse gases, as they are often saturated with methane. A post-treatment with methane-oxidizing bacterial consortia could mitigate diffuse emissions at such sites. Semi-continuously fed stirred reactors were used as model systems to characterize the influence of the key parameters on the activity of these mixed methanotrophic communities. The addition of 140 mg L(-1) NH (4) (+) -N had no significant influence on the activity nor did a temperature increase from 28 degrees C to 35 degrees C. On the other hand, addition of 0.64 mg L(-1) of copper(II) increased the methane removal rate by a factor of 1.5 to 1.7 since the activity of particulate methane monooxygenase was enhanced. The influence of different concentrations of NaCl was also tested, as effluents of anaerobic digesters often contain salt levels up to 10 g NaCl L(-1). At a concentration of 11 g NaCl L(-1), almost no methane-oxidizing activity was observed in the reactors without copper addition. Yet, reactors with copper addition exhibited a sustained activity in the presence of NaCl. A colorimetric test based on naphthalene oxidation showed that soluble methane monooxygenase was inhibited by copper, suggesting that the particulate methane monooxygenase was the active enzyme and thus more salt resistant. The results obtained demonstrate that the treatment of methane-saturated effluents, even those with increased ammonium (up to 140 mg L(-1) NH (4) (+) -N) and salt levels, can be mitigated by implementation of methane-oxidizing microbial consortia.