Topic
Bipolaron
About: Bipolaron is a research topic. Over the lifetime, 1335 publications have been published within this topic receiving 29154 citations. The topic is also known as: bipolarons.
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TL;DR: In this paper, the structure of a one-dimensional bipolaron was studied, taking into account three types of correlation effects: such as interelectronic correlations caused by the direct dependence of the wave function on the distance between electrons as well as the one-center and two-center correlations.
4 citations
TL;DR: The time constants (tau1) were found to be temperature dependent confirming the earlier findings in Na-NaI melts that ionic diffusion almost exclusively controls the dynamics of excess electrons in high temperature ionic liquids.
Abstract: Temperature-dependent investigations of excess electrons in molten solutions of cesium-doped cesium iodide (Cs-CsI) (mole fraction of Cs approximately 0.003) were performed applying femtosecond pump-probe absorption spectroscopy. The pulse-limited induced bleach observed at probe wavelengths from 600 to 1240 nm was attributed to the excitation of equilibrated excess electrons which were initially formed by melting a Cs-CsI mixture. The interpretation of the relaxation process is based on strongly localized polarons that constitute the majority of defect states in this melt. As expected, the bipolaron contribution was insignificant. The time constants (tau1) were found to be temperature dependent confirming our earlier findings in Na-NaI melts that ionic diffusion almost exclusively controls the dynamics of excess electrons in high temperature ionic liquids. Apart from this temperature dependence, the relaxation dynamics of excess electrons do not differ irrespective of the excitation regime (blue or red part of the respective stationary spectra).
4 citations
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TL;DR: In this paper, an exponentially large, low-field and necessarily positive magnetoresistance effect is predicted in the presence of Hubbard interaction and spin-dynamics under certain conditions.
Abstract: We develop a theory of magnetoresistance based on variable-range hopping. An exponentially large, low-field and necessarily positive magnetoresistance effect is predicted in the presence of Hubbard interaction and spin-dynamics under certain conditions. The theory was developed with the recently discovered organic magnetoresistance in mind. To account for the experimental observation that the organic magnetoresistance effect can also be negative, we tentatively amend the theory with a mechanism of bipolaron formation.
4 citations
TL;DR: In this article, the collision processes between two acoustic polarons, two acoustic bipolarons, and a polaron and a bipolaron in a one-dimensional electron-lattice system are analyzed by numerical simulations based on Su, Schrieffer and Heeger's model extended to include short-ranged Coulombic electron-electron interactions.
Abstract: The collision processes between two acoustic polarons, two acoustic bipolarons, and a polaron and a bipolaron in a one-dimensional electron-lattice system are analyzed by numerical simulations based on Su, Schrieffer and Heeger's model extended to include short-ranged Coulombic electron-electron interactions. The collisions between two polarons with the same spin and between two bipolarons are essentially elastic because of a rather strong repulsion due to the Pauli principle. On the other hand, those between two polarons with opposite spins and between a polaron and a bipolaron show some inelastic behaviors depending on the relative velocity of the two objects before the collision. This knowledge will serve to understand the dynamics of the system when many polarons and/or bipolarons are created in the system e.g. by photoexcitation.
4 citations
TL;DR: In this paper, a copolymer from polyacetylene and polyazine can be found on the metallic regime and it is shown that the bipolaron type of defect is formed on the copolymers.
4 citations