Topic
Charge ordering
About: Charge ordering is a research topic. Over the lifetime, 3575 publications have been published within this topic receiving 81615 citations.
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TL;DR: X-ray diffraction experiments reveal that spatial charge ordering occurs in the pseudogap state of YBa2Cu3O6.67 as discussed by the authors, which competes with high-temperature superconductivity, and their relative strengths can be tuned using a magnetic field.
Abstract: X-ray diffraction experiments reveal that spatial charge ordering occurs in the pseudogap state of YBa2Cu3O6.67. Moreover, this charge ordered state competes with high-temperature superconductivity, and their relative strengths can be tuned using a magnetic field.
830 citations
TL;DR: It is found that a minimum thickness of five LaTiO3 layers is required for the centre titanium site to recover bulk-like electronic properties, and this represents a framework within which the short-length-scale electronic response can be probed and incorporated in thin-film oxide heterostructures.
Abstract: The nature and length scales of charge screening in complex oxides are fundamental to a wide range of systems, spanning ceramic voltage-dependent resistors (varistors), oxide tunnel junctions and charge ordering in mixed-valence compounds. There are wide variations in the degree of charge disproportionation, length scale, and orientation in the mixed-valence compounds: these have been the subject of intense theoretical study, but little is known about the microscopic electronic structure. Here we have fabricated an idealized structure to examine these issues by growing atomically abrupt layers of LaTi(3+)O(3) embedded in SrTi(4+)O(3). Using an atomic-scale electron beam, we have observed the spatial distribution of the extra electron on the titanium sites. This distribution results in metallic conductivity, even though the superlattice structure is based on two insulators. Despite the chemical abruptness of the interfaces, we find that a minimum thickness of five LaTiO(3) layers is required for the centre titanium site to recover bulk-like electronic properties. This represents a framework within which the short-length-scale electronic response can be probed and incorporated in thin-film oxide heterostructures.
829 citations
TL;DR: In this article, a survey of microscopic factors determining the coexistence of magnetite and ferroelectricity is given, and different possible routes to combine them in one material are discussed, in particular, the role of the occupation of d-states in transition metal perovskites, possible role of spiral magnetic structures, and the mechanism of ferro electricity in magnetic systems due to combination of site-centered and bond-centred charge ordering.
812 citations
TL;DR: The manganese oxides of general formula RE1−xMxMnO3 (RE = rare earth, M = Ca, Sr, Ba, Pb) have remarkable interrelated structural, magnetic and transport properties induced by the mixed valence (3+−4+) of the Mn ions.
Abstract: The manganese oxides of general formula RE1−xMxMnO3 (RE = rare earth, M = Ca, Sr, Ba, Pb) have remarkable interrelated structural, magnetic and transport properties induced by the mixed valence (3+–4+) of the Mn ions. In particular, they exhibit very large negative magnetoresistance, called colossal magnetoresistance (CMR), in the vicinity of metal–insulator transition for certain compositions. In this review paper, we summarize the most important features of the physics of the CMR manganites. The growth techniques for manganese oxide thin films, which are the basic material for potential applications, are reviewed and their structure and morphology examined in relation to growth parameters. The effects of epitaxial strains on the physical properties are discussed. Early works on superlattices and devices are presented.
775 citations
TL;DR: Using density-functional calculations, a three-band spinless model Hamiltonian is suggested for the description of the Verwey transition using a Stoner model as well as from calculations within the framework of the local-spin-density approximation to the density- functional theory.
Abstract: Using density-functional calculations, we examine the electronic structure of magnetite in the spinel crystal structure in order to gain insight into the nature of the Verwey transition. The calculated cohesive and magnetic properties are in agreement with experimental results. The magnetic structure is analyzed using a Stoner model as well as from calculations within the framework of the local-spin-density approximation to the density-functional theory. The calculations show a minority-spin band at the Fermi energy consisting of ${\mathit{t}}_{2\mathit{g}}$ orbitals on the Fe(B) sublattice. These results suggest a three-band spinless model Hamiltonian for the description of the Verwey transition. The hopping integrals and the electron interaction parameters entering the model Hamiltonian are calculated using the ``constrained'' density-functional theory. The calculated parameters are consistent with the electronic origin of the Verwey transition.
610 citations