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Exciton

About: Exciton is a research topic. Over the lifetime, 31603 publications have been published within this topic receiving 810642 citations.


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Journal ArticleDOI
TL;DR: In this paper, a simple variational approach was applied to quantify the effect of exciton in carbon nanotubes, and the apower law with exponent ∼-0.6 was obtained for the binding energy dependence on nanotube radius.
Abstract: Excitons in quasi-one-dimensional semiconductors may lower the optical transition energies by a substantial amount. To quantify the effect in carbon nanotubes, we apply a simple variational approach. In excitonic units, apower law with exponent ∼-0.6 is obtained for the binding energy dependence on nanotube radius. When converted to ordinary units, the ratio of binding energy to tight-binding band gap yields a roughly constant value of nearly 40%. This substantial ratio implies that exciton effects are of prime importance for the optical properties of carbon nanotubes.

188 citations

Journal ArticleDOI
TL;DR: It is found that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton- phonon coupling, and a significant fraction of the spectral weight of the absorption peak is transferred to a distinct exciton+phonon sideband, which is peaked at around 200 meV above the main absorption peak.
Abstract: We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred to a distinct $\mathrm{\text{exciton}}+\mathrm{\text{phonon}}$ sideband, which is peaked at around 200 meV above the main absorption peak. This sideband provides a distinctive signature of the excitonic character of the optical transition. The exciton-phonon coupling is reflected in a dynamical structural distortion, which contributes a binding energy of up to 100 meV. The distortion is surprisingly long ranged, and is strongly dependent on chirality.

188 citations

Journal ArticleDOI
TL;DR: It is demonstrated that the observed renormalization of the Rabi frequency is induced by fluctuations in the bath of longitudinal acoustic phonons, an effect that is a phonon analogy of the Lamb shift.
Abstract: We study optically driven Rabi rotations of a quantum dot exciton transition between 5 and 50 K, and for pulse areas of up to 14 pi In a high driving field regime, the decay of the Rabi rotations is nonmonotonic, and the period decreases with pulse area and increases with temperature By comparing the experiments to a weak-coupling model of the exciton-phonon interaction, we demonstrate that the observed renormalization of the Rabi frequency is induced by fluctuations in the bath of longitudinal acoustic phonons, an effect that is a phonon analogy of the Lamb shift

187 citations

Journal ArticleDOI
TL;DR: In this article, the effect of confinement on the exciton binding energies has been systematically investigated for two series of ZnO/ZnMgO multiquantum wells with various well widths and barrier heights.
Abstract: The effect of confinement on the exciton binding energies has been systematically investigated for two series of ZnO/ZnMgO multiquantum wells with various well widths and barrier heights. The exciton binding energies were extracted from the energy difference between the stimulated emission band induced by inelastic exciton–exciton scattering and the free exciton absorption band. The binding energies of excitons are found to be sensitively dependent on the well widths. The experimental results of the well width dependence of binding energies are in good agreement with Coli and Bajaj’s theoretical calculations for these structures [G. Coli and K. K. Bajaj, Appl. Phys. Lett. 78, 2861 (2001)]. The remarkable reduction in coupling strength between excitons and longitudinal optical phonons is closely correlated with the enhancement of the exciton binding energy, indicating that the stability of excitons is greatly increased by the enhancement of exciton binding energy in quantum wells.

187 citations

Journal ArticleDOI
TL;DR: In this article, the authors investigated the competition between induced absorption in the singlet S 1 → S n and triplet T 1 → T n excited electronic configurations and bleaching of the S 0 → S 1 transition.

187 citations


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Performance
Metrics
No. of papers in the topic in previous years
YearPapers
20231,269
20222,623
20211,045
20201,157
20191,096
20181,057