Femtosecond

About: Femtosecond is a research topic. Over the lifetime, 35106 publications have been published within this topic receiving 691405 citations. The topic is also known as: 1 E-15 s & fs.

Micromachining of photonic devices by femtosecond laser pulses

Abstract: In this paper we review the micromachining of photonic devices in several materials by means of ultrashort laser pulses. The physical mechanisms underlying the refractive index modification and the different laser systems used to induce such modification are discussed. A thorough review of the photonic devices demonstrated with the femtosecond laser microfabrication technique is presented. In particular, this paper is focused on photonic devices based on optical waveguides. The devices are organized into two categories: passive and active devices. In the former category power splitters, directional couplers, interferometers and Bragg gratings are reviewed, while in the latter amplifiers and lasers are discussed. Finally, conclusions and future perspectives of femtosecond laser micromachining in photonics are provided.

Electrooptical generation and detection of femtosecond electrical transients

Abstract: Recent work on the generation of ultrashort electrical pulses by optical rectification of femtosecond optical pulses in electrooptic materials is summarized. This technique, which is called electrooptic Cherenkov radiation, is described in detail with particular emphasis on the effects of dispersion due to coupling to lattice vibrational resonances. Recent experimental results in lithium tantalate are described which illustrate these effects. When the duration of the exciting femto second optical pulse is comparable to the period of the lattice vibrations, a pronounced ringing is observed in the electrical waveforms. A coupled oscillator model is used to develop a theory that accurately accounts for these effects and can be used to predict the limiting speed of response and generation efficiency of different electrooptic materials. >

Femtosecond pulse shaping by an evolutionary algorithm with feedback

Abstract: We report on computer controlled compression of femtosecond laser pulses using a programmable liquid crys- tal spatial light modulator which is feedback-controlled by an evolutionary algorithm. This algorithm generates the opti- mal laser field on the basis of feedback from the experiment by optimizing the laser pulse iteratively. Without knowledge of the (chirped) input pulses, the experimental signal (second harmonic light=SHG) is maximized by the algorithm, thus re- sulting in fully compressed pulses. This method only makes use of the experiment's response (SHG signal) on the formed pulses. No other parameters need to be considered. This ap- proach leads to many experimental applications in all fields of optics and ultrafast spectroscopy where particularly shaped pulses are advantageous.

Vibrational cooling after ultrafast photoisomerization of azobenzene measured by femtosecond infrared spectroscopy

Abstract: The vibrational cooling of azobenzene after photoisomerization is investigated by time resolved IR spectroscopy with femtosecond time resolution. Transient difference spectra were obtained in a frequency range where phenyl ring modes and the central N=N-stretching mode absorbs. The experimental data are discussed in terms of a simple theoretical model which was derived in order to account for the off-diagonal anharmonicity between the investigated high-frequency modes and the bath of the remaining low-frequency modes in a polyatomic molecule. It is shown that these off-diagonal anharmonic constants dominate the observed transient absorbance changes while the anharmonicity of the high-frequency modes themselves (diagonal anharmonicity) causes only minor effects. Based on the transient IR spectra, the energy flow in the azobenzene molecule can be described as follows: After an initial ultrafast intramolecular energy redistribution process, the decay of the related intramolecular temperature occurs via intermolecular energy transfer to the solvent on a time scale of ca. 20 ps.