Four-wave mixing

About: Four-wave mixing is a research topic. Over the lifetime, 7530 publications have been published within this topic receiving 112702 citations.

Optical Frequency Combs Generated by Four-Wave Mixing in Optical Fibers for Astrophysical Spectrometer Calibration and Metrology

Abstract: Optical frequency combs generated by multiple four-wave mixing of two stabilized single-frequency lasers in optical fibers are proposed for use as high precision frequency markers, calibration of astrophysical spectrometers and metrology. Use of highly nonlinear and photonic crystal fibers with very short lengths and small group velocity dispersion, combined with energy and momentum conservation required by the parametric generation, assures negligible phase mismatch between comb frequencies. In contrast to combs from mode-locked lasers or microcavities, the absence of a resonator allows large tuning of the frequency spacing from tens of gigahertz to beyond teraHertz.

Self‐pumped phase conjugation with a new mechanism in KTa1−xNbxO3:Fe crystals

Abstract: A new model is proposed to explain the origin of the self‐pumped phase conjugation (SPPC) that we have observed in KTa1−xNbxO3:Fe crystals. In this model SPPC is generated by both four‐wave mixing and backscattering processes rather than by only one of them. The advantage of this kind of phase conjugator is also discussed.

100-Gb/s multiple-channel output all-optical OTDM demultiplexing using multichannel four-wave mixing in a semiconductor optical amplifier

Abstract: We present a successful demonstration of ultra-fast all-optical time-division demultiplexing with simultaneous multiple-channel output, a vital function for all-optical demultiplexers. The demultiplexing operation is based on multichannel four-wave mixing (FWM) in a semiconductor optical amplifier. Error-free, simultaneous live-channel-output, 100-6.3-Gb/s demultiplexing is successfully performed.

Combined third-harmonic generation and four-wave mixing microscopy of tissues and embryos

Abstract: Nonlinear microscopy can be used to probe the intrinsic optical properties of biological tissues. Using femtosecond pulses, third-harmonic generation (THG) and four-wave mixing (FWM) signals can be efficiently produced and detected simultaneously. Both signals probe a similar parameter, i.e. the real part of the third-order nonlinear susceptibility χ((3)). However THG and FWM images result from different phase matching conditions and provide complementary information. We analyze this complementarity using calculations, z-scan measurements on water and oils, and THG-FWM imaging of cell divisions in live zebrafish embryos. The two signals exhibit different sensitivity to sample size and clustering in the half-wavelength regime. Far from resonance, THG images reveal spatial variations |Δχ((3))(-3ω;ω,ω,ω)| with remarkable sensitivity while FWM directly reflects the distribution of χ((3))(-2ω(1) + ω(2);ω(1), -ω(2), ω(1)). We show that FWM images provide χ((3)) maps useful for proper interpretation of cellular THG signals, and that combined imaging carries additional structural information. Finally we present simultaneous imaging of intrinsic THG, FWM, second-harmonic (SHG) and two-photon-excited fluorescence (2PEF) signals in live Caenorhabditis elegans worms illustrating the information provided by multimodal nonlinear imaging of unstained tissue.

Time-resolved four-wave-mixing spectroscopy for inner-valence transitions

Abstract: Non-collinear four-wave mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between spatially localized inner-valence transitions among different sites of a molecule in the extreme ultraviolet (XUV) spectral range have not been observed yet. As an experimental step towards this goal we perform time-resolved FWM spectroscopy with femtosecond NIR and attosecond XUV pulses. The first two pulses (XUV-NIR) coincide in time and act as coherent excitation fields, while the third pulse (NIR) acts as a probe. As a first application we show how coupling dynamics between odd- and even-parity inner-valence excited states of neon can be revealed using a two-dimensional spectral representation. Experimentally obtained results are found to be in good agreement with ab initio time-dependent R-matrix calculations providing the full description of multi-electron interactions, as well as few-level model simulations. Future applications of this method also include site-specific probing of electronic processes in molecules.