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Showing papers on "Haze published in 2009"


Proceedings ArticleDOI
20 Jun 2009
TL;DR: A simple but effective image prior - dark channel prior to remove haze from a single input image is proposed, based on a key observation - most local patches in haze-free outdoor images contain some pixels which have very low intensities in at least one color channel.
Abstract: In this paper, we propose a simple but effective image prior - dark channel prior to remove haze from a single input image. The dark channel prior is a kind of statistics of the haze-free outdoor images. It is based on a key observation - most local patches in haze-free outdoor images contain some pixels which have very low intensities in at least one color channel. Using this prior with the haze imaging model, we can directly estimate the thickness of the haze and recover a high quality haze-free image. Results on a variety of outdoor haze images demonstrate the power of the proposed prior. Moreover, a high quality depth map can also be obtained as a by-product of haze removal.

847 citations


Journal ArticleDOI
TL;DR: In this paper, the characteristics of PAHs, organic carbon, elemental carbon and water-soluble inorganic ions were studied under four periods (summer normal, summer haze, winter normal and winter haze).

229 citations


Journal ArticleDOI
TL;DR: In this paper, the authors used transmission electron microscopy (TEM) coupled with energy-dispersive X-ray (EDX) microanalyses to analyze 332 mineral dust particles together with their coatings.
Abstract: . Nitrate compounds have received much attention because of their ability to alter the hygroscopic properties and cloud condensation nuclei (CCN) activity of mineral dust particles in the atmosphere. However, very little is known about specific characteristics of ambient nitrate-coated mineral particles on an individual particle scale. In this study, sample collection was conducted during brown haze and dust episodes between 24 May and 21 June 2007 in Beijing, northern China. Sizes, morphologies, and compositions of 332 mineral dust particles together with their coatings were analyzed using transmission electron microscopy (TEM) coupled with energy-dispersive X-ray (EDX) microanalyses. Structures of some mineral particles were verified using selected-area electron diffraction (SAED). TEM observation indicates that approximately 90% of the collected mineral particles are covered by visible coatings in haze samples whereas only 5% are coated in the dust sample. 92% of the analyzed mineral particles are covered with Ca-, Mg-, and Na-rich coatings, and 8% are associated with K- and S-rich coatings. The majority of coatings contain Ca, Mg, O, and N with minor amounts of S and Cl, suggesting that they are possibly nitrates mixed with small amounts of sulfates and chlorides. These nitrate coatings are strongly correlated with the presence of alkaline mineral components (e.g., calcite and dolomite). CaSO4 particles with diameters from 10 to 500 nm were also detected in the coatings including Ca(NO3)2 and Mg(NO3)2. Our results indicate that mineral particles in brown haze episodes were involved in atmospheric heterogeneous reactions with two or more acidic gases (e.g., SO2, NO2, HCl, and HNO3). Mineral particles that acquire hygroscopic nitrate coatings tend to be more spherical and larger, enhancing their light scattering and CCN activity, both of which have cooling effects on the climate.

206 citations


Journal ArticleDOI
TL;DR: In this paper, the authors analyzed multidecadal data of horizontal visibility, and found that the frequency of low-visibility conditions such as fog, mist and haze has declined in Europe over the past 30 years, for all seasons and all visibility ranges between distances of 0 and 8 km.
Abstract: Surface solar radiation has undergone decadal variations, producing global ‘dimming’ and ‘brightening’ effects, probably owing to changes in aerosol burden and clouds. An analysis of multidecadal data of horizontal visibility shows that the occurrence of fog, mist and haze has declined in Europe over the past 30 years. Surface solar radiation has undergone decadal variations since the middle of the twentieth century, producing global ‘dimming’ and ‘brightening’ effects1,2. These variations presumably result from changes in aerosol burden and clouds3, but the detailed processes involved have yet to be determined. Over Europe, the marked solar radiation increase since the 1980s is thought to have contributed to the observed large continental warming4, but this contribution has not been quantified. Here we analyse multidecadal data of horizontal visibility, and find that the frequency of low-visibility conditions such as fog, mist and haze has declined in Europe over the past 30 years, for all seasons and all visibility ranges between distances of 0 and 8 km. This decline is spatially and temporally correlated with trends in sulphur dioxide emissions, suggesting a significant contribution of air-quality improvements. Statistically linking local visibility changes with temperature variations, we estimate that the reduction in low-visibility conditions could have contributed on average to about 10–20% of Europe’s recent daytime warming and to about 50% of eastern European warming. Large improvements in air quality and visibility already achieved in Europe over the past decades may mean that future reductions in the frequency of low-visibility events will be limited, possibly leading to less rapid regional warming.

189 citations


Journal ArticleDOI
TL;DR: In this article, a near-infrared transit photometry of the nearby hot-Jupiter HD 189733b was performed using the NICMOS instrument during five transits, with three transits executed with a narrowband filter at 1.87 μm and two performed with a wideband filter on 1.66 μm.
Abstract: We present Hubble Space Telescope near-infrared transit photometry of the nearby hot-Jupiter HD 189733b. The observations were taken with the NICMOS instrument during five transits, with three transits executed with a narrowband filter at 1.87 μ ma nd two performed with a narrowband filter at 1.66 μm. Our observing strategy using narrowband filters is insensitive to the usual HST intraorbit and orbit-to-orbit measurement of systematic errors, allowing us to accurately and robustly measure the near-IR wavelength dependance of the planetary radius. Our measurements fail to reproduce the previously claimed detection of an absorption signature of atmospheric H2 Ob elow 2μ ma t a5 σ confidence level. We measure a planet-to-star radius contrast of 0.15498± 0.00035 at 1.66 μm and a contrast of 0.15517 ± 0.00019 at 1.87 μm. Both of our near-IR planetary radii values are in excellent agreement with the levels expected from Rayleigh scattering by sub-micron haze particles, observed at optical wavelengths, indicating that upper-atmospheric haze still dominates the near-IR transmission spectra over the absorption from gaseous molecular species at least below 2 μm.

183 citations


Journal ArticleDOI
01 Jul 2009-Icarus
TL;DR: In this paper, the authors analyzed a unique, three-dimensional data set of Uranus acquired with the STIS Hubble spectrograph on August 19, 2002, covering a full afternoon hemisphere at 300 and 1000 nm wavelength at 1 nm resolution.

181 citations


Journal ArticleDOI
TL;DR: Wang et al. as mentioned in this paper presented the patterns and trends of haze over 31 provincial capitals in China between 1980 and 2005, based on human visual range observations at 31 synoptic meteorological stations operated by the China Meteorological Administration.
Abstract: This paper presents the patterns and trends of haze over 31 provincial capitals in China between 1980 and 2005. The haze measurements were based on human visual range observations at 31 synoptic meteorological stations operated by the China Meteorological Administration (CMA). The high haze regions were found in largely populated cities such as Chongqing, Beijing, and Shenyang, while the low haze regions were located in the cities with small populations such as Lhasa, Kunming, and Guiyang in southwestern China and Haikou in southern China. The haziness of the 12 cities shows a significantly (95%) decreasing trend, while that of the 13 cities shows a significantly increasing trend over the 25-year study period. The increases are evident in the eastern and southwestern cities in China. It has also been found that there is a decreasing haze trend in winter but an increasing trend in summer for many cities. Nonetheless, the causality for the reduction of aerosol emissions has not been established. This report is the first survey and preliminary analysis done on haze patterns and trends from 1980 to 2005 over the capital cities of 31 provinces in Mainland China.

179 citations


Journal ArticleDOI
TL;DR: The result illustrated that the serious air pollution in haze episodes was strongly correlated with the meteorological conditions; the shorter air masses transport distance, the worse air quality and visibility in Guangzhou, indicating the strong domination of local sources contributing to haze formation.
Abstract: The chemical characteristics (water-soluble ions and carbonaceous species) of PM2.5 in Guangzhou were measured during a typical haze episode. Most of the chemical species in PM2.5 showed significant difference between normal and haze days. The highest contributors to PM2.5 were organic carbon (OC), nitrate, and sulfate in haze days and were OC, sulfate, and elemental carbon (EC) in normal days. The concentrations of secondary species such as, NO3(-), SO4(2-), and NH4(+) in haze days were 6.5, 3.9, and 5.3 times higher than those in normal days, respectively, while primary species (EC, Ca(2+), K(+)) show similar increase from normal to haze days by a factor about 2.2-2.4. OC/EC ratio ranged from 2.8 to 6.2 with an average of 4.7 and the estimation on a minimum OC/EC ratio showed that SOC (secondary organic carbon) accounted more than 36.6% for the total organic carbon in haze days. The significantly increase in the secondary species (SOC, NO3(-), SO4(2-), and NH4(+)), especially in NO3(-), caused the worst air quality in this region. Simultaneously, the result illustrated that the serious air pollution in haze episodes was strongly correlated with the meteorological conditions. During the sampling periods, air pollution and visibility had a good relationship with the air mass transport distance; the shorter air masses transport distance, the worse air quality and visibility in Guangzhou, indicating the strong domination of local sources contributing to haze formation. High concentration of the secondary aerosol in haze episodes was likely due to the higher oxidation rates of sulfur and nitrogen species.

164 citations


Journal ArticleDOI
TL;DR: In this paper, a near-infrared transit photometry of the nearby hot-Jupiter HD189733b was performed using the NICMOS instrument during five transits.
Abstract: We present Hubble Space Telescope near-infrared transit photometry of the nearby hot-Jupiter HD189733b. The observations were taken with the NICMOS instrument during five transits, with three transits executed with a narrowband filter at 1.87 microns and two performed with a narrowband filter at 1.66 microns. Our observing strategy using narrowband filters is insensitive to the usual HST intra-orbit and orbit-to-orbit measurement of systematic errors, allowing us to accurately and robustly measure the near-IR wavelength dependance of the planetary radius. Our measurements fail to reproduce the Swain et al. absorption signature of atmospheric water below 2 microns at a 5-sigma confidence level. We measure a planet-to-star radius contrast of 0.15498+/-0.00035 at 1.66 microns and a contrast of 0.15517+/-0.00019 at 1.87 microns. Both of our near-IR planetary radii values are in excellent agreement with the levels expected from Rayleigh scattering by sub-micron haze particles, observed at optical wavelengths, indicating that upper-atmospheric haze still dominates the near-IR transmission spectra over the absorption from gaseous molecular species at least below 2 microns.

153 citations


Journal ArticleDOI
TL;DR: In this paper, the authors focus on measurements of aerosol chemical composition to assess trends in Arctic haze aerosol and implications for source regions, the interaction between pollution-derived and ocean-derived aerosols and the resulting impacts on the chemistry of the Arctic boundary layer, and the response of aerosols to a changing climate.
Abstract: . Aerosol measurements at Barrow, Alaska during the past 30 years have identified the long range transport of pollution associated with Arctic Haze as well as ocean-derived aerosols of more local origin. Here, we focus on measurements of aerosol chemical composition to assess (1) trends in Arctic Haze aerosol and implications for source regions, (2) the interaction between pollution-derived and ocean-derived aerosols and the resulting impacts on the chemistry of the Arctic boundary layer, and (3) the response of aerosols to a changing climate. Aerosol chemical composition measured at Barrow, AK during the Arctic haze season is compared for the years 1976–1977 and 1997–2008. Based on these two data sets, concentrations of non-sea salt (nss) sulfate (SO4=) and non-crustal (nc) vanadium (V) have decreased by about 60% over this 30 year period. Consistency in the ratios of nss SO4=/ncV and nc manganese (Mn)/ncV between the two data sets indicates that, although emissions have decreased in the source regions, the source regions have remained the same over this time period. The measurements from 1997–2008 indicate that, during the haze season, the nss SO4= aerosol at Barrow is becoming less neutralized by ammonium (NH4+) yielding an increasing sea salt aerosol chloride (Cl−) deficit. The expected consequence is an increase in the release of Cl atoms to the atmosphere and a change in the lifetime of volatile organic compounds (VOCs) including methane. In addition, summertime concentrations of biogenically-derived methanesulfonate (MSA−) and nss SO4= are increasing at a rate of 12 and 8% per year, respectively. Further research is required to assess the environmental factors behind the increasing concentrations of biogenic aerosol.

108 citations


Journal ArticleDOI
TL;DR: In this paper, a data set acquired by eight particle-dedicated instruments set up on the SIRTA (Site Instrumental de Recherche par Teledetection Atmospherique, which is French for Instrumented Site for Atmospheric Remote Sensing Research) during the ParisFog field campaign is exploited to document microphysical properties of particles contributing to extinction of visible radiation in variable situations.

Book ChapterDOI
01 Jan 2009
TL;DR: In this paper, the authors review the photochemical and thermochemical equilibrium theories for the formation of condensate clouds and photochemical haze in Saturn's upper troposphere and stratosphere and show the relevant observations from ground-based and spacecraft instruments.
Abstract: In this chapter we review the photochemical and thermochemical equilibrium theories for the formation of condensate clouds and photochemical haze in Saturn's upper troposphere and stratosphere and show the relevant observations from ground-based and spacecraft instruments. Based on thermochemical equilibrium models we expect ammonia ice crystals to dominate in the high troposphere. There is very little spectral evidence to confirm this idea. Thanks to a stellar occultation observed by the Cassini VIMS instrument we now have spectral evidence for a hydrocarbon stratospheric haze component, and we still seek evidence for an expected diphosphine stratospheric haze component. The vertical distributions of stratospheric and upper tropospheric hazes have been mapped well with ground-based and Hubble Space telescope data, and Cassini data are beginning to add to this picture. Polar stratospheric aerosols are dark at UV wavelengths and exhibit strong Rayleigh-like polarization which suggests that auroral processes are important for their formation as is the case for the jovian polar stratospheric haze. The cloud and haze structure exhibits a variety of temporal variation, including seasonal change, long-term secular change near the equator, and short-term changes with a complicated latitudinal structure, and still not understood. Cassini instruments, especially the VIMS instrument, show an abundance of small-scale structure (convective clouds) at a pressure near 2 bar.

Journal ArticleDOI
TL;DR: In this article, the spectral properties of the upper haze of the Venus mesosphere were investigated using three spectrometers with a wavelength range from ultraviolet to mid-infrared and an altitude range from 70 to >100 km.
Abstract: The Spectroscopy for Investigation of Characteristics of the Atmosphere of Venus/Solar Occultation at Infrared (SPICAV/SOIR) suite of instruments onboard the Venus Express spacecraft comprises three spectrometers covering a wavelength range from ultraviolet to midinfrared and an altitude range from 70 to >100 km. However, it is only recently (more than 1 year after the beginning of the mission) that the three spectrometers can operate simultaneously in the solar occultation mode. These observations have enabled the study of the properties of the Venusian mesosphere over a broad spectral range. In this manuscript, we briefly describe the instrument characteristics and the method used to infer haze microphysical properties from a data set of three selected orbits. Discussion focuses on the wavelength dependence of the continuum, which is primarily shaped by the extinction caused by the aerosol particles of the upper haze. This wavelength dependence is directly related to the effective particle radius (cross section weighted mean radius) of the particles. Through independent analyses for the three channels, we demonstrate the potential to characterize the aerosols in the mesosphere of Venus. The classical assumption that the upper haze is only composed of submicron particles is not sufficient to explain the observations. We find that at high northern latitudes, two types of particles coexist in the upper haze of Venus: mode 1 of mean radius 0.1 ≤ rg ≤ 0.3 μm and mode 2 of 0.4 ≤ rg ≤ 1.0 μm. An additional population of micron-sized aerosols seems, therefore, needed to reconcile the data of the three spectrometers. Moreover, we observe substantial temporal variations of aerosol extinction over a time scale of 24 h.

Journal ArticleDOI
TL;DR: The geometric mean diameters (GMDs) of organic aerosols are larger in the fine mode during the hazy days, suggesting aerosols emitted from the wheat straw burning are larger than those from fossil fuel combustion, and fine particle coagulation and organic compound repartitioning were enhanced.
Abstract: Size-segregated aerosol samples were collected in urban Nanjing, China during summer and autumn of 2007 including a period of hazy days during June 1−5. Organic aerosols in the haze event were characterized by elevated concentrations of levoglucosan, high molecular weight (HMW) n-alkanes, and HMW fatty acids due to the emissions from field burning of wheat straw. In contrast, organic aerosols on nonhazy days were characterized by a predominance of fossil fuel combustion products. Levoglucosan (4030 ng m−3), n-alkanes (1520 ng m−3), fatty acids (2629 ng m−3), and PAHs (57 ng m−3) in the haze samples were 3−40 times more abundant than those in nonevent samples. Approximately 30−90% of the organics during the haze period can be attributed to wheat straw burning. Concentrations of particulate material (PM) mass, n-alkanes, and low molecular weight (LMW) PAHs showed a unimodal size distribution, peaking at 0.7−1.1 μm during the hazy days, and a bimodal distribution, peaking at 0.7−1.1 μm and 4.7−5.8 μm during ...

Journal ArticleDOI
01 Jun 2009-Icarus
TL;DR: By comparing observations from the Cassini imaging system, UV spectrometer, and Huygens atmospheric structure instrument, this article determined an apparent radius of ∼40 nm, an imaginary index < 0.3 at 187.5 nm and a number density of ∼30 particles at 520 km in Titan's mesosphere.

Journal ArticleDOI
TL;DR: This paper derives several methods for estimating parameters of the airlight, particularly its degree of polarization (DOP), when the sky is not in view, and proposes blind estimation of the DOP, based on the image data.
Abstract: Outdoor imaging in haze is plagued by poor visibility. A major problem is spatially-varying reduction of contrast by airlight, which is scattered by the haze particles towards the camera. However, images can be compensated for haze, and even yield a depth map of the scene. A key step in such scene recovery is subtraction of the airlight. In particular, this can be achieved by analyzing polarization-filtered images. This analysis requires parameters of the airlight, particularly its degree of polarization (DOP). These parameters were estimated in past studies by measuring pixels in sky areas. However, the sky is often unseen in the field of view. This paper derives several methods for estimating these parameters, when the sky is not in view. The methods are based on minor prior knowledge about a couple of scene points. Moreover, we propose blind estimation of the DOP, based on the image data. This estimation is based on independent component analysis (ICA). The methods were demonstrated in field experiments.

Journal ArticleDOI
TL;DR: In this article, the authors studied the trends of PM2.5 (particles with an aerodynamic diameter of 2.5 µm or less) concentrations and source apportionment in Lahore, Pakistan.
Abstract: The work reported in this paper was carried out to study the trends of PM2.5 (particles with an aerodynamic diameter of 2.5 µm or less) concentrations and source apportionment of PM2.5 monitored at an urban residential site in Lahore, Pakistan. PM2.5 aerosol samples were collected for 2 days in a week at 12 h interval in a day, both in dry and wet seasons, on ZefluorTM filter papers using Thermo-Electron Corporation Reference Ambient Air Sampler (RAAS). Total 310 samples were collected during the period under study, i.e., from November 2005 to December 2007. High PM2.5 loads were observed in winter, which were approximately 4 times greater than those observed in the summer, spring, fall and monsoon seasons in the yearlong measurements. Source apportionment was performed on short duration analysis results of November 2005 to March 2006 using Positive Matrix Factorization (PMF) model. The results derived from PMF model indicated that the major contributors to PM2.5 in Lahore are: soil/road dust, industrial emissions, vehicular emissions and secondary aerosols. It is, therefore, concluded that in addition to local vehicular and industrial emissions, the city is also affected from trans-boundary air pollutants particularly due to secondary aerosols (especially SO42-) during winter which increase PM2.5 concentrations manifold when relatively less mixing height exists. The sulfate particles also facilitate in haze/fog formation during calm highly humid conditions, thus reduce visibility and increase the incidents of respiratory diseases encountered in the city every year.

Journal ArticleDOI
TL;DR: In this paper, the optical and microphysical parameters from severe haze events observed in October 2005 at Gwangju, Korea (35.10°N, 126.53°E) were determined from the ground using a multi-wavelength Raman lidar, a sunphotometer, and a real-time carbon particle analyzer and from space using satellite retrievals.

Journal ArticleDOI
TL;DR: The presence of H(2) on early Earth could thus have favored warmer surface temperatures and yet allowed photochemical haze formation to deliver complex organic species to early Earth's surface.
Abstract: Recent attempts to resolve the faint young Sun paradox have focused on an early Earth atmosphere with elevated levels of the greenhouse gases methane (CH(4)) and carbon dioxide (CO(2)) that could have provided adequate warming to Earth's surface. On Titan, the photolysis of CH(4) has been shown to create a thick haze layer that cools its surface. Unlike Titan, however, early Earth's atmosphere likely contained high amounts of CO(2) and hydrogen (H(2)). In this work, we examine haze formation in an early Earth atmosphere composed of CO(2), H(2), N(2), and CH(4), with a CO(2)/CH(4) ratio of 10 and a H(2)/CO(2) ratio of up to 15. To initiate aerosol formation, a broad-spectrum ultraviolet (UV) energy source with emission at Lyman-alpha was used to simulate the solar spectrum. Aerosol composition and total aerosol mass produced as a function of reagent gas were measured with an aerosol mass spectrometer (AMS). Results show an order of magnitude decrease in haze production with the addition of H(2), with no significant change in the chemical composition of the haze. We calculate that the presence of H(2) on early Earth could thus have favored warmer surface temperatures and yet allowed photochemical haze formation to deliver complex organic species to early Earth's surface.

Journal ArticleDOI
Sönke Szidat1
23 Jan 2009-Science
TL;DR: Radiocarbon analysis elucidates the sources of the pollutants responsible for the "brown clouds" over South Asia.
Abstract: Radiocarbon analysis elucidates the sources of the pollutants responsible for the "brown clouds" over South Asia.

Journal ArticleDOI
TL;DR: In this paper, the satellite observations are used to heuristically separate polar thin ice clouds into two crystal size categories, and an aerosol index based on the attenuated backscattering and color ratio of the sampled volumes is used for identifying haze in cloud-free regions.
Abstract: [1] Data sets from CloudSat radar reflectivity and CALIPSO lidar backscattering measurements provide a new regard on Arctic and Antarctic winter cloud systems, as well as on the way aerosols determine their formation and evolution. Especially, links between the cloud ice crystal size and the surrounding aerosol field may be further investigated. In this study, the satellite observations are used to heuristically separate polar thin ice clouds into two crystal size categories, and an aerosol index based on the attenuated backscattering and color ratio of the sampled volumes is used for identifying haze in cloud-free regions. Statistics from 386 Arctic satellite overpasses during January 2007 and from 379 overpasses over Antarctica during July 2007 reveal that sectors with the highest proportion of thin ice clouds having large ice crystals at their top are those for which the aerosol index is highest. Moreover, a weak but significant correlation between the cloud top ice effective radius and the above-cloud aerosol index suggests that more polluted clouds tend to have higher ice effective radius, in 10 of the 11 sectors investigated. These results are interpreted in terms of a sulphate-induced freezing inhibition effect.

Journal ArticleDOI
TL;DR: Interface haze is associated with an ultra-thin femtosecond laser flap setting of 90 microm and younger age among eyes following LASIK for myopia.

Journal ArticleDOI
TL;DR: In this article, the authors used multivariate linear regression to determine the types of dust-causing events that contribute to low visibility at a given site when the sum of extinction from coarse mass (CM) and fine soil (FS) was larger than any other aerosol component and the reconstructed aerosol extinction coefficient was among the 20% highest (calculated on a calendar year basis) for that site.
Abstract: [1] Aerosol data from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, air mass backward trajectories, land use maps, soil characteristics maps, diagnostic ratios of elemental composition, and multivariate linear regression were utilized as part of a semiquantitative analysis. The purpose of the analysis was to determine the types of dust-causing events that contribute to low visibility at a given site when the sum of extinction from coarse mass (CM) and fine soil (FS) was larger than any other aerosol component and the reconstructed aerosol extinction coefficient was among the 20% highest (calculated on a calendar year basis) for that site. For these “worst dust days,” the above tools were used to ascribe the cause of low visibility to one of the following types of events: (1) transcontinental transport of dust originating from Asia; (2) windblown dust events from sources located nearby the site and; (3) transport of windblown dust from sources upwind of the site. Depending on the weight of evidence, a low or high level of confidence was associated with the assignment of one of these three events. Absence of convincing evidence resulted in ascribing the worst dust day to “undetermined events.” Of the 610 worst dust days over the 2001–2003 period, 51% were associated with one of the three event types with high confidence and an additional 30% were accounted for with low confidence. Of the 496 worst dust days associated with an event (either low or high confidence), Asian dust was the assigned event on 55 days (for 2001–2002), locally generated windblown dust on 201 days, and transport from upwind source areas susceptible to wind erosion on 240 days. Events associated with windblown episodes from source areas in the United States and Mexico exhibited the highest dust concentrations. Asian dust events were associated with lower dust concentrations and a larger FS-to-CM ratio. Some variations between Asian dust and continental North American dust were observed in organic matter (OMC), black carbon (LAC), and nitrate (NO3−) content. None of the tools used in this study was adequate for identifying events associated with mechanically released dust by anthropogenic activities including, agriculture, construction and motor vehicle travel on paved and unpaved roads. Some of the worst dust days may have been caused by these types of activities, especially in central Arizona and northern and Southern California, where the fraction of undetermined events was higher than in other regions within the western United States. All in all, the methods and results of this study can help improve the performance of large-scale dust emission models and provide insight into the distribution of the types of events that cause dust resultant haze in relatively remote areas of the western United States.

Book ChapterDOI
TL;DR: The nature of protein-polyphenol interaction and its effect on haze particles, analysis of haze constituents, and stabilization of beverages against haze formation are reviewed.
Abstract: Beverages such as beer, wine, clear fruit juices, teas, and formulated products with similar ingredients are generally expected by consumers to be clear (free of turbidity) and to remain so during the normal shelf life of the product. Hazy products are often regarded as defective and perhaps even potentially harmful. Since consumers are usually more certain of what they perceive visually than of what they taste or smell, the development of haze in a clear product can reduce the likelihood of repeat purchasing of a product and can have serious economic consequences to a producer. Hazes are caused by suspended insoluble particles of colloidal or larger size that can be perceived visually or by instruments. Hazes in clear beverages can arise from a number of causes, but are most often due to protein-polyphenol interaction. The nature of protein-polyphenol interaction and its effect on haze particles, analysis of haze constituents, and stabilization of beverages against haze formation are reviewed.

Journal ArticleDOI
TL;DR: Thermal measurements by the Cassini spacecraft show that the mixing ratios of all photochemical species, except ethylene, increase with altitude at equatorial and southern latitudes, reflecting transport from a high-altitude source to a condensation sink in the lower stratosphere.
Abstract: Our present knowledge of the composition and chemistry of Titan’s stratosphere is reviewed. Thermal measurements by the Cassini spacecraft show that the mixing ratios of all photochemical species, except ethylene, increase with altitude at equatorial and southern latitudes, reflecting transport from a high-altitude source to a condensation sink in the lower stratosphere. Most compounds are enriched at latitudes northward of 458 N, a consequence of subsidence in the winter polar vortex. This enrichment is much stronger for nitriles and complex hydrocarbons than for ethane and acetylene. Titan’s chemistry originates from breakdown of methane due to photodissociation in the upper atmosphere and catalytical reactions in the stratosphere, and from destruction of nitrogen both by UV photons and electrons. Photochemistry also produces haze particles made of complex refractory material, albeit at a lower rate than ethane, the most abundant gas product. Haze characteristics (vertical distribution, physical and spectral properties) inferred by several instruments aboard Cassini/Huygens are discussed here.

Journal ArticleDOI
TL;DR: In this article, the authors used the Models-3 Community Multi-scale Air Quality modeling system with meteorological fields simulated by the Fifth-generation National Center for Atmospheric Research/Penn State University Mesoscale Model (MM5) from September 26th to September 30th, 2004.
Abstract: The atmospheric haze over the Pearl River Delta (PRD) was investigated by using the Models-3 Community Multi-scale Air Quality modeling system with meteorological fields simulated by the Fifth-generation National Center for Atmospheric Research/Penn State University Mesoscale Model (MM5) from September 26th to September 30th, 2004. The model-simulated meteorological elements and particulate matter with aerodynamic diameter less than 10 μm (PM10) were compared with observations at four air quality-monitoring stations. The results showed that MM5 successfully reproduced the diurnal variations of temperature, wind speed, and wind directions at these stations. The temporal variations of the simulated values were consistent with those of the observed (such as temperature, wind speed, and wind direction). The correlation coefficient was 0.91 for temperature and 0.56 for wind speed. The modeling results show that the spatial distributions of simulated PM10 were closely related to the source emissions indicating three maxima of PM10 over the PRD. The sea–land breezes diurnal cycle played a significant role in the redistribution and transport of PM10. Nighttime land breeze could transport PM10 to the coast and the sea, while daytime sea breeze (SB) could carry the accumulated PM10 offshore back to the inland cities. PM10 could also be transported vertically to a height of up to about 1000 m because of strong turbulence in the SB front. Process analyses indicated that the emission sources and the vertical diffusion were the major processes to influence the concentrations of particulate matter with aerodynamic diameter less than 2.5 μm (PM2.5).

Journal ArticleDOI
TL;DR: This paper compares the measurement results from different methods, presents the effect of the white standard, and analyses the measurement uncertainty.
Abstract: Transmittance haze is increasingly important to the LCD and solar cell industry. Most commercial haze measurement instruments are designed according to the method recommended in the documentary standards like ASTM D 1003 (ASTM 2003 Standard Test Method for Haze and Luminous Transmittance of Transparent Plastics), JIS K 7361 (JIS 1997 Plastics—Determination of the Total Luminous Transmittance of Transparent Materials—Part 1: Single Beam Instrument) and ISO 14782 (ISO 1997 Plastics—Determination of Haze of Transparent Materials). To improve the measurement accuracy of the current standards, a new apparatus was designed by the Center for Measurement Standards (Yu et al 2006 Meas. Sci. Technol. 17 N29–36). Besides the methods mentioned above, a double-beam method is used in the design of some instruments. There are discrepancies between the various methods. But no matter which method is used, a white standard is always needed. This paper compares the measurement results from different methods, presents the effect of the white standard, and analyses the measurement uncertainty.

Journal ArticleDOI
TL;DR: SO2 emission reduction is the most beneficial control strategy in reducing summertime PM2.5 levels and improving visibility in the Southeast and electric generating utilities are the single largest source of SO2.

Posted Content
TL;DR: In this paper, the intensity and morphology of the WMAP haze using a multi-linear regression involving full-sky templates of the dominant forms of galactic foreground emission, using two different CMB sky signal estimators.
Abstract: Observations by the Wilkinson Microwave Anisotropy Probe (WMAP) satellite have identified an excess of microwave emission from the centre of the Milky Way. It has been suggested that this WMAP haze emission could potentially be synchrotron emission from relativistic electrons and positrons produced in the annihilations of one (or more) species of dark matter particles. In this paper we re-calculate the intensity and morphology of the WMAP haze using a multi-linear regression involving full-sky templates of the dominant forms of galactic foreground emission, using two different CMB sky signal estimators. The first estimator is a posterior mean CMB map, marginalized over a general foreground model using a Gibbs sampling technique, and the other is the ILC map produced by the WMAP team. Earlier analyses of the WMAP haze used the ILC map, which is more contaminated by galactic foregrounds than the Gibbs map. In either case, we re-confirm earlier results that a statistically significant residual emission remains after foreground subtraction that is concentrated around the galactic centre. However, we find that the significance of this emission can be significantly reduced by allowing for a subtle spatial variation in the frequency dependence of soft synchrotron emission in the inner and outer parts of the galaxy. We also re-investigate the prospect of a neutralino dark matter interpretation of the origin of the haze, and find that significant boosting in the dark matter annihilation rate is required, relative to that obtained with a smooth galactic dark matter distribution, in order to reproduce the inferred residual emission, contrary to that deduced in several recent studies.

Journal ArticleDOI
TL;DR: In this paper, synchrotron emission from electron-positron pairs injected into the interstellar medium by the galactic population of pulsars with energies in the 1 to 100 GeV range can explain the frequency spectrum of WMAP haze and the drop in the average haze power with latitude.
Abstract: The WMAP haze is an excess in the 22 to 93 GHz frequency bands of WMAP extending about 10 degrees from the galactic center We show that synchrotron emission from electron-positron pairs injected into the interstellar medium by the galactic population of pulsars with energies in the 1 to 100 GeV range can explain the frequency spectrum of the WMAP haze and the drop in the average haze power with latitude The same spectrum of high energy electron-positron pairs from pulsars, which gives rise to the haze, may also generate the observed excesses in AMS, HEAT and PAMELA We discuss the spatial morphology of the pulsar synchrotron signal and its deviation from spherical symmetry, which may provide an avenue to determine the pulsar contribution to the haze