High harmonic generation

About: High harmonic generation is a research topic. Over the lifetime, 11694 publications have been published within this topic receiving 222650 citations. The topic is also known as: HHG.

Polarization State of High-Order Harmonic Emission from Aligned Molecules

Abstract: High harmonic emission in isotropic gases is polarized in the same direction as the incident laser polarization. Laser-induced molecular alignment allows us to break the symmetry of the gas medium. By using aligned molecules in high harmonic generation experiments, we show that the polarization of the extreme ultraviolet emission depends strongly on the molecular alignment and the orbital structure. Polarization measurements give insight into the molecular orbital symmetry. Furthermore, molecular alignment will allow us to produce attosecond pulses with time-dependent polarization.

Harmonic generation in CO2 laser target interaction

Abstract: We report the observation of an extended series of integral harmonic lines in the spectrum of direct backscatter of 10.6‐μm radiation incident at intensities ≳1014 W/cm2 onto planar solid targets. We have observed and spectrally resolved up to the eleventh harmonic (0.95 μm) at intensities well above the plasma continuum background.

Attosecond localization of electrons in molecules

Abstract: Numerical solutions of the time-dependent Schrodinger equation for a 1D model non-Born–Oppenheimer H are used to illustrate the nonlinear nonperturbative response of molecules to intense (I ≥ 1013 W/cm2), ultrashort (t < 10 fs) laser pulses. Molecular high-order harmonic generation (MHOHG) is shown to be an example of such response and the resulting nonlinear photon emission spectrum is shown to lead to the synthesis of single attosecond (10−18 s) pulses. Application of such ultrashort pulses to the H system results in localized electron wavepackets whose motion can be detected by asymmetry in the photoelectron spectrum generated by a subsequent probe attosecond pulse, thus leading to measurement of electron motion in molecules on the attosecond time scale. © 2004 Wiley Periodicals, Inc. Int J Quantum Chem, 2004

Phase measurement for surface infrared-visible sum-frequency generation

Abstract: We present what are to our knowledge the first measurements of the phase of the infrared-visible sum-frequency generation signal. We introduce two techniques and apply the measurements to the determination of the polar orientation of a selected group of atoms within an adsorbed molecule.

Coulomb corrections and polarization effects in high-intensity high-harmonic emission

Abstract: We describe a quasiclassical approach to correct electron motion following tunneling ionization in intense laser fields, for the presence of the Coulomb potential. The technique is applied to model the dependence of high-harmonic generation on the ellipticity of the incident laser field. We present experimental data on the harmonics with photon energies close to the ionization potential of an atom, identify their source, and explain their unusual dependence on the ellipticity of the incident laser field. Our calculations are in good agreement with experimental data. \textcopyright{} 1996 The American Physical Society.