Optical microcavity

About: Optical microcavity is a research topic. Over the lifetime, 2599 publications have been published within this topic receiving 72125 citations. The topic is also known as: optical microcavities.

Guest-responsive polaritons in a porous framework: chromophoric sponges in optical QED cavities

Abstract: Introducing porous material into optical cavities is a critical step toward the utilization of quantum-electrodynamical (QED) effects for advanced technologies, e.g. in the context of sensing. We demonstrate that crystalline, porous metal–organic frameworks (MOFs) are well suited for the fabrication of optical cavities. In going beyond functionalities offered by other materials, they allow for the reversible loading and release of guest species into and out of optical resonators. For an all-metal mirror-based Fabry–Perot cavity we yield strong coupling (∼21% Rabi splitting). This value is remarkably large, considering that the high porosity of the framework reduces the density of optically active moieties relative to the corresponding bulk structure by ∼60%. Such a strong response of a porous chromophoric scaffold could only be realized by employing silicon-phthalocyanine (SiPc) dyes designed to undergo strong J-aggregation when assembled into a MOF. Integration of the SiPc MOF as active component into the optical microcavity was realized by employing a layer-by-layer method. The new functionality opens up the possibility to reversibly and continuously tune QED devices and to use them as optical sensors.

Real-time monitoring of the enzymatic reaction of urease by using whispering gallery mode lasing

Abstract: A new strategy is reported here to monitor the enzymatic reactions in real time by using whispering gallery mode (WGM) lasing. The optical microcavity is formed via the self-assembly of an ultraviolet (UV)-treated nematic liquid crystal (LC) 4-cyano-4’-pentylbiphenyl (5CB). The single UV-treated 5CB microdroplet serves as both optical resonator and sensing reactor. The microdroplet configuration transitions induced wavelength shift in the WGM lasing spectra can be used as an indicator for the enzymatic reaction. The proposed sensor has a sub-microgram detection limit of urease (∼0.5 µg/ml), which is lower than the detection limit of currently available urease sensor based on LC materials. Our experimental results demonstrate that WGM lasing has unique advantages in the real-time monitoring of enzymatic reactions compared, for instance, with observation of the optical appearance under a polarized optical microscope.

Optical spectra of a quantum dot in a microcavity in the nonlinear regime

Abstract: The optical emission spectrum of a quantum dot in strong coupling with the single mode of a microcavity is obtained in the nonlinear regime. We study how exciton-exciton interactions alter the emission spectrum of the system, bringing the linear Rabi doublet into a multiplet structure that is strongly dependent on the cavity-exciton energy detuning. We emphasize how nonlinearity can be used to evidence the genuine quantum nature of the coupling by producing satellites peaks of the Rabi doublet that originate from the quantized energy levels of the interactions.

One- and two-photon photocurrents from tunable organic microcavity photodiodes

Abstract: We have constructed multilayer thin-film organic microcavity photodiodes with the photoactive layer comprised of a spin-coated conjugated polymer and an evaporated C60 layer. The electrodes are designed as semitransparent mirrors which form a resonant cavity structure. The photocurrent spectra show distinct maxima at the optical resonances of the cavities, which are located up to 200 nm below the fundamental optical transition of the polymer. The design allows a simple tuning of the spectral response by varying the layer thickness. Microcavity photodiodes are also shown to be highly sensitive two-photon detectors, which exhibit a factor 500 improvement in the two-photon response compared to devices without photonic confinement.

Micro-cavity laser having increased sensitivity

Abstract: An optically pumped micro-cavity laser has an optical gain cavity and an optical resonant cavity. The optical gain cavity has a gain medium disposed that generates an optical output in response to an optical pump signal. The optical resonant cavity has an electro-optic material in which is disposed an electrode structure with first and second apertures disposed generally parallel to an optical signal propagating within the electro-optic material. Electrically conductive material is disposed within the apertures coupling an electrical signal to the optical cavity. Optically reflective material is disposed on the opposing surfaces of the micro-cavity laser and between the optical gain cavity and the optical resonant cavity.