Showing papers on "Quadrupole published in 2021"

Generalized hybrid anapole modes in all-dielectric ellipsoid particles[Invited]

Abstract: Numerous exciting optical effects in all-dielectric high-refractive-index structures are associated with so-called toroidal electrodynamics. Among these effects are anapoles, nonradiated states caused by interference phenomena, e.g. between electric dipole and toroidal dipole modes. For a spherical particle it is possible to reach simultaneous destructive interference for electric, magnetic, and corresponding toroidal dipole modes (so-called hybrid anapole mode), by varying the refractive index and/or particle size. However, there are no sufficient degrees of freedom within spherical geometry to extend the hybrid anapole mode effect to higher multipoles. Due to the optical theorem, it is also impossible to create the ideal anapole with destructive interference for all multipoles under plane wave illumination. In principle, it is possible to suppress radiation losses for the finite number of multipoles only by constructing the nanoantenna with complex geometry. Our approach of the hybrid anapole state excitation, we demonstrate in ellipsoidal all-dielectric particle providing cancellation of both electric and magnetic scattering up to quadrupole modes. This effect is achieved due to the optimised geometry of the ellipsoidal particle. Moreover, we provide classification of novel anapoles arising due to interference between moments and their mean- square radii (MSR) of electric, magnetic and toroidal family and introduce generalized anapoles for high order interaction between moments. Our concept is useful for the design of light controlling devices, reflectionless metasurfaces, high Q-factor opened resonators and nonscattering particle development.

Probing triaxial deformation of atomic nuclei in high-energy heavy ion collisions

Abstract: Most atomic nuclei are deformed with a quadrupole shape described by its overall strength $\beta_2$ and triaxiality $\gamma$. The deformation can be accessed in high-energy heavy-ion collisions by measuring the collective flow response of the produced quark-gluon plasma to the eccentricity $\varepsilon_2$ and the density gradient $d_{\perp}$ in the initial state. Using analytical estimate and a Glauber model, we show that the variances, $\langle\varepsilon_2^2\rangle$ or $\langle(\delta d_{\perp}/d_{\perp})^2\rangle$, and skewnesses, $\langle\varepsilon_2^2\delta d_{\perp}/d_{\perp}\rangle$ or $\langle(\delta d_{\perp}/d_{\perp})^3\rangle$, have a simple analytical form of $a'+b'\beta_2^2$ and $a'+(b'+c'\cos(3\gamma))\beta_2^3$, respectively. From these, we constructed several normalized skewnesses to isolate the $\gamma$ dependence from that of $\beta_2$, and show that the correlations between any normalized skewness and any variance can constrain simultaneously the $\beta_2$ and $\gamma$. Assuming a linear relation with elliptic flow $v_2$ and mean-transverse momentum $[p_{\mathrm{T}}]$ of final state particles, $v_2\propto \varepsilon_2$ and $\delta d_{\perp}/d_{\perp} \propto \delta[p_{\mathrm{T}}]/[p_{\mathrm{T}}]$, similar conclusions are also expected for the variances and skewnesses of $v_2$ and $[p_{\mathrm{T}}]$, which can be measured precisely in top RHIC and LHC energies. Our findings motivate a dedicated system scan of high-energy heavy ion collisions to measure triaxiality of atomic nuclei. This is better done by collisions of prolate, $\cos(3\gamma)=1$, and oblate nuclei, $\cos(3\gamma)=-1$, with well known $\beta_2$ values to calibrate the coefficients $b'$ and $c'$, followed by collisions of species of interest especially those with known $\beta_2$ but unknown $\gamma$.

Multipole expansion of gravitational waves: from harmonic to Bondi coordinates

Abstract: We transform the metric of an isolated matter source in the multipolar post-Minkowskian approximation from harmonic (de Donder) coordinates to radiative Newman-Unti (NU) coordinates. To linearized order, we obtain the NU metric as a functional of the mass and current multipole moments of the source, valid all-over the exterior region of the source. Imposing appropriate boundary conditions we recover the generalized Bondi-van der Burg-Metzner-Sachs residual symmetry group. To quadratic order, in the case of the mass-quadrupole interaction, we determine the contributions of gravitational-wave tails in the NU metric, and prove that the expansion of the metric in terms of the radius is regular to all orders. The mass and angular momentum aspects, as well as the Bondi shear, are read off from the metric. They are given by the radiative quadrupole moment including the tail terms.

Possible quadrupole density wave in the superconducting Kondo lattice CeRh2As2

Abstract: CeRh2As2 has recently been reported to be a rare case of multi-phase unconventional superconductor [S. Khim et al., arXiv:2101.09522] close to a quantum critical point (QCP). Here, we present a comprehensive study of its normal state properties and of the phase (I) below To ~ 0.4 K which preempts superconductivity at Tc = 0.26 K. The 2nd-order phase transition at To presents signatures in specific heat and thermal expansion, but none in magnetization and ac-susceptibility, indicating a non-magnetic origin of phase I. In addition, an upturn of the in-plane resistivity at To points to a gap opening at the Fermi level in the basal plane. Thermal expansion indicates a strong positive pressure dependence of To , dTo/dp = 1.5 K/GPa, in contrast to the strong negative pressure coefficient observed for magnetic order in Ce-based Kondo lattices close to a QCP. Similarly, an in-plane magnetic field shifts To to higher temperatures and transforms phase I into another non-magnetic phase (II) through a 1st-order phase transition at about 9 T. Using renormalized band structure calculations, we found that the Kondo effect (TK ~ 30 K) leads to substantial mixing of the excited crystalline-electric-field (CEF) states into the ground state. This allows quadrupolar degrees of freedom in the resulting heavy bands at the Fermi level which are prone to nesting. The huge sensitivity of the quadrupole moment on hybridization together with nesting would cause an unprecedented case of phase transition into a quadrupole-density-wave (QDW) state at a temperature To << TK , which would explain the nature of phase I and II.

Infrared spectroscopy of an endohedral water in fullerene.

Abstract: An infrared absorption spectroscopy study of the endohedral water molecule in a solid mixture of H2O@C60 and C60 was carried out at liquid helium temperature. From the evolution of the spectra during the ortho-para conversion process, the spectral lines were identified as para-H2O and ortho-H2O transitions. Eight vibrational transitions with rotational side peaks were observed in the mid-infrared: ω1, ω2, ω3, 2ω1, 2ω2, ω1 + ω3, ω2 + ω3, and 2ω2 + ω3. The vibrational frequencies ω2 and 2ω2 are lower by 1.6% and the rest by 2.4%, as compared to those of free H2O. A model consisting of a rovibrational Hamiltonian with the dipole and quadrupole moments of H2O interacting with the crystal field was used to fit the infrared absorption spectra. The electric quadrupole interaction with the crystal field lifts the degeneracy of the rotational levels. The finite amplitudes of the pure v1 and v2 vibrational transitions are consistent with the interaction of the water molecule dipole moment with a lattice-induced electric field. The permanent dipole moment of encapsulated H2O is found to be 0.50 ± 0.05 D as determined from the far-infrared rotational line intensities. The translational mode of the quantized center-of-mass motion of H2O in the molecular cage of C60 was observed at 110 cm-1 (13.6 meV).

High-resolution laser spectroscopy of 27-32Al

Abstract: Hyperfine spectra of $^\text{27-32}$Al ($Z=13$) have been measured at the ISOLDE-CERN facility via collinear laser spectroscopy using the $3s^23p\ ^2\text{P}^\text{o} _{3/2}\rightarrow 3s^24s\ ^2\text{S}_{1/2}$ atomic transition. For the first time, mean-square charge radii of radioactive aluminum isotopes have been determined alongside the previously unknown magnetic dipole moment of $^{29}$Al and electric quadrupole moments of $^{29,30}$Al. A potentially reduced charge radius at $N=19$ may suggest an effect of the $N=20$ shell closure, which is visible in the Al chain, contrary to other isotopic chains in the $sd$ shell. The experimental results are compared to theoretical calculations in the framework of the valence-space in-medium similarity renormalization group using multiple sets of two and three-nucleon forces from chiral effective field theory. While the trend of experimental magnetic dipole and electric quadrupole moments is well reproduced, the absolute values are underestimated by theory, consistent with earlier studies. Moreover, both the scale and trend of the charge radii appear to be very sensitive to the chosen interaction.

Onset of triaxial deformation in $^{66}$Zn and properties of its first excited $0^+$ state studied by means of Coulomb excitation

Abstract: The electromagnetic structure of Zn66 at low excitation energy was investigated via low-energy Coulomb excitation at INFN Legnaro National Laboratories, using the Gamma Array of Legnaro Infn Laboratories for nuclEar spectrOscopy (GALILEO) γ-ray spectrometer coupled to the SPIDER (Silicon PIe DEtectoR). A set of reduced E2, E3, and M1 matrix elements was extracted from the collected data using the gosia code, yielding 12 reduced transition probabilities between the low-spin states and the spectroscopic quadrupole moment of the 21+ state. The B(E2) values for transitions depopulating the 02+ state have been determined for the first time, allowing for the lifetime of this state to be deduced and, consequently, the ρ2(E0;02+→01+) monopole transition strength to be extracted. In addition, the B(E3;31−→01+) value has been determined for the first time in a Coulomb excitation experiment. The obtained results resolve the existing discrepancies between literature lifetimes and demonstrate that Zn66 cannot be described by using simple collective models. Therefore, new state-of-the-art beyond-mean-field and large-scale shell-model calculations were performed in order to interpret the structure of this nucleus. Both the experimental and theoretical results suggest that the triaxial degree of freedom has an important impact on electromagnetic properties of Zn66, while the unique features of the 02+ state indicate its distinct and rather isolated structure.

Magnetic dipole and electric quadrupole absorption in carbon dioxide

Abstract: Magnetic dipole and electric quadrupole absorption in carbon dioxide are addressed in details. The selection rules for both processes are presented. The equations for the line intensities are given. In the case of the quadrupole absorption the Herman-Wallis functions are derived. The results of the present paper were used in the analysis of the carbon dioxide absorption band at 3.3 µm in the atmosphere of Mars (Trokhimovskiy A, Perevalov V, Korablev O, Fedorova A, Olsen KS, Bertaux JL, Patrakeev A, Shakun A, Montmessin F, Lefevre F, Lukashevskaya A. First observation of the magnetic dipole CO2 absorption band at 3.3 µm in the atmosphere of Mars by ExoMars Trace Gas Orbiter ACS instrument. A&A 639, A142 (2020)). The retrieved from the Martian atmosphere spectra vibrational transition magnetic dipole moment for the 01111–00001 (ν2+ν3) band of 12C16O2 M 01111 ← 000001 | Δ l 2 | = 1 = 0.96 μ N (where μN is nuclear magneton) is one order of magnitude larger than the gyromagnetic ratio in the case of the rotation-induced magnetic dipole moment.

Post-Newtonian Waveforms from Spinning Scattering Amplitudes

Abstract: We derive the classical gravitational radiation from an aligned spin binary black hole on \textit{closed} orbits, using a dictionary built from the 5-point QFT scattering amplitude of two massive particles exchanging and emitting a graviton. We show explicitly the agreement of the transverse-traceless components of the radiative linear metric perturbations -- and the corresponding gravitational wave energy flux -- at future null infinity, derived from the scattering amplitude and those derived utilizing an effective worldline action in conjunction with multipolar post-Minkowskian matching. At the tree-level, this result holds at leading orders in the black holes' velocities and up to quadratic order in their spins. At sub-leading order in black holes' velocities, we demonstrate a matching of the radiation field for quasi-circular orbits in the no-spin limit. At the level of the radiation field, and to leading order in the velocities, there exists a one-to-one correspondence between the binary black hole mass and current quadrupole moments, and the scalar and linear-in-spin scattering amplitudes, respectively. Therefore, we show explicitly that waveforms, needed to detect gravitational waves from \textit{inspiraling} binary black holes, can be derived consistently, to the orders considered, from the classical limit of quantum \textit{scattering} amplitudes.

Theory of dipole insulators

Abstract: Insulating systems are characterized by their insensitivity to twisted boundary conditions as quantified by the charge stiffness and charge localization length. The latter quantity was shown to be related to the expectation value of the many-body position operator and serves as a universal criterion to distinguish between metals and insulators. In this work we extend these concepts to a new class of quantum systems having conserved charge and dipole moments. We refine the concept of a charge insulator by introducing notions of multipolar insulators, e.g., a charge insulator could be a dipole insulator or dipole metal. We develop a universal criterion to distinguish between these phases by extending the concept of charge stiffness and localization to analogous versions for multipole moments but with our focus on dipoles. We are able to relate the dipole localization scale to the expectation value of a recently introduced many-body quadrupole operator. This refined structure allows for the identification of phase transitions where charge remains localized but, e.g., dipoles delocalize. We illustrate the proposed criterion using several exactly solvable models that exemplify these concepts and discuss a possible realization in cold-atom systems.

Wide-angle invisible dielectric metasurface driven by transverse Kerker scattering

Abstract: Interference is the cornerstone of Huygens source design for reshaping and controlling scattering patterns. The conventional underpinning principle, such as for the Kerker effect, is the interference of electric and magnetic dipole and quadrupole modes. Here a route to realize transverse Kerker scattering through employing only the interference between the electric dipole and magnetic quadrupole is demonstrated. The proposed approach is numerically validated in an ultrathin Silicon square nanoplate metasurface, and is further verified by multipole decomposition. The metasurface is shown to be invisible for near-infrared wavelengths and with an enhanced electric field in the region of the nanoparticle. Additionally, we develop further the proposed approach with practical implementation for invisibility applications by exploring the effects of the aspect ratio of the square plate nanoresonator, the interparticle separation, and the presence of a substrate. Further it is demonstrated that invisibility can be observed at oblique incidence up to ${60}^{\ensuremath{\circ}}$ for a transverse magnetic plane wave. The results are relevant for Huygens metasurface design for perfect reflectors, invisibility, and devices for harmonic generation manipulation.

Gravitational-wave constraints on the GWTC-2 events by measuring the tidal deformability and the spin-induced quadrupole moment

Abstract: Gravitational waves from compact binary coalescences provide a unique laboratory to test properties of compact objects. As alternatives to the ordinary black holes in general relativity, various exotic compact objects have been proposed. Some of them have largely different values of the tidal deformability and spin-induced quadrupole moment from those of black holes, and their binaries could be distinguished from the binary black hole by using gravitational waves emitted during their inspiral regime, excluding the highly model-dependent merger and ringdown regimes. We reanalyze gravitational waves from low-mass merger events in the GWTC-2, detected by the Advanced LIGO and Advanced Virgo. Focusing on the influence of tidal deformability and spin-induced quadrupole moment in the inspiral waveform, we provide model-independent constraints on deviations from the standard binary black hole case. We find that all events that we have analyzed are consistent with the waveform of the binary black hole in general relativity. Bayesian model selection shows that the hypothesis that the binary is composed of exotic compact objects is disfavored by all events.

Multipole polarizabilities for hydrogen-like atoms in Hulthén potential with and without spherical confinement

Abstract: The multipole polarizabilities for hydrogen-like atoms with Hulthen potential are calculated with the sum-over-states formalism where the system bound and pseudocontinuum states are produced by employing the generalized pseudospectral method. Energies for nonzero angular momentum states, transition oscillator strengths, and dipole polarizabilities for the ground state of H atom with HP are calculated with high accuracy and compared with previous calculations. Quadrupole, octupole, and hexadecapole polarizabilities for both the ground and excited states are reported for the first time. The combined effect of Hulthen potential and impenetrable sphere on the polarizabilities is investigated, and the relation of such system with the confined H atom and particle in a box is discussed. Further comparison among Hulthen, screened Coulomb, and exponential cosine screened Coulomb potentials reveals that although the ground state energies follow the comparison theorem very well, their first-order energy corrections show complicated variations.

Electric quadrupole form factors of singly heavy baryons with spin 3/2

Abstract: We study the electromagnetic form factors of the lowest-lying singly heavy baryons in a pion mean-field approach, which is also known as the SU(3) chiral quark-soliton model. In the limit of the heavy-quark mass, the dynamics inside a singly heavy baryon is governed by the $N_c-1$ valence quarks, while the heavy quark remains as a mere static color source. In this framework, a singly heavy baryon is described by combining the colored soliton with the singly heavy quark. In the infinitely heavy-quark mass limit, we can compute the electric quadrupole form factors of the baryon sextet with spin 3/2 with the rotational $1/N_c$ and linear corrections of the explicit flavor SU(3) symmetry breaking taken into account. We find that the sea-quark contributions or the Dirac-sea level contributions dominate over the valence-quark contributions in lower $Q^2$ region. We examined the effects of explicit flavor SU(3) symmetry breaking in detail. The numerical results are also compared with the recent data from the lattice calculation with the unphysical value of the pion mass considered, which was used in the lattice calculation.

Possible quadrupole order in tetragonal Ba2CdReO6 and chemical trend in the ground states of 5d1 double perovskites

Abstract: The synthesis and physical properties of the double perovskite (DP) compound Ba2CdReO6 with the 5d1 electronic configuration are reported Three successive phases originating from a spin-orbit-entangled Jeff = 3/2 state, confirmed by the reduced effective magnetic moment of 072 {\mu}B, were observed upon cooling X-ray diffraction measurements revealed a structural transition from a high-temperature cubic structure to a low-temperature tetragonal structure at Ts = 170 K, below which the Jeff = 3/2 state was preserved Magnetization, heat capacity, and thermal expansion measurements showed two more electronic transitions to a possible quadrupole ordered state at Tq = 25 K, and an antiferromagnetic order of dipoles accompanied by a ferromagnetic moment of ~ 02 {\mu}B at Tm = 12 K These properties were compared with those of the sister compounds Ba2BReO6 (B = Mg, Zn, and Ca) and the chemical trend is discussed in terms of the mean-field theory for spin-orbit-coupled 5d electrons [G Chen et al, Phys Rev B 82, 174440 (2010)] The DP compound Ba2BReO6 provides a unique opportunity for a systematic investigation on symmetry breaking in the presence of multipolar degrees of freedom

New searches for continuous gravitational waves from seven fast pulsars

Abstract: We conduct searches for continuous gravitational waves from seven pulsars, that have not been targeted in continuous wave searches of Advanced LIGO data before. We target emission at exactly twice the rotation frequency of the pulsars and in a small band around such frequency. The former search assumes that the gravitational wave quadrupole is changing phase-locked with the rotation of the pulsar. The search over a range of frequencies allows for differential rotation between the component emitting the radio signal and the component emitting the gravitational waves, for example the crust or magnetosphere versus the core. Timing solutions derived from the Arecibo 327-MHz Drift-Scan Pulsar Survey (AO327) observations are used. No evidence of a signal is found and upper limits are set on the gravitational wave amplitude. For one of the pulsars we probe gravitational wave intrinsic amplitudes just a factor of 3.8 higher than the spin-down limit, assuming a canonical moment of inertia of $10^{38}$ kg m$^2$. Our tightest ellipticity is $1.7 \times 10^{-8}$, which is a value well within the range of what a neutron star crust could support.

Universal features of gravitational waves emitted by superkick binary black hole systems

Abstract: We use numerical relativity to study the merger and ringdown stages of ``superkick'' binary black hole systems (those with equal mass and antiparallel spins). We find a universal way to describe the mass and current quadrupole gravitational waves emitted by these systems during the merger and ringdown stage: (i) The time evolutions of these waves are insensitive to the progenitor's parameters (spins) after being normalized by their own peak values. (ii) The peak values, which encode all the spin information of the progenitor, can be consistently fitted to formulas inspired by post-Newtonian theory. We find that the universal evolution of the mass quadrupole wave can be accurately modeled by the so-called Backwards One-Body (BOB) model. However, the BOB model, in its present form, leads to a lower waveform match and a significant parameter-estimation bias for the current quadrupole wave. We also decompose the ringdown signal into seven overtones, and study the dependence of mode amplitudes on the progenitor's parameters. Such dependence is found to be insensitive to the overtone index (up to a scaling factor). Finally, we use the Fisher matrix technique to investigate how the ringdown waveform can be at least as important for parameter estimation as the inspiral stage. Assuming the Cosmic Explorer, we find the contribution of ringdown portion dominates as the total mass exceeds $\ensuremath{\sim}250\text{ }\text{ }{M}_{\ensuremath{\bigodot}}$. For massive binary black hole (BBH) systems, the accuracy of parameter measurement is improved by incorporating the information of ringdown---the ringdown sector gives rise to a different parameter correlation from inspiral stage; hence, the overall parameter correlation is reduced in full signal.

Microscopic description of quadrupole-octupole coupling in actinides with the Gogny-D1M energy density functional

Abstract: The interplay between quadrupole and octupole degrees of freedom is discussed in a series of U, Pu, Cm and Cf isotopes both at the mean-field level and beyond. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the parametrization D1M of the Gogny energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and $B(E3)$ are discussed in detail and compared with the available experimental data. It is shown that, for the studied nuclei, the quadrupole-octupole coupling is weak and to a large extent the properties of negative parity states can be reasonably well described in terms of the octupole degree of freedom alone.

Science with the TianQin Observatory: Preliminary results on testing the no-hair theorem with extreme mass ratio inspirals

Abstract: Constituted with a massive black hole and a stellar mass compact object, extreme mass ratio inspiral (EMRI) events hold unique opportunity for the study of massive black holes, such as by measuring and checking the relations among the mass, spin and quadrupole moment of a massive black hole, putting the no-hair theorem to test. TianQin is a planned space-based gravitational wave observatory and EMRI is one of its main types of sources. It is important to estimate the capacity of TianQin on testing the no-hair theorem with EMRIs. In this work, we use the analytic kludge waveform with quadrupole moment corrections and study how the quadrupole moment can be constrained with TianQin. We find that TianQin can measure the dimensionless quadrupole moment parameter with accuracy to the level of ${10}^{\ensuremath{-}5}$ under suitable scenarios. The choice of the waveform cutoff is found to have significant effect on the result: if the Schwarzschild cutoff is used, the accuracy depends strongly on the mass of the massive black hole, while the spin has negligible impact; if the Kerr cutoff is used, however, the dependence on the spin is more significant. We have also analyzed the cases when TianQin is observing simultaneously with other detectors such as LISA.

Equation of motion coupled-cluster study of core excitation spectra II: Beyond the dipole approximation.

Abstract: We present the time-independent (TI) and time-dependent (TD) equation of motion coupled-cluster (EOM-CC) oscillator strengths not limited to those obtained by the dipole approximation. For the conventional TI-EOM-CC, we implement all the terms in the multipole expansion through second order that contributes to the oscillator strength. These include contributions such as magnetic dipole, electric quadrupole, electric octupole, and magnetic quadrupole. In TD-EOM-CC, we only include the quadrupole moment contributions. This augments our previous work [Y. C. Park, A. Perera, and R. J. Bartlett, J. Chem. Phys. 151, 164117 (2019)]. The inclusion of the quadrupole contributions (and all the other contributions through second order in the case of TI-EOM-CCSD) enables us to obtain the intensities for the pre-edge transitions in the metal K-edge spectra, which are dipole inactive. The TI-EOM-CCSD and TD-EOM-CCSD spectra of Ti4+ atoms are used to showcase the implementation of the second-order oscillator strengths. The origin of 1s → e and 1s → t2 in core spectra from iron tetrachloride and titanium tetrachloride is discussed and compared with the experiment.

Local vs global approaches to treat two equivalent methyl internal rotations and 14N nuclear quadrupole coupling of 2,5-dimethylpyrrole

Abstract: The microwave spectrum of 2,5-dimethylpyrrole was recorded using a molecular jet Fourier transform microwave spectrometer operating in the frequency range from 2 to 26.5 GHz. Only one stable conformer was observed as expected and confirmed by quantum chemical calculations carried out to complement the experimental analysis. The two equivalent methyl groups cause each rotational transition to split into four torsional species, which is combined with the quadrupole hyperfine splittings in the same order of magnitude arising from the 14N nucleus. This results in a complicated spectrum feature. The spectral assignment was done separately for each torsional species. Two global fits were carried out using the XIAM code and the BELGI-C2v-2Tops-hyperfine code, a modified version of the BELGI-C2v-2Tops code, giving satisfactory root-mean-square deviations. The potential barriers to internal rotation of the two methyl groups were determined to be V3 = 317.208(16) cm−1. The molecular parameters were obtained with high accuracy, providing all necessary ground state information for further investigations in higher frequency ranges and on excited torsional-vibrational states.

Investigation on the Cs 6 S 1/2 to 7 D electric quadrupole transition via monochromatic two-photon process at 767 nm

Abstract: We experimentally demonstrate the cesium electric quadrupole transition from the 6S1/2 ground state to the 7D3/2,5/2 excited state through a virtual level by using a single laser at 767 nm. The excited state energy level population is characterized by varying the laser power, the temperature of the vapor, and the polarization combinations of the laser beams. The optimized experimental parameters are obtained for a high resolution transition interval identification. The magnetic dipole coupling constant A and electric quadrupole coupling constant B for the 7D3/2,5/2 states are precisely determined by using the hyperfine levels intervals. The results, A = 7.39 (0.06) MHz, B = −0.19 (0.18) MHz for the 7D3/2 state, and A = −1.79 (0.05) MHz, B =1.05 (0.29) MHz for the 7D5/2 state, are in good agreement with the previous reported results. This work is beneficial for the determination of atomic structure information and parity non-conservation, which paves the way for the field of precision measurements and atomic physics.

Hybridization and Dehybridization of Plasmonic Modes

Abstract: The plasmon resonances (modes) of a metal nanostructure can be defined as a dipole, a quadrupole, or high-order modes depending on the surface charge distribution induced by the incident field. In ...