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Showing papers on "Quantum published in 2008"


Journal ArticleDOI
06 Jun 2008-Science
TL;DR: It is shown that the opacity of suspended graphene is defined solely by the fine structure constant, a = e2/hc � 1/137 (where c is the speed of light), the parameter that describes coupling between light and relativistic electrons and that is traditionally associated with quantum electrodynamics rather than materials science.
Abstract: There are few phenomena in condensed matter physics that are defined only by the fundamental constants and do not depend on material parameters. Examples are the resistivity quantum, h/e2 (h is Planck's constant and e the electron charge), that appears in a variety of transport experiments and the magnetic flux quantum, h/e, playing an important role in the physics of superconductivity. By and large, sophisticated facilities and special measurement conditions are required to observe any of these phenomena. We show that the opacity of suspended graphene is defined solely by the fine structure constant, a = e2/hc feminine 1/137 (where c is the speed of light), the parameter that describes coupling between light and relativistic electrons and that is traditionally associated with quantum electrodynamics rather than materials science. Despite being only one atom thick, graphene is found to absorb a significant (pa = 2.3%) fraction of incident white light, a consequence of graphene's unique electronic structure.

7,952 citations


Journal ArticleDOI
18 Apr 2008-Science
TL;DR: This work reports on electron transport in quantum dot devices carved entirely from graphene, demonstrating the possibility of molecular-scale electronics based on graphene.
Abstract: The exceptional electronic properties of graphene, with its charge carriers mimicking relativistic quantum particles and its formidable potential in various applications, have ensured a rapid growth of interest in this new material. We report on electron transport in quantum dot devices carved entirely from graphene. At large sizes (>100 nanometers), they behave as conventional single-electron transistors, exhibiting periodic Coulomb blockade peaks. For quantum dots smaller than 100 nanometers, the peaks become strongly nonperiodic, indicating a major contribution of quantum confinement. Random peak spacing and its statistics are well described by the theory of chaotic neutrino billiards. Short constrictions of only a few nanometers in width remain conductive and reveal a confinement gap of up to 0.5 electron volt, demonstrating the possibility of molecular-scale electronics based on graphene.

2,032 citations


BookDOI
01 Jul 2008
TL;DR: In this paper, the authors used the nonequilibrium Green function theory for the derivation of the quantum kinetic equations for femtosecond laser-pulse spectroscopy.
Abstract: Nanoscale miniaturization and femtosecond laser-pulse spectroscopy require a quantum mechanical description of the carrier kinetics that goes beyond the conventional Boltzmann theory. On these extremely short length and time scales the electrons behave like partially coherent waves. This monograph deals with quantum kinetics for transport in low-dimensional microstructures and for ultra-short laser pulse spectroscopy. The nonequilibrium Green function theory is described and used for the derivation of the quantum kinetic equations. Numerical methods for the solution of the retarded quantum kinetic equations are discussed and results are presented for high-field transport and for mesoscopic transport phenomena. Quantum beats, polarization decay, and non-Markovian behaviour are treated for femtosecond spectroscopy on a microscopic basis. Since the publishing of the first edition in 1996 the nonequilibrium Green function technique has been applied to a large number of new research topics, and the revised edition introduces the reader to some of these areas, such as molecular electronics, noise calculations, build-up of screening and polaron correlations, and non-Markovian relaxation, among others. Connection to recent experiments is made, and it is emphasized how the quantum kinetic theory is essential in their interpretation. (orig.)

1,908 citations


Journal ArticleDOI
06 Mar 2008-Nature
TL;DR: A cavity which is detuned by the motion of a 50-nm-thick dielectric membrane placed between two macroscopic, rigid, high-finesse mirrors is demonstrated, which segregates optical and mechanical functionality to physically distinct structures and avoids compromising either.
Abstract: In recent years micromechanical devices have been developed that can strongly couple to light, by integrating them within optical cavities. A main goal has been to cool the devices optomechanically, freezing out all thermal vibrations, so that the object's motion eventually becomes limited by quantum mechanical fluctuations. This would make it possible to study a new range of quantum behaviour of mechanical objects. Thompson et al. report an improved design of such a system, involving a movable membrane sandwiched between two rigid high-quality mirrors. In previous designs one of the mirrors had to double-up as a microresonator. The new device achieves substantial cooling, from room temperature to 6.8 mK. It should eventually be possible to reach the quantum-limited ground state with this system. A report on an improved design of an optomechanical system in which a movable membrane is placed between two rigid high-quality mirrors, as opposed to previous designs where one of the mirrors has a double function as the microresonator; it's claimed that it is feasible to reach the quantum-limited ground state with this new design. Macroscopic mechanical objects and electromagnetic degrees of freedom can couple to each other through radiation pressure. Optomechanical systems in which this coupling is sufficiently strong are predicted to show quantum effects and are a topic of considerable interest. Devices in this regime would offer new types of control over the quantum state of both light and matter1,2,3,4, and would provide a new arena in which to explore the boundary between quantum and classical physics5,6,7. Experiments so far have achieved sufficient optomechanical coupling to laser-cool mechanical devices8,9,10,11,12, but have not yet reached the quantum regime. The outstanding technical challenge in this field is integrating sensitive micromechanical elements (which must be small, light and flexible) into high-finesse cavities (which are typically rigid and massive) without compromising the mechanical or optical properties of either. A second, and more fundamental, challenge is to read out the mechanical element’s energy eigenstate. Displacement measurements (no matter how sensitive) cannot determine an oscillator’s energy eigenstate13, and measurements coupling to quantities other than displacement14,15,16 have been difficult to realize in practice. Here we present an optomechanical system that has the potential to resolve both of these challenges. We demonstrate a cavity which is detuned by the motion of a 50-nm-thick dielectric membrane placed between two macroscopic, rigid, high-finesse mirrors. This approach segregates optical and mechanical functionality to physically distinct structures and avoids compromising either. It also allows for direct measurement of the square of the membrane’s displacement, and thus in principle the membrane’s energy eigenstate. We estimate that it should be practical to use this scheme to observe quantum jumps of a mechanical system, an important goal in the field of quantum measurement.

1,201 citations


Journal ArticleDOI
TL;DR: A theoretical framework for studying the role of quantum interference effects in energy transfer dynamics of molecular arrays interacting with a thermal bath within the Lindblad formalism is developed and an effective interplay between the free Hamiltonian evolution and the thermal fluctuations in the environment is demonstrated.
Abstract: Energy transfer within photosynthetic systems can display quantum effects such as delocalized excitonic transport. Recently, direct evidence of long-lived coherence has been experimentally demonstrated for the dynamics of the Fenna-Matthews-Olson (FMO) protein complex [Engel et al., Nature (London) 446, 782 (2007)]. However, the relevance of quantum dynamical processes to the exciton transfer efficiency is to a large extent unknown. Here, we develop a theoretical framework for studying the role of quantum interference effects in energy transfer dynamics of molecular arrays interacting with a thermal bath within the Lindblad formalism. To this end, we generalize continuous-time quantum walks to nonunitary and temperature-dependent dynamics in Liouville space derived from a microscopic Hamiltonian. Different physical effects of coherence and decoherence processes are explored via a universal measure for the energy transfer efficiency and its susceptibility. In particular, we demonstrate that for the FMO complex, an effective interplay between the free Hamiltonian evolution and the thermal fluctuations in the environment leads to a substantial increase in energy transfer efficiency from about 70% to 99%.

1,145 citations


Journal ArticleDOI
TL;DR: In this paper, the authors summarize some of the basic issues, including the extent to which the quantum criticality in heavy-fermion metals goes beyond the standard theory of order-parameter fluctuations, the nature of the Kondo effect in the quantum-critical regime, the non-Fermi-liquid phenomena that accompany quantum criticalities and the interplay between quantum criticalness and unconventional superconductivity.
Abstract: Quantum criticality describes the collective fluctuations of matter undergoing a second-order phase transition at zero temperature. Heavy-fermion metals have in recent years emerged as prototypical systems to study quantum critical points. There have been considerable efforts, both experimental and theoretical, that use these magnetic systems to address problems that are central to the broad understanding of strongly correlated quantum matter. Here, we summarize some of the basic issues, including the extent to which the quantum criticality in heavy-fermion metals goes beyond the standard theory of order-parameter fluctuations, the nature of the Kondo effect in the quantum-critical regime, the non-Fermi-liquid phenomena that accompany quantum criticality and the interplay between quantum criticality and unconventional superconductivity. At a zero-temperature phase transition from one ordered state to another, fluctuations between the two states lead to quantum critical behaviour that can lead to unexpected physics. Metals with ‘heavy’ electrons often harbour such weird states.

1,055 citations


Journal ArticleDOI
TL;DR: An open quantum system, the time evolution of which is governed by a master equation, can be driven into a given pure quantum state by an appropriate design of the coupling between the system and t...
Abstract: An open quantum system, the time evolution of which is governed by a master equation, can be driven into a given pure quantum state by an appropriate design of the coupling between the system and t ...

969 citations


Journal ArticleDOI
TL;DR: It is shown that the interaction between trapped electromagnetic modes can lead to scattering resonances with practically zero width, which are the bound states in the radiation continuum first discovered in quantum systems by von Neumann and Wigner.
Abstract: With examples of two parallel dielectric gratings and two arrays of thin parallel dielectric cylinders, it is shown that the interaction between trapped electromagnetic modes can lead to scattering resonances with practically zero width. Such resonances are the bound states in the radiation continuum first discovered in quantum systems by von Neumann and Wigner. Potential applications of such photonic systems include: large amplification of electromagnetic fields within photonic structures and, hence, enhancement of nonlinear phenomena, biosensing, as well as perfect filters and waveguides for a particular frequency, and impurity detection.

674 citations


Journal ArticleDOI
TL;DR: It is shown that the existence of a minimum measurable length and the related generalized uncertainty principle (GUP), predicted by theories of quantum gravity, influence all quantum Hamiltonians, and they predict quantum gravity corrections to various quantum phenomena.
Abstract: We show that the existence of a minimum measurable length and the related generalized uncertainty principle (GUP), predicted by theories of quantum gravity, influence all quantum Hamiltonians. Thus, they predict quantum gravity corrections to various quantum phenomena. We compute such corrections to the Lamb shift, the Landau levels, and the tunneling current in a scanning tunneling microscope. We show that these corrections can be interpreted in two ways: (a) either that they are exceedingly small, beyond the reach of current experiments, or (b) that they predict upper bounds on the quantum gravity parameter in the GUP, compatible with experiments at the electroweak scale. Thus, more accurate measurements in the future should either be able to test these predictions, or further tighten the above bounds and predict an intermediate length scale between the electroweak and the Planck scale.

664 citations


01 Jan 2008
TL;DR: Several quantities of interest in quantum information, including entanglement and purity, are nonlinear functions of the density matrix and cannot, even in principle, correspond to proper quantum information.
Abstract: Several quantities of interest in quantum information, including entanglement and purity, are nonlinear functions of the density matrix and cannot, even in principle, correspond to proper quantum o...

660 citations


Journal ArticleDOI
TL;DR: In this paper, a quantum theory of membranes designed such that the ground-state wavefunction of the membrane with compact spatial topology reproduces the partition function of the bosonic string on worldsheet is presented.
Abstract: We propose a quantum theory of membranes designed such that the ground-state wavefunction of the membrane with compact spatial topology \Sigma_h reproduces the partition function of the bosonic string on worldsheet \Sigma_h. The construction involves worldvolume matter at quantum criticality, described in the simplest case by Lifshitz scalars with dynamical critical exponent z=2. This matter system must be coupled to a novel theory of worldvolume gravity, also exhibiting quantum criticality with z=2. We first construct such a nonrelativistic "gravity at a Lifshitz point" with z=2 in D+1 spacetime dimensions, and then specialize to the critical case of D=2 suitable for the membrane worldvolume. We also show that in the second-quantized framework, the string partition function is reproduced if the spacetime ground state takes the form of a Bose-Einstein condensate of membranes in their first-quantized ground states, correlated across all genera.


Journal ArticleDOI
22 Feb 2008-Science
TL;DR: This work has demonstrated a robust, efficient mechanism for the regulated transport of photons one by one using a microscopic optical resonator and verified the transformation from a Poissonian to a sub-Poissonian photon stream by photon counting measurements of the input and output fields.
Abstract: Beyond traditional nonlinear optics with large numbers of atoms and photons, qualitatively new phenomena arise in a quantum regime of strong interactions between single atoms and photons. By using a microscopic optical resonator, we achieved such interactions and demonstrated a robust, efficient mechanism for the regulated transport of photons one by one. With critical coupling of the input light, a single atom within the resonator dynamically controls the cavity output conditioned on the photon number at the input, thereby functioning as a photon turnstile. We verified the transformation from a Poissonian to a sub-Poissonian photon stream by photon counting measurements of the input and output fields. The results have applications in quantum information science, including for controlled interactions of single light quanta and for scalable quantum processing on atom chips.

Journal ArticleDOI
Ali Mostafazadeh1
TL;DR: A diagonalizable non-Hermitian Hamiltonian having a real spectrum can be used to define a unitary quantum system, if one modifies the inner product of the Hilbert space properly as discussed by the authors.
Abstract: A diagonalizable non-Hermitian Hamiltonian having a real spectrum may be used to define a unitary quantum system, if one modifies the inner product of the Hilbert space properly. We give a comprehensive and essentially self-contained review of the basic ideas and techniques responsible for the recent developments in this subject. We provide a critical assessment of the role of the geometry of the Hilbert space in conventional quantum mechanics to reveal the basic physical principle motivating our study. We then offer a survey of the necessary mathematical tools and elaborate on a number of relevant issues of fundamental importance. In particular, we discuss the role of the antilinear symmetries such as PT, the true meaning and significance of the charge operators C and the CPT-inner products, the nature of the physical observables, the equivalent description of such models using ordinary Hermitian quantum mechanics, the pertaining duality between local-non-Hermitian versus nonlocal-Hermitian descriptions of their dynamics, the corresponding classical systems, the pseudo-Hermitian canonical quantization scheme, various methods of calculating the (pseudo-) metric operators, subtleties of dealing with time-dependent quasi-Hermitian Hamiltonians and the path-integral formulation of the theory, and the structure of the state space and its ramifications for the quantum Brachistochrone problem. We also explore some concrete physical applications of the abstract concepts and tools that have been developed in the course of this investigation. These include applications in nuclear physics, condensed matter physics, relativistic quantum mechanics and quantum field theory, quantum cosmology, electromagnetic wave propagation, open quantum systems, magnetohydrodynamics, quantum chaos, and biophysics.

Proceedings ArticleDOI
29 May 2008
TL;DR: In this paper, the effects of the Casimir effect in quantum electrodynamics on the dimensions of the five-dimensional Kaluza-Klein model were investigated and the one-loop effective potential, as a function of five-five component of the metric, was computed.
Abstract: The phenomenon of dimensional reduction in quantum theories of gravity is described. The five‐dimensional Kaluza‐Klein model is studied and the one‐loop effective potential, as a function of the five‐five component of the metric, is computed. For values of this field such that the distance around the fifth dimension is larger than the Planck length, the loop expansion for the effective potential is reliable. The form of the potential then implies the existence of a force tending to make the fifth dimension contract to a size on the order of the Planck length. This result can be interpreted as a gravitational version of the Casimir effect in quantum electrodynamics.

Journal ArticleDOI
TL;DR: From a snapshot of a quantum evolution, it can be decided whether or not a channel is consistent with a time (in)dependent Markovian evolution, for which a computable measure of "Markovianity" is introduced.
Abstract: We investigate what a snapshot of a quantum evolution--a quantum channel reflecting open system dynamics--reveals about the underlying continuous time evolution. Remarkably, from such a snapshot, and without imposing additional assumptions, it can be decided whether or not a channel is consistent with a time (in)dependent Markovian evolution, for which we provide computable necessary and sufficient criteria. Based on these, a computable measure of "Markovianity" is introduced. We discuss how the consistency with Markovian dynamics can be checked in quantum process tomography. The results also clarify the geometry of the set of quantum channels with respect to being solutions of time (in)dependent master equations.

Journal ArticleDOI
17 Jul 2008-Nature
TL;DR: Measuring the photonic degree of freedom of the coupled system, the measurements provide unambiguous spectroscopic evidence for the quantum nature of the resonant atom–field interaction in cavity QED.
Abstract: The field of cavity quantum electrodynamics (QED), traditionally studied in atomic systems1,2,3, has gained new momentum by recent reports of quantum optical experiments with solid-state semiconducting4,5,6,7,8 and superconducting9,10,11 systems. In cavity QED, the observation of the vacuum Rabi mode splitting is used to investigate the nature of matter–light interaction at a quantum-mechanical level. However, this effect can, at least in principle, be explained classically as the normal mode splitting of two coupled linear oscillators12. It has been suggested that an observation of the scaling of the resonant atom–photon coupling strength in the Jaynes–Cummings energy ladder13 with the square root of photon number n is sufficient to prove that the system is quantum mechanical in nature14. Here we report a direct spectroscopic observation of this characteristic quantum nonlinearity. Measuring the photonic degree of freedom of the coupled system, our measurements provide unambiguous spectroscopic evidence for the quantum nature of the resonant atom–field interaction in cavity QED. We explore atom–photon superposition states involving up to two photons, using a spectroscopic pump and probe technique. The experiments have been performed in a circuit QED set-up15, in which very strong coupling is realized by the large dipole coupling strength and the long coherence time of a superconducting qubit embedded in a high-quality on-chip microwave cavity. Circuit QED systems also provide a natural quantum interface between flying qubits (photons) and stationary qubits for applications in quantum information processing and communication16.

Journal ArticleDOI
TL;DR: This work rigorously proves that the evolving state locally relaxes to a steady state with maximum entropy constrained by second moments--thus maximizing the entanglement.
Abstract: A reasonable physical intuition in the study of interacting quantum systems says that, independent of the initial state, the system will tend to equilibrate. In this work we introduce an experimentally accessible setting where relaxation to a steady state is exact, namely, for the Bose-Hubbard model quenched from a Mott quantum phase to the free strong superfluid regime. We rigorously prove that the evolving state locally relaxes to a steady state with maximum entropy constrained by second moments--thus maximizing the entanglement. Remarkably, for this to be true, no time average is necessary. Our argument includes a central limit theorem and exploits the finite speed of information transfer. We also show that for all periodic initial configurations (charge density waves) the system relaxes locally, and identify experimentally accessible signatures in optical lattices as well as implications for the foundations of statistical mechanics.

Journal ArticleDOI
TL;DR: In this paper, the authors survey recent theoretical studies concerning the use of cavity quantum electrodynamics to create quantum many-body systems, including the Bose-Hubbard and anisotropic Heisenberg models.
Abstract: The increasing level of experimental control over atomic and optical systems gained in the past years have paved the way for the exploration of new physical regimes in quantum optics and atomic physics, characterised by the appearance of quantum many-body phenomena, originally encountered only in condensed-matter physics, and the possibility of experimentally accessing them in a more controlled manner. In this review article we survey recent theoretical studies concerning the use of cavity quantum electrodynamics to create quantum many-body systems. Based on recent experimental progress in the fabrication of arrays of interacting micro-cavities and on their coupling to atomic-like structures in several different physical architectures, we review proposals on the realisation of paradigmatic many-body models in such systems, such as the Bose-Hubbard and the anisotropic Heisenberg models. Such arrays of coupled cavities offer interesting properties as simulators of quantum many-body physics, including the full addressability of individual sites and the accessibility of inhomogeneous models.

Journal ArticleDOI
Subir Sachdev1
TL;DR: In this article, the phase transitions between magnetic spin states, including quantum criticality and entangled electron states, are discussed, and a review article covers phase transition between these states, and the phase transition is discussed in detail.
Abstract: Quantum magnetism describes systems of magnetic spins in which quantum mechanical effects dominate, often in surprising ways. This review article covers phase transitions between these states, including quantum criticality and entangled electron states.

Journal ArticleDOI
TL;DR: In this article, a simple choice of the proportionality constants reproduces the one loop back reaction effect in the spacetime, found by conformal field theory methods, which modifies the Hawking temperature of the black hole.
Abstract: Hawking radiation as tunneling by Hamilton-Jacobi method beyond semiclassical approximation is analysed. We compute all quantum corrections in the single particle action revealing that these are proportional to the usual semiclassical contribution. We show that a simple choice of the proportionality constants reproduces the one loop back reaction effect in the spacetime, found by conformal field theory methods, which modifies the Hawking temperature of the black hole. Using the law of black hole mechanics we give the corrections to the Bekenstein-Hawking area law following from the modified Hawking temperature. Some examples are explicitly worked out.

Journal ArticleDOI
19 Jun 2008-Nature
TL;DR: At nanokelvin temperatures, ultracold quantum gases can be stored in optical lattices, which are arrays of microscopic trapping potentials formed by laser light, providing opportunities for investigating quantum coherence and generating large-scale entanglement, ultimately leading to quantum information processing in these artificial crystal structures.
Abstract: At nanokelvin temperatures, ultracold quantum gases can be stored in optical lattices, which are arrays of microscopic trapping potentials formed by laser light. Such large arrays of atoms provide opportunities for investigating quantum coherence and generating large-scale entanglement, ultimately leading to quantum information processing in these artificial crystal structures. These arrays can also function as versatile model systems for the study of strongly interacting many-body systems on a lattice.

Journal ArticleDOI
TL;DR: In this article, the authors find an interpretation of the recent connection found between topological strings on Calabi-Yau threefolds and crystal melting: summing over statistical mechanical configuration of melting crystal is equivalent to a quantum gravitational path integral involving fluctuations of Kahler geometry and topology.
Abstract: We find an interpretation of the recent connection found between topological strings on Calabi-Yau threefolds and crystal melting: Summing over statistical mechanical configuration of melting crystal is equivalent to a quantum gravitational path integral involving fluctuations of Kahler geometry and topology. We show how the limit shape of the melting crystal emerges as the average geometry and topology of the quantum foam at the string scale. The geometry is classical at large length scales, modified to a smooth limit shape dictated by mirror geometry at string scale and is a quantum foam at area scales ~ gsα'.

Journal ArticleDOI
TL;DR: In this article, a quantum hydrodynamic (fluid) model derived from the Wigner-Poisson equations is used to investigate the ultrafast electron dynamics in thin metal films.
Abstract: A quantum hydrodynamic (fluid) model, derived from the Wigner-Poisson equations, is used to investigate the ultrafast electron dynamics in thin metal films. The hydrodynamic equations, which include exchange and correlation effects, can be combined into a single nonlinear Schr\"odinger-type equation. The fluid model is first benchmarked against a density-functional calculation for the ground state, with good agreement between the two approaches. The ultrafast nonlinear electron dynamics is then investigated and compared to recent semiclassical results obtained with a Vlasov-Poisson approach.

Journal ArticleDOI
TL;DR: In this article, the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems was investigated, mimicking a light harvesting antenna connected to a reaction center as it is found in natural photosynthetic systems.
Abstract: We investigate the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems, mimicking a light-harvesting antenna connected to a reaction center as it is found in natural photosynthetic systems. By using a quantum jump approach, we demonstrate that in the presence of quantum coherent energy transfer and energetic disorder, the efficiency of excitation transfer from the antenna to the reaction center depends intimately on the quantum superposition properties of the initial state. In particular, we find that efficiency is sensitive to symmetric and asymmetric superposition of states in the basis of localized excitations, indicating that initial-state properties can be used as an efficiency control parameter at low temperatures.

Journal ArticleDOI
TL;DR: In this paper, the authors studied the quantum measurement of a cantilever using a parametrically coupled electromagnetic cavity which is driven at the two sidebands corresponding to the mechanical motion.
Abstract: We study the quantum measurement of a cantilever using a parametrically coupled electromagnetic cavity which is driven at the two sidebands corresponding to the mechanical motion. This scheme, originally due to Braginsky et al (Braginsky V, Vorontsov Y I and Thorne K P 1980 Science 209 547), allows a back-action free measurement of one quadrature of the cantilever's motion, and hence the possibility of generating a squeezed state. We present a complete quantum theory of this system, and derive simple conditions on when the quantum limit on the added noise can be surpassed. We also study the conditional dynamics of the measurement, and discuss how such a scheme (when coupled with feedback) can be used to generate and detect squeezed states of the oscillator. Our results are relevant to experiments in optomechanics, and to experiments in quantum electromechanics employing stripline resonators coupled to mechanical resonators.

Journal ArticleDOI
TL;DR: Numerical tests show that quantum coherence can cause significant changes in steady state donor/acceptor populations from those predicted by the FD theory and illustrate delicate cooperation of nonequilibrium and quantum coherent effects on the transient population dynamics.
Abstract: A theory of coherent resonance energy transfer is developed combining the polaron transformation and a time-local quantum master equation formulation, which is valid for arbitrary spectral densities including common modes. The theory contains inhomogeneous terms accounting for nonequilibrium initial preparation effects and elucidates how quantum coherence and nonequilibrium effects manifest themselves in the coherent energy transfer dynamics beyond the weak resonance coupling limit of the Forster and Dexter (FD) theory. Numerical tests show that quantum coherence can cause significant changes in steady state donor/acceptor populations from those predicted by the FD theory and illustrate delicate cooperation of nonequilibrium and quantum coherence effects on the transient population dynamics.

Journal ArticleDOI
TL;DR: In this article, the role of quantum coherence and the environment in the dynamics of excitation energy transfer is not fully understood, and the concept of dynamical contributions of various physical processes to the energy transfer efficiency is introduced.
Abstract: The role of quantum coherence and the environment in the dynamics of excitation energy transfer is not fully understood. In this work, we introduce the concept of dynamical contributions of various physical processes to the energy transfer efficiency. We develop two complementary approaches, based on a Green's function method and energy transfer susceptibilities, and quantify the importance of the Hamiltonian evolution, phonon-induced decoherence, and spatial relaxation pathways. We investigate the Fenna-Matthews-Olson protein complex, where we find a contribution of coherent dynamics of about 10% and of relaxation of 80%.

Posted Content
01 Jan 2008
TL;DR: In this paper, a quantum controller synthesis problem for non-commutative linear stochastic systems with quantum commutation relations is formulated and a quantum version of the Strict Bounded Real Lemma is derived.
Abstract: The purpose of this paper is to formulate and solve a H∞ controller synthesis problem for a class of non-commutative linear stochastic systems which includes many examples of interest in quantum technology. The paper includes results on the class of such systems for which the quantum commutation relations are preserved (such a requirement must be satisfied in a physical quantum system). A quantum version of standard (classical) dissipativity results are presented and from this a quantum version of the Strict Bounded Real Lemma is derived. This enables a quantum version of the two Riccati solution to the H∞ control problem to be presented. This result leads to controllers which may be realized using purely quantum, purely classical or a mixture of quantum and classical elements. This issue of physical realizability of the controller is examined in detail, and necessary and sufficient conditions are given. Our results are constructive in the sense that we provide explicit formulas for the Hamiltonian function and coupling operator corresponding to the controller.

Journal ArticleDOI
TL;DR: In this paper, it has been shown that this method has a previously overlooked temporal contribution to the quasi-classical amplitude, which lies in different character of time in general relativity versus quantum mechanics, and when one takes into account this temporal contribution does one obtain the canonical temperature for the radiation.