Showing papers on "Radiative transfer published in 2018"

An update on the RTTOV fast radiative transfer model (currently at version 12)

Abstract: . This paper gives an update of the RTTOV (Radiative Transfer for TOVS) fast radiative transfer model, which is widely used in the satellite retrieval and data assimilation communities. RTTOV is a fast radiative transfer model for simulating top-of-atmosphere radiances from passive visible, infrared and microwave downward-viewing satellite radiometers. In addition to the forward model, it also optionally computes the tangent linear, adjoint and Jacobian matrix providing changes in radiances for profile variable perturbations assuming a linear relationship about a given atmospheric state. This makes it a useful tool for developing physical retrievals from satellite radiances, for direct radiance assimilation in NWP models, for simulating future instruments, and for training or teaching with a graphical user interface. An overview of the RTTOV model is given, highlighting the updates and increased capability of the latest versions, and it gives some examples of its current performance when compared with more accurate line-by-line radiative transfer models and a few selected observations. The improvement over the original version of the model released in 1999 is demonstrated.

Correction: Corrigendum: Control of Radiative Exciton Recombination by Charge Transfer Induced Surface Dipoles in MoS 2 and WS 2 Monolayers

Abstract: Scientific Reports 6: Article number: 24105; published online: 07 April 2016; updated: 05 April 2018. This article contains an error in Figure 2, where the same image was inadvertently shown in both panel (a) and (b). The correct Figure 2 appears below:

Constraints on the neutron star equation of state from AT2017gfo using radiative transfer simulations

Abstract: The detection of the binary neutron star merger GW170817 together with the observation of electromagnetic counterparts across the entire spectrum inaugurated a new era of multimessenger astronomy. In this study, we incorporate wavelength-dependent opacities and emissivities calculated from atomic-structure data enabling us to model both the measured light curves and spectra of the electromagnetic transient AT2017gfo. Best fits of the observational data are obtained by Gaussian Process Regression, which allows us to present posterior samples for the kilonova and source properties connected to GW170817. Incorporating constraints obtained from the gravitational wave signal measured by the LIGO-Virgo Scientific Collaboration, we present a 90 per cent upper bound on the mass ratio q ≲ 1.38 and a lower bound on the tidal deformability of Λ ≳ 197, which rules out sufficiently soft equations of state. Our analysis is a path-finder for more realistic kilonova models and shows how the combination of gravitational wave and electromagnetic measurements allow for stringent constraints on the source parameters and the supranuclear equation of state.

High Purcell factor generation of indistinguishable on-chip single photons

Abstract: On-chip single-photon sources are key components for integrated photonic quantum technologies. Semiconductor quantum dots can exhibit near-ideal single-photon emission, but this can be significantly degraded in on-chip geometries owing to nearby etched surfaces. A long-proposed solution to improve the indistinguishablility is to use the Purcell effect to reduce the radiative lifetime. However, until now only modest Purcell enhancements have been observed. Here we use pulsed resonant excitation to eliminate slow relaxation paths, revealing a highly Purcell-shortened radiative lifetime (22.7 ps) in a waveguide-coupled quantum dot–photonic crystal cavity system. This leads to near-lifetime-limited single-photon emission that retains high indistinguishablility (93.9%) on a timescale in which 20 photons may be emitted. Nearly background-free pulsed resonance fluorescence is achieved under π-pulse excitation, enabling demonstration of an on-chip, on-demand single-photon source with very high potential repetition rates.

Structured thermal surface for radiative camouflage.

Abstract: Thermal camouflage has been successful in the conductive regime, where thermal metamaterials embedded in a conductive system can manipulate heat conduction inside the bulk. Most reported approaches are background-dependent and not applicable to radiative heat emitted from the surface of the system. A coating with engineered emissivity is one option for radiative camouflage, but only when the background has uniform temperature. Here, we propose a strategy for radiative camouflage of external objects on a given background using a structured thermal surface. The device is non-invasive and restores arbitrary background temperature distributions on its top. For many practical candidates of the background material with similar emissivity as the device, the object can thereby be radiatively concealed without a priori knowledge of the host conductivity and temperature. We expect this strategy to meet the demands of anti-detection and thermal radiation manipulation in complex unknown environments and to inspire developments in phononic and photonic thermotronics.

Radiative control of dark excitons at room temperature by nano-optical antenna-tip Purcell effect.

Abstract: Excitons, Coulomb-bound electron–hole pairs, are elementary photo-excitations in semiconductors that can couple to light through radiative relaxation. In contrast, dark excitons (XD) show anti-parallel spin configuration with generally forbidden radiative emission. Because of their long lifetimes, these dark excitons are appealing candidates for quantum computing and optoelectronics. However, optical read-out and control of XD states has remained challenging due to their decoupling from light. Here, we present a tip-enhanced nano-optical approach to induce, switch and programmably modulate the XD emission at room temperature. Using a monolayer transition metal dichalcogenide (TMD) WSe2 on a gold substrate, we demonstrate ~6 × 105-fold enhancement in dark exciton photoluminescence quantum yield achieved through coupling of the antenna-tip to the dark exciton out-of-plane optical dipole moment, with a large Purcell factor of ≥2 × 103 of the tip–sample nano-cavity. Our approach provides a facile way to harness excitonic properties in low-dimensional semiconductors offering new strategies for quantum optoelectronics. Tip-enhanced photoluminescence spectroscopy allows for modulation and radiative control of dark exciton emission at room temperature.

Entropy generation in magnetohydrodynamic radiative flow due to rotating disk in presence of viscous dissipation and Joule heating

Abstract: Simultaneous effects of viscous dissipation and Joule heating in flow by rotating disk of variable thickness are examined. Radiative flow saturating porous space is considered. Much attention is given to entropy generation outcome. Developed nonlinear ordinary differential systems are computed for the convergent series solutions. Specifically, the results of velocity, temperature, entropy generation, Bejan number, coefficient of skin friction, and local Nusselt number are discussed. Clearly the entropy generation rate depends on velocity and temperature distributions. Moreover the entropy generation rate is a decreasing function of Hartmann number, Eckert number, and Reynolds number, while they gave opposite behavior for Bejan numbers.

Color Centers in Hexagonal Boron Nitride Monolayers: A Group Theory and Ab Initio Analysis

Abstract: We theoretically study physical properties of the most promising color center candidates for the recently observed single-photon emissions in hexagonal boron nitride (h-BN) monolayers. Through our group theory analysis combined with density functional theory (DFT) calculations we provide several pieces of evidence that the electronic properties of the color centers match the characters of the experimentally observed emitters. We calculate the symmetry-adapted multielectron wave functions of the defects using group theory methods and analyze the spin–orbit and spin–spin interactions in detail. We also identify the radiative and nonradiative transition channels for each color center. An advanced ab initio DFT method is then used to compute energy levels of the color centers and their zero-phonon-line (ZPL) emissions. The computed ZPLs, the profile of excitation and emission dipole polarizations, and the competing relaxation processes are discussed and matched with the observed emission lines. By providing e...

Entropy generation minimization (EGM) of nanofluid flow by a thin moving needle with nonlinear thermal radiation

Abstract: Entropy generation minimization (EGM) and heat transport in nonlinear radiative flow of nanomaterials over a thin moving needle has been discussed. Nonlinear thermal radiation and viscous dissipation terms are merged in the energy expression. Water is treated as ordinary fluid while nanomaterials comprise titanium dioxide, copper and aluminum oxide. The nonlinear governing expressions of flow problems are transferred to ordinary ones and then tackled for numerical results by Built-in-shooting technique. In first section of this investigation, the entropy expression is derived as a function of temperature and velocity gradients. Geometrical and physical flow field variables are utilized to make it nondimensionalized. An entropy generation analysis is utilized through second law of thermodynamics. The results of temperature, velocity, concentration, surface drag force and heat transfer rate are explored. Our outcomes reveal that surface drag force and Nusselt number (heat transfer) enhanced linearly for higher nanoparticle volume fraction. Furthermore drag force decays for aluminum oxide and it enhances for copper nanoparticles. In addition, the lowest heat transfer rate is achieved for higher radiative parameter. Temperature field is enhanced with increase in temperature ratio parameter.

New Spectral Model for Constraining Torus Covering Factors from Broadband X-Ray Spectra of Active Galactic Nuclei

Abstract: The basic unified model of active galactic nuclei (AGNs) invokes an anisotropic obscuring structure, usually referred to as a torus, to explain AGN obscuration as an angle-dependent effect. We present a new grid of X-ray spectral templates based on radiative transfer calculations in neutral gas in an approximately toroidal geometry, appropriate for CCD-resolution X-ray spectra (FWHM ≥ 130 eV). Fitting the templates to broadband X-ray spectra of AGNs provides constraints on two important geometrical parameters of the gas distribution around the supermassive black hole: the average column density and the covering factor. Compared to the currently available spectral templates, our model is more flexible, and capable of providing constraints on the main torus parameters in a wider range of AGNs. We demonstrate the application of this model using hard X-ray spectra from NuSTAR (3–79 keV) for four AGNs covering a variety of classifications: 3C 390.3, NGC 2110, IC 5063, and NGC 7582. This small set of examples was chosen to illustrate the range of possible torus configurations, from disk-like to sphere-like geometries with column densities below, as well as above, the Compton-thick threshold. This diversity of torus properties challenges the simple assumption of a standard geometrically and optically thick toroidal structure commonly invoked in the basic form of the unified model of AGNs. Finding broad consistency between our constraints and those from infrared modeling, we discuss how the approach from the X-ray band complements similar measurements of AGN structures at other wavelengths.

Observation of Polarization Vortices in Momentum Space.

Abstract: The vortex, a fundamental topological excitation featuring the in-plane winding of a vector field, is important in various areas such as fluid dynamics, liquid crystals, and superconductors. Although commonly existing in nature, vortices were observed exclusively in real space. Here, we experimentally observed momentum-space vortices as the winding of far-field polarization vectors in the first Brillouin zone of periodic plasmonic structures. Using homemade polarization-resolved momentum-space imaging spectroscopy, we mapped out the dispersion, lifetime, and polarization of all radiative states at the visible wavelengths. The momentum-space vortices were experimentally identified by their winding patterns in the polarization-resolved isofrequency contours and their diverging radiative quality factors. Such polarization vortices can exist robustly on any periodic systems of vectorial fields, while they are not captured by the existing topological band theory developed for scalar fields. Our work provides a new way for designing high-Q plasmonic resonances, generating vector beams, and studying topological photonics in the momentum space.

Suppressed Quenching and Strong-Coupling of Purcell-Enhanced Single-Molecule Emission in Plasmonic Nanocavities

Abstract: An emitter in the vicinity of a metal nanostructure is quenched by its decay through nonradiative channels, leading to the belief in a zone of inactivity for emitters placed within <10 nm of a plasmonic nanostructure. Here we demonstrate and explain why in tightly coupled plasmonic resonators forming nanocavities “quenching is quenched” due to plasmon mixing. Unlike isolated nanoparticles, such plasmonic nanocavities show mode hybridization, which can massively enhance emitter excitation and decay via radiative channels, here experimentally confirmed by laterally dependent emitter placement through DNA-origami. We explain why this enhancement of excitation and radiative decay can be strong enough to facilitate single-molecule strong coupling, as evident in dynamic Rabi-oscillations.

Evolved Climates and Observational Discriminants for the TRAPPIST-1 Planetary System

Abstract: The TRAPPIST-1 planetary system provides an unprecedented opportunity to study terrestrial exoplanet evolution with the James Webb Space Telescope (JWST) and ground-based observatories. Since M dwarf planets likely experience extreme volatile loss, the TRAPPIST-1 planets may have highly-evolved, possibly uninhabitable atmospheres. We used a versatile, 1D terrestrial-planet climate model with line-by-line radiative transfer and mixing length convection (VPL Climate) coupled to a terrestrial photochemistry model to simulate environmental states for the TRAPPIST-1 planets. We present equilibrium climates with self-consistent atmospheric compositions, and observational discriminants of post-runaway, desiccated, 10-100 bar O2- and CO2-dominated atmospheres, including interior outgassing, as well as for water-rich compositions. Our simulations show a range of surface temperatures, most of which are not habitable, although an aqua-planet TRAPPIST-1 e could maintain a temperate surface given Earth-like geological outgassing and CO2. We find that a desiccated TRAPPIST-1 h may produce habitable surface temperatures beyond the maximum greenhouse distance. Potential observational discriminants for these atmospheres in transmission and emission spectra are influenced by photochemical processes and aerosol formation, and include collision-induced oxygen absorption (O2-O2), and O3, CO, SO2, H2O, and CH4 absorption features, with transit signals of up to 200 ppm. Our simulated transmission spectra are consistent with K2, HST, and Spitzer observations of the TRAPPIST-1 planets. For several terrestrial atmospheric compositions, we find that TRAPPIST-1 b is unlikely to produce aerosols. These results can inform JWST observation planning and data interpretation for the TRAPPIST-1 system and other M dwarf terrestrial planets.

Photonic thermal management of coloured objects

Abstract: The colours of outdoor structures, such as automobiles, buildings and clothing, are typically chosen for functional or aesthetic reasons. With a chosen colour, however, one must control the radiative thermal load for heating or cooling purposes. Here we provide a comprehensive calculation of the tunable range of radiative thermal load for all colours. The range exceeds 680 Wm−2 for all colours, and can be as high as 866 Wm−2, resulting from effects of metamerism, infrared solar absorption and radiative cooling. We experimentally demonstrate that two photonic structures with the same pink colour can have their temperatures differ by 47.6 °C under sunlight. These structures are over 20 °C either cooler or hotter than a commercial paint with a comparable colour. Furthermore, the hotter pink structure is 10 °C hotter than a commercial black paint. These results elucidate the fundamental potentials of photonic thermal management for coloured objects.

Generalized hydrodynamics of classical integrable field theory: the sinh-Gordon model

Abstract: Using generalized hydrodynamics (GHD), we develop the Euler hydrodynamics of classical integrable field theory. Classical field GHD is based on a known formalism for Gibbs ensembles of classical fields, that resembles the thermodynamic Bethe ansatz of quantum models, which we extend to generalized Gibbs ensembles (GGEs). In general, GHD must take into account both solitonic and radiative modes of classical fields. We observe that the quasi-particle formulation of GHD remains valid for radiative modes, even though these do not display particle-like properties in their precise dynamics. We point out that because of a UV catastrophe similar to that of black body radiation, radiative modes suffer from divergences that restrict the set of finite-average observables; this set is larger for GGEs with higher conserved charges. We concentrate on the sinh-Gordon model, which only has radiative modes, and study transport in the domain-wall initial problem as well as Euler-scale correlations in GGEs. We confirm a variety of exact GHD predictions, including those coming from hydrodynamic projection theory, by comparing with Metropolis numerical evaluations.

STiC -- A multi-atom non-LTE PRD inversion code for full-Stokes solar observations.

Abstract: The inference of the underlying state of the plasma in the solar chromosphere remains extremely challenging because of the nonlocal character of the observed radiation and plasma conditions in this layer. Inversion methods allow us to derive a model atmosphere that can reproduce the observed spectra by undertaking several physical assumptions. The most advanced approaches involve a depth-stratified model atmosphere described by temperature, line-of-sight velocity, turbulent velocity, the three components of the magnetic field vector, and gas and electron pressure. The parameters of the radiative transfer equation are computed from a solid ground of physical principles. To apply these techniques to spectral lines that sample the chromosphere, NLTE effects must be included in the calculations. We developed a new inversion code STiC to study spectral lines that sample the upper chromosphere. The code is based the RH synthetis code, which we modified to make the inversions faster and more stable. For the first time, STiC facilitates the processing of lines from multiple atoms in non-LTE, also including partial redistribution effects. Furthermore, we include a regularization strategy that allows for model atmospheres with a complex stratification, without introducing artifacts in the reconstructed physical parameters, which are usually manifested in the form of oscillatory behavior. This approach takes steps toward a node-less inversion, in which the value of the physical parameters at each grid point can be considered a free parameter. In this paper we discuss the implementation of the aforementioned techniques, the description of the model atmosphere, and the optimizations that we applied to the code. We carry out some numerical experiments to show the performance of the code and the regularization techniques that we implemented. We made STiC publicly available to the community.

IPOLE - semi-analytic scheme for relativistic polarized radiative transport

Abstract: We describe ${\\tt ipole}$, a new public ray-tracing code for covariant, polarized radiative transport. The code extends the ${\\tt ibothros}$ scheme for covariant, unpolarized transport using two representations of the polarized radiation field: in the coordinate frame, it parallel transports the coherency tensor; in the frame of the plasma it evolves the Stokes parameters under emission, absorption, and Faraday conversion. The transport step is implemented to be as spacetime- and coordinate- independent as possible. The emission, absorption, and Faraday conversion step is implemented using an analytic solution to the polarized transport equation with constant coefficients. As a result, ${\\tt ipole}$ is stable, efficient, and produces a physically reasonable solution even for a step with high optical depth and Faraday depth. We show that the code matches analytic results in flat space, and that it produces results that converge to those produced by Dexter's ${\\tt grtrans}$ polarized transport code on a complicated model problem. We expect ${\\tt ipole}$ will mainly find applications in modeling Event Horizon Telescope sources, but it may also be useful in other relativistic transport problems such as modeling for the IXPE mission.

Colored, Daytime Radiative Coolers with Thin-Film Resonators for Aesthetic Purposes

Abstract: DOI: 10.1002/adom.201800707 sunlight. The features of an accurate radiative model, strong selective emission in the atmospheric transparency window, and broadband high reflectance to solar irradiation are each formulated individually and then configured collectively to accomplish this outcome. Because all of the successful examples of daytime radiative coolers possess high solar reflectivity, they are white or silver in color and are thus not visually appealing,[5–7,9] thereby restricting the possible installation locations and limiting their net cooling capacity. Although previous efforts have been paid to incorporate colors into the radiative cooler,[26] the research only dealt with theoretical calculations without experimental demonstrations, and structural optimization of colored radiative coolers has not been performed. Here, we present concepts and strategies for daytime radiative cooling systems that involve comparable attention to engineering design but with the goal of achieving systems that offer aesthetically desired colors and patterns and functional purposes, thus enabling more widespread installation. The experimental demonstration exhibits subambient cooling behaviors under a clear sky while preserving its color. The approaches reported here can address application concepts for wearable electronic devices whose operational temperature is lowered by radiative cooling. Figure 1a exhibits a schematic of a decorative colored passive radiative cooler (CPRC) for aesthetic purposes featuring areas with subtractive primary colors (i.e., cyan, magenta, and yellow) on a silvery background, where the latter area represents a conventional daytime radiative cooler. The CPRC consists of a SE comprising a bilayer of SiO2 (650 nm) and Si3N4 (910 nm), whose thicknesses are defined by extensive numerical optimization; and a metal reflector comprising an Ag film (100 nm) deposited on a silicon substrate (Figure 1b, left). Additional photonic nanostructures were inserted below the SE to generate vivid colors at specific desired areas (Figure 1b, right), which comprised a thin-film resonator composed of a metal–insulator–metal (MIM) structure. The MIM structure determined each color via interference in the 1D stacked layers, where the color generation was precisely controlled by tuning the thickness of the insulator layer (i.e., SiO2 cavity) in the MIM. In this study, the MIM structure was chosen as the colorant structure because it provided minimal loss of solar reflectance and a narrow spectral width compared with other additive color filters such as metal gratings and 1D photonic crystals (1D PhC), Recently developed approaches in passive radiative cooling enable daytime cooling via engineered photonic structure layouts. However, the use of these daytime radiative coolers is restricted owing to their nonaesthetic appearance resulted from strong solar reflection. Therefore, this article introduces a colored passive radiative cooler (CPRC) capable of generating potential cooling power, based on a thin-film optical resonator embedded in an efficient thermal emission structure. This CPRC not only selectively emits infrared wave through the atmospheric transparency window but also displays subtractive primary colors to exhibit the desired appearance. Theoretical analysis and systematic experiments prove the possibility of subambient cooling via CPRC by lowering the temperature to 3.9 °C below the ambient air in the daylight. This is the first example of coloring radiative cooler by photonic structures. Successful demonstration of cooling/coloring behavior with wearable electronic devices under solar irradiation represents a major step forward in the field of temperature-sensitive, flexible, wearable electronic/optoelectronic devices.

The role of electron heating physics in images and variability of the Galactic Centre black hole Sagittarius A

Abstract: The accretion flow around the Galactic Center black hole Sagittarius A* (Sgr A*) is expected to have an electron temperature that is distinct from the ion temperature, due to weak Coulomb coupling in the low-density plasma. We present four two-temperature general relativistic radiative magnetohydrodynamic (GRRMHD) simulations of Sgr A* performed with the code KORAL. These simulations use different electron heating prescriptions, motivated by different models of the underlying plasma microphysics. We compare the Landau-damped turbulent cascade model used in previous work with a new prescription we introduce based on the results of particle-in-cell simulations of magnetic reconnection. With the turbulent heating model, electrons are preferentially heated in the polar outflow, whereas with the reconnection model electrons are heated by nearly the same fraction everywhere in the accretion flow. The spectra of the two models are similar around the submillimetre synchrotron peak, but the models heated by magnetic reconnection produce variability more consistent with the level observed from Sgr A*. All models produce 230~GHz images with distinct black hole shadows which are consistent with the image size measured by the Event Horizon Telescope, but only the turbulent heating produces an anisotropic `disc-jet' structure where the image is dominated by a polar outflow or jet at frequencies below the synchrotron peak. None of our models can reproduce the observed radio spectral slope, the large near-infrared and X-ray flares, or the near-infrared spectral index, all of which suggest non-thermal electrons are needed to fully explain the emission from Sgr A*.