Scanning tunneling spectroscopy

About: Scanning tunneling spectroscopy is a research topic. Over the lifetime, 7886 publications have been published within this topic receiving 213828 citations.

Observation Of Atomic Tunneling From An Accelerating Optical Potential

Abstract: ~Received 30 October 1996! We observe quantum tunneling of cold sodium atoms from an accelerating one-dimensional standing wave of light. Atoms are trapped in a far-detuned standing wave that is accelerated for a controlled duration. For sufficiently large values of the acceleration, we observe an exponential decay in the number of atoms that remain trapped as a function of the interaction time. We show that this loss is due to quantum tunneling, and compare the decay rates with Landau-Zener theory. We also observe oscillations in the tunneling rate as a function of the acceleration which are due to quantum interference effects. @S1050-2947~97!50702-5# PACS number~s!: 03.75.Be, 32.80.Pj, 42.50.Vk Tunneling in the center-of mass motion of atoms should become an important process at the low temperatures that are now achieved with laser cooling. This can appear, for example, as a loss mechanism for atoms confined in an optical lattice constructed from interfering beams of light. While atomic motion in these structures has become an active area of research @1,2#, tunneling has been obscured by spontaneous scattering @3#. An alternative atom optics system where tunneling can be significant has appeared in our efforts to develop a cold atomic beam for interferometry. Our approach has been to launch laser-cooled atoms in the potential created by an accelerating, far-detuned, standing wave of light. This system was previously used to study Wannier-Stark ladders @4# and Bloch oscillations @5#. The results reported in this Rapid Communications provide an observation of tunneling in atom optics, and the high degree of experimental control has enabled a quantitative comparison with theory. We consider atomic motion in an accelerating standing wave of light. For sufficiently large detuning from atomic resonance, the atoms remain in their internal ground state and experience an effective one-dimensional potential given by V0cos@2kL(x2at 2 /2)#, where k L52p/l L is the wave number, and a is the acceleration of the standing wave @6#. The well depth V0 is the amplitude of the optical dipole potential. It is proportional to the laser intensity and inversely proportional to detuning from atomic resonance. We neglect variations of the potential in the two transverse directions, which is justified for beams that are sufficiently

Measurement of Electronic States of PbS Nanocrystal Quantum Dots Using Scanning Tunneling Spectroscopy: The Role of Parity Selection Rules in Optical Absorption

Abstract: We study the structure of electronic states in individual PbS nanocrystal quantum dots by scanning tunneling spectroscopy (STS) using one-to-two monolayer nanocrystal films treated with 1, 2-ethanedithiols (EDT). Up to six individual valence and conduction band states are resolved for a range of quantum dot sizes. The measured states' energies are in good agreement with calculations using the k · p four-band envelope function formalism. A comparison of STS and optical absorption spectra indicates that some of the absorption features can only be explained by asymmetric transitions involving the states of different symmetries (e.g., S and P or P and D), which points towards the relaxation of the parity selection rules in these nanostructures. STS measurements also reveal a midgap feature, which is likely similar to one observed in previous charge transport studies of EDT-treated quantum dot films.

Adsorbate-induced alloy phase separation: a direct view by high-pressure scanning tunneling microscopy.

Abstract: The influence of high pressures of carbon monoxide (CO) on the stability of a Au/Ni(111) surface alloy has been studied by high-pressure scanning tunneling microscopy. We show that CO induces a phase separation of the surface alloy at high pressures, and by means of time-lapsed STM movies we find that Ni atoms are removed from the surface layer during the process. Density functional theory calculations reveal the thermodynamic driving force for the phase separation to be the Au-induced compression of the CO overlayer with a resulting CO-CO repulsion. Furthermore, the atomistic mechanism of the process is shown to be kink-site carbonyl formation and evaporation which is found to be enhanced by the presence of Au.

First-principles theory of atom extraction by scanning tunneling microscopy.

Abstract: A new method to provide a self-consistent electronic structure, field, and current distribution for an atomistic bielectrode system with applied bias voltages is presented. In our method the scattering waves are calculated by a step-by-step recursion-matrix method and two different Fermi levels are assigned to each electrode in accord with a given applied bias voltage. The method is applied to the scanning tunneling microscope (STM) system around the contact region. The tip-surface chemical interaction induced by the electric fields is shown to be important for the extreme specificity of atom extraction by STM.

Layered Antiferromagnetism Induces Large Negative Magnetoresistance in the van der Waals Semiconductor CrSBr.

Abstract: The recent discovery of magnetism within the family of exfoliatable van der Waals (vdW) compounds has attracted considerable interest in these materials for both fundamental research and technological applications. However, current vdW magnets are limited by their extreme sensitivity to air, low ordering temperatures, and poor charge transport properties. Here the magnetic and electronic properties of CrSBr are reported, an air-stable vdW antiferromagnetic semiconductor that readily cleaves perpendicular to the stacking axis. Below its Neel temperature, TN = 132 ± 1 K, CrSBr adopts an A-type antiferromagnetic structure with each individual layer ferromagnetically ordered internally and the layers coupled antiferromagnetically along the stacking direction. Scanning tunneling spectroscopy and photoluminescence (PL) reveal that the electronic gap is ΔE = 1.5 ± 0.2 eV with a corresponding PL peak centered at 1.25 ± 0.07 eV. Using magnetotransport measurements, strong coupling between magnetic order and transport properties in CrSBr is demonstrated, leading to a large negative magnetoresistance response that is unique among vdW materials. These findings establish CrSBr as a promising material platform for increasing the applicability of vdW magnets to the field of spin-based electronics.