Showing papers on "Scattering published in 2018"

General Relativity from Scattering Amplitudes.

Abstract: Weoutline the program to apply modern quantum field theory methods to calculate observables in classical general relativity through a truncation to classical terms of the multigraviton, two-body, on-shell scattering amplitudes between massive fields. Since only long-distance interactions corresponding to nonanalytic pieces need to be included, unitarity cuts provide substantial simplifications for both post-Newtonian and post-Minkowskian expansions. We illustrate this quantum field theoretic approach to classical general relativity by computing the interaction potentials to second order in the post-Newtonian expansion, as well as the scattering functions for two massive objects to second order in the post-Minkowskian expansion. We also derive an all-order exact result for gravitational light-by-light scattering.

Topologically Enabled Ultra-high-Q Guided Resonances Robust to Out-of-plane Scattering

Abstract: Due to their ability to confine light, optical resonators are of great importance to science and technology, yet their performances are often limited by out-of-plane scattering losses from inevitable fabrication imperfections. Here, we theoretically propose and experimentally demonstrate a class of guided resonances in photonic crystal slabs, where out-of-plane scattering losses are strongly suppressed due to their topological nature. Specifically, these resonances arise when multiple bound states in the continuum - each carrying a topological charge - merge in the momentum space and enhance the quality factors of all resonances nearby. We experimentally achieve quality factors as high as $4.9\times 10^5$ based on these resonances in the telecommunication regime, which is 12-times higher than ordinary designs. We further show this enhancement is robust across the samples we fabricated.Our work paves the way for future explorations of topological photonics in systems with open boundary condition and their applications in improving optoelectronic devices in photonic integrated circuits.

Constraints on sub-GeV dark matter-electron scattering from the DarkSide-50 experiment

Abstract: We present new constraints on sub-GeV dark-matter particles scattering off electrons based on 6780.0 kg d of data collected with the DarkSide-50 dual-phase argon time projection chamber. This analysis uses electroluminescence signals due to ionized electrons extracted from the liquid argon target. The detector has a very high trigger probability for these signals, allowing for an analysis threshold of three extracted electrons, or approximately 0.05 keVee. We calculate the expected recoil spectra for dark matter-electron scattering in argon and, under the assumption of momentum-independent scattering, improve upon existing limits from XENON10 for dark-matter particles with masses between 30 and 100 MeV/c^{2}.

Grain boundary dominated charge transport in Mg3Sb2-based compounds

Abstract: Thermally activated mobility near room temperature is a signature of detrimental scattering that limits the efficiency and figure-of-merit zT in thermoelectric semiconductors. This effect has been observed dramatically in Mg3Sb2-based compounds, but also to a lesser extent in other thermoelectric compounds. Processing samples differently or adding impurities such that this effect is less noticeable produces materials with a higher zT. Experiments suggest that the behavior is related to grain boundaries, but impurity scattering has also been proposed. However, conventional models using Matthissen's rule are not able to explain the dramatic change in the temperature dependency of conductivity or drift mobility which is observed in Mg3Sb2-based compounds. We find that it is essential to consider the grain boundary region as an effectively separate phase rather than a scattering center, taking into account the weaker screening in semiconductors compared with classical metals. By modeling a grain boundary phase with a band offset, we successfully reproduce the experimentally observed conductivity versus temperature and thermopower versus conductivity relations, which indicate an improved description of transport. The model shows good agreement with measured grain size dependencies of conductivity, opening up avenues for quantitatively engineering materials with similar behavior. Model estimates predict room for >60% improvement in the room temperature zT of Mg3.2Sb1.5Bi0.49Te0.01 if the grain boundary resistance could be eliminated.

Quantum Oscillation from In-Gap States and a Non-Hermitian Landau Level Problem

Abstract: Motivated by recent experiments on Kondo insulators, we theoretically study quantum oscillations from disorder-induced in-gap states in small-gap insulators By solving a non-Hermitian Landau level problem that incorporates the imaginary part of electron's self-energy, we show that the oscillation period is determined by the Fermi surface area in the absence of the hybridization gap, and we derive an analytical formula for the oscillation amplitude as a function of the indirect band gap, scattering rates, and temperature Over a wide parameter range, we find that the effective mass is controlled by scattering rates, while the Dingle factor is controlled by the indirect band gap We also show the important effect of scattering rates in reshaping the quasiparticle dispersion in connection with angle-resolved photoemission measurements on heavy fermion materials

Early-Universe constraints on dark matter-baryon scattering and their implications for a global 21 cm signal

Abstract: We present and compare several cosmological constraints on the cross section for elastic scattering between dark matter (DM) and baryons, for cross sections with a range of power-law dependences on the DM-baryon relative velocity $v$, especially focusing on the case of $\sigma \propto v^{-4}$. We study constraints spanning a wide range of epochs in cosmological history, from pre-recombination distortions to the blackbody spectrum and anisotropies of the cosmic microwave background (CMB), to modifications to the intergalactic medium temperature and the resulting 21cm signal, and discuss the allowed signals in the latter channels given the constraints from the former. We improve previous constraints on DM-baryon scattering from the CMB anisotropies, demonstrate via principal component analysis that the effect on the CMB can be written as a simple function of DM mass, and map out the redshifts dominating this signal. We show that given high-redshift constraints on DM-baryon scattering, a $v^{-4}$ scaling of the cross section for light DM would be sufficient to explain the deep 21cm absorption trough recently claimed by the EDGES experiment, if 100% of the DM scatters with baryons. For millicharged DM models proposed to explain the observation, where only a small fraction of the DM interacts, we estimate that a PIXIE-like future experiment measuring CMB spectral distortion could test the relevant parameter space.

Uncovering electron scattering mechanisms in NiFeCoCrMn derived concentrated solid solution and high entropy alloys

Abstract: Whilst it has long been known that disorder profoundly affects transport properties, recent measurements on a series of solid solution 3d-transition metal alloys reveal two orders of magnitude variations in the residual resistivity. Using ab-initio methods, we demonstrate that, while the carrier density of all alloys is as high as in normal metals, the electron mean-free-path can vary from ~10 A (strong scattering limit) to ~10$^3$ A (weak scattering limit). Here, we delineate the underlying electron scattering mechanisms responsible for this disparate behavior. While spin dependent site-diagonal disorder is always dominant, for alloys containing only Fe, Co, and Ni the majority spin channel experiences negligible disorder scattering, thereby providing a short circuit, while for Cr/Mn containing alloys both spin channels experience strong disorder scattering due to an electron filling effect. Unexpectedly, other scattering mechanisms (e.g. displacement scattering) are found to be relatively weak in most cases.

UV complete me: Positivity Bounds for Particles with Spin

Abstract: For a low energy effective theory to admit a standard local, unitary, analytic and Lorentz-invariant UV completion, its scattering amplitudes must satisfy certain inequalities. While these bounds are known in the forward limit for real polarizations, any extension beyond this for particles with nonzero spin is subtle due to their non-trivial crossing relations. Using the transversity formalism (i.e. spin projections orthogonal to the scattering plane), in which the crossing relations become diagonal, these inequalities can be derived for 2-to-2 scattering between any pair of massive particles, for a complete set of polarizations at and away from the forward scattering limit. This provides a set of powerful criteria which can be used to restrict the parameter space of any effective field theory, often considerably more so than its forward limit subset alone.

Strong coupling and induced transparency at room temperature with single quantum dots and gap plasmons

Abstract: Coherent coupling between plasmons and transition dipole moments in emitters can lead to two distinct spectral effects: vacuum Rabi splitting at strong coupling strengths, and induced transparency (also known as Fano interference) at intermediate coupling strengths. Achieving either strong or intermediate coupling between a single emitter and a localized plasmon resonance has the potential to enable single-photon nonlinearities and other extreme light-matter interactions, at room temperature and on the nanometer scale. Both effects produce two peaks in the spectrum of scattering from the plasmon resonance, and can thus be confused if scattering measurements alone are performed. Here we report measurements of scattering and photoluminescence from individual coupled plasmon-emitter systems that consist of a single colloidal quantum dot in the gap between a gold nanoparticle and a silver film. The measurements unambiguously demonstrate weak coupling (the Purcell effect), intermediate coupling (Fano interference), and strong coupling (Rabi splitting) at room temperature.

Silicon Mie resonators for highly directional light emission from monolayer MoS 2

Abstract: Controlling light emission from quantum emitters has important applications, ranging from solid-state lighting and displays to nanoscale single-photon sources. Optical antennas have emerged as promising tools to achieve such control right at the location of the emitter, without the need for bulky, external optics. Semiconductor nanoantennas are particularly practical for this purpose because simple geometries such as wires and spheres support multiple, degenerate optical resonances. Here, we start by modifying Mie scattering theory developed for plane wave illumination to describe scattering of dipole emission. We then use this theory and experiments to demonstrate several pathways to achieve control over the directionality, polarization state and spectral emission that rely on a coherent coupling of an emitting dipole to optical resonances of a silicon nanowire. A forward-to-backward ratio of 20 was demonstrated for the electric dipole emission at 680 nm from a monolayer MoS2 by optically coupling it to a silicon nanowire.

A multipurpose instrument for time-resolved ultra-small-angle and coherent X-ray scattering

Abstract: This article presents the main technical features and performance of the upgraded beamline ID02 at the ESRF. The beamline combines different small-angle X-ray scattering techniques in one unique instrument, enabling static and kinetic investigations from angstrom to micrometre size scales and time resolution down to the sub-millisecond range. The main component of the instrument is an evacuated detector tube of length 34 m and diameter 2 m. Several different detectors are housed inside a motorized wagon that travels along a rail system, allowing an automated change of the sample–detector distance from about 1 to 31 m as well as selection of the desired detector. For optional combined wide-angle scattering measurements, a wide-angle detector is installed at the entrance cone of the tube. A scattering vector (of magnitude q) range of 0.002 ≤ q ≤ 50 nm−1 is covered with two sample–detector distances and a single-beam setting for an X-ray wavelength of 1 A. In the high-resolution mode, two-dimensional ultra-small-angle X-ray scattering patterns down to q < 0.001 nm−1 can be recorded, and the resulting one-dimensional profiles have superior quality as compared to those measured with an optimized Bonse–Hart instrument. In the highest-resolution mode, the beam is nearly coherent, thereby permitting multispeckle ultra-small-angle X-ray photon correlation spectroscopy measurements. The main applications of the instrument include the elucidation of static and transient hierarchical structures, and nonequilibrium dynamics in soft matter and biophysical systems.

Constraining Baryon-Dark-Matter Scattering with the Cosmic Dawn 21-cm Signal.

Abstract: The recent detection of an anomalously strong 21-cm signal of neutral hydrogen from cosmic dawn by the EDGES low-band radio experiment can be explained if cold dark matter particles scattered off the baryons draining excess energy from the gas. In this Letter we explore the expanded range of the 21-cm signal that is opened up by this interaction, varying the astrophysical parameters as well as the properties of dark matter particles in the widest possible range. We identify models consistent with current data by comparing to both the detection in the low-band region and the upper limits from the EDGES high-band antenna. We find that consistent models predict a 21-cm fluctuation during cosmic dawn that is between 3 and 30 times larger than the largest previously expected without dark matter scattering. The expected power spectrum exhibits strong baryon acoustic oscillations imprinted by the velocity-dependent cross section. The latter signature is a conclusive evidence of the velocity-dependent scattering and could be used by interferometers to verify the dark matter explanation of the EDGES detection.

Giant Electron-Phonon Coupling and Deep Conduction Band Resonance in Metal Halide Double Perovskite.

Abstract: The room-temperature charge carrier mobility and excitation–emission properties of metal halide perovskites are governed by their electronic band structures and intrinsic lattice phonon scattering mechanisms. Establishing how charge carriers interact within this scenario will have far-reaching consequences for developing high-efficiency materials for optoelectronic applications. Herein we evaluate the charge carrier scattering properties and conduction band environment of the double perovskite Cs2AgBiBr6 via a combinatorial approach; single crystal X-ray diffraction, optical excitation and temperature-dependent emission spectroscopy, resonant and nonresonant Raman scattering, further supported by first-principles calculations. We identify deep conduction band energy levels and that scattering from longitudinal optical phonons—via the Frohlich interaction—dominates electron scattering at room temperature, manifesting within the nominally nonresonant Raman spectrum as multiphonon processes up to the fourth ...

Inverse scattering transform for the nonlocal nonlinear Schrödinger equation with nonzero boundary conditions

Abstract: In 2013, a new nonlocal symmetry reduction of the well-known AKNS (an integrable system of partial differential equations, introduced by and named after Mark J. Ablowitz, David J. Kaup, and Alan C. Newell et al. (1974)) scattering problem was found. It was shown to give rise to a new nonlocal PT symmetric and integrable Hamiltonian nonlinear Schrodinger (NLS) equation. Subsequently, the inverse scattering transform was constructed for the case of rapidly decaying initial data and a family of spatially localized, time periodic one-soliton solutions was found. In this paper, the inverse scattering transform for the nonlocal NLS equation with nonzero boundary conditions at infinity is presented in four different cases when the data at infinity have constant amplitudes. The direct and inverse scattering problems are analyzed. Specifically, the direct problem is formulated, the analytic properties of the eigenfunctions and scattering data and their symmetries are obtained. The inverse scattering problem, which...

Optical tweezers and their applications

Abstract: Optical tweezers, tools based on strongly focused light, enable optical trapping, manipulation, and characterisation of a wide range of microscopic and nanoscopic materials. In the limiting cases of spherical particles either much smaller or much larger than the trapping wavelength, the force in optical tweezers separates into a conservative gradient force, which is proportional to the light intensity gradient and responsible for trapping, and a non-conservative scattering force, which is proportional to the light intensity and is generally detrimental for trapping, but fundamental for optical manipulation and laser cooling. For non-spherical particles or at intermediate (meso)scales, the situation is more complex and this traditional identification of gradient and scattering force is more elusive. Moreover, shape and composition can have dramatic consequences for optically trapped particle dynamics. Here, after an introduction to the theory and practice of optical forces with a focus on the role of shape and composition, we give an overview of some recent applications to biology, nanotechnology, spectroscopy, stochastic thermodynamics, critical Casimir forces, and active matter.

First look at two-loop five-gluon scattering in QCD

Abstract: We compute the leading-color contributions to five-gluon scattering at two loops in massless QCD. The integrands of all independent helicity amplitudes are evaluated using d -dimensional generalized unitarity cuts and finite field reconstruction techniques. Numerical evaluation of the integral basis is performed with sector decomposition methods to obtain the first benchmark results for all helicity configurations of a 2 → 3 scattering process in QCD.

Migdal Effect in Dark Matter Direct Detection Experiments

Abstract: The elastic scattering of an atomic nucleus plays a central role in dark matter direct detection experiments. In those experiments, it is usually assumed that the atomic electrons around the nucleus of the target material immediately follow the motion of the recoil nucleus. In reality, however, it takes some time for the electrons to catch up, which results in ionization and excitation of the atoms. In previous studies, those effects are taken into account by using the so-called Migdal’s approach, in which the final state ionization/excitation are treated separately from the nuclear recoil. In this paper, we reformulate the Migdal’s approach so that the “atomic recoil” cross section is obtained coherently, where we make transparent the energy-momentum conservation and the probability conservation. We show that the final state ionization/excitation can enhance the detectability of rather light dark matter in the GeV mass range via the nuclear scattering. We also discuss the coherent neutrino-nucleus scattering, where the same effects are expected.

Directly detecting sub-GeV dark matter with electrons from nuclear scattering

Abstract: Dark matter (DM) particles with mass in the sub-GeV range are an attractive alternative to heavier weakly interacting massive particles, but direct detection of such light particles is challenging. If, however, DM-nucleus scattering leads to ionization of the recoiling atom, the resulting electron may be detected even if the nuclear recoil is unobservable. We demonstrate that including this effect significantly enhances direct detection sensitivity to sub-GeV DM. Existing experiments set world-leading limits, and future experiments may probe the cross sections relevant for thermal freeze-out.

Light Scattering by a Dielectric Sphere: Perspectives on the Mie Resonances

Abstract: Light scattering by a small spherical particle, a central topic for electromagnetic scattering theory, is here considered. In this short review, some of the basic features of its resonant scattering behavior are covered. First, a general physical picture is described by a full electrodynamic perspective, the Lorenz–Mie theory. The resonant spectrum of a dielectric sphere reveals the existence of two distinctive types of polarization enhancement: the plasmonic and the dielectric resonances. The corresponding electrostatic (Rayleigh) picture is analyzed and the polarizability of a homogeneous spherical inclusion is extracted. This description facilitates the identification of the first type of resonance, i.e., the localized surface plasmon (plasmonic) resonance, as a function of the permittivity. Moreover, the electrostatic picture is linked with the plasmon hybridization model through the case of a step-inhomogeneous structure, i.e., a core–shell sphere. The connections between the electrostatic and electrodynamic models are reviewed in the small size limit and details on size-induced aspects, such as the dynamic depolarization and the radiation reaction on a small sphere are exposed through the newly introduced Mie–Pade approximative perspective. The applicability of this approximation is further expanded including the second type of resonances, i.e., the dielectric resonances. For this type of resonances, the Mie–Pade approximation reveals the main character of the two different cases of resonances of either magnetic or electric origin. A unified picture is therefore described encompassing both plasmonic and dielectric resonances, and the resonant conditions of all three different types are extracted as functions of the permittivity and the size of the sphere. Lastly, the directional scattering behavior of the first two dielectric resonances is exposed in a simple manner, namely the Kerker conditions for maximum forward and backscattering between the first magnetic and electric dipole contributions of a dielectric sphere. The presented results address several prominent functional features, aiming at readers with either theoretical or applied interest for the scattering aspects of a resonant sphere.

Ab initio electron density determination directly from solution scattering data.

Abstract: Using a novel iterative structure factor retrieval algorithm, here I show that electron density can be directly calculated from solution scattering data without modeling The algorithm was validated with experimental data from 12 different biological macromolecules This approach avoids many of the assumptions limiting the resolution and accuracy of modeling algorithms by explicitly calculating electron density This algorithm can be applied to a wide variety of molecular systems

First Observation of Coherent Elastic Neutrino-Nucleus Scattering

Abstract: The coherent elastic scattering of neutrinos off nuclei has eluded detection for four decades, even though its predicted cross section is by far the largest of all low-energy neutrino couplings. This mode of interaction offers new opportunities to study neutrino properties and leads to a miniaturization of detector size, with potential technological applications. We observed this process at a 6.7σ confidence level, using a low-background, 14.6-kilogram CsI[Na] scintillator exposed to the neutrino emissions from the Spallation Neutron Source at Oak Ridge National Laboratory. Characteristic signatures in energy and time, predicted by the standard model for this process, were observed in high signal-to-background conditions. Improved constraints on nonstandard neutrino interactions with quarks are derived from this initial data set.

Four-phonon scattering reduces intrinsic thermal conductivity of graphene and the contributions from flexural phonons

Abstract: We have developed a formalism of the exact solution to linearized phonon Boltzmann transport equation (BTE) for thermal conductivity calculation including three- and four-phonon scattering. We find strikingly high four-phonon scattering rates in single-layer graphene (SLG) based on the optimized Tersoff potential. The reflection symmetry in graphene, which forbids the three-ZA (out-of-plane acoustic) scattering, allows the four-ZA processes $\mathrm{ZA}+\mathrm{ZA}\ensuremath{\rightleftharpoons}\mathrm{ZA}+\mathrm{ZA}$ and $\mathrm{ZA}\ensuremath{\rightleftharpoons}\mathrm{ZA}+\mathrm{ZA}$ + ZA. As a result, the large phonon population of the low-energy ZA branch originated from the quadratic phonon dispersion leads to high four-phonon scattering rates, even much higher than the three-phonon scattering rates at room temperature. These four-phonon processes are dominated by the normal processes, which lead to a failure of the single mode relaxation time approximation. Therefore, we have solved the exact phonon BTE using an iterative scheme and then calculated the length- and temperature-dependent thermal conductivities. We find that the predicted thermal conductivity of SLG is lower than the previously predicted value from the three-phonon scattering only. The relative contribution of the ZA branch is reduced from 70% to 30% when four-phonon scattering is included. Furthermore, we have demonstrated that the four-phonon scattering in multilayer graphene and graphite is not strong due to the ZA splitting by interlayer van der Waals interaction. We also demonstrate that the five-phonon process in SLG is not strong due to the restriction of reflection symmetry.

Three-body spectrum in a finite volume: the role of cubic symmetry

Abstract: The three-particle quantization condition is partially diagonalized in the center-of-mass frame by using cubic symmetry on the lattice. To this end, instead of spherical harmonics, the kernel of the Bethe-Salpeter equation for particle-dimer scattering is expanded in the basis functions of different irreducible representations of the octahedral group. Such a projection is of particular importance for the three-body problem in the finite volume due to the occurrence of three-body singularities above breakup. Additionally, we study the numerical solution and properties of such a projected quantization condition in a simple model. It is shown that, for large volumes, these solutions allow for an instructive interpretation of the energy eigenvalues in terms of bound and scattering states.

What Limits the Intrinsic Mobility of Electrons and Holes in Two Dimensional Metal Dichalcogenides

Abstract: Two-dimensional (2D) metal dichalcogenides (MX2) are the most common type of 2D semiconductors and have shown great potential for a wide range of chemical and physical applications. However, they are limited by a low electron/hole mobility, which has been recognized as one of the major challenges impeding their further developments, and urges efforts to understand the mobility-limiting factors and discovery of higher-mobility alternatives. Here using density functional perturbation theory and Wannier interpolation of the electron–phonon matrix to study a wide range of MX2, we find that the intrinsic carrier mobility, in contrast to common belief, neither correlates with the effective mass nor can be assessed by the widely used deformation potential theory; instead it is limited by the longitudinal optical (LO) phonon scattering for most MX2, while for MoS2 and WS2, the mobility is limited by the longitudinal acoustic (LA) phonon scattering. Furthermore, we find that the LO scattering strength is strongly ...

Three-dimensional collective charge excitations in electron-doped copper oxide superconductors

Abstract: High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides5–7 reveals their charge origin, that is, without mixing with magnetic components5–7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought ‘acoustic plasmon’, which is a branch of distinct charge collective modes predicted for layered systems8–12 and argued to play a substantial part in mediating high-temperature superconductivity10–12. Resonant inelastic X-ray scattering on electron-doped copper oxide superconductors reveals a three-dimensional charge collective mode, which has properties suggestive of the long-sought acoustic plasmon.

Brillouin Light Scattering by Magnetic Quasivortices in Cavity Optomagnonics.

Abstract: A ferromagnetic sphere can support optical vortices in the form of whispering gallery modes and magnetic quasivortices in the form of magnetostatic modes with nontrivial spin textures. These vortices can be characterized by their orbital angular momenta. We experimentally investigate Brillouin scattering of photons in the whispering gallery modes by magnons in the magnetostatic modes, zeroing in on the exchange of the orbital angular momenta between the optical vortices and magnetic quasivortices. We find that the conservation of the orbital angular momentum results in different nonreciprocal behavior in the Brillouin light scattering. New avenues for chiral optics and optospintronics can be opened up by taking the orbital angular momenta as a new degree of freedom for cavity optomagnonics.