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Showing papers on "Spin wave published in 2011"


Journal ArticleDOI
TL;DR: In this article, the spin Hall effect in a thin film with strong spin-orbit scattering can excite magnetic precession in an adjacent ferromagnetic film, and the ratio of these two signals allows a quantitative determination of the spin current and spin Hall angle.
Abstract: We demonstrate that the spin Hall effect in a thin film with strong spin-orbit scattering can excite magnetic precession in an adjacent ferromagnetic film. The flow of alternating current through a Pt/NiFe bilayer generates an oscillating transverse spin current in the Pt, and the resultant transfer of spin angular momentum to the NiFe induces ferromagnetic resonance dynamics. The Oersted field from the current also generates a ferromagnetic resonance signal but with a different symmetry. The ratio of these two signals allows a quantitative determination of the spin current and the spin Hall angle.

1,421 citations


Journal ArticleDOI
TL;DR: Fully relativistic first-principles calculations based on density functional theory are performed to study the spin-orbit-induced spin splitting in monolayer systems of the transition-metal dichalcogenides MoS${}_{2}$, MoSe${}-2}, WS${} -2}, and WSe${] -2] as mentioned in this paper.
Abstract: Fully relativistic first-principles calculations based on density functional theory are performed to study the spin-orbit-induced spin splitting in monolayer systems of the transition-metal dichalcogenides MoS${}_{2}$, MoSe${}_{2}$, WS${}_{2}$, and WSe${}_{2}$. All these systems are identified as direct-band-gap semiconductors. Giant spin splittings of 148--456 meV result from missing inversion symmetry. Full out-of-plane spin polarization is due to the two-dimensional nature of the electron motion and the potential gradient asymmetry. By suppression of the Dyakonov-Perel spin relaxation, spin lifetimes are expected to be very long. Because of the giant spin splittings, the studied materials have great potential in spintronics applications.

1,374 citations


Journal ArticleDOI
TL;DR: In this paper, the magnetic component of terahertz transients enables ultrafast control of the spin degree of freedom in the NiO at frequencies as high as 1.5 GHz.
Abstract: Ultrafast charge and spin excitations in the elusive terahertz regime1,2 of the electromagnetic spectrum play a pivotal role in condensed matter3,4,5,6,7,8,9,10,11,12,13. The electric field of free-space terahertz pulses has provided a direct gateway to manipulating the motion of charges on the femtosecond timescale6,7,8,9. Here, we complement this process by showing that the magnetic component of intense terahertz transients enables ultrafast control of the spin degree of freedom. Single-cycle terahertz pulses switch on and off coherent spin waves in antiferromagnetic NiO at frequencies as high as 1 THz. An optical probe pulse with a duration of 8 fs follows the terahertz-induced magnetic dynamics directly in the time domain and verifies that the terahertz field addresses spins selectively by means of the Zeeman interaction. This concept provides a universal ultrafast means to control previously inaccessible magnetic excitations in the electronic ground state. Researchers report the direct observation of ultrafast magnetic dynamics using the magnetic component of highly intense terahertz wave pulses with a time resolution of 8 fs. This concept provides a universal ultrafast method of visualizing magnetic excitations in the electronic ground state.

817 citations


Journal ArticleDOI
TL;DR: This work directly observes a propagating spin wave launched from a spin torque oscillator with a nanoscale electrical contact into an extended Permalloy (nickel iron) film through the spin transfer torque effect, and shows that spin waves with tunable frequencies can propagate for several micrometres.
Abstract: Spin torque oscillators with nanoscale electrical contacts are able to produce coherent spin waves in extended magnetic films, and offer an attractive combination of electrical and magnetic field control, broadband operation, fast spin-wave frequency modulation, and the possibility of synchronizing multiple spin-wave injection sites. However, many potential applications rely on propagating (as opposed to localized) spin waves, and direct evidence for propagation has been lacking. Here, we directly observe a propagating spin wave launched from a spin torque oscillator with a nanoscale electrical contact into an extended Permalloy (nickel iron) film through the spin transfer torque effect. The data, obtained by wave-vector-resolved micro-focused Brillouin light scattering, show that spin waves with tunable frequencies can propagate for several micrometres. Micromagnetic simulations provide the theoretical support to quantitatively reproduce the results.

353 citations


Journal ArticleDOI
TL;DR: In this paper, the spin Hall effects in 4$d$ and 5€d$ transition metals, Nb, Ta, Mo, Pd, and Pt, were investigated by incorporating the spin absorption method in the lateral spin valve structure.
Abstract: We have investigated spin Hall effects in 4$d$ and 5$d$ transition metals, Nb, Ta, Mo, Pd, and Pt, by incorporating the spin absorption method in the lateral spin valve structure, where large spin current preferably relaxes into the transition metals, exhibiting strong spin-orbit interactions. Thereby nonlocal spin valve measurements enable us to evaluate their spin Hall conductivities. The sign of the spin Hall conductivity changes systematically depending on the number of $d$ electrons. This tendency is in good agreement with the recent theoretical calculation based on the intrinsic spin Hall effect.

338 citations


Journal ArticleDOI
TL;DR: The Berry curvature effect in the classical limit of long-wavelength magnetostatic spin waves having macroscopic coherence length is discussed, which is caused by the Berry phase in momentum space from the magnon band structure.
Abstract: We theoretically show that the magnon wave packet has a rotational motion in two ways: a self-rotation and a motion along the boundary of the sample (edge current). They are similar to the cyclotron motion of electrons, but unlike electrons the magnons have no charge and the rotation is not due to the Lorentz force. These rotational motions are caused by the Berry phase in momentum space from the magnon band structure. Furthermore, the rotational motion of the magnon gives an additional correction term to the magnon Hall effect. We also discuss the Berry curvature effect in the classical limit of long-wavelength magnetostatic spin waves having macroscopic coherence length.

304 citations


Journal ArticleDOI
TL;DR: First-principles calculations well describe both low α and large K(u) for these alloys, and the damping constant α, characterizing macroscopic spin relaxation and being a key factor in spin-transfer-torque systems, is not larger than 0.008 for the δ=1.46 (0.88) film.
Abstract: Spin precession with frequencies up to 280 GHz is observed in Mn(3-δ)Ga alloy films with a perpendicular magnetic anisotropy constant K(u)∼15 M erg/cm(3). The damping constant α, characterizing macroscopic spin relaxation and being a key factor in spin-transfer-torque systems, is not larger than 0.008 (0.015) for the δ=1.46 (0.88) film. Those are about one-tenth of α values for known materials with large K(u). First-principles calculations well describe both low α and large K(u) for these alloys.

293 citations


Journal ArticleDOI
TL;DR: It is experimentally show that exchange magnons can be detected by using a combination of spin pumping and the inverse spin-Hall effect proving its wavelength integrating capability down to the submicrometer scale.
Abstract: We experimentally show that exchange magnons can be detected by using a combination of spin pumping and the inverse spin-Hall effect proving its wavelength integrating capability down to the submicrometer scale. The magnons were injected in a ferrite yttrium iron garnet film by parametric pumping and the inverse spin-Hall effect voltage was detected in an attached Pt layer. The role of the density, wavelength, and spatial localization of the magnons for the spin pumping efficiency is revealed.

265 citations


Journal ArticleDOI
14 Apr 2011-Nature
TL;DR: It is demonstrated that interactions can be strong enough to reverse spin currents, with components of opposite spin reflecting off each other, and obtained the spin drag coefficient, the spin diffusivity and the spin susceptibility as a function of temperature on resonance and shown that they obey universal laws at high temperatures.
Abstract: Strongly interacting Fermi gases are ubiquitous in nature, from electrons in high-temperature superconductors, to nuclear matter. Their transport properties, such as the speed of diffusion, are poorly understood. Sommer et al. use controlled collisions of ultracold atomic clouds to investigate spin transport in a strongly interacting Fermi gas. They find that the spin excitations are maximally damped (leading to high spin drag), and that interactions are strong enough to reverse spin currents so that opposite spin components reflect off each other. The speed of diffusion is set by a fundamental quantum limit. The results have implications for any area involving fermion transport, from spintronics to studies of the early Universe. Transport of fermions, particles with half-integer spin, is central to many fields of physics. Electron transport runs modern technology, defining states of matter such as superconductors and insulators, and electron spin is being explored as a new carrier of information1. Neutrino transport energizes supernova explosions following the collapse of a dying star2, and hydrodynamic transport of the quark–gluon plasma governed the expansion of the early Universe3. However, our understanding of non-equilibrium dynamics in such strongly interacting fermionic matter is still limited. Ultracold gases of fermionic atoms realize a pristine model for such systems and can be studied in real time with the precision of atomic physics4. Even above the superfluid transition, such gases flow as an almost perfect fluid with very low viscosity when interactions are tuned to a scattering resonance3,5,6,7,8. In this hydrodynamic regime, collective density excitations are weakly damped6,7. Here we experimentally investigate spin excitations in a Fermi gas of 6Li atoms, finding that, in contrast, they are maximally damped. A spin current is induced by spatially separating two spin components and observing their evolution in an external trapping potential. We demonstrate that interactions can be strong enough to reverse spin currents, with components of opposite spin reflecting off each other. Near equilibrium, we obtain the spin drag coefficient, the spin diffusivity and the spin susceptibility as a function of temperature on resonance and show that they obey universal laws at high temperatures. In the degenerate regime, the spin diffusivity approaches a value set by ℏ/m, the quantum limit of diffusion, where ℏ/m is Planck’s constant divided by 2π and m the atomic mass. For repulsive interactions, our measurements seem to exclude a metastable ferromagnetic state9,10,11.

257 citations


Journal ArticleDOI
TL;DR: These findings quantitatively corroborate the present theoretical understanding of spin pumping in combination with the inverse spin Hall effect and the spin mixing conductance derived from the experimental data.
Abstract: We systematically measured the dc voltage V(ISH) induced by spin pumping together with the inverse spin Hall effect in ferromagnet-platinum bilayer films. In all our samples, comprising ferromagnetic 3d transition metals, Heusler compounds, ferrite spinel oxides, and magnetic semiconductors, V(ISH) invariably has the same polarity, and scales with the magnetization precession cone angle. These findings, together with the spin mixing conductance derived from the experimental data, quantitatively corroborate the present theoretical understanding of spin pumping in combination with the inverse spin Hall effect.

249 citations


Journal ArticleDOI
TL;DR: In this article, a linear response theory of the spin Seebeck effect was proposed, i.e., a spin voltage generation from heat current flowing in a ferromagnet.
Abstract: We formulate a linear response theory of the spin Seebeck effect, i.e., a spin voltage generation from heat current flowing in a ferromagnet. Our approach focuses on the collective magnetic excitation of spins, i.e., magnons. We show that the linear-response formulation provides us with a qualitative as well as quantitative understanding of the spin Seebeck effect observed in a prototypical magnet, yttrium iron garnet.

Journal ArticleDOI
TL;DR: It is demonstrated experimentally that the unidirectional vortex core reversal process also occurs when such azimuthal modes are excited and is confirmed by micromagnetic simulations, which clearly show the selection rules for this novel reversal mechanism.
Abstract: Micron-sized magnetic platelets in the flux-closed vortex state are characterized by an in-plane curling magnetization and a nanometer-sized perpendicularly magnetized vortex core. Having the simplest non-trivial configuration, these objects are of general interest to micromagnetics and may offer new routes for spintronics applications. Essential progress in the understanding of nonlinear vortex dynamics was achieved when low-field core toggling by excitation of the gyrotropic eigenmode at sub-GHz frequencies was established. At frequencies more than an order of magnitude higher vortex state structures possess spin wave eigenmodes arising from the magneto-static interaction. Here we demonstrate experimentally that the unidirectional vortex core reversal process also occurs when such azimuthal modes are excited. These results are confirmed by micromagnetic simulations, which clearly show the selection rules for this novel reversal mechanism. Our analysis reveals that for spin-wave excitation the concept of a critical velocity as the switching condition has to be modified.

Journal ArticleDOI
TL;DR: In this paper, the spin-wave transportation through a transverse magnetic domain wall (DW) in a magnetic nanowire is studied and it is found that the spin wave passes through a DW without reflection.
Abstract: The spin-wave transportation through a transverse magnetic domain wall (DW) in a magnetic nanowire is studied. It is found that the spin wave passes through a DW without reflection. A magnon, the quantum of the spin wave, carries opposite spins on the two sides of the DW. As a result, there is a spin angular momentum transfer from the propagating magnons to the DW. This magnonic spin-transfer torque can efficiently drive a DW to propagate in the opposite direction to that of the spin wave.

Journal ArticleDOI
TL;DR: In this paper, it was shown that the magnon wave packet undergoes two types of orbital motions in analogy with the electron system: the self-rotation motion and a motion along the boundary of the sample (edge current).
Abstract: Due to the Berry curvature in momentum space, the magnon wave packet undergoes two types of orbital motions in analogy with the electron system: the self-rotation motion and a motion along the boundary of the sample (edge current). The magnon edge current causes the thermal Hall effect, and these orbital motions give corrections to the thermal transport coefficients. We also apply our theory to the magnetostatic spin wave in a thin-film ferromagnet and derive expression for the Berry curvature.

Journal ArticleDOI
03 Jun 2011-Science
TL;DR: The excitation spectrum in a magnetic field is probed, identifying collective modes that emerged from the Coulomb interaction in the artificial lattice, as predicted by the Mott-Hubbard model and suggesting the existence of a Coulomb-driven ground state.
Abstract: Artificial crystal lattices can be used to tune repulsive Coulomb interactions between electrons. We trapped electrons, confined as a two-dimensional gas in a gallium arsenide quantum well, in a nanofabricated lattice with honeycomb geometry. We probed the excitation spectrum in a magnetic field, identifying collective modes that emerged from the Coulomb interaction in the artificial lattice, as predicted by the Mott-Hubbard model. These observations allow us to determine the Hubbard gap and suggest the existence of a Coulomb-driven ground state.

Journal ArticleDOI
TL;DR: In this article, a micromagnetic study on domain wall (DW) propagation in ferromagnetic nanotubes was conducted and it was found that DWs in a tubular geometry are much more robust than ones in flat strips.
Abstract: We report on a micromagnetic study on domain wall (DW) propagation in ferromagnetic nanotubes. It is found that DWs in a tubular geometry are much more robust than ones in flat strips. This is explained by topological considerations. Our simulations show that the Walker breakdown of the DW can be completely suppressed. Constant DW velocities above 1000 m/s are achieved by small fields. A different velocity barrier of the DW propagation is encountered, which significantly reduces the DW mobility. This effect occurs as the DW reaches the phase velocity of spin waves (SWs), thereby triggering a Cherenkov-like emission of SWs.

Journal ArticleDOI
TL;DR: It is shown that lateral spin valves with low-resistivity NiFe/MgO/Ag junctions enable efficient spin injection with high applied current density, which leads to the spin-valve voltage increasing 100-fold, suggesting a route to faster and manipulable spin transport for the development of pure spin-current-based memory, logic and sensing devices.
Abstract: The non-local spin injection in lateral spin valves is strongly expected to be an effective method to generate a pure spin current for potential spintronic application. However, the spin-valve voltage, which determines the magnitude of the spin current flowing into an additional ferromagnetic wire, is typically of the order of 1 μV. Here we show that lateral spin valves with low-resistivity NiFe/MgO/Ag junctions enable efficient spin injection with high applied current density, which leads to the spin-valve voltage increasing 100-fold. Hanle effect measurements demonstrate a long-distance collective 2π spin precession along a 6-μm-long Ag wire. These results suggest a route to faster and manipulable spin transport for the development of pure spin-current-based memory, logic and sensing devices.

Journal ArticleDOI
TL;DR: In this article, the first experimental demonstration of electrical spin injection, transport, and detection in bulk germanium (Ge) was reported and the nonlocal magnetoresistance (MR) in n-type Ge was observable up to 225 K.
Abstract: We report the first experimental demonstration of electrical spin injection, transport, and detection in bulk germanium (Ge). The nonlocal magnetoresistance (MR) in n-type Ge is observable up to 225 K. Our results indicate that the spin relaxation rate in the n-type Ge is closely related to the momentum scattering rate, which is consistent with the predicted Elliot-Yafet spin relaxation mechanism for Ge. The bias dependence of the nonlocal MR and the spin lifetime in n-type Ge is also investigated.

Journal ArticleDOI
TL;DR: In this paper, inelastic neutron scattering was used to study spin waves below and above T{sub N} in iron-arsenide BaFe{sub 2}As{sub2}.
Abstract: We use inelastic neutron scattering to study spin waves below and above T{sub N} in iron-arsenide BaFe{sub 2}As{sub 2}. In the low-temperature orthorhombic phase, we find highly anisotropic spin waves with a large damping along the antiferromagnetic a-axis direction. On warming the system to the paramagnetic tetragonal phase, the low-energy spin waves evolve into quasi-elastic excitations, while the anisotropic spin excitations near the zone boundary persist. These results strongly suggest the presence of a spin nematic fluid in the tetragonal phase of BaFe{sub 2}As{sub 2}, which may cause the electronic and orbital anisotropy observed in these materials.

Journal ArticleDOI
TL;DR: In this article, the spin Seebeck effect (SSE) was investigated in half-metallic Heusler compound (CMS)/Pt thin films to investigate the effect of spin polarization of ferromagnetic layer on SSE.
Abstract: The recently discovered spin Seebeck effect (SSE) which generates spin voltage due to a temperature gradient in ferromagnets, was systematically studied in half-metallic Heusler compound ${\mathrm{Co}}_{2}\mathrm{MnSi}$ (CMS)/Pt thin films to investigate the effect of spin polarization of ferromagnetic layer on SSE. An epitaxial thin film of CMS with an almost perfect $B$2-ordered structure was prepared directly on a MgO(001) substrate. The measurement was performed at room temperature for various temperature differences, \ensuremath{\Delta}$T$ $=$ 0--20 K between higher (300 K$+$\ensuremath{\Delta}$T$) and lower (300 K) temperature ends along the film. The clear sign reversal of the thermally induced spin voltage due to SSE at the higher and lower temperature ends of the CMS film was detected by means of inverse spin-Hall effect in a Pt wire. The SSE was also investigated in a Py thin film deposited on a MgO(001) substrate and compared to that with CMS to verify the effect of spin polarization on SSE. Comparable signals of SSE in CMS and Py thin films suggested that thermal excitation of magnons might have more vital effects in SSE than the degree of spin polarization in ferromagnetic metals.

Journal ArticleDOI
TL;DR: In this article, a holographic description of a system of strongly coupled fermions in 2 + 1 dimensions based on a D7-brane probe in the background of D3-branes is considered.
Abstract: We consider a holographic description of a system of strongly-coupled fermions in 2 + 1 dimensions based on a D7-brane probe in the background of D3-branes. The black hole embedding represents a Fermi-like liquid. We study the excitations of the Fermi liquid system. Above a critical density which depends on the temperature, the system becomes unstable towards an inhomogeneous modulated phase which is similar to a charge density and spin wave state. The essence of this instability can be effectively described by a Maxwell-axion theory with a background electric field. We also consider the fate of zero sound at non-zero temperature.

Journal ArticleDOI
TL;DR: In this article, the collective picosecond magnetization dynamics in [Co/Pd]8 multilayers with perpendicular magnetic anisotropy was observed and the damping coefficient α was found to be inversely proportional to the Co layer thickness.
Abstract: We report the experimental observation of collective picosecond magnetization dynamics in [Co/Pd]8 multilayers with perpendicular magnetic anisotropy. The precession frequency shows large and systematic variation from about 5 GHz to about 90 GHz with the decrease in the Co layer thickness from 1.0 to 0.22 nm due to the linear increase in the perpendicular magnetic anisotropy. The damping coefficient α is found to be inversely proportional to the Co layer thickness and a linear relation between the perpendicular magnetic anisotropy and α is established. We discuss the possible reasons behind the enhanced damping as the d-d hybridization at the interface and spin pumping. These observations are significant for the applications of these materials in spintronics and magnonic crystals.

Journal ArticleDOI
TL;DR: The spin torque effect in nanoferromagnets is described by a generalization of the Landau-Lifshitz-Gilbert (LLG) equation which forms a basic dynamical equation in the field of spintronics as discussed by the authors.
Abstract: The Landau-Lifshitz-Gilbert (LLG) equation is a fascinating nonlinear evolution equation both from mathematical and physical points of view. It is related to the dynamics of several important physical systems such as ferromagnets, vortex filaments, moving space curves, etc. and has intimate connections with many of the well known integrable soliton equations, including nonlinear Schr\"odinger and sine-Gordon equations. It can admit very many dynamical structures including spin waves, elliptic function waves, solitons, dromions, vortices, spatio-temporal patterns, chaos, etc. depending on the physical and spin dimensions and the nature of interactions. An exciting recent development is that the spin torque effect in nanoferromagnets is described by a generalization of the LLG equation which forms a basic dynamical equation in the field of spintronics. This article will briefly review these developments as a tribute to Robin Bullough who was a great admirer of the LLG equation.

Journal ArticleDOI
TL;DR: In this paper, the authors propose a concept of magnetic logic circuits engineering, which takes an advantage of magnetization as a computational state variable and exploits spin waves for information transmission, and present a library of logic gates consisting of magnetoelectric cells and spin wave buses providing 0 or π phase shifts.
Abstract: We propose a concept of magnetic logic circuits engineering, which takes an advantage of magnetization as a computational state variable and exploits spin waves for information transmission. The circuits consist of magneto-electric cells connected via spin wave buses. We present the result of numerical modeling showing the magneto-electric cell switching as a function of the amplitude as well as the phase of the spin wave. The phase-dependent switching makes it possible to engineer logic gates by exploiting spin wave buses as passive logic elements providing a certain phase-shift to the propagating spin waves. We present a library of logic gates consisting of magneto-electric cells and spin wave buses providing 0 or π phase shifts. The utilization of phases in addition to amplitudes is a powerful tool which let us construct logic circuits with a fewer number of elements than required for CMOS technology. As an example, we present the design of the magnonic Full Adder circuit comprising only 5 magneto-elec...

Journal ArticleDOI
TL;DR: Control of spin waves in a ferrite thin film via interfacial spin scattering was demonstrated, and the spin scattering affects the saturation behavior of high-power spin waves.
Abstract: Control of spin waves in a ferrite thin film via interfacial spin scattering was demonstrated. The experiments used a 4.6 μm-thick yttrium iron garnet (YIG) film strip with a 20-nm thick Pt capping layer. A dc current pulse was applied to the Pt layer and produced a spin current across the Pt thickness. As the spin current scatters off the YIG surface, it can either amplify or attenuate spin-wave pulses that travel in the YIG strip, depending on the current or field configuration. The spin scattering also affects the saturation behavior of high-power spin waves.

Journal ArticleDOI
TL;DR: In this paper, the authors used a material with an ordering temperature near room temperature to study the thermal properties of the artificial spin ice arrays of micromagnetic islands, and they confirmed a dynamical pre-melting of the spin ice structure at a temperature well below the intrinsic ordering temperature of the island material.
Abstract: Artificial spin ice arrays of micromagnetic islands are a means of engineering additional energy scales and frustration into magnetic materials. Despite much progress in elucidating the properties of such arrays, the `spins' in the systems studied so far have no thermal dynamics as the kinetic constraints are too high. Here we address this problem by using a material with an ordering temperature near room temperature. By measuring the temperature dependent magnetization in different principal directions, and comparing with simulations of idealized statistical mechanical models, we confirm a dynamical `pre-melting' of the artificial spin ice structure at a temperature well below the intrinsic ordering temperature of the island material. We thus create a spin ice array that has real thermal dynamics of the artificial spins over an extended temperature range.

Journal ArticleDOI
TL;DR: A theoretical approach is presented for the study of this combined process using a density matrix formalism, and the effect of the spin lattice relaxation times on the polarization buildup times and the resulting end polarization are discussed and the quenching of the polarizations by the hyperfine interaction is demonstrated.
Abstract: The dynamic nuclear polarization (DNP) process in solids depends on the magnitudes of hyperfine interactions between unpaired electrons and their neighboring (core) nuclei, and on the dipole-dipole interactions between all nuclei in the sample. The polarization enhancement of the bulk nuclei has been typically described in terms of a hyperfine-assisted polarization of a core nucleus by microwave irradiation followed by a dipolar-assisted spin diffusion process in the core-bulk nuclear system. This work presents a theoretical approach for the study of this combined process using a density matrix formalism. In particular, solid effect DNP on a single electron coupled to a nuclear spin system is considered, taking into account the interactions between the spins as well as the main relaxation mechanisms introduced via the electron, nuclear, and cross-relaxation rates. The basic principles of the DNP-assisted spin diffusion mechanism, polarizing the bulk nuclei, are presented, and it is shown that the polarization of the core nuclei and the spin diffusion process should not be treated separately. To emphasize this observation the coherent mechanism driving the pure spin diffusion process is also discussed. In order to demonstrate the effects of the interactions and relaxation mechanisms on the enhancement of the nuclear polarization, model systems of up to ten spins are considered and polarization buildup curves are simulated. A linear chain of spins consisting of a single electron coupled to a core nucleus, which in turn is dipolar coupled to a chain of bulk nuclei, is considered. The interaction and relaxation parameters of this model system were chosen in a way to enable a critical analysis of the polarization enhancement of all nuclei, and are not far from the values of (13)C nuclei in frozen (glassy) organic solutions containing radicals, typically used in DNP at high fields. Results from the simulations are shown, demonstrating the complex dependences of the DNP-assisted spin diffusion process on variations of the relevant parameters. In particular, the effect of the spin lattice relaxation times on the polarization buildup times and the resulting end polarization are discussed, and the quenching of the polarizations by the hyperfine interaction is demonstrated.

Journal ArticleDOI
TL;DR: In this article, a short spin-wave packet is excited in a yttrium-iron garnet (YIG) waveguide by a microwave signal and is detected at a distance of 3 mm by an attached Pt layer as a delayed spin Hall effect (ISHE) voltage pulse.
Abstract: Conversion of traveling magnons into an electron carried spin current is demonstrated in a time resolved experiment using a spatially separated inductive spin-wave source and an inverse spin Hall effect (ISHE) detector. A short spin-wave packet is excited in a yttrium-iron garnet (YIG) waveguide by a microwave signal and is detected at a distance of 3 mm by an attached Pt layer as a delayed ISHE voltage pulse. The delay in the detection appears due to the finite spin-wave group velocity and proves the magnon spin transport. The experiment suggests utilization of spin waves for the information transfer over macroscopic distances in spintronic devices and circuits.

Journal ArticleDOI
TL;DR: In this article, the authors reported measurements of the anisotropic magnetic susceptibility chi versus temperature T from 300 to 1000 K of single crystals of BaMn2As2, and magnetic inelastic neutron scattering measurements at 8 K and 75As NMR measurements from 4 to 300 K of polycrystalline samples.
Abstract: BaMn2As2 is unique among BaT2As2 compounds crystallizing in the body-centered-tetragonal ThCr2Si2 structure, which contain stacked square lattices of 3d transition metal T atoms, since it has an insulating large-moment (3.9 muB/Mn) G-type (checkerboard) antiferromagnetic AF ground state. We report measurements of the anisotropic magnetic susceptibility chi versus temperature T from 300 to 1000 K of single crystals of BaMn2As2, and magnetic inelastic neutron scattering measurements at 8 K and 75As NMR measurements from 4 to 300 K of polycrystalline samples. The Neel temperature determined from the chi(T) measurements is TN = 618(3) K. The measurements are analyzed using the J1-J2-Jc Heisenberg model. Linear spin wave theory for G-type AF ordering and classical and quantum Monte Carlo simulations and molecular field theory calculations of chi(T) and of the magnetic heat capacity Cmag(T) are presented versus J1, J2 and Jc. We also obtain band theoretical estimates of the exchange couplings in BaMn2As2. From analyses of our chi(T), NMR, neutron scattering, and previously published heat capacity data for BaMn2As2 on the basis of the above theories for the J1-J2-Jc Heisenberg model and our band-theoretical results, our best estimates of the exchange constants in BaMn2As2 are J1 = 13 meV, J2/J1 = 0.3 and Jc/J1 = 0.1, which are all antiferromagnetic. From our classical Monte Carlo simulations of the G-type AF ordering transition, these exchange parameters predict TN = 640 K for spin S = 5/2, in close agreement with experiment. Using spin wave theory, we also utilize these exchange constants to estimate the suppression of the ordered moment due to quantum fluctuations for comparison with the observed value and again obtain S = 5/2 for the Mn spin.

Journal ArticleDOI
Zhi-Gang Yu1
TL;DR: In this paper, the authors developed a systematic approach of quantifying spin-orbit coupling (SOC) and a rigorous theory of carrier spin relaxation caused by the SOC in disordered organic solids.
Abstract: We develop a systematic approach of quantifying spin-orbit coupling (SOC) and a rigorous theory of carrier spin relaxation caused by the SOC in disordered organic solids. The SOC mixes up and down spin in the polaron states and can be characterized by an admixture parameter γ2. This mixing effects spin flips as polarons hop from one molecule to another. The spin relaxation time is τ(sf) = R2/(16γ2 D), and the spin diffusion length is L(s) = R/4|γ|, where R is the mean polaron hopping distance and D the carrier diffusion constant. The SOC in tris-(8-hydroxyquinoline) aluminum (Alq3) is particularly strong due to the orthogonal arrangement of the three ligands. The theory quantitatively explains the temperature-dependent spin diffusion in Alq3 from recent muon measurements.