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Spontaneous emission
About: Spontaneous emission is a research topic. Over the lifetime, 12855 publications have been published within this topic receiving 323684 citations.
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TL;DR: A review of current research on the optical properties of ZnO nanostructures and results of nonlinear optical studies, such as second-harmonic generation, are presented.
Abstract: We present a review of current research on the optical properties of ZnO nanostructures. We provide a brief introduction to different fabrication methods for various ZnO nanostructures and some general guidelines on how fabrication parameters (temperature, vapor-phase versus solution-phase deposition, etc.) affect their properties. A detailed discussion of photoluminescence, both in the UV region and in the visible spectral range, is provided. In addition, different gain (excitonic versus electron hole plasma) and feedback (random lasing versus individual nanostructures functioning as Fabry-Perot resonators) mechanisms for achieving stimulated emission are described. The factors affecting the achievement of stimulated emission are discussed, and the results of time-resolved studies of stimulated emission are summarized. Then, results of nonlinear optical studies, such as second-harmonic generation, are presented. Optical properties of doped ZnO nanostructures are also discussed, along with a concluding outlook for research into the optical properties of ZnO.
1,746 citations
TL;DR: Comparisons with three-dimensional calculations guide us to decipher the contributions of the excitation enhancement, spontaneous emission modification, and quenching in the molecular excitation and emission processes.
Abstract: We investigate the coupling of a single molecule to a single spherical gold nanoparticle acting as a nanoantenna. Using scanning probe technology, we position the particle in front of the molecule with nanometer accuracy and measure a strong enhancement of more than 20 times in the fluorescence intensity simultaneous to a 20-fold shortening of the excited state lifetime. Comparisons with three-dimensional calculations guide us to decipher the contributions of the excitation enhancement, spontaneous emission modification, and quenching. Furthermore, we provide direct evidence for the role of the particle plasmon resonance in the molecular excitation and emission processes.
1,513 citations
TL;DR: It is shown that under the influence of pure vacuum noise two entangled qubits become completely disentangled in a finite-time, and in a specific example the time to be given by ln((2+sqrt[2] / 2) times the usual spontaneous lifetime).
Abstract: We show that under the influence of pure vacuum noise two entangled qubits become completely disentangled in a finite-time, and in a specific example we find the time to be given by ln((2+sqrt[2] / 2) times the usual spontaneous lifetime.
1,487 citations
Book•
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27 Aug 2012
TL;DR: In this paper, the authors present a survey of the most commonly used line-broadening and line-switching techniques for laser beams, including the following: 1.1.1 Semiclassical approach, 2.2.2 Allowed and Forbidden Transitions, and 3.3.3 Pumping Schemes.
Abstract: 1 Introductory Concepts.- 1.1 Spontaneous and Stimulated Emission, Absorption.- 1.1.1 Spontaneous Emission.- 1.1.2 Stimulated Emission.- 1.1.3 Absorption.- 1.2 The Laser Idea.- 1.3 Pumping Schemes.- 1.4 Properties of Laser Beams.- 1.4.1 Monochromaticity.- 1.4.2 Coherence.- 1.4.3 Directionality.- 1.4.4 Brightness.- Problems.- 2 Interaction of Radiation with Matter.- 2.1 Summary of Blackbody Radiation Theory.- 2.2 Absorption and Stimulated Emission.- 2.2.1 Rates of Absorption and Stimulated Emission.- 2.2.2 Allowed and Forbidden Transitions.- 2.2.3 Transition Cross Section, Absorption and Gain Coefficient.- 2.3 Spontaneous Emission.- 2.3.1 Semiclassical Approach.- 2.3.2 Quantum Electrodynamic Approach.- 2.3.3 Einstein Thermodynamic Treatment.- 2.3.4 Radiation Trapping, Superradiance, Superfluorescence, and Amplified Spontaneous Emission.- 2.4 Nonradiative Decay.- 2.5 Line Broadening Mechanisms.- 2.5.1 Homogeneous Broadening.- 2.5.2 Inhomogeneous Broadening.- 2.5.3 Combined Effect of Line Broadening Mechanisms.- 2.6 Saturation.- 2.6.1 Saturation of Absorption: Homogeneous Line.- 2.6.2 Gain Saturation: Homogeneous Line.- 2.6.3 Inhomogeneously Broadened Line.- 2.7 Degenerate Levels.- 2.8 Relation between Cross Section and Spontaneous Radiative Lifetime.- 2.9 Molecular Systems.- 2.9.1 Energy Levels of a Molecule.- 2.9.2 Level Occupation at Thermal Equilibrium.- 2.9.3 Radiative and Nonradiative Transitions.- Problems.- References.- 3 Pumping Processes.- 3.1 Introduction.- 3.2 Optical Pumping.- 3.2.1 Pumping Efficiency.- 3.2.2 Pump Light Distribution.- 3.2.3 Pumping Rate.- 3.3 Electrical Pumping.- 3.3.1 Electron Impact Excitation.- 3.3.2 Spatial Distribution of the Pump Rate.- 3.3.3 Pumping Efficiency.- 3.3.4 Excitation by (Near) Resonant Energy Transfer.- Problems.- References.- 4 Passive Optical Resonators.- 4.1 Introduction.- 4.2 Plane-Parallel Resonator.- 4.2.1 Approximate Treatment of Schawlow and Townes.- 4.2.2 Fox and Li Treatment.- 4.3 Confocal Resonator.- 4.4 Generalized Spherical Resonator.- 4.4.1 Mode Amplitudes, Diffraction Losses, and Resonance Frequencies.- 4.4.2 Stability Condition.- 4.5 Unstable Resonators.- Problems.- References.- 5 Continuous Wave and Transient Laser Behavior.- 5.1 Introduction.- 5.2 Rate Equations.- 5.2.1 Four-Level Laser.- 5.2.2 Three-Level Laser.- 5.3 CW Laser Behavior.- 5.3.1 Four-Level Laser.- 5.3.2 Three-Level Laser.- 5.3.3 Optimum Output Coupling.- 5.3.4 Reasons for Multimode Oscillation.- 5.3.5 Single-Line and Single-Mode Oscillation.- 5.3.6 Two Numerical Examples.- 5.3.7 Frequency Pulling and Limit to Monochromaticity.- 5.3.8 Lamb Dip and Active Stabilization of Laser Frequency.- 5.4 Transient Laser Behavior.- 5.4.1 Spiking Behavior of Single-Mode and Multimode Lasers.- 5.4.2 Q-Switching.- 5.4.2.1 Methods of Q-Switching.- 5.4.2.2 Operating Regimes.- 5.4.2.3 Theory of Q-Switching.- 5.4.2.4 A Numerical Example.- 5.4.3 Mode Locking.- 5.4.3.1 Methods of Mode Locking.- 5.4.3.2 Operating Regimes.- 5 5 Limits to the Rate Equations.- Problems.- References.- 6 Types of Lasers.- 6.1 Introduction.- 6.2 Solid-State Lasers.- 6.2.1 The Ruby Laser.- 6.2.2 Neodymium Lasers.- 6.3 Gas Lasers.- 6.3.1 Neutral Atom Lasers.- 6.3.2 Ion Lasers.- 6.3.2.1 Ion Gas Lasers.- 6.3.2.2 Metal Vapor Lasers.- 6.3.3 Molecular Gas Lasers.- 6.3.3.1 Vibrational-Rotational Lasers.- 6.3.3.2 Vibronic Lasers.- 6.3.3.3 Excimer Lasers.- 6.4 Liquid Lasers (Dye Lasers).- 6.4.1 Photophysical Properties of Organic Dyes.- 6.4.2 Characteristics of Dye Lasers.- 6.5 Chemical Lasers.- 6.6 Semiconductor Lasers.- 6.6.1 Photophysical Properties of Semiconductor Lasers.- 6.6.2 Characteristics of Semiconductor Lasers.- 6.7 Color-Center Lasers.- 6.8 The Free-Electron Laser.- 6.9 Summary of Performance Data.- Problems.- References.- 7 Properties of Laser Beams.- 7.1 Introduction.- 7.2 Monochromaticity.- 7.3 First-Order Coherence.- 7.3.1 Complex Representation of Polychromatic Fields.- 7.3.2 Degree of Spatial and Temporal Coherence.- 7.3.3 Measurement of Spatial and Temporal Coherence.- 7.3.4 Relation between Temporal Coherence and Monochromaticity.- 7.3.5 Some Numerical Examples.- 7.4 Directionality.- 7.5 Laser Speckle.- 7.6 Brightness.- 7.7 Higher-Order Coherence.- Problems.- References.- 8 Laser Beam Transformation.- 8.1 Introduction.- 8.2 Transformation in Space. Gaussian Beam Propagation.- 8.3 Transformation in Amplitude: Laser Amplification.- 8.4 Transformation in Frequency: Second-Harmonic Generation and Parametric Oscillation.- 8.4.1 Physical Picture.- 8.4.1.1 Second-Harmonic Generation.- 8.4.1.2 Parametric Oscillation.- 8.4.2 Analytical Treatment.- 8.4.2.1 Parametric Oscillation.- 8.4.2.2 Second-Harmonic Generation.- Problems.- References.- 9 Applications of Lasers.- 9.1 Introduction.- 9.2 Applications in Physics and Chemistry.- 9.3 Applications in Biology and Medicine.- 9.4 Material Working.- 9.5 Optical Communications.- 9.6 Measurement and Inspection.- 9.7 Thermonuclear Fusion.- 9.8 Information Processing and Recording.- 9.9 Military Applications.- 9.10 Holography.- 9.11 Concluding Remarks.- References.- Appendixes.- A Space-Dependent Rate Equations.- B Physical Constants.- Answers to Selected Problems.
1,483 citations
TL;DR: This work demonstrates a cavity-free, broadband approach for engineering photon–emitter interactions via subwavelength confinement of optical fields near metallic nanostructures and shows that efficient coupling is accompanied by more than 2.5-fold enhancement of the quantum dot spontaneous emission, in good agreement with theoretical predictions.
Abstract: Control over the interaction between single photons and individual optical emitters is an outstanding problem in quantum science and engineering. It is of interest for ultimate control over light quanta, as well as for potential applications such as efficient photon collection, single-photon switching and transistors, and long-range optical coupling of quantum bits. Recently, substantial advances have been made towards these goals, based on modifying photon fields around an emitter using high-finesse optical cavities. Here we demonstrate a cavity-free, broadband approach for engineering photon-emitter interactions via subwavelength confinement of optical fields near metallic nanostructures. When a single CdSe quantum dot is optically excited in close proximity to a silver nanowire, emission from the quantum dot couples directly to guided surface plasmons in the nanowire, causing the wire's ends to light up. Non-classical photon correlations between the emission from the quantum dot and the ends of the nanowire demonstrate that the latter stems from the generation of single, quantized plasmons. Results from a large number of devices show that efficient coupling is accompanied by more than 2.5-fold enhancement of the quantum dot spontaneous emission, in good agreement with theoretical predictions.
1,412 citations