Spontaneous emission

About: Spontaneous emission is a research topic. Over the lifetime, 12855 publications have been published within this topic receiving 323684 citations.

Control of emission characteristics in organic thin‐film electroluminescent diodes using an optical‐microcavity structure

Abstract: An electroluminescent diode with a microcavity structure which comprised a reflective Ag anode (36 nm), a hole transport dye layer (250 nm), an emission dye laser (15 nm), an electron transport dye layer (240 nm), and a reflective MgAg cathode was fabricated. A diode without the microcavity structure with a transparent ITO anode was also prepared for reference. The diode with microcavity was driven in the electric excitation mode and emission spectra at fixed detection angles were measured together with the angular dependence of emission intensity at fixed wavelengths. A sharpening of emission spectra and a marked alteration of emission patterns in the diode with microcavity were observed.

Room temperature continuous wave operation and controlled spontaneous emission in ultrasmall photonic crystal nanolaser.

Abstract: Photonic crystal slab enables us to form an ultrasmall laser cavity with a modal volume close to the diffraction limit of light. However, the thermal resistance of such nanolasers, as high as 10(6) K/W, has prevented continuous-wave operation at room temperature. The present paper reports on the first successful continuous-wave operation at room temperature for the smallest nanolaser reported to date, achieved through fabrication of a laser with a low threshold of 1.2 muW. Near-thresholdless lasing and spontaneous emission enhancement due to the Purcell effect are also demonstrated in a moderately low Q nanolaser, both of which are well explained by a detailed rate equation analysis.

Highly efficient light-emitting diodes with microcavities

Abstract: One-dimensional microcavities are optical resonators with coplanar reflectors separated by a distance on the order of the optical wavelength. Such structures quantize the energy of photons propagating along the optical axis of the cavity and thereby strongly modify the spontaneous emission properties of a photon-emitting medium inside a microcavity. This report concerns semiconductor light-emitting diodes with the photon-emitting active region of the light-emitting diodes placed inside a microcavity. These devices are shown to have strongly modified emission properties including experimental emission efficiencies that are higher by more than a factor of 5 and theoretical emission efficiencies that are higher by more than a factor of 10 than the emission efficiencies in conventional light-emitting diodes.

Imaging chromophores with undetectable fluorescence by stimulated emission microscopy

Abstract: Fluorescence, that is, spontaneous emission, is generally more sensitive than absorption measurement, and is widely used in optical imaging. However, many chromophores, such as haemoglobin and cytochromes, absorb but have undetectable fluorescence because the spontaneous emission is dominated by their fast non-radiative decay. Yet the detection of their absorption is difficult under a microscope. Here we use stimulated emission, which competes effectively with the nonradiative decay, to make the chromophores detectable, and report a new contrast mechanism for optical microscopy. In a pump-probe experiment, on photoexcitation by a pump pulse, the sample is stimulated down to the ground state by a time-delayed probe pulse, the intensity of which is concurrently increased. We extract the miniscule intensity increase with shot-noise-limited sensitivity by using a lock-in amplifier and intensity modulation of the pump beam at a high megahertz frequency. The signal is generated only at the laser foci owing to the nonlinear dependence on the input intensities, providing intrinsic three-dimensional optical sectioning capability. In contrast, conventional one-beam absorption measurement exhibits low sensitivity, lack of three-dimensional sectioning capability, and complication by linear scattering of heterogeneous samples. We demonstrate a variety of applications of stimulated emission microscopy, such as visualizing chromoproteins, non-fluorescent variants of the green fluorescent protein, monitoring lacZ gene expression with a chromogenic reporter, mapping transdermal drug distributions without histological sectioning, and label-free microvascular imaging based on endogenous contrast of haemoglobin. For all these applications, sensitivity is orders of magnitude higher than for spontaneous emission or absorption contrast, permitting nonfluorescent reporters for molecular imaging.

Spontaneous and induced atomic decay in photonic band structures

Abstract: We present a comprehensive quantum electrodynamical analysis of the interaction between a continuum with photonic band gaps (PBGs) or frequency cut-off and an excited two-level atom, which can be either ‘bare’ or ‘dressed’ by coupling to a near-resonant field mode. A diversity of novel features in the atom and field dynamics is shown to arise from the non-Markovian character of radiative decay into such a continuum of modes. Firstly the excited atom is shown to evolve, by spontaneous decay, into a superposition of non-decaying single-photon dressed states, each having an energy in a different PBG, and a decaying component. This superposition is determined by the atomic resonance shift, induced by the spontaneously emitted photon, into or out of a PBG. The main novel feature exhibited by the decaying excited-state component is the occurrence of beats between the shifted atomic resonance frequency and the PBG cut-off frequencies, corresponding to a non-Lorentzian emission spectrum. Secondly the ind...