Showing papers on "Synchrotron radiation published in 2003"

Polarization of the prompt gamma-ray emission from the gamma-ray burst of 6 december 2002

Abstract: Observations of the afterglows of gamma-ray bursts (GRBs) have revealed that they lie at cosmological distances, and so correspond to the release of an enormous amount of energy. The nature of the central engine that powers these events and the prompt gamma-ray emission mechanism itself remain enigmatic because, once a relativistic fireball is created, the physics of the afterglow is insensitive to the nature of the progenitor. Here we report the discovery of linear polarization in the prompt gamma-ray emission from GRB021206, which indicates that it is synchrotron emission from relativistic electrons in a strong magnetic field. The polarization is at the theoretical maximum, which requires a uniform, large-scale magnetic field over the gamma-ray emission region. A large-scale magnetic field constrains possible progenitors to those either having or producing organized fields. We suggest that the large magnetic energy densities in the progenitor environment (comparable to the kinetic energy densities of the fireball), combined with the large-scale structure of the field, indicate that magnetic fields drive the GRB explosion.

High resolution-high energy x-ray photoelectron spectroscopy using third-generation synchrotron radiation source, and its application to Si-high k insulator systems

Abstract: High-resolution x-ray photoelectron spectroscopy (XPS) at 6 keV photon energy has been realized utilizing high-flux-density x rays from the third generation high-energy synchrotron radiation facility, SPring-8. The method has been applied to analysis of high-k HfO2/interlayer/Si complementary metal–oxide–semiconductor gate-dielectric structures. With the high energy resolution and high throughput of our system, chemical-state differences were observed in the Si 1s, Hf 3d, and O 1s peaks for as-deposited and annealed samples. The results revealed that a SiOxNy interlayer is more effective in controlling the interface structure than SiO2. Our results show the wide applicability of high resolution XPS with hard x rays from a synchrotron source.

Recent experiments on a small-angle/wide-angle X-ray scattering beam line at the ESRF

Abstract: Recent results using a new combined small-angle/wide-angle X-ray scattering (SAXS/WAXS) beam line at the European Synchrotron Radiation Source (ESRF) will be presented. This beam line is specifically designed to be able to handle complicated sample environments required to perform time-resolved experiments mimicking processing conditions used in material science. Besides the attention that has been given to the interfacing of these sample environments to the beam line data acquisition system also the developments in detector technology will be discussed. The influence that a high count rate and low noise WAXS detector can have on the accuracy of experimental results in polymer crystallisation will be shown. It is shown that it is feasible to detect crystalline volume fractions as low as 10 -3 -10 -4 in polymeric systems.

Brilliant, Coherent Far-Infrared (THz) Synchrotron Radiation

Abstract: A new technology for generating steady state, brilliant, broadband, coherent, far-infrared (FIR) radiation in electron storage rings is presented, suitable for FIR spectroscopy. An FIR power increase of up to 100 000 compared to the normal, incoherent synchrotron radiation in the range of approximately 5 to approximately 40 cm(-1) could be achieved. The source is up to 1000 times more brillant compared to a standard Hg arc lamp. The coherent synchrotron radiation is produced in a "low alpha" optics mode of the synchrotron light source BESSY, by bunch shortening and non-Gaussian bunch deformation.

A γ-ray burst with a high-energy spectral component inconsistent with the synchrotron shock model

Abstract: Gamma-ray bursts are among the most powerful events in nature. These events release most of their energy as photons with energies in the range from 30 keV to a few MeV, with a smaller fraction of the energy radiated in radio, optical, and soft X-ray afterglows. The data are in general agreement with a relativistic shock model, where the prompt and afterglow emissions correspond to synchrotron radiation from shock-accelerated electrons. Here we report an observation of a high-energy (multi-MeV) spectral component in the burst of 17 October 1994 that is distinct from the previously observed lower-energy gamma-ray component. The flux of the high-energy component decays more slowly and its fluence is greater than the lower-energy component; it is described by a power law of differential photon number index approximately -1 up to about 200 MeV. This observation is difficult to explain with the standard synchrotron shock model, suggesting the presence of new phenomena such as a different non-thermal electron process, or the interaction of relativistic protons with photons at the source.

Relations between the Photoluminescence Efficiency of CdTe Nanocrystals and Their Surface Properties Revealed by Synchrotron XPS

Abstract: The surface of colloidally prepared CdTe nanocrystals capped with thioglycolic acid has been studied by photoelectron spectroscopy with tunable synchrotron radiation excitation. Colloidally prepare...

Linear polarization in gamma-ray bursts: the case for an ordered magnetic field

Abstract: Linear polarization at the level of ~1%-3% has by now been measured in several gamma-ray burst afterglows. Whereas the degree of polarization, P, was found to vary in some sources, the position angle, θp, was roughly constant in all cases. Until now, the polarization has been commonly attributed to synchrotron radiation from a jet with a tangled magnetic field that is viewed somewhat off-axis. However, this model predicts either a peak in P or a 90° change in θp around the "jet break" time in the light curve, for which there has so far been no observational confirmation. We propose an alternative interpretation, wherein the polarization is attributed, at least in part, to a large-scale, ordered magnetic field in the ambient medium. The ordered component may dominate the polarization even if the total emissivity is dominated by a tangled field generated by postshock turbulence. In this picture, θp is roughly constant because of the uniformity of the field, whereas P varies as a result of changes in the ratio of the ordered-to-random mean-squared field amplitudes. We point out that variable afterglow light curves should be accompanied by a variable polarization. The radiation from the original ejecta, which includes the prompt γ-ray emission and the emission from the reverse shock (the "optical flash" and "radio flare"), could potentially exhibit a high degree of polarization (up to ~60%) induced by an ordered transverse magnetic field advected from the central source.

Electron density measurement with dual-energy x-ray CT using synchrotron radiation

Abstract: Monochromatic x-ray computed tomography (CT) at two different energies provides information about electron density of human tissue without ambiguity due to the beam hardening effect. This information makes the treatment planning for proton and heavy-ion radiotherapy more precise. We have started a feasibility study on dual energy x-ray CT by using synchrotron radiation. A translation-rotation scanning CT system was developed for quantitative measurement in order to clarify what precision in the measurement was achieved. Liquid samples of solutions of K2HPO4 and solid samples of tissue equivalent materials were used to simulate human tissue. The experiments were carried out using monochromatic x-rays with energies of 40, 70 and 80 keV produced by monochromatizing synchrotron radiation. The solid samples were also measured in a complementary method using high-energy carbon beams to evaluate the electron densities. The measured electron densities were compared with the theoretical values or the values measured in the complementary method. It was found that these values were in agreement in 0.9% on average. Effective atomic numbers were obtained as well from dual-energy x-ray CT. The tomographic image based on each of the electron densities and the effective atomic number presents a different feature of the material, and its contrast drastically differs from that in a conventional CT image.

X-ray generation in an ion channel

Abstract: X-ray generation by relativistic electrons in an ion channel is studied. The emission process is analyzed in the regime of high harmonic generation when the plasma wiggler strength is large. Like for the conventional free electron laser, the synchrotron-like broadband spectrum is generated in this regime. An asymptotic expression for the radiation spectrum of the spontaneous emission is derived. The radiation spectrum emitted from an axisymmetric monoenergetic electron beam is analyzed. The stimulated emission in the ion channel is studied and the gain of the ion-channel synchrotron-radiation laser is calculated. It is shown that the use of laser-produced ion channels leads to a much higher power of x-ray radiation than the one in a self-generated channel. In addition, the mean photon energy, the number of emitted photons and the brilliance of the photon beam increase dramatically. Three-dimensional particle-in-cell simulations of a 25-GeV electron bunch propagating in a laser-produced ion channel are mad...

High-resolution inner-shell spectroscopies of free atoms and molecules using soft-x-ray beamlines at the third-generation synchrotron radiation sources

Abstract: This article reviews the current status of inner-shell spectroscopies of free atoms and molecules using high-resolution soft-x-ray monochromators installed in the soft-x-ray beamlines at the third-generation synchrotron radiation facilities. Beamlines and endstations devoted to atomic and molecular inner-shell spectroscopies and various types of experimental techniques, such as ion yield spectroscopy, resonant photoemission spectroscopy and multiple-coincidence momentum imaging, are described. Experimental results for K-shell excitation of Ne, O K-shell excitation of H2O and CO2, C K-shell excitation and ionization of CO2 and B K-shell excitation of BF3, obtained at beamline 27SU of SPring-8 in Japan, are discussed as examples of atomic and molecular inner-shell spectroscopies using the third-generation synchrotron radiation sources.

Circular dichroism in the photoelectron angular distribution from randomly oriented enantiomers of camphor

Abstract: Circular dichroism in the angular distribution of valence photoelectrons emitted from randomly oriented chiral molecules has been observed in experiments that use circularly polarized VUV synchrotron radiation. Photoionization of the outermost carbonyl oxygen lone pair electrons from pure enantiomers of the prototype chiral molecule camphor is shown to have an asymmetry in the forward–backward scattering of photoelectrons (relative to the propagation direction of the light beam) of magnitude approaching 3% at 9.2 eV photon energy. The asymmetry reverses on exchange of either the helicity of the radiation or of the molecular enantiomer, confirming theoretical predictions of an effect that arises in the pure electric-dipole approximation.

Single-element elliptical hard x-ray micro-optics.

Abstract: Using micro-fabrication techniques, we have manufactured a single element kinoform lens in single-crystal silicon with an elliptical profile for 12.398 keV (1A) x-rays. By fabricating a lens that is optimized at fixed wavelengths, absorption in the lens material can be significantly reduced by removing 2π phase-shifting regions. This permits short focal length devices to be fabricated with small radii of curvatures at the lens apex. This feature allows one to obtain a high demagnification of a finite synchrotron electron source size. The reduced absorption loss also enables optics with a larger aperture, and hence improved resolution for focussing and imaging applications. Our first trial of these lenses has resulted in a one micron line focus (fwhm) at the National Synchrotron Light Source X13B beamline.

Measurement of gigawatt radiation pulses from a vacuum and extreme ultraviolet free-electron laser

Abstract: In order to measure the photon flux of highly intense and extremely pulsed vacuum ultraviolet (VUV) and extreme ultraviolet (EUV) radiation in absolute terms, we have developed a gas-monitor detector which is based on the atomic photoionization of a rare gas at low particle density. The device is indestructible and almost transparent. By first pulse-resolved measurements of VUV free-electron laser radiation at the TESLA test facility in Hamburg, a peak power of more than 100 MW was detected. Moreover, the extended dynamic range of the detector allowed its accurate calibration using spectrally dispersed synchrotron radiation at much lower photon intensities.

A high-resolution synchrotron-radiation angle-resolved photoemission spectrometer with in situ oxide thin film growth capability

Abstract: We have constructed a high-resolution synchrotron-radiation angle-resolved photoemission (ARPES) spectrometer combined with a combinatorial laser molecular-beam epitaxy (laser MBE) thin film growth system in order to investigate the electronic structure of transition metal oxide thin films. An ARPES spectrometer GAMMADATA SCIENTA SES-100 was selected for the high-throughput and high-energy and angular-resolution ARPES measurements. A total energy resolution of 6.3 meV and a momentum (an angular) resolution of 0.02 A−1 (0.2°) were obtained at a photon energy of 40 eV. The system is installed at the high-resolution vacuum-ultraviolet beamline BL-1C or the soft-x-ray undulator beamline BL-2C at the Photon Factory as an end-station. Another distinctive feature of this system is the direct connection from the spectrometer to a laser MBE chamber. Thin film samples can be transferred quickly into the photoemission chamber without breaking ultrahigh vacuum. Laser MBE is one of the best methods to grow thin films ...

Synchrotron texture analysis with area detectors

Abstract: The wide availability of X-ray area detectors provides an opportunity for using synchrotron radiation based X-ray diffraction for the determination of preferred crystallite orientation in polycrystalline materials. These measurements are very fast compared to other techniques. Texture is immediately recognized as intensity variations along Debye rings in diffraction images, yet in many cases this information is not used because the quantitative treatment of texture information has not yet been developed into a standard technique. In special cases it is possible to interpret the texture information contained in these intensity variations intuitively. However, diffraction studies focused on the effects of texture on materials properties often require the full orientation distribution function (ODF) which can be obtained from spherical tomography analysis. In cases of high crystal symmetry (cubic and hexagonal) an approximation to the full ODF can be reconstructed from single diffraction images, as is demonstrated for textures in rolled copper and titanium sheets. Combined with area detectors, the reconstruction methods make the measurements fast enough to study orientation changes during phase transformations, recrystallization and deformation in situ, and even in real time, at a wide range of temperature and pressure conditions. The present work focuses on practical aspects of texture measurement and data processing procedures to make the latter available for the growing community of synchrotron users. It reviews previous applications and highlights some opportunities for synchrotron texture analysis based on case studies on different materials.

Gamma‐ray bursts: optical afterglows in the deep Newtonian phase

Abstract: Gamma-ray burst remnants become trans-relativistic typically in days to tens of days, and they enter the deep Newtonian phase in tens of days to months, during which the majority of shock-accelerated electrons will no longer be highly relativistic. However, a small portion of electrons are still accelerated to ultra-relativistic speeds and are capable of emitting synchrotron radiation. The distribution function for electrons is re-derived here so that synchrotron emission from these relativistic electrons can be calculated. Based on the revised model, optical afterglows from both isotropic fireballs and highly collimated jets are studied numerically, and compared to analytical results. In the beamed cases, it is found that, in addition to the steepening due to the edge effect and the lateral expansion effect, the light curves are universally characterized by a flattening during the deep Newtonian phase.

X-ray and gamma-ray emission from millisecond pulsars

Abstract: We present a self-consistent model to describe X-ray and γ-ray emission from millisecond pulsars (MSPs). The X-rays of MSPs are produced by the backflow of primary charged particles from the outer gap and most likely consist of three components, two thermal components and one power law component if there is a strong multipole magnetic field on the stellar surface. The backflow of ultra-relativistic particles emits photons with energies about several tens of GeV via curvature radiation. These photons cause an electromagnetic cascade about 2-3 stellar radii above the polar cap. The synchrotron radiation of these cascade e γ pairs produces hard X-rays with a power law index ∼1.5. Near 10 5 cm above the stellar surface, the primary charged particles encounter the strong surface magnetic field, which alters the local radius of curvature greatly, and they quickly loose more than half of their remaining energies to curvature radiation. These curvature photons heat up the polar cap area with a radius ∼10 5 cm, which produce the softer thermal X-ray component. Finally, the primary charged particles deposit their remaining energies in a much smaller polar cap area, which corresponds to the footprints of outer gap and produce the medium hard X-ray component. γ-rays are produced in the outer gap through synchro-curvature radiation. We have applied this model to the MSPs which emit pulsed X-rays and likely γ-rays such as PSR J0437-4715, PSR J2124-3358, PSR J0218+4232 and PSR B 1821-24. Our results give an agreement between predicted spectrum and the observed spectrum of MSP emission.

Implications of the -ray polarization of GRB 021206

Abstract: We compare two possible scenarios for the production of a high level of polarization within the prompt emission of a GRB: synchrotron emission from a relativistic jet with a uniform (in space and time) magnetic field and synchrotron emission from a jet with a random magnetic field in the plane of the shock. Somewhat surprisingly we find that both scenarios can produce a comparable level of polarization (~45–50% for the uniform field and ~30–35% for a random field). A uniform time independent field most naturally arises by expansion of the field from the compact object. It requires a 1012 G field at the source and a transport of the field R−1. It does not imply Poynting flux domination of the energy of the wind. There is a serious difficulty however, within this scenario, in accounting for particle acceleration (which requires random magnetic fields) both for Poynting flux and non-Poynting flux domination. Significant polarization can also arise from a random field provided that the observer is located within a 1/Γ orientation from a narrow (θj ~ 1/Γ) jet. While most jets are wider, the jet of GRB 021206 from which strong polarization was recently observed is most likely very narrow. GRB 021206 is among the strongest bursts ever. Adopting the energy–angle relation we find an estimated angle of <1/40 rad or even smaller. Thus, for this particular burst the required geometry is not unusual. We conclude that the RHESSI observations suggest that the prompt emission results from synchrotron radiation. However, in view of the comparable levels of polarization predicted by both the random field and the homogeneous field scenarios, these observations are insufficient to rule out or confirm either one. An important difference between the two scenarios is that any observer will measure high polarization from a uniform magnetic field while only some of the observers will measure high polarization from a random magnetic field. Thus, future observations will enable us to distinguish between the two scenarios.

X-ray synchrotron study of liquid-vapor interfaces at short length scales: effect of long-range forces and bending energies.

Abstract: We have investigated the small-scale structure of the liquid-vapor interface using synchrotron x-ray scattering for liquids with different molecular structures and interactions. The effective momentum-dependent surface energy first decreases from its macroscopic value due to the effect of long-range forces, and then increases with increasing wave vector. The results are analyzed using a recent density functional theory. The large wave-vector increase is attributed to a bending energy for which local and nonlocal contributions are equally important.

Anomalous small-angle X-ray scattering in materials science

Abstract: After the exploratory studies of the 1980s, anomalous small-angle X-ray scattering (ASAXS) is now a mature technique to disentangle complex subjects in materials science: this is illustrated through selected examples.

The multifrequency variability of Mrk 421

Abstract: We present a model of the multifrequency variability of the blazar Mrk 421. The model explains correlated variability observed from Very High Energy (VHE) gamma rays to radio frequencies. We assume that the dominant part of the stationary emission from the radio frequencies to the X-rays is generated by the synchrotron radiation of relativistic electrons ejected from the central engine. The particles move from the center of the source with relativistic velocities and form an inhomogeneous jet. We perform detailed calculations of the radiation transfer and calculate evolution of the electron energy spectrum along the jet. We explain the observed variability by the evolving synchrotron and Inverse-Compton (IC) radiation of a compact component (a blob) which travels along the jet. Two scenarios have been considered as mechanisms to generate VHE flares. The first scenario assumes that the high energy electrons, necessary for generation of the VHE flares, are injected into the jet, directly from the central engine or from an acceleration zone (e.g., a shock wave). The second scheme assumes that the high energy electrons are generated in situ by acceleration, for example by diffusive shock waves or a localized turbulence inside the jet. The particles evolve along the jet. They are cooled by the radiative processes and by the adiabatic expansion which compete with the acceleration process and the injection of high energy electrons. We present new observations we obtained in the radio domain for Mrk 421. The radio data gathered in February–April 2001 show a well defined radio outburst which corresponds to an X-ray outburst observed by RXTE-ASM and a gamma-ray flare detected by HEGRA in the TeV range. The best of our knowledge, this is the first direct observational evidence for a flare observed simultaneously in the radio range and at very high energies. Our scenario with acceleration of electrons in the middle part of the jet describes well the temporal evolution of such multispectral flare.

Implications of the $\gamma$-ray Polarization of GRB 021206

Abstract: We compare two possible scenarios for the producing of high level of polarization within the prompt emission of a GRB: synchrotron emission from a relativistic jet with a uniform (in space and time) magnetic field and synchrotron emission from a jet with a random magnetic field in the plane of the shock. Somewhat surprisingly we find that both scenarios can produce a comparable level of polarization ($\sim 45-50$% for the uniform field and $\sim 30-35$% for a random field). Uniform time independent field most naturally arises by expansion of the field from the compact object. It requires a $10^{12}$G field at the source and a transport of the field as $\propto R^{-1}$. It {\it does not} imply Poynting flux domination of the energy of the wind. There is a serious difficulty however, within this scenario, accounting for particle acceleration (which requires random magnetic fields) both for Poynting flux and non-Poynting flux domination. Significant polarization can also arise from a random field provided that the observer is located within $1/\Gamma$ orientation from a narrow ($\theta_j \sim 1/\Gamma$) jet. While most jets are wider, the jet of GRB 021206 from which strong polarization was recently observed, was most likely very narrow. GRB 021206 is among the strongest bursts ever. Adopting the energy-angle relation we find an estimated angle of $<1/40$rad or even smaller. Thus, for this particular burst the required geometry is not unusual. We conclude that the RHESSI observations suggest that the prompt emission results from synchrotron radiation. However, in view of the comparable levels of polarizations predicted by both the random field and the homogeneous field scenarios these observations are insufficient to rule out or confirm either one.

Structural Change of Li1−xNi0.5Mn0.5O2 Cathode Materials for Lithium-ion Batteries by Synchrotron Radiation

Abstract: Synchrotron X-ray diffraction and XAFS measurement have been employed to investigate structural change and the charging process of a layered LiNi0.5Mn0.5O2 cathode material. The structure of charged Li1−xNi0.5Mn0.5O2 (x=0.5), which corresponds to the composition for showing rechargeable capacity, was determined. The results showed that divalent nickel metal was oxidized to trivalent after charging, in association with the phase transition from hexagonal (R3-m) to monoclinic (C2/m) resulting from the ordering of cations in the layered structure.

Helicity switching of circularly polarized undulator radiation by local orbit bumps

Abstract: Helicity switching of circularly polarized undulator radiation provides a valuable tool in synchrotron radiation experiments, particularly in the study of circular dichroism. At SPring-8, we have developed a helicity switching system by means of selecting radiation from two helical undulators. Right and left circular photon beams are alternately supplied to the beamline using electron beam orbit bumps. Instead of reversing the magnetic field applied to a sample, helicity switched light was used in magnetic circular dichroism measurements and the measuring time was reduced by 1 3 .

Radiometry with synchrotron radiation

Abstract: Electron storage rings are nearly ideal radiation sources for radiometry over a broad spectral range from the infrared to the x-ray region. Many national metrology institutes make extensive use of synchrotron radiation for radiometry. The Synchrotron Ultraviolet Radiation Facility SURF III, which has recently been upgraded, is used by the National Institute of Standards and Technology (NIST), and the Physikalisch-Technische Bundesanstalt (PTB) operates a European radiometry laboratory at the third-generation storage ring BESSY II. The storage rings are used as calculable broadband radiation sources (primary source standards) and in combination with primary detector standards as sources of continuously tunable monochromatic radiation for detector calibration. The use of cryogenic electrical-substitution radiometers as primary detector standards has made it possible to considerably extend high-accuracy calibrations from the ultraviolet (UV) to the x-ray regime. Radiometry in the extreme UV (EUV) range, and in particular reflectometry, has become increasingly important for the development of EUV lithography. An overview of synchrotron radiation based radiometry will be given.